Abstract

Active control of metamaterial properties with high tunability of both resonant intensity and frequency is essential for advanced terahertz (THz) applications, ranging from spectroscopy and sensing to communications. Among varied metamaterials, plasmon-induced transparency (PIT) has enabled active control with giant sensitivity by embedding semiconducting materials. However, there is still a stringent challenge to achieve dynamic responses in both intensity and frequency modulation. Here, an anisotropic THz active metamaterial device with an ultrasensitive modulation feature is proposed and experimentally studied. A radiative-radiative-coupled PIT system is established, with a frequency shift of 0.26 THz in its sharp transparent windows by polarization rotation. Enabled by high charge-carrier mobility and longer diffusion lengths, we utilize a straightforwardly spin-coated MAPbI3 film acting as a photoactive medium to endow the device with high sensitivity and ultrafast speed. When the device is pumped by an ultralow laser fluence, the PIT transmission windows at 0.86 and 1.12 THz demonstrate a significant reduction for two polarizations, respectively, with a full recovery time of 561 ps. In addition, we numerically prove the validity that the investigated resonator structure is sensitive to the optically induced conductivity. The hybrid system not only achieves resonant intensity and frequency modulations simultaneously, but also preserves the all-optical-induced switching merits with high sensitivity and speed, which enriches multifunctional subwavelength metamaterial devices at THz frequencies.

© 2019 Chinese Laser Press

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2019 (7)

J. Liu, Y. Zhou, Y. Lin, M. Li, H. Cai, Y. Liang, M. Liu, Z. Huang, F. Lai, F. Huang, and W. Zheng, “Anisotropic photo-response of the ultrathin GeSe nanoplates grown by rapid physical vapor deposition,” ACS Appl. Mater. Interfaces 11, 4123–4130 (2019).
[Crossref]

Y. S. Jonathan, F. Kebin, and J. P. A. Willie, “Zero-rank, maximum nullity perfect electromagnetic wave absorber,” Adv. Opt. Mater. 7, 1801632 (2019).
[Crossref]

X. Zhao, Y. Wang, J. Schalch, G. Duan, K. Cremin, J. Zhang, C. Chen, D. R. Averitt, and X. Zhang, “Optically modulated ultra-broadband all-silicon metamaterial terahertz absorbers,” ACS Photon. 6, 830–837 (2019).
[Crossref]

M. T. Nouman, J. Hwang, M. Faiyaz, G. Lee, D. Y. Noh, and J.-H. Jang, “Dynamic metasurface based cavity structures for enhanced absorption and phase modulation,” ACS Photon. 6, 374–381 (2019).
[Crossref]

G. P. Neupane, K. Zhou, S. Chen, T. Yildirim, P. Zhang, and Y. Lu, “In-plane isotropic/anisotropic 2D van der Waals heterostructures for future devices,” Small 15, 1804733 (2019).
[Crossref]

P. Pitchappa, A. Kumar, S. Prakash, H. Jani, T. Venkatesan, and R. Singh, “Chalcogenide phase change material for active terahertz photonics,” Adv. Mater. 31, 1808157 (2019).
[Crossref]

J. Zhen, W. Zhou, M. Chen, B. Li, L. Jia, M. Wang, and S. Yang, “Pyridine-functionalized fullerene additive enabling coordination interactions with CH3NH3PbI3 perovskite towards highly efficient bulk heterojunction solar cells,” J. Mater. Chem. A 7, 2754–2763 (2019).
[Crossref]

2018 (24)

A. Kumar, Y. K. Srivastava, M. Manjappa, and R. Singh, “Color-sensitive ultrafast optical modulation and switching of terahertz plasmonic devices,” Adv. Opt. Mater. 6, 1800030 (2018).
[Crossref]

W. X. Lim, M. Manjappa, Y. K. Srivastava, L. Cong, A. Kumar, K. F. MacDonald, and R. Singh, “Ultrafast all-optical switching of germanium-based flexible metaphotonic devices,” Adv. Mater. 30, 1705331 (2018).
[Crossref]

S.-F. Leung, K.-T. Ho, P.-K. Kung, V. K. S. Hsiao, H. N. Alshareef, Z. L. Wang, and J.-H. He, “A self-powered and flexible organometallic halide perovskite photodetector with very high detectivity,” Adv. Mater. 30, 1704611 (2018).
[Crossref]

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
[Crossref]

L. Cong, Y. K. Srivastava, H. Zhang, X. Zhang, J. Han, and S. Ranjan, “All-optical active THz metasurfaces for ultrafast polarization switching and dynamic beam splitting,” Light Sci. Appl. 7, 28 (2018).
[Crossref]

H. Jung, H. Jo, W. Lee, B. Kim, H. Choi, M. S. Kang, and H. Lee, “Electrical control of electromagnetically induced transparency by terahertz metamaterial funneling,” Adv. Opt. Mater. 7, 1801205 (2018).
[Crossref]

Z. Chen, X. Chen, L. Tao, K. Chen, M. Long, X. Liu, K. Yan, R. I. Stantchev, E. Pickwell-MacPherson, and J.-B. Xu, “Graphene controlled Brewster angle device for ultra-broadband terahertz modulation,” Nat. Commun. 9, 4909 (2018).
[Crossref]

T.-T. Kim, H.-D. Kim, R. Zhao, S. S. Oh, T. Ha, D. S. Chung, Y. H. Lee, B. Min, and S. Zhang, “Electrically tunable slow light using graphene metamaterials,” ACS Photon. 5, 1800–1807 (2018).
[Crossref]

S. J. Kindness, N. W. Almond, B. Wei, R. Wallis, W. Michailow, V. S. Kamboj, P. Braeuniger-Weimer, S. Hofmann, H. E. Beere, D. A. Ritchie, and R. Degl’Innocenti, “Active control of electromagnetically induced transparency in a terahertz metamaterial array with graphene for continuous resonance frequency tuning,” Adv. Opt. Mater. 6, 1800570 (2018).
[Crossref]

H. Jung, J. Koo, E. Heo, B. Cho, C. In, W. Lee, H. Jo, J. H. Cho, H. Choi, M. S. Kang, and H. Lee, “Electrically controllable molecularization of terahertz meta-atoms,” Adv. Mater. 30, 1802760 (2018).
[Crossref]

X. Chen, S. Ghosh, Q. Xu, C. Ouyang, Y. Li, X. Zhang, Z. Tian, J. Gu, L. Liu, A. K. Azad, J. Han, and W. Zhang, “Active control of polarization-dependent near-field coupling in hybrid metasurfaces,” Appl. Phys. Lett. 113, 061111 (2018).
[Crossref]

H. Cai, Q. Huang, X. Hu, Y. Liu, Z. Fu, Y. Zhao, H. He, and Y. Lu, “All-optical and ultrafast tuning of terahertz plasmonic metasurfaces,” Adv. Opt. Mater. 6, 1800143 (2018).
[Crossref]

W. Zhou, J. Chen, H. Gao, T. Hu, S. Ruan, A. Stroppa, and W. Ren, “Anomalous and polarization-sensitive photo-response of Td-WTe2 from visible to infrared light,” Adv. Mater. 31, 1804629 (2018).
[Crossref]

Y. Zhao, Y. Zhang, Q. Shi, S. Liang, W. Huang, W. Kou, and Z. Yang, “Dynamic photoinduced controlling of the large phase shift of terahertz waves via vanadium dioxide coupling nanostructures,” ACS Photon. 5, 3040–3050 (2018).
[Crossref]

M. Manjappa, P. Pitchappa, N. Wang, C. Lee, and R. Singh, “Active control of resonant cloaking in a terahertz MEMS metamaterial,” Adv. Opt. Mater. 6, 1800141 (2018).
[Crossref]

L. Cheng, Z. Jin, Z. Ma, F. Su, Y. Zhao, Y. Zhang, T. Su, Y. Sun, X. Xu, Z. Meng, Y. Bian, and Z. Sheng, “Mechanical terahertz modulation based on single-layered graphene,” Adv. Opt. Mater. 6, 1700877 (2018).
[Crossref]

Z. Wang, B. Ai, Z. Zhou, Y. Guan, H. Möhwald, and G. Zhang, “Free-standing plasmonic chiral metamaterials with 3D resonance cavities,” ACS Nano 12, 10914–10923 (2018).
[Crossref]

Z. Zhou, M. Long, L. Pan, X. Wang, M. Zhong, M. Blei, J. Wang, J. Fang, S. Tongay, W. Hu, J. Li, and Z. Wei, “Perpendicular optical reversal of the linear dichroism and polarized photodetection in 2D GeAs,” ACS Nano 12, 12416–12423 (2018).
[Crossref]

S. Yoo, S. Lee, and Q.-H. Park, “Loss-free negative-index metamaterials using forward light scattering in dielectric meta-atoms,” ACS Photon. 5, 1370–1374 (2018).
[Crossref]

K. Wei, T. Jiang, Z. Xu, J. Zhou, J. You, Y. Tang, H. Li, R. Chen, X. Zheng, S. Wang, K. Yin, Z. Wang, J. Wang, and X. Cheng, “Ultrafast carrier transfer promoted by interlayer Coulomb coupling in 2D/3D perovskite heterostructures,” Laser Photon. Rev. 12, 1800128 (2018).
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H. Li, X. Zheng, Y. Liu, Z. P. Zhang, and T. Jiang, “Ultrafast interfacial energy transfer and interlayer excitons in the monolayer WS2/CsPbBr3 quantum dot heterostructure,” Nanoscale 10, 1650–1659 (2018).
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B. Jeong, H. Han, Y. J. Choi, S. H. Cho, E. H. Kim, S. W. Lee, J. S. Kim, C. Park, D. Kim, and C. Park, “All-inorganic CsPbI3 perovskite phase-stabilized by poly(ethylene oxide) for red-light-emitting diodes,” Adv. Funct. Mater. 28, 1706401 (2018).
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R. Macedo, T. Dumelow, R. E. Camley, and R. L. Stamps, “Oriented asymmetric wave propagation and refraction bending in hyperbolic media,” ACS Photon. 5, 5086–5094 (2018).
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Y. K. Srivastava, M. Manjappa, L. Cong, H. N. S. Krishnamoorthy, V. Savinov, P. Pitchappa, and R. Singh, “A superconducting dual-channel photonic switch,” Adv. Mater. 30, 1801257 (2018).
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2017 (8)

C. La-o-vorakiat, L. Cheng, T. Salim, R. A. Marcus, M. E. M. Beyerle, Y. M. Lam, and E. E. M. Chia, “Hybrid tandem quantum dot/organic photovoltaic cells with complementary near infrared absorption,” Appl. Phys. Lett. 110, 123901 (2017).
[Crossref]

M. R. Shcherbakov, S. Liu, V. V. Zubyuk, A. Vaskin, P. P. Vabishchevich, G. Keeler, T. Pertsch, T. V. Dolgova, I. Staude, I. Brener, and A. A. Fedyanin, “Ultrafast all-optical tuning of direct-gap semiconductor metasurfaces,” Nat. Commun. 8, 17 (2017).
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Q. Yang, J. Gu, Y. Xu, X. Zhang, Y. Li, C. Ouyang, Z. Tian, J. Han, and W. Zhang, “Broadband and robust metalens with nonlinear phase profiles for efficient terahertz wave control,” Adv. Opt. Mater. 5, 1601084 (2017).
[Crossref]

Y. K. Srivastava, A. Chaturvedi, M. Manjappa, A. Kumar, G. Dayal, C. Kloc, and R. Singh, “MoS2 for ultrafast all-optical switching and modulation of THz Fano metaphotonic devices,” Adv. Opt. Mater. 5, 1700762 (2017).
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M. Liu, Z. Tian, X. Zhang, J. Gu, C. Ouyang, J. Han, and W. Zhang, “Tailoring the plasmon-induced transparency resonances in terahertz metamaterials,” Opt. Express 25, 19844–19855 (2017).
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L. Q. Cong, K. S. Yogesh, S. Ankur, C. S. Tze, and S. Ranjan, “Perovskite as a platform for active flexible metaphotonic devices,” ACS Photon. 4, 1595–1601 (2017).
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T. W. Crothers, R. L. Milot, J. B. Patel, E. S. Parrott, J. Schlipf, P. Müller-Buschbaum, M. B. Johnston, and L. M. Herz, “Photon reabsorption masks intrinsic bimolecular charge-carrier recombination in CH3NH3PbI3 perovskite,” Nano Lett. 17, 5782–5789 (2017).
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M. Manjappa, Y. K. Srivastava, A. Solanki, A. Kumar, T. C. Sum, and R. Singh, “Hybrid lead halide perovskites for ultrasensitive photoactive switching in terahertz metamaterial devices,” Adv. Mater. 29, 1605881 (2017).
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2016 (6)

M. H. Laura, “Charge-carrier dynamics in organic-inorganic metal halide perovskites,” Annu. Rev. Phys. Chem. 67, 65–89 (2016).
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A. S. Roberts, D. Wang, D. Fei, D. Wang, P. K. Kristensen, S. I. Bozhevolnyi, and K. Pedersen, “Multilayer tungsten-alumina-based broadband light absorbers for high-temperature applications,” Opt. Mater. Express 6, 2704–2714 (2016).
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C. Laovorakiat, J. M. Kadro, T. Salim, D. Zhao, T. Ahmed, Y. M. Lam, J. X. Zhu, R. A. Marcus, M. E. Michel-Beyerle, and E. E. M. Chia, “Phonon mode transformation across the orthohombic-tetragonal phase transition in a lead-iodide perovskite CH3NH3PbI3: a terahertz time-domain spectroscopy approach,” J. Phys. Chem. Lett. 7, 1–6 (2016).
[Crossref]

M. Bokdam, T. Sander, A. Stroppa, S. Picozzi, D. D. Sarma, C. Franchini, and G. Kresse, “Role of polar phonons in the photo excited state of metal halide perovskites,” Sci. Rep. 6, 28618 (2016).
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K. Wei, Z. J. Xu, R. Z. Chen, X. Zheng, X. A. Cheng, and T. Jiang, “Temperature-dependent excitonic photoluminescence excited by two-photon absorption in perovskite CsPbBr3 quantum dots,” Opt. Lett. 41, 3821–3824 (2016).
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O. E. Semonin, G. A. Elbaz, D. B. Straus, T. D. Hull, D. W. Paley, A. M. van der Zande, J. C. Hone, I. Kymissis, C. R. Kagan, X. Roy, and J. S. Owen, “Limits of carrier diffusion in n-type and p-type CH3NH3PbI3 perovskite single crystals,” J. Phys. Chem. Lett. 7, 3510–3518 (2016).
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2015 (7)

Y. Kim, E. Yassitepe, O. Voznyy, R. Comin, G. Walters, X. Gong, P. Kanjanaboos, A. F. Nogueira, and E. H. Sargent, “Efficient luminescence from perovskite quantum dot solids,” ACS Appl. Mater. Interfaces 7, 25007–25013 (2015).
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F. Zhang, H. Zhong, C. Chen, X.-G. Wu, X. Hu, H. Huang, J. Han, B. Zou, and Y. Dong, “Brightly luminescent and color-tunable colloidal CH3NH3PbX3 (X = Br, I, Cl) quantum dots: potential alternatives for display technology,” ACS Nano 9, 4533–4542 (2015).
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Q. A. Akkerman, V. D’Innocenzo, S. Accornero, A. Scarpellini, A. Petrozza, M. Prato, and L. Manna, “Tuning the optical properties of cesium lead halide perovskite nanocrystals by anion exchange reactions,” J. Am. Chem. Soc. 137, 10276–10281 (2015).
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X. Zhang, N. Xu, K. Qu, Z. Tian, R. Singh, J. Han, and W. L. Zhang, “Electromagnetically induced absorption in a three-resonator metasurface system,” Sci. Rep. 5, 10737 (2015).
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H. Cho, S.-H. Jeong, M.-H. Park, Y.-H. Kim, C. Wolf, C.-L. Lee, J. H. Heo, A. Sadhanala, N. Myoung, S. Yoo, S. H. Im, R. H. Friend, and T.-W. Lee, “Overcoming the electroluminescence efficiency limitations of perovskite light-emitting diodes,” Science 350, 1222–1225 (2015).
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D. A. Valverde-Chávez, C. S. Ponseca, C. C. Stoumpos, A. Yartsev, M. G. Kanatzidis, V. Sundström, and D. G. Cooke, “Intrinsic femtosecond charge generation dynamics in single crystal CH3NH3PbI3,” Energy Environ. Sci. 8, 3700–3707 (2015).
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Q. Dong, Y. Fang, Y. Shao, P. Mulligan, J. Qiu, L. Cao, and J. Huang, “Electron-hole diffusion lengths > 175  μm in solution-grown CH3NH3PbI3 single crystals,” Science 347, 967–970 (2015).
[Crossref]

2014 (4)

R. Schittny, M. Kadic, T. Buckmann, and M. Wegener, “Invisibility cloaking in a diffusive light scattering medium,” Science 345, 427–429 (2014).
[Crossref]

W. Christian, E. E. Giles, B. J. Michael, J. S. Henry, and M. H. Laura, “High charge carrier mobilities and lifetimes in organolead trihalide perovskites,” Energy Environ. Sci. 7, 2269 (2014).
[Crossref]

W. S. De, J. Holovsky, S. J. Moon, P. L. Per, B. Niesen, M. Ledinsky, F. J. Haug, J.-H. Yum, and C. Ballif, “Organometallic halide perovskites: sharp optical absorption edge and its relation to photovoltaic performance,” J. Phys. Chem. Lett. 5, 1035–1039 (2014).
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X. Guichuan, M. Nripan, S. L. Swee, Y. Natalia, L. Xinfeng, S. Dharani, G. Michael, M. Subodh, and C. S. Tze, “Low-temperature solution-processed wavelength-tunable perovskites for lasing,” Nat. Mater. 13, 476–480 (2014).
[Crossref]

2013 (2)

J. H. Heo, S. H. Im, J. H. Noh, T. N. Mandal, C. S. Lim, J. A. Chang, Y. H. Lee, H.-J. Kim, A. Sarkar, M. K. Nazeeruddin, M. Grätzel, and S. Seok, “Efficient inorganic-organic hybrid heterojunction solar cells containing perovskite compound and polymeric hole conductors,” Nat. Photonics 7, 486–491 (2013).
[Crossref]

C. W. Singh, R. Zhang, C. J. G. Han, M. Tonouchi, and W. L. Zhang, “Plasmon-induced transparency in metamaterials: active near field coupling between bright superconducting and dark metallic mode resonators,” Appl. Phys. Lett. 103, 101106 (2013).
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2012 (4)

P. Tassin, L. Zhang, R. Zhao, A. Jain, T. Koschny, and C. M. Soukoulis, “Electromagnetically induced transparency and absorption in metamaterials: the radiating two-oscillator model and its experimental confirmation,” Phys. Rev. Lett. 109, 187401 (2012).
[Crossref]

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

M. M. Lee, J. Teuscher, T. Miyasaka, T. N. Murakami, and H. J. Snaith, “Efficient hybrid solar cells based on meso-superstructured organometal halide perovskites,” Science 338, 643–647 (2012).
[Crossref]

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

Accornero, S.

Q. A. Akkerman, V. D’Innocenzo, S. Accornero, A. Scarpellini, A. Petrozza, M. Prato, and L. Manna, “Tuning the optical properties of cesium lead halide perovskite nanocrystals by anion exchange reactions,” J. Am. Chem. Soc. 137, 10276–10281 (2015).
[Crossref]

Agresti, A.

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
[Crossref]

Ahmed, T.

C. Laovorakiat, J. M. Kadro, T. Salim, D. Zhao, T. Ahmed, Y. M. Lam, J. X. Zhu, R. A. Marcus, M. E. Michel-Beyerle, and E. E. M. Chia, “Phonon mode transformation across the orthohombic-tetragonal phase transition in a lead-iodide perovskite CH3NH3PbI3: a terahertz time-domain spectroscopy approach,” J. Phys. Chem. Lett. 7, 1–6 (2016).
[Crossref]

Ai, B.

Z. Wang, B. Ai, Z. Zhou, Y. Guan, H. Möhwald, and G. Zhang, “Free-standing plasmonic chiral metamaterials with 3D resonance cavities,” ACS Nano 12, 10914–10923 (2018).
[Crossref]

Akkerman, Q. A.

Q. A. Akkerman, V. D’Innocenzo, S. Accornero, A. Scarpellini, A. Petrozza, M. Prato, and L. Manna, “Tuning the optical properties of cesium lead halide perovskite nanocrystals by anion exchange reactions,” J. Am. Chem. Soc. 137, 10276–10281 (2015).
[Crossref]

Almond, N. W.

S. J. Kindness, N. W. Almond, B. Wei, R. Wallis, W. Michailow, V. S. Kamboj, P. Braeuniger-Weimer, S. Hofmann, H. E. Beere, D. A. Ritchie, and R. Degl’Innocenti, “Active control of electromagnetically induced transparency in a terahertz metamaterial array with graphene for continuous resonance frequency tuning,” Adv. Opt. Mater. 6, 1800570 (2018).
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Alshareef, H. N.

S.-F. Leung, K.-T. Ho, P.-K. Kung, V. K. S. Hsiao, H. N. Alshareef, Z. L. Wang, and J.-H. He, “A self-powered and flexible organometallic halide perovskite photodetector with very high detectivity,” Adv. Mater. 30, 1704611 (2018).
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Ankur, S.

L. Q. Cong, K. S. Yogesh, S. Ankur, C. S. Tze, and S. Ranjan, “Perovskite as a platform for active flexible metaphotonic devices,” ACS Photon. 4, 1595–1601 (2017).
[Crossref]

Averitt, D. R.

X. Zhao, Y. Wang, J. Schalch, G. Duan, K. Cremin, J. Zhang, C. Chen, D. R. Averitt, and X. Zhang, “Optically modulated ultra-broadband all-silicon metamaterial terahertz absorbers,” ACS Photon. 6, 830–837 (2019).
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Azad, A. K.

X. Chen, S. Ghosh, Q. Xu, C. Ouyang, Y. Li, X. Zhang, Z. Tian, J. Gu, L. Liu, A. K. Azad, J. Han, and W. Zhang, “Active control of polarization-dependent near-field coupling in hybrid metasurfaces,” Appl. Phys. Lett. 113, 061111 (2018).
[Crossref]

Azad, K.

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

Ballif, C.

W. S. De, J. Holovsky, S. J. Moon, P. L. Per, B. Niesen, M. Ledinsky, F. J. Haug, J.-H. Yum, and C. Ballif, “Organometallic halide perovskites: sharp optical absorption edge and its relation to photovoltaic performance,” J. Phys. Chem. Lett. 5, 1035–1039 (2014).
[Crossref]

Beere, H. E.

S. J. Kindness, N. W. Almond, B. Wei, R. Wallis, W. Michailow, V. S. Kamboj, P. Braeuniger-Weimer, S. Hofmann, H. E. Beere, D. A. Ritchie, and R. Degl’Innocenti, “Active control of electromagnetically induced transparency in a terahertz metamaterial array with graphene for continuous resonance frequency tuning,” Adv. Opt. Mater. 6, 1800570 (2018).
[Crossref]

Bellani, S.

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
[Crossref]

Beyerle, M. E. M.

C. La-o-vorakiat, L. Cheng, T. Salim, R. A. Marcus, M. E. M. Beyerle, Y. M. Lam, and E. E. M. Chia, “Hybrid tandem quantum dot/organic photovoltaic cells with complementary near infrared absorption,” Appl. Phys. Lett. 110, 123901 (2017).
[Crossref]

Bian, Y.

L. Cheng, Z. Jin, Z. Ma, F. Su, Y. Zhao, Y. Zhang, T. Su, Y. Sun, X. Xu, Z. Meng, Y. Bian, and Z. Sheng, “Mechanical terahertz modulation based on single-layered graphene,” Adv. Opt. Mater. 6, 1700877 (2018).
[Crossref]

Blei, M.

Z. Zhou, M. Long, L. Pan, X. Wang, M. Zhong, M. Blei, J. Wang, J. Fang, S. Tongay, W. Hu, J. Li, and Z. Wei, “Perpendicular optical reversal of the linear dichroism and polarized photodetection in 2D GeAs,” ACS Nano 12, 12416–12423 (2018).
[Crossref]

Bokdam, M.

M. Bokdam, T. Sander, A. Stroppa, S. Picozzi, D. D. Sarma, C. Franchini, and G. Kresse, “Role of polar phonons in the photo excited state of metal halide perovskites,” Sci. Rep. 6, 28618 (2016).
[Crossref]

Bonaccorso, F.

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
[Crossref]

Bozhevolnyi, S. I.

Braeuniger-Weimer, P.

S. J. Kindness, N. W. Almond, B. Wei, R. Wallis, W. Michailow, V. S. Kamboj, P. Braeuniger-Weimer, S. Hofmann, H. E. Beere, D. A. Ritchie, and R. Degl’Innocenti, “Active control of electromagnetically induced transparency in a terahertz metamaterial array with graphene for continuous resonance frequency tuning,” Adv. Opt. Mater. 6, 1800570 (2018).
[Crossref]

Brener, I.

M. R. Shcherbakov, S. Liu, V. V. Zubyuk, A. Vaskin, P. P. Vabishchevich, G. Keeler, T. Pertsch, T. V. Dolgova, I. Staude, I. Brener, and A. A. Fedyanin, “Ultrafast all-optical tuning of direct-gap semiconductor metasurfaces,” Nat. Commun. 8, 17 (2017).
[Crossref]

Buckmann, T.

R. Schittny, M. Kadic, T. Buckmann, and M. Wegener, “Invisibility cloaking in a diffusive light scattering medium,” Science 345, 427–429 (2014).
[Crossref]

Cai, H.

J. Liu, Y. Zhou, Y. Lin, M. Li, H. Cai, Y. Liang, M. Liu, Z. Huang, F. Lai, F. Huang, and W. Zheng, “Anisotropic photo-response of the ultrathin GeSe nanoplates grown by rapid physical vapor deposition,” ACS Appl. Mater. Interfaces 11, 4123–4130 (2019).
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H. Cai, Q. Huang, X. Hu, Y. Liu, Z. Fu, Y. Zhao, H. He, and Y. Lu, “All-optical and ultrafast tuning of terahertz plasmonic metasurfaces,” Adv. Opt. Mater. 6, 1800143 (2018).
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Calabro, E.

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
[Crossref]

Camley, R. E.

R. Macedo, T. Dumelow, R. E. Camley, and R. L. Stamps, “Oriented asymmetric wave propagation and refraction bending in hyperbolic media,” ACS Photon. 5, 5086–5094 (2018).
[Crossref]

Cao, L.

Q. Dong, Y. Fang, Y. Shao, P. Mulligan, J. Qiu, L. Cao, and J. Huang, “Electron-hole diffusion lengths > 175  μm in solution-grown CH3NH3PbI3 single crystals,” Science 347, 967–970 (2015).
[Crossref]

Carlo, A. D.

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
[Crossref]

Castillo, A. E. D. R.

L. Najafi, B. Taheri, B. Martín-García, S. Bellani, D. D. Girolamo, A. Agresti, R. Oropesa-Nunez, S. Pescetelli, L. Vesce, E. Calabro, M. Prato, A. E. D. R. Castillo, A. D. Carlo, and F. Bonaccorso, “MoS2 quantum dot/graphene hybrids for advanced interface engineering of a CH3NH3PbI3 perovskite solar cell with an efficiency of over 20%,” ACS Nano 12, 10736–10754 (2018).
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Chang, J. A.

J. H. Heo, S. H. Im, J. H. Noh, T. N. Mandal, C. S. Lim, J. A. Chang, Y. H. Lee, H.-J. Kim, A. Sarkar, M. K. Nazeeruddin, M. Grätzel, and S. Seok, “Efficient inorganic-organic hybrid heterojunction solar cells containing perovskite compound and polymeric hole conductors,” Nat. Photonics 7, 486–491 (2013).
[Crossref]

Chaturvedi, A.

Y. K. Srivastava, A. Chaturvedi, M. Manjappa, A. Kumar, G. Dayal, C. Kloc, and R. Singh, “MoS2 for ultrafast all-optical switching and modulation of THz Fano metaphotonic devices,” Adv. Opt. Mater. 5, 1700762 (2017).
[Crossref]

Chen, A.

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

Chen, C.

X. Zhao, Y. Wang, J. Schalch, G. Duan, K. Cremin, J. Zhang, C. Chen, D. R. Averitt, and X. Zhang, “Optically modulated ultra-broadband all-silicon metamaterial terahertz absorbers,” ACS Photon. 6, 830–837 (2019).
[Crossref]

F. Zhang, H. Zhong, C. Chen, X.-G. Wu, X. Hu, H. Huang, J. Han, B. Zou, and Y. Dong, “Brightly luminescent and color-tunable colloidal CH3NH3PbX3 (X = Br, I, Cl) quantum dots: potential alternatives for display technology,” ACS Nano 9, 4533–4542 (2015).
[Crossref]

Chen, H.-T.

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
[Crossref]

J. Gu, R. Singh, X. Liu, X. Zhang, Y. Ma, S. Zhang, A. S. Maier, Z. Tian, K. Azad, A. Chen, H.-T. Chen, A. Taylor, J. Han, and W. Zhang, “Active control of electromagnetically induced transparency analogue in terahertz metamaterials,” Nat. Commun. 3, 1151 (2012).
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Chen, J.

W. Zhou, J. Chen, H. Gao, T. Hu, S. Ruan, A. Stroppa, and W. Ren, “Anomalous and polarization-sensitive photo-response of Td-WTe2 from visible to infrared light,” Adv. Mater. 31, 1804629 (2018).
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Chen, K.

Z. Chen, X. Chen, L. Tao, K. Chen, M. Long, X. Liu, K. Yan, R. I. Stantchev, E. Pickwell-MacPherson, and J.-B. Xu, “Graphene controlled Brewster angle device for ultra-broadband terahertz modulation,” Nat. Commun. 9, 4909 (2018).
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Q. Dong, Y. Fang, Y. Shao, P. Mulligan, J. Qiu, L. Cao, and J. Huang, “Electron-hole diffusion lengths > 175  μm in solution-grown CH3NH3PbI3 single crystals,” Science 347, 967–970 (2015).
[Crossref]

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Small (1)

G. P. Neupane, K. Zhou, S. Chen, T. Yildirim, P. Zhang, and Y. Lu, “In-plane isotropic/anisotropic 2D van der Waals heterostructures for future devices,” Small 15, 1804733 (2019).
[Crossref]

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Figures (11)

Fig. 1.
Fig. 1. (a) Schematic of the polarization-dependent metamaterial-perovskite THz device. A periodic array of CRRs and SRRs tailors the PIT resonance at different frequencies determined by incident polarizations. A thin perovskite film is deposited on the quartz substrate acting as a photoactive layer illuminated by optical pump pulses (400 nm). (b) Schematic view of the functional unit cell. The thickness of the quartz substrate is H=2  mm, the height of the Au metamaterial is h=127  nm, and the period is Px=150  μm, Py=110  μm. Geometric parameters of the structure are L1=120  μm, L2=50  μm, L11=26  μm, L12=25  μm, L21=50  μm, L22=18  μm, respectively. Inset presentation shows the crystal structure of T−CH3NH3PbI3 phases. Optical microscopic images of fabricated Au structures (c) before and (d) after covering a 55 nm perovskite thin film, where the scale bar represents 100 μm, and the inset picture shows the thickness of the perovskite film.
Fig. 2.
Fig. 2. (a) Simulated and (b) measured amplitude transmissions of the designed polarization-related metamaterial under illuminations of x-polarized (blue) and y-polarized (red) THz electric fields without perovskite coating. Dashed lines represent Fano-resonant frequencies for two polarized THz electric fields.
Fig. 3.
Fig. 3. Results of the optical modulation of anisotropic THz wave. Measured transmission spectra of the designed perovskite-based device of the (a) x-polarized and (c) y-polarized incident THz electric field under different pump powers. Corresponding numerically simulated transmission spectra of the (b) x-polarized and (d) y-polarized incident THz electric field under different conductivities of the perovskite thin film. The dashed lines mark the frequencies corresponding to the Fano resonance peaks.
Fig. 4.
Fig. 4. Calculated z-component field distributions in the transverse plane of the Au metasurface varying the conductivity of the perovskite film under the x-polarized THz electric field from 0 S/m to 960 S/m. Incident fields are normalized as 1 V/m.
Fig. 5.
Fig. 5. Calculated z-component field distributions in the transverse plane of the Au metasurface varying the conductivity of the perovskite film under the y-polarized THz electric field from 0 S/m to 1440 S/m. Incident fields are normalized as 1 V/m.
Fig. 6.
Fig. 6. Time-evolution dynamics of the metasurface-perovskite device. (a) Transient transmission spectra of the y-polarized THz electric field at different pump-probe delay values for an average pump fluence of 30  μJ/cm2. (b) Measured transient THz excitation dynamics for perovskite (CH3NH3PbI3) thin film spin-coated on the Fano-resonant metasurface implemented by using OPTP measurements for various pump fluences. Solid curves represent the fittings of recombination processes utilizing rate equations, where the dotted lines are measured by experiment.
Fig. 7.
Fig. 7. Normalized linear absorption and PL spectra of the spin-coated perovskite (CH3NH3PbI3) film. The PL and absorption peaks are located at 760 and 740 nm, respectively.
Fig. 8.
Fig. 8. Intrinsic THz spectra of SRR and CRR resonators along (a) x and (b) y directions. The near-field coupling effect between CRR and SRR is the origin of PIT resonance.
Fig. 9.
Fig. 9. Theoretical calculation results of the Lorentzian mechanical oscillator model along the (a) x-polarized and (b) y-polarized incident THz electric field.
Fig. 10.
Fig. 10. Group delay data extracted from experiment results as a function of pump fluence: (a) x-direction and (b) y-direction.
Fig. 11.
Fig. 11. Simulated results with a phonon mode at 1.0 THz in the perovskite thin film as a function of optical conductivity of the perovskite thin film.

Tables (1)

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Table 1. Some Reported Active Modulation of the Optically Controlled THz Modulator

Equations (5)

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EtEonEoffEon×100%,
ΔTT(t)=A1ett1+A2ett2+A3ett3+A0,
ΔTT(t)=A1ett1+A2ett2+A0,
ω12p¨(t)+Γ1ω11p˙(t)+p(t)=f(t)κq(t),ω22q¨(t)+Γ2ω21q˙(t)+q(t)=κp(t),
σ(ω)=iε0ω(ε1)+m=1ε0ωp,m2ωi(ω0,m2ω2)+ωΓm+iσωε0,