Abstract

Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we experimentally demonstrate the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi-photon wavelengths, and when excited by a pump beam it generates photon pairs with a rate of 35 Hz. Normalized to the pump energy stored by the nanoantenna, this rate corresponds to 1.4 GHz/Wm, being 1 order of magnitude higher than conventional on-chip or bulk photon-pair sources. Our experiments open the way for multiplexing several antennas for coherent generation of multi-photon quantum states with complex spatial-mode entanglement and applications in free-space quantum communications and sensing.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2019 (1)

G. Marino, C. Gigli, D. Rocco, A. Lemaítre, I. Favero, C. De Angelis, and G. Leo, “Zero-order second harmonic generation from AlGaAs-on-insulator metasurfaces,” ACS Photon. 6, 1226–1231 (2019).
[Crossref]

2018 (9)

F. Lenzini, A. N. Poddubny, J. Titchener, P. Fisher, A. Boes, S. Kasture, B. Haylock, M. Villa, A. Mitchell, A. S. Solntsev, A. A. Sukhorukov, and M. Lobino, “Direct characterization of a nonlinear photonic circuit’s wave function with laser light,” Light Sci. Appl. 7, 17143 (2018).
[Crossref]

A. S. Solntsev, P. Kumar, T. Pertsch, A. A. Sukhorukov, and F. Setzpfandt, “LiNbO3 waveguides for integrated SPDC spectroscopy,” APL Photon. 3, 021301 (2018).
[Crossref]

G. Marino, P. Segovia, A. V. Krasavin, P. Ginzburg, N. Olivier, G. A. Wurtz, and A. V. Zayats, “Second-harmonic generation from hyperbolic plasmonic nanorod metamaterial slab,” Laser Photon. Rev. 12, 1700189 (2018).
[Crossref]

S. Liu, P. P. Vabishchevich, A. Vaskin, J. L. Reno, G. A. Keeler, M. B. Sinclair, I. Staude, and I. Brener, “An all-dielectric metasurface as a broadband optical frequency mixer,” Nat. Commun. 9, 2506–2507 (2018).
[Crossref]

F. J. Löchner, A. N. Fedotova, S. Liu, G. A. Keeler, G. M. Peake, S. Saravi, M. R. Shcherbakov, S. Burger, A. A. Fedyanin, I. Brener, T. Pertsch, F. Setzpfandt, and I. Staude, “Polarization-dependent second harmonic diffraction from resonant GaAs metasurfaces,” ACS Photon. 5, 1786–1793 (2018).
[Crossref]

P. P. Vabishchevich, S. Liu, M. B. Sinclair, G. A. Keeler, G. M. Peake, and I. Brener, “Enhanced second-harmonic generation using broken symmetry III–V semiconductor Fano metasurfaces,” ACS Photon. 5, 1685–1690 (2018).
[Crossref]

K. Wang, J. G. Titchener, S. S. Kruk, L. Xu, H.-P. Chung, M. Parry, I. I. Kravchenko, Y.-H. Chen, A. S. Solntsev, Y. S. Kivshar, D. N. Neshev, and A. A. Sukhorukov, “Quantum metasurface for multiphoton interference and state reconstruction,” Science 361, 1104–1108 (2018).
[Crossref]

T. Stav, A. Faerman, E. Maguid, D. Oren, V. Kleiner, E. Hasman, and M. Segev, “Quantum entanglement of the spin and orbital angular momentum of photons using metamaterials,” Science 361, 1101–1104 (2018).
[Crossref]

H. Liu, C. Guo, G. Vampa, J. L. Zhang, T. Sarmiento, M. Xiao, P. H. Bucksbaum, J. Vučković, S. Fan, and D. A. Reis, “Enhanced high-harmonic generation from an all-dielectric metasurface,” Nat. Phys. 14, 1006 (2018).
[Crossref]

2017 (6)

L. Carletti, D. Rocco, A. Locatelli, C. De Angelis, V. F. Gili, M. Ravaro, I. Favero, G. Leo, M. Finazzi, L. Ghirardini, M. Celebrano, G. Marino, and A. V. Zayats, “Controlling second-harmonic generation at the nanoscale with monolithic AlGaAs-on-AlOx antennas,” Nanotechnology 28, 114005 (2017).
[Crossref]

G. Grinblat, Y. Li, M. P. Nielsen, R. F. Oulton, and S. A. Maier, “Efficient third harmonic generation and nonlinear subwavelength imaging at a higher-order anapole mode in a single germanium nanodisk,” ACS Nano 11, 953–960 (2017).
[Crossref]

P. Senellart, G. Solomon, and A. White, “High-performance semiconductor quantum-dot single-photon sources,” Nat. Nanotechnol. 12, 1026–1039 (2017).
[Crossref]

A. S. Solntsev and A. A. Sukhorukov, “Path-entangled photon sources on nonlinear chips,” Rev. Phys. 2, 19–31 (2017).
[Crossref]

X. Guo, C. L. Zou, C. Schuck, H. Jung, R. S. Cheng, and H. X. Tang, “Parametric down-conversion photon-pair source on a nanophotonic chip,” Light Sci. Appl. 6, e16249 (2017).
[Crossref]

M. Baselli, A. L. Baudrion, L. Ghirardini, G. Pellegrini, E. Sakat, L. Carletti, A. Locatelli, C. De Angelis, P. Biagioni, L. Duo, M. Finazzi, P. M. Adam, and M. Celebrano, “Plasmon-enhanced second harmonic generation: from individual antennas to extended arrays,” Plasmonics 12, 1595–1600 (2017).
[Crossref]

2016 (13)

A. Sipahigil, R. E. Evans, D. D. Sukachev, M. J. Burek, J. Borregaard, M. K. Bhaskar, C. T. Nguyen, J. L. Pacheco, H. A. Atikian, C. Meuwly, R. M. Camacho, F. Jelezko, E. Bielejec, H. Park, M. Loncar, and M. D. Lukin, “An integrated diamond nanophotonics platform for quantum-optical networks,” Science 354, 847–850 (2016).
[Crossref]

N. Somaschi, V. Giesz, L. De Santis, J. C. Loredo, M. P. Almeida, G. Hornecker, S. L. Portalupi, T. Grange, C. Anton, J. Demory, C. Gomez, I. Sagnes, N. D. Lanzillotti-Kimura, A. Lemaitre, A. Auffeves, A. G. White, L. Lanco, and P. Senellart, “Near-optimal single-photon sources in the solid state,” Nat. Photonics 10, 340–345 (2016).
[Crossref]

I. Aharonovich, D. Englund, and M. Toth, “Solid-state single-photon emitters,” Nat. Photonics 10, 631–641 (2016).
[Crossref]

T. T. Tran, K. Bray, M. J. Ford, M. Toth, and I. Aharonovich, “Quantum emission from hexagonal boron nitride monolayers,” Nat. Nanotechnol. 11, 37–42 (2016).
[Crossref]

C. Reimer, M. Kues, P. Roztocki, B. Wetzel, F. Grazioso, B. E. Little, S. T. Chu, T. Johnston, Y. Bromberg, L. Caspani, D. J. Moss, and R. Morandotti, “Generation of multiphoton entangled quantum states by means of integrated frequency combs,” Science 351, 1176–1180 (2016).
[Crossref]

S. Liu, M. B. Sinclair, S. Saravi, G. A. Keeler, Y. M. Yang, J. Reno, G. M. Peake, F. Setzpfandt, I. Staude, T. Pertsch, and I. Brener, “Resonantly enhanced second-harmonic generation using III-V semiconductor all-dielectric metasurfaces,” Nano Lett. 16, 5426–5432 (2016).
[Crossref]

R. Camacho-Morales, M. Rahmani, S. Kruk, L. Wang, L. Xu, D. A. Smirnova, A. S. Solntsev, A. Miroshnichenko, H. H. Tan, F. Karouta, S. Naureen, K. Vora, L. Carletti, C. De Angelis, C. Jagadish, Y. S. Kivshar, and D. N. Neshev, “Nonlinear generation of vector beams from AlGaAs nanoantennas,” Nano Lett. 16, 7191–7197 (2016).
[Crossref]

A. S. Shorokhov, E. V. Melik-Gaykazyan, D. A. Smirnova, B. Hopkins, K. E. Chong, D. Y. Choi, M. R. Shcherbakov, A. E. Miroshnichenko, D. N. Neshev, A. A. Fedyanin, and Y. S. Kivshar, “Multifold enhancement of third-harmonic generation in dielectric nanoparticles driven by magnetic Fano resonances,” Nano Lett. 16, 4857–4861 (2016).
[Crossref]

L. Carletti, A. Locatelli, D. Neshev, and C. De Angelis, “Shaping the radiation pattern of second-harmonic generation from AlGaAs dielectric nanoantennas,” ACS Photon. 3, 1500–1507 (2016).
[Crossref]

S. Rogers, D. Mulkey, X. Y. Lu, W. C. Jiang, and Q. Lin, “High visibility time-energy entangled photons from a silicon nanophotonic chip,” ACS Photon. 3, 1754–1761 (2016).
[Crossref]

A. I. Kuznetsov, A. E. Miroshnichenko, M. L. Brongersma, Y. S. Kivshar, and B. Luk’yanchuk, “Optically resonant dielectric nanostructures,” Science 354, aag2472 (2016).
[Crossref]

A. N. Poddubny, I. V. Iorsh, and A. A. Sukhorukov, “Generation of photon-plasmon quantum states in nonlinear hyperbolic metamaterials,” Phys. Rev. Lett. 117, 123901 (2016).
[Crossref]

V. F. Gili, L. Carletti, A. Locatelli, D. Rocco, M. Finazzi, L. Ghirardini, I. Favero, C. Gomez, A. Lemaitre, M. Celebrano, C. De Angelis, and G. Leo, “Monolithic AlGaAs second-harmonic nanoantennas,” Opt. Express 24, 15965–15971 (2016).
[Crossref]

2015 (3)

L. Carletti, A. Locatelli, O. Stepanenko, G. Leo, and C. De Angelis, “Enhanced second-harmonic generation from magnetic resonance in AlGaAs nanoantennas,” Opt. Express 23, 26544–26550 (2015).
[Crossref]

Y. M. Yang, W. Y. Wang, A. Boulesbaa, I. I. Kravchenko, D. P. Briggs, A. Puretzky, D. Geohegan, and J. Valentine, “Nonlinear Fano-resonant dielectric metasurfaces,” Nano Lett. 15, 7388–7393 (2015).
[Crossref]

M. Celebrano, X. F. Wu, M. Baselli, S. Grossmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duo, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10, 412–417 (2015).
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2014 (4)

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2013 (3)

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2012 (2)

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2010 (2)

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2009 (1)

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2007 (1)

2001 (1)

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2000 (1)

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Supplementary Material (1)

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Figures (3)

Fig. 1.
Fig. 1. Nonlinear nanoantenna for generation of spontaneous photon pairs. (a) Schematic representation of the nanoantenna-based source of photon pairs through the SPDC process. The inset depicts the energy diagram of the SPDC process. The SPDC pump is horizontally polarized along the [100] AlGaAs crystallographic axis. The signal and idler photons are generated by entangled magnetic dipole moments inside the volume of the AlGaAs nanoantenna, namely, mx and mz (sketched below the emitted photons). (b) Typical SEM images of [100] AlGaAs monolithic nanocylinders, 10 μm apart, such that each disk can be excited individually. (c) Simulated scattering efficiency Qsca and multipolar decomposition in terms of the two leading electric (ED) and magnetic dipoles (MD) for a nanocylinder with diameter d=430nm and height h=400nm. The vertical blue and orange bars show the spectral ranges of the pump light and the generated SPDC light (signal and idler), respectively.
Fig. 2.
Fig. 2. SFG nonlinear characterization of polarization correlations in the nanoantenna. (a) Schematic of the experimental arrangement and energy conservation diagram of the SFG process in the inset. (b) Signal (orange line) and idler (red line) spectra filtered from the femtossecond laser source. (c) Spectrum of the nonlinear wave mixing in the AlGaAs nanocylinder as a function of the time delay between the signal and idler pulses. The SFG only happens when the two pulses overlap, while the spectral features at 760 and 780 nm correspond to SHG from the individual signal and idler pulses. (d) Intensity of H-polarized reflected SFG at 770 nm measured with 16 combinations of horizontal (H), vertical (V), right circular (R), and left circular (L) polarizations of the signal and idler beams for the nanocylinder geometry in Fig. 1. (e) Measured reflected SFG images in k-space for the polarization combinations shown in (d) and SFG detected with NA=0.7.
Fig. 3.
Fig. 3. Generation of photon pairs in an AlGaAs disk nanoantenna. IR coincidence counts integrated over 24 h on two single-photon detectors after a beam splitter (shown in Fig. S8 of Supplement 1). A significant statistical increase, marked by the red bar, is apparent at a time difference of 26.5 ns, corresponding to the temporal delay between both detectors. Black dots are the measured coincidences, the yellow shadowed area indicates correlation due to thermal excitation of the semiconductor materials, while the green line is its fitted Gaussian curve. The light blue shading represents the statistical error of the background. The inset shows a schematic of the SPDC process and energy correlation. (b) and (c) Numerically simulated fields inside the nanocylinder when exciting mx and mz modes, respectively. The white arrows indicate the electric field vector. Different color bar scales are used, following the different intensities of mx, mz inside the nanocylinder, in contrast to the symmetric case of a nanosphere.

Equations (1)

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1ΦpdNpairdt=2πΞSFGλp4λs3λi3cΔλλs2.

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