Abstract

There is an increasing scientific and technological interest in the design and implementation of nanoscale sources of quantum light. Here, we investigate the quantum statistics of the light scattered from a plasmonic nanocavity coupled to a mesoscopic ensemble of emitters under low coherent pumping. We present an analytical description of the intensity correlations taking place in these systems and unveil the fingerprint of plasmon-exciton-polaritons in them. Our findings reveal that plasmonic cavities are able to retain and enhance excitonic nonlinearities, even when the number of emitters is large. This makes plasmonic strong coupling a promising route for generating nonclassical light beyond the single-emitter level.

© 2017 Optical Society of America

Full Article  |  PDF Article
OSA Recommended Articles
Plasmon-exciton-polariton lasing

Mohammad Ramezani, Alexei Halpin, Antonio I. Fernández-Domínguez, Johannes Feist, Said Rahimzadeh-Kalaleh Rodriguez, Francisco J. Garcia-Vidal, and Jaime Gómez Rivas
Optica 4(1) 31-37 (2017)

Effect of pure dephasing on the Jaynes-Cummings nonlinearities

A. Gonzalez-Tudela, E. del Valle, E. Cancellieri, C. Tejedor, D. Sanvitto, and F. P. Laussy
Opt. Express 18(7) 7002-7009 (2010)

References

  • View by:
  • |
  • |
  • |

  1. P. Törmä and W. L. Barnes, “Strong coupling between surface plasmon polaritons and emitters: a review,” Rep. Prog. Phys. 78, 013901 (2015).
    [Crossref]
  2. J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
    [Crossref]
  3. T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
    [Crossref]
  4. A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
    [Crossref]
  5. A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
    [Crossref]
  6. G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
    [Crossref]
  7. F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
    [Crossref]
  8. J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
    [Crossref]
  9. J. Galego, F. J. García-Vidal, and J. Feist, “Cavity-induced modifications of molecular structure in the strong-coupling regime,” Phys. Rev. X 5, 041022 (2015).
    [Crossref]
  10. E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
    [Crossref]
  11. J. Feist and F. J. García-Vidal, “Extraordinary exciton conductance induced by strong coupling,” Phys. Rev. Lett. 114, 196402 (2015).
    [Crossref]
  12. T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
    [Crossref]
  13. M. Ramezani, A. Halpin, A. I. Fernández-Domínguez, J. Feist, S. R.-K. Rodriguez, F. J. García-Vidal, and J. Gómez-Rivas, “Plasmon-exciton-polariton lasing,” Optica 4, 31–37 (2017).
    [Crossref]
  14. M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
    [Crossref]
  15. T. Holstein and H. Primakoff, “Field dependence of the intrinsic domain magnetization of a ferromagnet,” Phys. Rev. 58, 1098–1113 (1940).
    [Crossref]
  16. R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
    [Crossref]
  17. K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
    [Crossref]
  18. R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
    [Crossref]
  19. M. Tavis and F. W. Cummings, “Exact solution for an N-molecule-radiation-field Hamiltonian,” Phys. Rev. 170, 379–384 (1968).
    [Crossref]
  20. M. O. Scully and M. S. Zubairy, Quantum Optics (Cambridge University, 1997).
  21. B. R. Mollow, “Power spectrum of light scattered by two-level systems,” Phys. Rev. 188, 1969–1975 (1969).
    [Crossref]
  22. F. Miftasani and P. Machnikowski, “Photon–photon correlation statistics in the collective emission from ensembles of self-assembled quantum dots,” Phys. Rev. B 93, 075311 (2016).
    [Crossref]
  23. A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
    [Crossref]
  24. A. N. Poddubny, M. M. Glazov, and N. S. Averkiev, “Nonlinear emission spectra of quantum dots strongly coupled to a photonic mode,” Phys. Rev. B 82, 205330 (2010).
    [Crossref]
  25. P. M. Visser and G. Nienhuis, “Solution of quantum master equations in terms of a non-Hermitian Hamiltonian,” Phys. Rev. A 52, 4727–4736 (1995).
    [Crossref]
  26. R. J. Brecha, P. R. Rice, and M. Xiao, “N two-level atoms in a driven optical cavity: quantum dynamics of forward photon scattering for weak incident fields,” Phys. Rev. A 59, 2392–2417 (1999).
    [Crossref]
  27. K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
    [Crossref]
  28. A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
    [Crossref]
  29. H. Habibian, S. Zippilli, and G. Morigi, “Quantum light by atomic arrays in optical resonators,” Phys. Rev. A 84, 033829 (2011).
    [Crossref]
  30. A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
    [Crossref]
  31. F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
    [Crossref]

2017 (2)

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

M. Ramezani, A. Halpin, A. I. Fernández-Domínguez, J. Feist, S. R.-K. Rodriguez, F. J. García-Vidal, and J. Gómez-Rivas, “Plasmon-exciton-polariton lasing,” Optica 4, 31–37 (2017).
[Crossref]

2016 (4)

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
[Crossref]

R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
[Crossref]

F. Miftasani and P. Machnikowski, “Photon–photon correlation statistics in the collective emission from ensembles of self-assembled quantum dots,” Phys. Rev. B 93, 075311 (2016).
[Crossref]

2015 (7)

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

J. Galego, F. J. García-Vidal, and J. Feist, “Cavity-induced modifications of molecular structure in the strong-coupling regime,” Phys. Rev. X 5, 041022 (2015).
[Crossref]

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

J. Feist and F. J. García-Vidal, “Extraordinary exciton conductance induced by strong coupling,” Phys. Rev. Lett. 114, 196402 (2015).
[Crossref]

P. Törmä and W. L. Barnes, “Strong coupling between surface plasmon polaritons and emitters: a review,” Rep. Prog. Phys. 78, 013901 (2015).
[Crossref]

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

2014 (1)

A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
[Crossref]

2013 (2)

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

2012 (2)

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

2011 (3)

T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
[Crossref]

H. Habibian, S. Zippilli, and G. Morigi, “Quantum light by atomic arrays in optical resonators,” Phys. Rev. A 84, 033829 (2011).
[Crossref]

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

2010 (2)

A. N. Poddubny, M. M. Glazov, and N. S. Averkiev, “Nonlinear emission spectra of quantum dots strongly coupled to a photonic mode,” Phys. Rev. B 82, 205330 (2010).
[Crossref]

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

2008 (1)

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

2004 (1)

J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
[Crossref]

1999 (1)

R. J. Brecha, P. R. Rice, and M. Xiao, “N two-level atoms in a driven optical cavity: quantum dynamics of forward photon scattering for weak incident fields,” Phys. Rev. A 59, 2392–2417 (1999).
[Crossref]

1995 (1)

P. M. Visser and G. Nienhuis, “Solution of quantum master equations in terms of a non-Hermitian Hamiltonian,” Phys. Rev. A 52, 4727–4736 (1995).
[Crossref]

1969 (1)

B. R. Mollow, “Power spectrum of light scattered by two-level systems,” Phys. Rev. 188, 1969–1975 (1969).
[Crossref]

1968 (1)

M. Tavis and F. W. Cummings, “Exact solution for an N-molecule-radiation-field Hamiltonian,” Phys. Rev. 170, 379–384 (1968).
[Crossref]

1940 (1)

T. Holstein and H. Primakoff, “Field dependence of the intrinsic domain magnetization of a ferromagnet,” Phys. Rev. 58, 1098–1113 (1940).
[Crossref]

Antosiewicz, T. J.

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Auffeves, A.

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

Averkiev, N. S.

A. N. Poddubny, M. M. Glazov, and N. S. Averkiev, “Nonlinear emission spectra of quantum dots strongly coupled to a photonic mode,” Phys. Rev. B 82, 205330 (2010).
[Crossref]

Ballarini, D.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Barnes, W. L.

P. Törmä and W. L. Barnes, “Strong coupling between surface plasmon polaritons and emitters: a review,” Rep. Prog. Phys. 78, 013901 (2015).
[Crossref]

Barrow, S. J.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Baumberg, J. J.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Bellessa, J.

J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
[Crossref]

Benz, F.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Bitton, O.

K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
[Crossref]

Bonnand, C.

J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
[Crossref]

Bravo-Abad, J.

A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
[Crossref]

Brecha, R. J.

R. J. Brecha, P. R. Rice, and M. Xiao, “N two-level atoms in a driven optical cavity: quantum dynamics of forward photon scattering for weak incident fields,” Phys. Rev. A 59, 2392–2417 (1999).
[Crossref]

Chikkaraddy, R.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Chuntonov, L.

K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
[Crossref]

Cummings, F. W.

M. Tavis and F. W. Cummings, “Exact solution for an N-molecule-radiation-field Hamiltonian,” Phys. Rev. 170, 379–384 (1968).
[Crossref]

Cuscuna, M.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

D’Agostino, S.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Dayen, J. F.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

De Giorgi, M.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

de Nijs, B.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

del Valle, E.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

Delga, A.

A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
[Crossref]

Della Sala, F.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Demetriadou, A.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Devaux, E.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

Di Stefano, O.

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

Dominici, L.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Doudin, B.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Drezet, A.

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

Ebbesen, T. W.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
[Crossref]

Englund, D.

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Esposito, M.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Faraon, A.

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Feist, J.

M. Ramezani, A. Halpin, A. I. Fernández-Domínguez, J. Feist, S. R.-K. Rodriguez, F. J. García-Vidal, and J. Gómez-Rivas, “Plasmon-exciton-polariton lasing,” Optica 4, 31–37 (2017).
[Crossref]

J. Galego, F. J. García-Vidal, and J. Feist, “Cavity-induced modifications of molecular structure in the strong-coupling regime,” Phys. Rev. X 5, 041022 (2015).
[Crossref]

J. Feist and F. J. García-Vidal, “Extraordinary exciton conductance induced by strong coupling,” Phys. Rev. Lett. 114, 196402 (2015).
[Crossref]

A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
[Crossref]

Fernández-Domínguez, A. I.

M. Ramezani, A. Halpin, A. I. Fernández-Domínguez, J. Feist, S. R.-K. Rodriguez, F. J. García-Vidal, and J. Gómez-Rivas, “Plasmon-exciton-polariton lasing,” Optica 4, 31–37 (2017).
[Crossref]

R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
[Crossref]

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Fina, N.

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

Finley, J. J.

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

Fisher, K. A.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Fox, P.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

França Santos, M.

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

Fushman, I.

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Galego, J.

J. Galego, F. J. García-Vidal, and J. Feist, “Cavity-induced modifications of molecular structure in the strong-coupling regime,” Phys. Rev. X 5, 041022 (2015).
[Crossref]

García-Vidal, F. J.

M. Ramezani, A. Halpin, A. I. Fernández-Domínguez, J. Feist, S. R.-K. Rodriguez, F. J. García-Vidal, and J. Gómez-Rivas, “Plasmon-exciton-polariton lasing,” Optica 4, 31–37 (2017).
[Crossref]

R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
[Crossref]

J. Feist and F. J. García-Vidal, “Extraordinary exciton conductance induced by strong coupling,” Phys. Rev. Lett. 114, 196402 (2015).
[Crossref]

J. Galego, F. J. García-Vidal, and J. Feist, “Cavity-induced modifications of molecular structure in the strong-coupling regime,” Phys. Rev. X 5, 041022 (2015).
[Crossref]

A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
[Crossref]

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

Genes, C.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Genet, C.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
[Crossref]

George, J.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Gerace, D.

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

Gigli, G.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Glazov, M. M.

A. N. Poddubny, M. M. Glazov, and N. S. Averkiev, “Nonlinear emission spectra of quantum dots strongly coupled to a photonic mode,” Phys. Rev. B 82, 205330 (2010).
[Crossref]

Gómez-Rivas, J.

González-Tudela, A.

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

Habibian, H.

H. Habibian, S. Zippilli, and G. Morigi, “Quantum light by atomic arrays in optical resonators,” Phys. Rev. A 84, 033829 (2011).
[Crossref]

Hakala, T. K.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Halpin, A.

Haran, G.

K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
[Crossref]

Hernangómez-Pérez, D.

R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
[Crossref]

Hess, O.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Holstein, T.

T. Holstein and H. Primakoff, “Field dependence of the intrinsic domain magnetization of a ferromagnet,” Phys. Rev. 58, 1098–1113 (1940).
[Crossref]

Huidobro, P. A.

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

Hutchison, J. A.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
[Crossref]

Käll, M.

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Kelaita, Y. A.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Kim, M. S.

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

Lagoudakis, K. G.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Laucht, A.

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

Laussy, F. P.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

Lee, J.

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

Li, R.-Q.

R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
[Crossref]

Machnikowski, P.

F. Miftasani and P. Machnikowski, “Photon–photon correlation statistics in the collective emission from ensembles of self-assembled quantum dots,” Phys. Rev. B 93, 075311 (2016).
[Crossref]

Maier, S. A.

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

Martikainen, J.-P.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Martín-Moreno, L.

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

McEnery, K. R.

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

Miftasani, F.

F. Miftasani and P. Machnikowski, “Photon–photon correlation statistics in the collective emission from ensembles of self-assembled quantum dots,” Phys. Rev. B 93, 075311 (2016).
[Crossref]

Moilanen, A. J.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Mollow, B. R.

B. R. Mollow, “Power spectrum of light scattered by two-level systems,” Phys. Rev. 188, 1969–1975 (1969).
[Crossref]

Morigi, G.

H. Habibian, S. Zippilli, and G. Morigi, “Quantum light by atomic arrays in optical resonators,” Phys. Rev. A 84, 033829 (2011).
[Crossref]

Mugnier, J.

J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
[Crossref]

Müller, K.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Necada, M.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Nienhuis, G.

P. M. Visser and G. Nienhuis, “Solution of quantum master equations in terms of a non-Hermitian Hamiltonian,” Phys. Rev. A 52, 4727–4736 (1995).
[Crossref]

Nilsson, S.

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Orgiu, E.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Özdemir, S. K.

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

Petroff, P.

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Plenet, J. C.

J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
[Crossref]

Poddubny, A. N.

A. N. Poddubny, M. M. Glazov, and N. S. Averkiev, “Nonlinear emission spectra of quantum dots strongly coupled to a photonic mode,” Phys. Rev. B 82, 205330 (2010).
[Crossref]

Portolan, S.

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

Primakoff, H.

T. Holstein and H. Primakoff, “Field dependence of the intrinsic domain magnetization of a ferromagnet,” Phys. Rev. 58, 1098–1113 (1940).
[Crossref]

Pupillo, G.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Ramezani, M.

Rekola, H. T.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Rice, P. R.

R. J. Brecha, P. R. Rice, and M. Xiao, “N two-level atoms in a driven optical cavity: quantum dynamics of forward photon scattering for weak incident fields,” Phys. Rev. A 59, 2392–2417 (1999).
[Crossref]

Ridolfo, A.

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

Rodriguez, S. R.-K.

Rosta, E.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Rundquist, A.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Saija, R.

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

Samorì, P.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Sánchez-Muñoz, C.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Santhosh, K.

K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
[Crossref]

Sanvitto, D.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Sarmiento, T.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

Savasta, S.

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

Schachenmayer, J.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Scherman, O. A.

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

Schrapp, M.

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

Schwartz, T.

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
[Crossref]

Scully, M. O.

M. O. Scully and M. S. Zubairy, Quantum Optics (Cambridge University, 1997).

Shegai, T.

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Stellacci, F.

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Stoltz, N.

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Tame, M. S.

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

Tarantini, I.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Tavis, M.

M. Tavis and F. W. Cummings, “Exact solution for an N-molecule-radiation-field Hamiltonian,” Phys. Rev. 170, 379–384 (1968).
[Crossref]

Tejedor, C.

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

Todisco, F.

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Törmä, P.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

P. Törmä and W. L. Barnes, “Strong coupling between surface plasmon polaritons and emitters: a review,” Rep. Prog. Phys. 78, 013901 (2015).
[Crossref]

Väkeväinen, A. I.

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Visser, P. M.

P. M. Visser and G. Nienhuis, “Solution of quantum master equations in terms of a non-Hermitian Hamiltonian,” Phys. Rev. A 52, 4727–4736 (1995).
[Crossref]

Vuckovic, J.

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Wersäll, M.

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Xiao, M.

R. J. Brecha, P. R. Rice, and M. Xiao, “N two-level atoms in a driven optical cavity: quantum dynamics of forward photon scattering for weak incident fields,” Phys. Rev. A 59, 2392–2417 (1999).
[Crossref]

Zengin, G.

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Zippilli, S.

H. Habibian, S. Zippilli, and G. Morigi, “Quantum light by atomic arrays in optical resonators,” Phys. Rev. A 84, 033829 (2011).
[Crossref]

Zubairy, M. S.

M. O. Scully and M. S. Zubairy, Quantum Optics (Cambridge University, 1997).

ACS Nano (1)

F. Todisco, S. D’Agostino, M. Esposito, A. I. Fernández-Domínguez, M. De Giorgi, D. Ballarini, L. Dominici, I. Tarantini, M. Cuscuna, F. Della Sala, G. Gigli, and D. Sanvitto, “Exciton–plasmon coupling enhancement via metal oxidation,” ACS Nano 9, 9691–9699 (2015).
[Crossref]

Angew. Chem. (1)

J. A. Hutchison, T. Schwartz, C. Genet, E. Devaux, and T. W. Ebbesen, “Modifying chemical landscapes by coupling to vacuum fields,” Angew. Chem. 124, 1624–1628 (2012).
[Crossref]

J. Nanophoton. (1)

F. P. Laussy, E. del Valle, M. Schrapp, A. Laucht, and J. J. Finley, “Climbing the Jaynes–Cummings ladder by photon counting,” J. Nanophoton. 6, 061803 (2012).
[Crossref]

Nat. Commun. (2)

K. Santhosh, O. Bitton, L. Chuntonov, and G. Haran, “Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit,” Nat. Commun. 7, 11823 (2016).
[Crossref]

T. K. Hakala, H. T. Rekola, A. I. Väkeväinen, J.-P. Martikainen, M. Nečada, A. J. Moilanen, and P. Törmä, “Lasing in dark and bright modes of a finite-sized plasmonic lattice,” Nat. Commun. 8, 13687 (2017).
[Crossref]

Nat. Mater. (1)

E. Orgiu, J. George, J. A. Hutchison, E. Devaux, J. F. Dayen, B. Doudin, F. Stellacci, C. Genet, J. Schachenmayer, C. Genes, G. Pupillo, P. Samorì, and T. W. Ebbesen, “Conductivity in organic semiconductors,” Nat. Mater. 14, 1123–1129 (2015).
[Crossref]

Nat. Phys. (2)

M. S. Tame, K. R. McEnery, S. K. Özdemir, J. Lee, S. A. Maier, and M. S. Kim, “Quantum plasmonics,” Nat. Phys. 9, 329–340 (2013).
[Crossref]

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vučković, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

Nature (1)

R. Chikkaraddy, B. de Nijs, F. Benz, S. J. Barrow, O. A. Scherman, E. Rosta, A. Demetriadou, P. Fox, O. Hess, and J. J. Baumberg, “Single-molecule strong coupling at room temperature in plasmonic nanocavities,” Nature 535, 127–130 (2016).
[Crossref]

New J. Phys. (1)

A. Auffeves, D. Gerace, S. Portolan, A. Drezet, and M. França Santos, “Few emitters in a cavity: from cooperative emission to individualization,” New J. Phys. 13, 093020 (2011).
[Crossref]

Optica (1)

Phys. Rev. (3)

T. Holstein and H. Primakoff, “Field dependence of the intrinsic domain magnetization of a ferromagnet,” Phys. Rev. 58, 1098–1113 (1940).
[Crossref]

M. Tavis and F. W. Cummings, “Exact solution for an N-molecule-radiation-field Hamiltonian,” Phys. Rev. 170, 379–384 (1968).
[Crossref]

B. R. Mollow, “Power spectrum of light scattered by two-level systems,” Phys. Rev. 188, 1969–1975 (1969).
[Crossref]

Phys. Rev. A (3)

P. M. Visser and G. Nienhuis, “Solution of quantum master equations in terms of a non-Hermitian Hamiltonian,” Phys. Rev. A 52, 4727–4736 (1995).
[Crossref]

R. J. Brecha, P. R. Rice, and M. Xiao, “N two-level atoms in a driven optical cavity: quantum dynamics of forward photon scattering for weak incident fields,” Phys. Rev. A 59, 2392–2417 (1999).
[Crossref]

H. Habibian, S. Zippilli, and G. Morigi, “Quantum light by atomic arrays in optical resonators,” Phys. Rev. A 84, 033829 (2011).
[Crossref]

Phys. Rev. B (2)

A. N. Poddubny, M. M. Glazov, and N. S. Averkiev, “Nonlinear emission spectra of quantum dots strongly coupled to a photonic mode,” Phys. Rev. B 82, 205330 (2010).
[Crossref]

F. Miftasani and P. Machnikowski, “Photon–photon correlation statistics in the collective emission from ensembles of self-assembled quantum dots,” Phys. Rev. B 93, 075311 (2016).
[Crossref]

Phys. Rev. Lett. (9)

R.-Q. Li, D. Hernangómez-Pérez, F. J. García-Vidal, and A. I. Fernández-Domínguez, “Transformation optics approach to plasmon-exciton strong coupling in nanocavities,” Phys. Rev. Lett. 117, 107401 (2016).
[Crossref]

K. Müller, A. Rundquist, K. A. Fisher, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez-Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

A. Ridolfo, O. Di Stefano, N. Fina, R. Saija, and S. Savasta, “Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics,” Phys. Rev. Lett. 105, 263601 (2010).
[Crossref]

J. Feist and F. J. García-Vidal, “Extraordinary exciton conductance induced by strong coupling,” Phys. Rev. Lett. 114, 196402 (2015).
[Crossref]

J. Bellessa, C. Bonnand, J. C. Plenet, and J. Mugnier, “Strong coupling between surface plasmons and excitons in an organic semicoductor,” Phys. Rev. Lett. 93, 036404 (2004).
[Crossref]

T. Schwartz, J. A. Hutchison, C. Genet, and T. W. Ebbesen, “Reversible switching of ultrastrong light–molecule coupling,” Phys. Rev. Lett. 106, 196405 (2011).
[Crossref]

A. González-Tudela, P. A. Huidobro, L. Martín-Moreno, C. Tejedor, and F. J. García-Vidal, “Theory of strong coupling between quantum emitters and propagating surface plasmons,” Phys. Rev. Lett. 110, 126801 (2013).
[Crossref]

A. Delga, J. Feist, J. Bravo-Abad, and F. J. García-Vidal, “Quantum emitters near a metal nanoparticle: strong coupling and quenching,” Phys. Rev. Lett. 112, 253601 (2014).
[Crossref]

G. Zengin, M. Wersäll, S. Nilsson, T. J. Antosiewicz, M. Käll, and T. Shegai, “Realizing strong light–matter interactions between single-nanoparticle plasmons and molecular excitons at ambient conditions,” Phys. Rev. Lett. 114, 157401 (2015).
[Crossref]

Phys. Rev. X (1)

J. Galego, F. J. García-Vidal, and J. Feist, “Cavity-induced modifications of molecular structure in the strong-coupling regime,” Phys. Rev. X 5, 041022 (2015).
[Crossref]

Rep. Prog. Phys. (1)

P. Törmä and W. L. Barnes, “Strong coupling between surface plasmon polaritons and emitters: a review,” Rep. Prog. Phys. 78, 013901 (2015).
[Crossref]

Other (1)

M. O. Scully and M. S. Zubairy, Quantum Optics (Cambridge University, 1997).

Supplementary Material (1)

NameDescription
» Supplement 1       Supplemental document

Cited By

OSA participates in Crossref's Cited-By Linking service. Citing articles from OSA journals and other participating publishers are listed here.

Alert me when this article is cited.


Figures (4)

Fig. 1.
Fig. 1.

QE ensemble resonantly coupled to a generic plasmonic cavity. The right inset depicts the two-level QE model.

Fig. 2.
Fig. 2.

Correlation function g(2)(0) versus laser detuning for SP (black dashed–dotted line) and QEs (colored lines) uncoupled. Various ensemble sizes are shown, with (solid) and without (dashed) the inclusion of QE nonradiative decay, γQEnr.

Fig. 3.
Fig. 3.

(a1)–(d1) Scattering intensity I and (a2)–(d2) correlation function g(2)(0) versus laser frequency and single emitter cooperativity for various QE–SP systems. In the upper (lower) panels dotted (dashed) lines plot the PEP frequencies (half-frequencies) in the one-excitation (two-excitation) manifold.

Fig. 4.
Fig. 4.

Maximum (top) and minimum (bottom) correlation functions as functions of the QE ensemble size for several values of the single emitter cooperativity. The inset in the upper panel shows the map of photon positive (yellow) and negative (violet) correlations as functions of N and C.

Equations (5)

Equations on this page are rendered with MathJax. Learn more.

i[ρ^,H^]+γSP2La^[ρ^]+γQEr2LS^[ρ^]+γQEnr2i=1NLσ^i[ρ^]=0,
H^=ΔSPa^a^+ΔQES^z+λ(S^+a^+S^a^)+ΩSP(a^+a^)+ΩQE(S^++S^),
H^eff=H^iγSP2a^a^iγQEnr2S^ziγQEr2S^+S^,
I=(ηNμSPΩSP)2|ηΔ˜SP+Δ˜QE/ηN2λΔ˜SPΔ˜QENλ2|2,
g(2)(0)=|11N(ηΔ˜SPληΔ˜SP+Δ˜QE/ηN2λ)2(Δ˜QE+iNγQEr/2)[Δ˜QEΔ˜SP+(Δ˜SPλ/η)2Nλ2](Δ˜QE+iγQEr/2)[Δ˜QEΔ˜SP+Δ˜SP2Nλ2]Δ˜SP(N1)λ2|2.

Metrics