Abstract

Arrays of identical and individually addressable qubits lay the foundation for the creation of scalable quantum hardware such as quantum processors and repeaters. Silicon-vacancy (SiV) centers in diamond offer excellent physical properties such as low inhomogeneous broadening, fast photon emission, and a large Debye–Waller factor. The possibility for all-optical ultrafast manipulation and techniques to extend the spin coherence times makes them promising candidates for qubits. Here, we have developed arrays of nanopillars containing single (SiV) centers with high yield, and we demonstrate ultrafast all-optical complete coherent control of the excited state population of a single SiV center at the optical transition frequency. The high quality of the chemical vapor deposition (CVD) grown SiV centers provides excellent spectral stability, which allows us to coherently manipulate and quasi-resonantly read out the excited state population of individual SiV centers on picosecond timescales using ultrafast optical pulses. This work opens new opportunities to create a scalable on-chip diamond platform for quantum information processing and scalable nanophotonics applications.

© 2017 Optical Society of America

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References

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2017 (4)

Y.-C. Chen, P. S. Salter, S. Knauer, L. Weng, A. C. Frangeskou, C. J. Stephen, S. N. Ishmael, P. R. Dolan, S. Johnson, B. L. Green, G. W. Morley, M. E. Newton, J. G. Rarity, M. J. Booth, and J. M. Smith, “Laser writing of coherent colour centres in diamond,” Nat. Photonics 11, 77–80 (2017).
[Crossref]

T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
[Crossref]

Y. Zhou, A. Rasmita, K. Li, Q. Xiong, I. Aharonovich, and W. B. Gao, “Coherent control of a strongly driven silicon vacancy optical transition in diamond,” Nat. Commun. 8, 14451 (2017).
[Crossref]

B. Pingault, D. D. Jarausch, C. Hepp, L. Klintberg, J. N. Becker, M. Markham, C. Becher, and M. Atature, “Coherent control of the silicon-vacancy spin in diamond,” Nat. Commun. 8, 15579 (2017).
[Crossref]

2016 (7)

J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
[Crossref]

J. N. Becker, J. Gorlitz, C. Arend, M. Markham, and C. Becher, “Ultrafast all-optical coherent control of single silicon vacancy colour centres in diamond,” Nat. Commun. 7, 13512 (2016).
[Crossref]

C. Arend, J. N. Becker, H. Sternschulte, D. Steinmüller-Nethl, and C. Becher, “Photoluminescence excitation and spectral hole burning spectroscopy of silicon vacancy centers in diamond,” Phys. Rev. B 94, 045203 (2016).
[Crossref]

K. G. Lagoudakis, P. L. McMahon, C. Dory, K. A. Fischer, K. Müller, V. Borish, D. Dalacu, P. J. Poole, M. E. Reimer, V. Zwiller, Y. Yamamoto, and J. Vučković, “Ultrafast coherent manipulation of trions in site-controlled nanowire quantum dots,” Optica 3, 1430–1435 (2016).
[Crossref]

K. G. Lagoudakis, P. L. McMahon, K. A. Fischer, S. Puri, K. Müller, D. Dan, P. J. Poole, M. E. Reimer, V. Zwiller, Y. Yamamoto, and J. Vučković, “Initialization of a spin qubit in a site-controlled nanowire quantum dot,” New J. Phys. 18, 053024 (2016).
[Crossref]

R. E. Evans, A. Sipahigil, D. D. Sukachev, A. S. Zibrov, and M. D. Lukin, “Narrow-linewidth homogeneous optical emitters in diamond nanostructures via silicon ion implantation,” Phys. Rev. Appl. 5, 044010 (2016).
[Crossref]

A. Sipahigil, R. E. Evans, D. D. Sukachev, M. J. Burek, J. Borregaard, M. K. Bhaskar, C. T. Nguyen, J. L. Pacheco, H. A. Atikian, C. Meuwly, R. M. Camacho, F. Jelezko, E. Bielejec, H. Park, M. Lončar, and M. D. Lukin, “An integrated diamond nanophotonics platform for quantum optical networks,” Science 354, 847–850 (2016).
[Crossref]

2015 (2)

S. Unsleber, S. Maier, D. P. S. McCutcheon, Y.-M. He, M. Dambach, M. Gschrey, N. Gregersen, J. Mørk, S. Reitzenstein, S. Höfling, C. Schneider, and M. Kamp, “Observation of resonance fluorescence and the Mollow triplet from a coherently driven site-controlled quantum dot,” Optica 2, 1072–1077 (2015).
[Crossref]

K. D. Jahnke, A. Sipahigil, J. M. Binder, M. W. Doherty, M. Metsch, L. J. Rogers, N. B. Manson, M. D. Lukin, and F. Jelezko, “Electron-phonon processes of the silicon-vacancy centre in diamond,” New J. Phys. 17, 043011 (2015).
[Crossref]

2014 (5)

L. J. Rogers, K. D. Jahnke, M. H. Metsch, A. Sipahigil, J. M. Binder, T. Teraji, H. Sumiya, J. Isoya, M. D. Lukin, P. Hemmer, and F. Jelezko, “All-optical initialization, readout, and coherent preparation of single silicon-vacancy spins in diamond,” Phys. Rev. Lett. 113, 263602 (2014).
[Crossref]

B. Pingault, J. N. Becker, C. H. Schulte, C. Arend, C. Hepp, T. Godde, A. I. Tartakovskii, M. Markham, C. Becher, and M. Atature, “All-optical formation of coherent dark states of silicon-vacancy spins in diamond,” Phys. Rev. Lett. 113, 263601 (2014).
[Crossref]

J. Riedrich-Moller, C. Arend, C. Pauly, F. Mucklich, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “Deterministic coupling of a single silicon-vacancy color center to a photonic crystal cavity in diamond,” Nano Lett. 14, 5281–5287 (2014).
[Crossref]

A. Sipahigil, K. D. Jahnke, L. J. Rogers, T. Teraji, J. Isoya, A. S. Zibrov, F. Jelezko, and M. D. Lukin, “Indistinguishable photons from separated silicon-vacancy centers in diamond,” Phys. Rev. Lett. 113, 113602 (2014).
[Crossref]

L. J. Rogers, K. D. Jahnke, T. Teraji, L. Marseglia, C. Muller, B. Naydenov, H. Schauffert, C. Kranz, J. Isoya, L. P. McGuinness, and F. Jelezko, “Multiple intrinsically identical single-photon emitters in the solid state,” Nat. Commun. 5, 4739 (2014).
[Crossref]

2013 (2)

B. J. Hausmann, I. B. Bulu, P. B. Deotare, M. McCutcheon, V. Venkataraman, M. L. Markham, D. J. Twitchen, and M. Loncar, “Integrated high-quality factor optical resonators in diamond,” Nano Lett. 13, 1898–1902 (2013).
[Crossref]

M. J. Burek, D. Ramos, P. Patel, I. W. Frank, and M. Lončar, “Nanomechanical resonant structures in single-crystal diamond,” Appl. Phys. Lett. 103, 131904 (2013).
[Crossref]

2012 (4)

M. J. Burek, N. P. de Leon, B. J. Shields, B. J. Hausmann, Y. Chu, Q. Quan, A. S. Zibrov, H. Park, M. D. Lukin, and M. Loncar, “Free-standing mechanical and photonic nanostructures in single-crystal diamond,” Nano Lett. 12, 6084–6089 (2012).
[Crossref]

A. Faraon, C. Santori, Z. Huang, V. M. Acosta, and R. G. Beausoleil, “Coupling of nitrogen-vacancy centers to photonic crystal cavities in monocrystalline diamond,” Phys. Rev. Lett. 109, 033604 (2012).
[Crossref]

J. Riedrich-Moller, L. Kipfstuhl, C. Hepp, E. Neu, C. Pauly, F. Mucklich, A. Baur, M. Wandt, S. Wolff, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “One- and two-dimensional photonic crystal microcavities in single crystal diamond,” Nat. Nanotechnol. 7, 69–74 (2012).
[Crossref]

P. C. Maurer, G. Kucsko, C. Latta, L. Jiang, N. Y. Yao, S. D. Bennett, F. Pastawski, D. Hunger, N. Chisholm, M. Markham, D. J. Twitchen, J. I. Cirac, and M. D. Lukin, “Room-temperature quantum bit memory exceeding one second,” Science 336, 1283–1286 (2012).
[Crossref]

2011 (1)

E. Neu, D. Steinmetz, J. Riedrich-Möller, S. Gsell, M. Fischer, M. Schreck, and C. Becher, “Single photon emission from silicon-vacancy colour centres in chemical vapour deposition nano-diamonds on iridium,” New J. Phys. 13, 025012 (2011).
[Crossref]

2010 (3)

D. de Lange, Z. H. Wang, D. Riste, V. V. Dobrovitski, and R. Hanson, “Universal dynamical decoupling of a single solid-state spin from a spin bath,” Science 330, 60–63 (2010).
[Crossref]

D. M. Toyli, C. D. Weis, G. D. Fuchs, T. Schenkel, and D. D. Awschalom, “Chip-scale nanofabrication of single spins and spin arrays in diamond,” Nano Lett. 10, 3168–3172 (2010).
[Crossref]

E. D. Kim, K. Truex, X. Xu, B. Sun, D. G. Steel, A. S. Bracker, D. Gammon, and L. J. Sham, “Fast spin rotations by optically controlled geometric phases in a charge-tunable InAs quantum dot,” Phys. Rev. Lett. 104, 167401 (2010).
[Crossref]

2009 (1)

G. Balasubramanian, P. Neumann, D. Twitchen, M. Markham, R. Kolesov, N. Mizuochi, J. Isoya, J. Achard, J. Beck, J. Tissler, V. Jacques, P. R. Hemmer, F. Jelezko, and J. Wrachtrup, “Ultralong spin coherence time in isotopically engineered diamond,” Nat. Mater. 8, 383–387 (2009).
[Crossref]

2008 (1)

H. J. Kimble, “The quantum internet,” Nature 453, 1023–1030 (2008).
[Crossref]

Achard, J.

G. Balasubramanian, P. Neumann, D. Twitchen, M. Markham, R. Kolesov, N. Mizuochi, J. Isoya, J. Achard, J. Beck, J. Tissler, V. Jacques, P. R. Hemmer, F. Jelezko, and J. Wrachtrup, “Ultralong spin coherence time in isotopically engineered diamond,” Nat. Mater. 8, 383–387 (2009).
[Crossref]

Acosta, V. M.

A. Faraon, C. Santori, Z. Huang, V. M. Acosta, and R. G. Beausoleil, “Coupling of nitrogen-vacancy centers to photonic crystal cavities in monocrystalline diamond,” Phys. Rev. Lett. 109, 033604 (2012).
[Crossref]

Aharonovich, I.

Y. Zhou, A. Rasmita, K. Li, Q. Xiong, I. Aharonovich, and W. B. Gao, “Coherent control of a strongly driven silicon vacancy optical transition in diamond,” Nat. Commun. 8, 14451 (2017).
[Crossref]

Alassaad, K.

M. Radulaski, Y.-K. Tzeng, J. L. Zhang, K. G. Lagoudakis, H. Ishiwata, C. Dory, K. A. Fischer, Y. A. Kelaita, S. Sun, P. C. Maurer, K. Alassaad, G. Ferro, Z.-X. Shen, N. Melosh, S. Chu, and J. Vučković, “Diamond color center integration with a silicon carbide photonics platform,” arXiv: 1610.03183 (2017).

Arend, C.

J. N. Becker, J. Gorlitz, C. Arend, M. Markham, and C. Becher, “Ultrafast all-optical coherent control of single silicon vacancy colour centres in diamond,” Nat. Commun. 7, 13512 (2016).
[Crossref]

C. Arend, J. N. Becker, H. Sternschulte, D. Steinmüller-Nethl, and C. Becher, “Photoluminescence excitation and spectral hole burning spectroscopy of silicon vacancy centers in diamond,” Phys. Rev. B 94, 045203 (2016).
[Crossref]

B. Pingault, J. N. Becker, C. H. Schulte, C. Arend, C. Hepp, T. Godde, A. I. Tartakovskii, M. Markham, C. Becher, and M. Atature, “All-optical formation of coherent dark states of silicon-vacancy spins in diamond,” Phys. Rev. Lett. 113, 263601 (2014).
[Crossref]

J. Riedrich-Moller, C. Arend, C. Pauly, F. Mucklich, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “Deterministic coupling of a single silicon-vacancy color center to a photonic crystal cavity in diamond,” Nano Lett. 14, 5281–5287 (2014).
[Crossref]

Atature, M.

B. Pingault, D. D. Jarausch, C. Hepp, L. Klintberg, J. N. Becker, M. Markham, C. Becher, and M. Atature, “Coherent control of the silicon-vacancy spin in diamond,” Nat. Commun. 8, 15579 (2017).
[Crossref]

B. Pingault, J. N. Becker, C. H. Schulte, C. Arend, C. Hepp, T. Godde, A. I. Tartakovskii, M. Markham, C. Becher, and M. Atature, “All-optical formation of coherent dark states of silicon-vacancy spins in diamond,” Phys. Rev. Lett. 113, 263601 (2014).
[Crossref]

Atikian, H. A.

A. Sipahigil, R. E. Evans, D. D. Sukachev, M. J. Burek, J. Borregaard, M. K. Bhaskar, C. T. Nguyen, J. L. Pacheco, H. A. Atikian, C. Meuwly, R. M. Camacho, F. Jelezko, E. Bielejec, H. Park, M. Lončar, and M. D. Lukin, “An integrated diamond nanophotonics platform for quantum optical networks,” Science 354, 847–850 (2016).
[Crossref]

Awschalom, D. D.

D. M. Toyli, C. D. Weis, G. D. Fuchs, T. Schenkel, and D. D. Awschalom, “Chip-scale nanofabrication of single spins and spin arrays in diamond,” Nano Lett. 10, 3168–3172 (2010).
[Crossref]

Babinec, T. M.

J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
[Crossref]

Balasubramanian, G.

G. Balasubramanian, P. Neumann, D. Twitchen, M. Markham, R. Kolesov, N. Mizuochi, J. Isoya, J. Achard, J. Beck, J. Tissler, V. Jacques, P. R. Hemmer, F. Jelezko, and J. Wrachtrup, “Ultralong spin coherence time in isotopically engineered diamond,” Nat. Mater. 8, 383–387 (2009).
[Crossref]

Baur, A.

J. Riedrich-Moller, L. Kipfstuhl, C. Hepp, E. Neu, C. Pauly, F. Mucklich, A. Baur, M. Wandt, S. Wolff, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “One- and two-dimensional photonic crystal microcavities in single crystal diamond,” Nat. Nanotechnol. 7, 69–74 (2012).
[Crossref]

Beausoleil, R. G.

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A. Sipahigil, R. E. Evans, D. D. Sukachev, M. J. Burek, J. Borregaard, M. K. Bhaskar, C. T. Nguyen, J. L. Pacheco, H. A. Atikian, C. Meuwly, R. M. Camacho, F. Jelezko, E. Bielejec, H. Park, M. Lončar, and M. D. Lukin, “An integrated diamond nanophotonics platform for quantum optical networks,” Science 354, 847–850 (2016).
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T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
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T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
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P. C. Maurer, G. Kucsko, C. Latta, L. Jiang, N. Y. Yao, S. D. Bennett, F. Pastawski, D. Hunger, N. Chisholm, M. Markham, D. J. Twitchen, J. I. Cirac, and M. D. Lukin, “Room-temperature quantum bit memory exceeding one second,” Science 336, 1283–1286 (2012).
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M. Radulaski, Y.-K. Tzeng, J. L. Zhang, K. G. Lagoudakis, H. Ishiwata, C. Dory, K. A. Fischer, Y. A. Kelaita, S. Sun, P. C. Maurer, K. Alassaad, G. Ferro, Z.-X. Shen, N. Melosh, S. Chu, and J. Vučković, “Diamond color center integration with a silicon carbide photonics platform,” arXiv: 1610.03183 (2017).

Chu, Y.

M. J. Burek, N. P. de Leon, B. J. Shields, B. J. Hausmann, Y. Chu, Q. Quan, A. S. Zibrov, H. Park, M. D. Lukin, and M. Loncar, “Free-standing mechanical and photonic nanostructures in single-crystal diamond,” Nano Lett. 12, 6084–6089 (2012).
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P. C. Maurer, G. Kucsko, C. Latta, L. Jiang, N. Y. Yao, S. D. Bennett, F. Pastawski, D. Hunger, N. Chisholm, M. Markham, D. J. Twitchen, J. I. Cirac, and M. D. Lukin, “Room-temperature quantum bit memory exceeding one second,” Science 336, 1283–1286 (2012).
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Dambach, M.

Dan, D.

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M. J. Burek, N. P. de Leon, B. J. Shields, B. J. Hausmann, Y. Chu, Q. Quan, A. S. Zibrov, H. Park, M. D. Lukin, and M. Loncar, “Free-standing mechanical and photonic nanostructures in single-crystal diamond,” Nano Lett. 12, 6084–6089 (2012).
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B. J. Hausmann, I. B. Bulu, P. B. Deotare, M. McCutcheon, V. Venkataraman, M. L. Markham, D. J. Twitchen, and M. Loncar, “Integrated high-quality factor optical resonators in diamond,” Nano Lett. 13, 1898–1902 (2013).
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Y.-C. Chen, P. S. Salter, S. Knauer, L. Weng, A. C. Frangeskou, C. J. Stephen, S. N. Ishmael, P. R. Dolan, S. Johnson, B. L. Green, G. W. Morley, M. E. Newton, J. G. Rarity, M. J. Booth, and J. M. Smith, “Laser writing of coherent colour centres in diamond,” Nat. Photonics 11, 77–80 (2017).
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J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
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J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
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T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
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T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
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A. Sipahigil, R. E. Evans, D. D. Sukachev, M. J. Burek, J. Borregaard, M. K. Bhaskar, C. T. Nguyen, J. L. Pacheco, H. A. Atikian, C. Meuwly, R. M. Camacho, F. Jelezko, E. Bielejec, H. Park, M. Lončar, and M. D. Lukin, “An integrated diamond nanophotonics platform for quantum optical networks,” Science 354, 847–850 (2016).
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R. E. Evans, A. Sipahigil, D. D. Sukachev, A. S. Zibrov, and M. D. Lukin, “Narrow-linewidth homogeneous optical emitters in diamond nanostructures via silicon ion implantation,” Phys. Rev. Appl. 5, 044010 (2016).
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A. Faraon, C. Santori, Z. Huang, V. M. Acosta, and R. G. Beausoleil, “Coupling of nitrogen-vacancy centers to photonic crystal cavities in monocrystalline diamond,” Phys. Rev. Lett. 109, 033604 (2012).
[Crossref]

Ferro, G.

J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
[Crossref]

M. Radulaski, Y.-K. Tzeng, J. L. Zhang, K. G. Lagoudakis, H. Ishiwata, C. Dory, K. A. Fischer, Y. A. Kelaita, S. Sun, P. C. Maurer, K. Alassaad, G. Ferro, Z.-X. Shen, N. Melosh, S. Chu, and J. Vučković, “Diamond color center integration with a silicon carbide photonics platform,” arXiv: 1610.03183 (2017).

Fischer, K. A.

K. G. Lagoudakis, P. L. McMahon, C. Dory, K. A. Fischer, K. Müller, V. Borish, D. Dalacu, P. J. Poole, M. E. Reimer, V. Zwiller, Y. Yamamoto, and J. Vučković, “Ultrafast coherent manipulation of trions in site-controlled nanowire quantum dots,” Optica 3, 1430–1435 (2016).
[Crossref]

K. G. Lagoudakis, P. L. McMahon, K. A. Fischer, S. Puri, K. Müller, D. Dan, P. J. Poole, M. E. Reimer, V. Zwiller, Y. Yamamoto, and J. Vučković, “Initialization of a spin qubit in a site-controlled nanowire quantum dot,” New J. Phys. 18, 053024 (2016).
[Crossref]

M. Radulaski, Y.-K. Tzeng, J. L. Zhang, K. G. Lagoudakis, H. Ishiwata, C. Dory, K. A. Fischer, Y. A. Kelaita, S. Sun, P. C. Maurer, K. Alassaad, G. Ferro, Z.-X. Shen, N. Melosh, S. Chu, and J. Vučković, “Diamond color center integration with a silicon carbide photonics platform,” arXiv: 1610.03183 (2017).

Fischer, M.

J. Riedrich-Moller, C. Arend, C. Pauly, F. Mucklich, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “Deterministic coupling of a single silicon-vacancy color center to a photonic crystal cavity in diamond,” Nano Lett. 14, 5281–5287 (2014).
[Crossref]

J. Riedrich-Moller, L. Kipfstuhl, C. Hepp, E. Neu, C. Pauly, F. Mucklich, A. Baur, M. Wandt, S. Wolff, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “One- and two-dimensional photonic crystal microcavities in single crystal diamond,” Nat. Nanotechnol. 7, 69–74 (2012).
[Crossref]

E. Neu, D. Steinmetz, J. Riedrich-Möller, S. Gsell, M. Fischer, M. Schreck, and C. Becher, “Single photon emission from silicon-vacancy colour centres in chemical vapour deposition nano-diamonds on iridium,” New J. Phys. 13, 025012 (2011).
[Crossref]

Fokin, A. A.

J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
[Crossref]

Frangeskou, A. C.

Y.-C. Chen, P. S. Salter, S. Knauer, L. Weng, A. C. Frangeskou, C. J. Stephen, S. N. Ishmael, P. R. Dolan, S. Johnson, B. L. Green, G. W. Morley, M. E. Newton, J. G. Rarity, M. J. Booth, and J. M. Smith, “Laser writing of coherent colour centres in diamond,” Nat. Photonics 11, 77–80 (2017).
[Crossref]

Frank, I. W.

M. J. Burek, D. Ramos, P. Patel, I. W. Frank, and M. Lončar, “Nanomechanical resonant structures in single-crystal diamond,” Appl. Phys. Lett. 103, 131904 (2013).
[Crossref]

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D. M. Toyli, C. D. Weis, G. D. Fuchs, T. Schenkel, and D. D. Awschalom, “Chip-scale nanofabrication of single spins and spin arrays in diamond,” Nano Lett. 10, 3168–3172 (2010).
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E. D. Kim, K. Truex, X. Xu, B. Sun, D. G. Steel, A. S. Bracker, D. Gammon, and L. J. Sham, “Fast spin rotations by optically controlled geometric phases in a charge-tunable InAs quantum dot,” Phys. Rev. Lett. 104, 167401 (2010).
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Y. Zhou, A. Rasmita, K. Li, Q. Xiong, I. Aharonovich, and W. B. Gao, “Coherent control of a strongly driven silicon vacancy optical transition in diamond,” Nat. Commun. 8, 14451 (2017).
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B. Pingault, J. N. Becker, C. H. Schulte, C. Arend, C. Hepp, T. Godde, A. I. Tartakovskii, M. Markham, C. Becher, and M. Atature, “All-optical formation of coherent dark states of silicon-vacancy spins in diamond,” Phys. Rev. Lett. 113, 263601 (2014).
[Crossref]

Gorlitz, J.

J. N. Becker, J. Gorlitz, C. Arend, M. Markham, and C. Becher, “Ultrafast all-optical coherent control of single silicon vacancy colour centres in diamond,” Nat. Commun. 7, 13512 (2016).
[Crossref]

Green, B. L.

Y.-C. Chen, P. S. Salter, S. Knauer, L. Weng, A. C. Frangeskou, C. J. Stephen, S. N. Ishmael, P. R. Dolan, S. Johnson, B. L. Green, G. W. Morley, M. E. Newton, J. G. Rarity, M. J. Booth, and J. M. Smith, “Laser writing of coherent colour centres in diamond,” Nat. Photonics 11, 77–80 (2017).
[Crossref]

Gregersen, N.

Gschrey, M.

Gsell, S.

J. Riedrich-Moller, C. Arend, C. Pauly, F. Mucklich, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “Deterministic coupling of a single silicon-vacancy color center to a photonic crystal cavity in diamond,” Nano Lett. 14, 5281–5287 (2014).
[Crossref]

J. Riedrich-Moller, L. Kipfstuhl, C. Hepp, E. Neu, C. Pauly, F. Mucklich, A. Baur, M. Wandt, S. Wolff, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “One- and two-dimensional photonic crystal microcavities in single crystal diamond,” Nat. Nanotechnol. 7, 69–74 (2012).
[Crossref]

E. Neu, D. Steinmetz, J. Riedrich-Möller, S. Gsell, M. Fischer, M. Schreck, and C. Becher, “Single photon emission from silicon-vacancy colour centres in chemical vapour deposition nano-diamonds on iridium,” New J. Phys. 13, 025012 (2011).
[Crossref]

Hanson, R.

D. de Lange, Z. H. Wang, D. Riste, V. V. Dobrovitski, and R. Hanson, “Universal dynamical decoupling of a single solid-state spin from a spin bath,” Science 330, 60–63 (2010).
[Crossref]

Hausmann, B. J.

B. J. Hausmann, I. B. Bulu, P. B. Deotare, M. McCutcheon, V. Venkataraman, M. L. Markham, D. J. Twitchen, and M. Loncar, “Integrated high-quality factor optical resonators in diamond,” Nano Lett. 13, 1898–1902 (2013).
[Crossref]

M. J. Burek, N. P. de Leon, B. J. Shields, B. J. Hausmann, Y. Chu, Q. Quan, A. S. Zibrov, H. Park, M. D. Lukin, and M. Loncar, “Free-standing mechanical and photonic nanostructures in single-crystal diamond,” Nano Lett. 12, 6084–6089 (2012).
[Crossref]

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G. Balasubramanian, P. Neumann, D. Twitchen, M. Markham, R. Kolesov, N. Mizuochi, J. Isoya, J. Achard, J. Beck, J. Tissler, V. Jacques, P. R. Hemmer, F. Jelezko, and J. Wrachtrup, “Ultralong spin coherence time in isotopically engineered diamond,” Nat. Mater. 8, 383–387 (2009).
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P. C. Maurer, G. Kucsko, C. Latta, L. Jiang, N. Y. Yao, S. D. Bennett, F. Pastawski, D. Hunger, N. Chisholm, M. Markham, D. J. Twitchen, J. I. Cirac, and M. D. Lukin, “Room-temperature quantum bit memory exceeding one second,” Science 336, 1283–1286 (2012).
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J. L. Zhang, H. Ishiwata, T. M. Babinec, M. Radulaski, K. Muller, K. G. Lagoudakis, C. Dory, J. Dahl, R. Edgington, V. Souliere, G. Ferro, A. A. Fokin, P. R. Schreiner, Z. X. Shen, N. A. Melosh, and J. Vuckovic, “Hybrid group IV nanophotonic structures incorporating diamond silicon-vacancy color centers,” Nano Lett. 16, 212–217 (2016).
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T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
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K. G. Lagoudakis, P. L. McMahon, K. A. Fischer, S. Puri, K. Müller, D. Dan, P. J. Poole, M. E. Reimer, V. Zwiller, Y. Yamamoto, and J. Vučković, “Initialization of a spin qubit in a site-controlled nanowire quantum dot,” New J. Phys. 18, 053024 (2016).
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K. G. Lagoudakis, P. L. McMahon, C. Dory, K. A. Fischer, K. Müller, V. Borish, D. Dalacu, P. J. Poole, M. E. Reimer, V. Zwiller, Y. Yamamoto, and J. Vučković, “Ultrafast coherent manipulation of trions in site-controlled nanowire quantum dots,” Optica 3, 1430–1435 (2016).
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M. J. Burek, D. Ramos, P. Patel, I. W. Frank, and M. Lončar, “Nanomechanical resonant structures in single-crystal diamond,” Appl. Phys. Lett. 103, 131904 (2013).
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M. J. Burek, N. P. de Leon, B. J. Shields, B. J. Hausmann, Y. Chu, Q. Quan, A. S. Zibrov, H. Park, M. D. Lukin, and M. Loncar, “Free-standing mechanical and photonic nanostructures in single-crystal diamond,” Nano Lett. 12, 6084–6089 (2012).
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Nat. Commun. (5)

T. Schröder, M. E. Trusheim, M. Walsh, L. Li, J. Zheng, M. Schukraft, R. M. Camacho, J. L. Pacheco, E. S. Bielejec, A. Sipahigil, R. E. Evans, D. D. Sukachev, C. T. Nguyen, M. D. Lukin, and D. Englund, “Scalable focused ion beam creation of nearly lifetime-limited single quantum emitters in diamond nanostructures,” Nat. Commun. 8, 15376 (2017).
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Nat. Mater. (1)

G. Balasubramanian, P. Neumann, D. Twitchen, M. Markham, R. Kolesov, N. Mizuochi, J. Isoya, J. Achard, J. Beck, J. Tissler, V. Jacques, P. R. Hemmer, F. Jelezko, and J. Wrachtrup, “Ultralong spin coherence time in isotopically engineered diamond,” Nat. Mater. 8, 383–387 (2009).
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J. Riedrich-Moller, L. Kipfstuhl, C. Hepp, E. Neu, C. Pauly, F. Mucklich, A. Baur, M. Wandt, S. Wolff, M. Fischer, S. Gsell, M. Schreck, and C. Becher, “One- and two-dimensional photonic crystal microcavities in single crystal diamond,” Nat. Nanotechnol. 7, 69–74 (2012).
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Nat. Photonics (1)

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K. D. Jahnke, A. Sipahigil, J. M. Binder, M. W. Doherty, M. Metsch, L. J. Rogers, N. B. Manson, M. D. Lukin, and F. Jelezko, “Electron-phonon processes of the silicon-vacancy centre in diamond,” New J. Phys. 17, 043011 (2015).
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E. Neu, D. Steinmetz, J. Riedrich-Möller, S. Gsell, M. Fischer, M. Schreck, and C. Becher, “Single photon emission from silicon-vacancy colour centres in chemical vapour deposition nano-diamonds on iridium,” New J. Phys. 13, 025012 (2011).
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R. E. Evans, A. Sipahigil, D. D. Sukachev, A. S. Zibrov, and M. D. Lukin, “Narrow-linewidth homogeneous optical emitters in diamond nanostructures via silicon ion implantation,” Phys. Rev. Appl. 5, 044010 (2016).
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Phys. Rev. B (1)

C. Arend, J. N. Becker, H. Sternschulte, D. Steinmüller-Nethl, and C. Becher, “Photoluminescence excitation and spectral hole burning spectroscopy of silicon vacancy centers in diamond,” Phys. Rev. B 94, 045203 (2016).
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Phys. Rev. Lett. (5)

E. D. Kim, K. Truex, X. Xu, B. Sun, D. G. Steel, A. S. Bracker, D. Gammon, and L. J. Sham, “Fast spin rotations by optically controlled geometric phases in a charge-tunable InAs quantum dot,” Phys. Rev. Lett. 104, 167401 (2010).
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B. Pingault, J. N. Becker, C. H. Schulte, C. Arend, C. Hepp, T. Godde, A. I. Tartakovskii, M. Markham, C. Becher, and M. Atature, “All-optical formation of coherent dark states of silicon-vacancy spins in diamond,” Phys. Rev. Lett. 113, 263601 (2014).
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A. Sipahigil, K. D. Jahnke, L. J. Rogers, T. Teraji, J. Isoya, A. S. Zibrov, F. Jelezko, and M. D. Lukin, “Indistinguishable photons from separated silicon-vacancy centers in diamond,” Phys. Rev. Lett. 113, 113602 (2014).
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Science (3)

D. de Lange, Z. H. Wang, D. Riste, V. V. Dobrovitski, and R. Hanson, “Universal dynamical decoupling of a single solid-state spin from a spin bath,” Science 330, 60–63 (2010).
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M. Radulaski, Y.-K. Tzeng, J. L. Zhang, K. G. Lagoudakis, H. Ishiwata, C. Dory, K. A. Fischer, Y. A. Kelaita, S. Sun, P. C. Maurer, K. Alassaad, G. Ferro, Z.-X. Shen, N. Melosh, S. Chu, and J. Vučković, “Diamond color center integration with a silicon carbide photonics platform,” arXiv: 1610.03183 (2017).

Supplementary Material (1)

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Figures (4)

Fig. 1.
Fig. 1. (a) Scanning electron microscopy (SEM) image of a nanopillar array. Scale bar, 10 μm. (b) SEM image of a 165 nm diameter, 200 nm tall nanopillar. Scale bar, 400 nm. (c) Photoluminescence spectrum from a single nanopillar (red) compared with that from a SiV ensemble in bulk diamond (black). (d) Scanning confocal microscopy map of a representative portion of a nanopillar array on a higher SiV center density sample. The bright areas with higher photon count rate correspond to the areas containing SiV centers, while the background is SiV center free. The count rates observed in the nanopillars are 5001000cps.
Fig. 2.
Fig. 2. (a) Excitation and detection scheme of the coherent control experiment. Transition |2|4 of the single SiV center (our qubit) is resonantly addressed with a pulsed Ti:Sapphire laser (blue shaded line), while the radiative emission from transition |3|1 is detected through a double monochromator by an SPCM (yellow shaded area). Inset shows the energy levels of the SiV center. The double-sided thick blue arrow denotes the coherent interaction of the SiV with the resonant pulses and the red wavy downward arrow denotes the detected photons coming from transition |3|1. (b) Demonstration of Rabi rotations. Varying the area of the resonant pulses rotates the qubit around the x-axis with a direct impact on the detected photon counts from transition |3|1, which shows clear oscillations in detected photon counts as a function of the pulse area. The fit function used is f(p)=a+b·sin(c·p+d)+e·p2, with {a,b,c,d,e}={161.05,58.239,186.71,1.4371,17804}. These terms were not independently measured.
Fig. 3.
Fig. 3. (a) Ramsey interference for coarse interpulse delays ranging from 66.7 to 667.2 ps. At each coarse delay, we record the Ramsey interference by varying the fine delay over 10 fs, and then fit it with a sinusoidal function as shown in the inset. Fitted amplitude of the Ramsey interference at each coarse delay is shown by the red envelope. (b) Decay of the Ramsey fringe contrast extracted from the data in (a) (red filled circles). The contrast decay is fitted with a single exponential decay function that yields a decay time T2* of 240 ps for the qubit.
Fig. 4.
Fig. 4. Experimental (a) and simulated (b) SU(2) control of the upper excited state population. Detected counts for dual pulse excitation with variable pulse area and delay. Here, the angle of rotation per pulse on the Bloch sphere is varied with the pulse area, while the axis around which the state is rotated is controlled with the delay between pulses. The data was taken for a coarse interpulse delay of 66.7 ps.

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