Abstract

The rapid generation of non-classical light serves as the foundation for exploring quantum optics and developing applications such as secure communications or the generation of NOON states. While strongly coupled quantum dot-photonic crystal resonator systems have great potential as non-classical light sources due to their promise of tailored output statistics, the generation of indistinguishable photons has been obscured due to the strongly dissipative nature of such systems. Here, we demonstrate that the recently discovered self-homodyne suppression technique can be used to overcome this limitation and tune the quantum statistics of transmitted light, achieving indistinguishable photon emission competitive with state-of-the-art metrics. Furthermore, our nanocavity-based platform directly lends itself to scalable on-chip architectures for quantum information.

© 2016 Optical Society of America

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    [Crossref]

2016 (6)

A. Thoma, P. Schnauber, M. Gschrey, M. Seifried, J. Wolters, J.-H. Schulze, A. Strittmatter, S. Rodt, A. Carmele, A. Knorr, T. Heindel, and S. Reitzenstein, “Exploring dephasing of a solid-state quantum emitter via time- and temperature-dependent Hong-Ou-Mandel experiments,” Phys. Rev. Lett. 116, 033601 (2016).
[Crossref]

N. Somaschi, V. Giesz, L. De Santis, J. C. Loredo, M. P. Almeida, G. Hornecker, S. L. Portalupi, T. Grange, C. Antón, J. Demory, C. Gómez, I. Sagnes, N. D. Lanzillotti-Kimura, A. Lematre, A. Auffeves, A. G. White, L. Lanco, and P. Senellart, “Near-optimal single-photon sources in the solid state,” Nat. Photonics 10, 340–345 (2016).
[Crossref]

X. Ding, Y. He, Z.-C. Duan, N. Gregersen, M.-C. Chen, S. Unsleber, S. Maier, C. Schneider, M. Kamp, S. Höfling, C.-Y. Lu, and J.-W. Pan, “On-demand single photons with high extraction efficiency and near-unity indistinguishability from a resonantly driven quantum dot in a micropillar,” Phys. Rev. Lett. 116, 020401 (2016).
[Crossref]

S. Unsleber, Y.-M. He, S. Gerhardt, S. Maier, C.-Y. Lu, J.-W. Pan, N. Gregersen, M. Kamp, C. Schneider, and S. Höfling, “Highly indistinguishable on-demand resonance fluorescence photons from a deterministic quantum dot micropillar device with 74% extraction efficiency,” Opt. Express 24, 8539–8546 (2016).
[Crossref]

V. Giesz, N. Somaschi, G. Hornecker, T. Grange, B. Reznychenko, L. De Santis, J. Demory, C. Gomez, I. Sagnes, A. Lemaitre, O. Krebs, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffeves, and P. Senellart, “Coherent manipulation of a solid-state artificial atom with few photons,” Nat. Commun. 7, 11986 (2016).
[Crossref]

K. A. Fischer, K. Müller, A. Rundquist, T. Sarmiento, A. Y. Piggott, Y. Kelaita, C. Dory, K. G. Lagoudakis, and J. Vučković, “Self-homodyne measurement of a dynamic mollow triplet in the solid state,” Nat. Photonics 10, 163–166 (2016).
[Crossref]

2015 (6)

K. Müller, A. Rundquist, K. A. Fischer, T. Sarmiento, K. G. Lagoudakis, Y. A. Kelaita, C. Sánchez Muñoz, E. del Valle, F. P. Laussy, and J. Vučković, “Coherent generation of nonclassical light on chip via detuned photon blockade,” Phys. Rev. Lett. 114, 233601 (2015).
[Crossref]

K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

G. Reithmaier, M. Kaniber, F. Flassig, S. Lichtmannecker, K. Müller, A. Andrejew, J. Vučković, R. Gross, and J. J. Finley, “On-chip generation, routing, and detection of resonance fluorescence,” Nano Lett. 15, 5208–5213 (2015).
[Crossref]

M. Gschrey, A. Thoma, P. Schnauber, M. Seifried, R. Schmidt, B. Wohlfeil, L. Kruger, J. H. Schulze, T. Heindel, S. Burger, F. Schmidt, A. Strittmatter, S. Rodt, and S. Reitzenstein, “Highly indistinguishable photons from deterministic quantum-dot microlenses utilizing three-dimensional in situ electron-beam lithography,” Nat. Commun. 6, 7662 (2015).
[Crossref]

A. V. Kuhlmann, J. H. Prechtel, J. Houel, A. Ludwig, D. Reuter, A. D. Wieck, and R. J. Warburton, “Transform-limited single photons from a single quantum dot,” Nat. Commun. 6, 8204 (2015).
[Crossref]

S. Unsleber, S. Maier, D. P. S. McCutcheon, Y.-M. He, M. Dambach, M. Gschrey, N. Gregersen, J. Mørk, S. Reitzenstein, S. Höfling, C. Schneider, and M. Kamp, “Observation of resonance fluorescence and the mollow triplet from a coherently driven site-controlled quantum dot,” Optica 2, 1072–1077 (2015).
[Crossref]

2014 (5)

J. Hansom, C. H. H. Schulte, C. Matthiesen, M. J. Stanley, and M. Atatüre, “Frequency stabilization of the zero-phonon line of a quantum dot via phonon-assisted active feedback,” Appl. Phys. Lett. 105, 172107 (2014).
[Crossref]

R. Trotta, J. S. Wildmann, E. Zallo, O. G. Schmidt, and A. Rastelli, “Highly entangled photons from hybrid piezoelectric-semiconductor quantum dot devices,” Nano Lett. 14, 3439–3444 (2014).
[Crossref]

M. Müller, S. Bounouar, K. D. Jöns, M. Glässl, and P. Michler, “On-demand generation of indistinguishable polarization-entangled photon pairs,” Nat. Photonics 8, 224–228 (2014).
[Crossref]

Y.-J. Wei, Y.-M. He, M.-C. Chen, Y.-N. Hu, Y. He, D. Wu, C. Schneider, M. Kamp, S. Höfling, C.-Y. Lu, and J.-W. Pan, “Deterministic and robust generation of single photons from a single quantum dot with 99.5% indistinguishability using adiabatic rapid passage,” Nano Lett. 14, 6515–6519 (2014).
[Crossref]

C. S. Muñoz, E. del Valle, A. G. Tudela, K. Müller, S. Lichtmannecker, M. Kaniber, C. Tejedor, J. J. Finley, and F. P. Laussy, “Emitters of N-photon bundles,” Nat. Photonics 8, 550–555 (2014).
[Crossref]

2013 (6)

G. Reithmaier, S. Lichtmannecker, T. Reichert, P. Hasch, K. Muller, M. Bichler, R. Gross, and J. J. Finley, “On-chip time resolved detection of quantum dot emission using integrated superconducting single photon detectors,” Sci. Rep. 3, 1901 (2013).
[Crossref]

O. Gazzano, S. Michaelis de Vasconcellos, C. Arnold, A. Nowak, E. Galopin, I. Sagnes, L. Lanco, A. Lemaître, and P. Senellart, “Bright solid-state sources of indistinguishable single photons,” Nat. Commun. 4, 1425 (2013).
[Crossref]

Y.-M. He, Y. He, Y.-J. Wei, D. Wu, M. Atature, C. Schneider, S. Hofling, M. Kamp, C.-Y. Lu, and J.-W. Pan, “On-demand semiconductor single-photon source with near-unity indistinguishability,” Nat. Nanotechnol. 8, 213–217 (2013).
[Crossref]

J. H. Prechtel, A. V. Kuhlmann, J. Houel, L. Greuter, A. Ludwig, D. Reuter, A. D. Wieck, and R. J. Warburton, “Frequency-stabilized source of single photons from a solid-state qubit,” Phys. Rev. X 3, 041006 (2013).

J. P. Vasco, H. Vinck-Posada, P. T. Valentim, and P. S. S. Guimãraes, “Modeling of fano resonances in the reflectivity of photonic crystal cavities with finite spot size excitation,” Opt. Express 21, 31336–31346 (2013).
[Crossref]

M. K. Yakes, L. Yang, A. S. Bracker, T. M. Sweeney, P. G. Brereton, M. Kim, C. S. Kim, P. M. Vora, D. Park, S. G. Carter, and D. Gammon, “Leveraging crystal anisotropy for deterministic growth of InAs quantum dots with narrow optical linewidths,” Nano Lett. 13, 4870–4875 (2013).
[Crossref]

2011 (1)

A. Reinhard, T. Volz, M. Winger, A. Badolato, K. J. Hennessy, E. L. Hu, and A. Imamoglu, “Strongly correlated photons on a chip,” Nat. Photonics 6, 93–96 (2011).
[Crossref]

2009 (2)

A. Nick Vamivakas, Y. Zhao, C.-Y. Lu, and M. Atature, “Spin-resolved quantum-dot resonance fluorescence,” Nat. Phys. 5, 198–202 (2009).
[Crossref]

E. B. Flagg, A. Muller, J. W. Robertson, S. Founta, D. G. Deppe, M. Xiao, W. Ma, G. J. Salamo, and C. K. Shih, “Resonantly driven coherent oscillations in a solid-state quantum emitter,” Nat. Phys. 5, 203–207 (2009).
[Crossref]

2008 (1)

A. Faraon, I. Fushman, D. Englund, N. Stoltz, P. Petroff, and J. Vuckovic, “Coherent generation of non-classical light on a chip via photon-induced tunnelling and blockade,” Nat. Phys. 4, 859–863 (2008).
[Crossref]

2007 (4)

D. Englund, A. Faraon, I. Fushman, N. Stoltz, P. Petroff, and J. Vuckovic, “Controlling cavity reflectivity with a single quantum dot,” Nature 450, 857–861 (2007).
[Crossref]

K. Hennessy, A. Badolato, M. Winger, D. Gerace, M. Atatüre, S. Gulde, S. Fält, E. L. Hu, and A. Imamoğlu, “Quantum nature of a strongly coupled single quantum dot-cavity system,” Nature 445, 896–899 (2007).
[Crossref]

N. Gisin and R. Thew, “Quantum communication,” Nat. Photonics 1, 165–171 (2007).
[Crossref]

J. L. O’Brien, “Optical quantum computing,” Science 318, 1567–1570 (2007).
[Crossref]

2006 (1)

N. Akopian, N. H. Lindner, E. Poem, Y. Berlatzky, J. Avron, D. Gershoni, B. D. Gerardot, and P. M. Petroff, “Entangled photon pairs from semiconductor quantum dots,” Phys. Rev. Lett. 96, 130501 (2006).
[Crossref]

2005 (1)

D. Englund, D. Fattal, E. Waks, G. Solomon, B. Zhang, T. Nakaoka, Y. Arakawa, Y. Yamamoto, and J. Vučković, “Controlling the spontaneous emission rate of single quantum dots in a two-dimensional photonic crystal,” Phys. Rev. Lett. 95, 013904 (2005).
[Crossref]

2004 (2)

T. Yoshie, A. Scherer, J. Hendrickson, G. Khitrova, H. M. Gibbs, G. Rupper, C. Ell, O. B. Shchekin, and D. G. Deppe, “Vacuum Rabi splitting with a single quantum dot in a photonic crystal nanocavity,” Nature 432, 200–203 (2004).
[Crossref]

V. Giovannetti, S. Lloyd, and L. Maccone, “Quantum-enhanced measurements: beating the standard quantum limit,” Science 306, 1330–1336 (2004).
[Crossref]

2002 (2)

C. Santori, D. Fattal, J. Vučković, G. S. Solomon, and Y. Yamamoto, “Indistinguishable photons from a single-photon device,” Nature 419, 594–597 (2002).
[Crossref]

N. Gisin, G. Ribordy, W. Tittel, and H. Zbinden, “Quantum cryptography,” Rev. Mod. Phys. 74, 145–195 (2002).
[Crossref]

2000 (2)

A. N. Boto, P. Kok, D. S. Abrams, S. L. Braunstein, C. P. Williams, and J. P. Dowling, “Quantum interferometric optical lithography: exploiting entanglement to beat the diffraction limit,” Phys. Rev. Lett. 85, 2733–2736 (2000).
[Crossref]

O. Benson, C. Santori, M. Pelton, and Y. Yamamoto, “Regulated and entangled photons from a single quantum dot,” Phys. Rev. Lett. 84, 2513–2516 (2000).
[Crossref]

1987 (1)

C. K. Hong, Z. Y. Ou, and L. Mandel, “Measurement of subpicosecond time intervals between two photons by interference,” Phys. Rev. Lett. 59, 2044–2046 (1987).
[Crossref]

Abrams, D. S.

A. N. Boto, P. Kok, D. S. Abrams, S. L. Braunstein, C. P. Williams, and J. P. Dowling, “Quantum interferometric optical lithography: exploiting entanglement to beat the diffraction limit,” Phys. Rev. Lett. 85, 2733–2736 (2000).
[Crossref]

Akopian, N.

N. Akopian, N. H. Lindner, E. Poem, Y. Berlatzky, J. Avron, D. Gershoni, B. D. Gerardot, and P. M. Petroff, “Entangled photon pairs from semiconductor quantum dots,” Phys. Rev. Lett. 96, 130501 (2006).
[Crossref]

Almeida, M. P.

N. Somaschi, V. Giesz, L. De Santis, J. C. Loredo, M. P. Almeida, G. Hornecker, S. L. Portalupi, T. Grange, C. Antón, J. Demory, C. Gómez, I. Sagnes, N. D. Lanzillotti-Kimura, A. Lematre, A. Auffeves, A. G. White, L. Lanco, and P. Senellart, “Near-optimal single-photon sources in the solid state,” Nat. Photonics 10, 340–345 (2016).
[Crossref]

Andrejew, A.

G. Reithmaier, M. Kaniber, F. Flassig, S. Lichtmannecker, K. Müller, A. Andrejew, J. Vučković, R. Gross, and J. J. Finley, “On-chip generation, routing, and detection of resonance fluorescence,” Nano Lett. 15, 5208–5213 (2015).
[Crossref]

Antón, C.

N. Somaschi, V. Giesz, L. De Santis, J. C. Loredo, M. P. Almeida, G. Hornecker, S. L. Portalupi, T. Grange, C. Antón, J. Demory, C. Gómez, I. Sagnes, N. D. Lanzillotti-Kimura, A. Lematre, A. Auffeves, A. G. White, L. Lanco, and P. Senellart, “Near-optimal single-photon sources in the solid state,” Nat. Photonics 10, 340–345 (2016).
[Crossref]

Arakawa, Y.

D. Englund, D. Fattal, E. Waks, G. Solomon, B. Zhang, T. Nakaoka, Y. Arakawa, Y. Yamamoto, and J. Vučković, “Controlling the spontaneous emission rate of single quantum dots in a two-dimensional photonic crystal,” Phys. Rev. Lett. 95, 013904 (2005).
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Supplementary Material (1)

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Figures (3)

Fig. 1.
Fig. 1.

Resonantly excited strongly coupled system. (a) Schematic illustration of the QD-photonic crystal cavity platform. (b) Schematic illustration of the Jaynes–Cummings (JC) ladder of dressed states that describes the energy level structure of a strongly coupled system. The arrows illustrate the resonant excitation of UP1 and subsequent relaxation. (c) Cross-polarized reflectivity spectrum of the coupled quantum dot-cavity system obtained by temperature tuning the QD through the cavity resonance. An anticrossing of the peaks clearly demonstrates the strong coupling. (d) Typical spectrum for resonantly exciting UP1 with a 16 ps long pulse at a QD-cavity detuning of Δ = 4.5 g and in the presence of self-homodyne suppression. The red shaded region indicates the spectral filter used in subsequent experiments.

Fig. 2.
Fig. 2.

Indistinguishability measurements. (a) Schematic illustration of the setup used to extract Hong–Ou–Mandel interference. (b) Measured correlation function of the emission using the same excitation conditions as in Fig. 1(d). Due to the quantum character of the light, the amplitude of the three center peaks surrounding zero time delay is reduced. (c) Amplitudes around zero delay obtained from binning the data presented in (b) with a temporal width of 384 ps about the center of each peak (represented as diamond data points). The error bars result from the N variation of the photocount distribution. Fits to the data are presented as blue columns and reveal g ( 2 ) [ 0 ] = 0.24 ± 0.03 and | g ( 1 ) [ 0 ] | 2 = 0.25 ± 0.03 . (d) Same as (c) but under spectral filtering of the emission from UP1, resulting in g ( 2 ) [ 0 ] = 0.05 ± 0.04 and | g ( 1 ) [ 0 ] | 2 = 0.96 ± 0.05 .

Fig. 3.
Fig. 3.

Quantum optical simulations. (a) Simulated spectrum for resonant excitation of UP1 by a 16 ps long π pulse at a QD-cavity detuning Δ = 4.5 g , with and without SHS. (b)  g ( 2 ) [ 0 ] (second-order coherence) for the excitation conditions of (a) (resonant excitation of UP1) as a function of the SHS tuning parameter with and without spectral filtering on UP1 (red region in (a). (c, d) g HOM ( 2 ) [ 0 ] as a function of the filtering wavelength excluding (c) and including (d) SHS. Only the central wavelength of the filter changes, but bandwidth remains the same. The shaded area below the curves visualizes 1 2 ( 1 | g ( 1 ) [ 0 ] | 2 ) , while the white area visualizes 1 2 g ( 2 ) [ 0 ] . Green lines denote the non-classical threshold. All wavelengths are referenced to that of the bare cavity.

Equations (2)

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g HOM ( 2 ) [ 0 ] = 1 2 g ( 2 ) [ 0 ] + 1 2 [ 1 | g ( 1 ) [ 0 ] | 2 ] ,
g MZ ( 2 ) [ 0 ] = 2 3 g ( 2 ) [ 0 ] + 1 3 [ 1 | g ( 1 ) [ 0 ] | 2 ] .

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