Abstract

Pattern formation often reveals constituent nonlinear mechanisms of a complex system. Here, we study self-synchronizing, light-induced thermal cycles in plasmonically absorbing nanofluids, whose anomalous thermal, optomechanical, electrochemical, and hydrodynamic responses are not yet well understood. We show that the oscillatory behavior—caused by light grazing the nanofluid meniscus—exhibits a strong dependence on hydrogen bonding in the solvent environment and that there are low-intensity optical thresholds in alcohol–water binary-solvent nanofluids. Moreover, these thermal cycles occur with a periodic, vertically discharging heat-dissipation mechanism, which could be facilitated by nanobubbles or thermophoresis. We show that an incoherent white-light source, such as sunlight, will also induce self-synchronizing thermal cycles; in this demonstration, we illustrate new methods of energy storage, transfer, and harvesting that will not alter the natural carbon cycle of life.

© 2015 Optical Society of America

Full Article  |  PDF Article
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References

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    [Crossref]
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    [Crossref]
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    [Crossref]
  36. M. Chaplin, “Theory vs experiment: what is the surface charge of water?” Water 1, 1–28 (2009).
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  38. M. Sedlak, D. Rak, “On the origin of mesoscale structures in aqueous solutions of tertiary butyl alcohol: the mystery resolved,” J. Phys. Chem. B 118, 2726–2737 (2014).
    [Crossref]
  39. E. Ruckenstein, I. Shulgin, “Hydrophobic self-assembling in dilute aqueous solutions of alcohols and hydrocarbons,” Chem. Eng. Sci. 56, 5675–5680 (2001).
    [Crossref]
  40. H. Hayashi, K. Nishikawa, T. Iijima, “Small-angle x-ray scattering study of fluctuations in 1-propanol–water and 2-propanol–water systems,” J. Phys. Chem. 94, 8334–8338 (1990).
    [Crossref]
  41. B. L. Smorodin, I. N. Cherepanov, B. I. Myznikova, M. I. Shliomis, “Traveling-wave convection in colloids stratified by gravity,” Phys. Rev. E 84, 026305 (2011).
    [Crossref]
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    [Crossref]
  43. A. Bricard, J.-B. Caussin, N. Desreumaux, O. Dauchot, D. Bartolo, “Emergence of macroscopic directed motion in populations of motile colloids,” Nature 503, 95–98 (2013).
    [Crossref]
  44. H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
    [Crossref]
  45. E. Palleau, D. Morales, M. D. Dickey, O. D. Velev, “Reversible patterning and actuation of hydrogels by electrically assisted ionoprinting,” Nat. Commun. 4, 2257 (2013).
    [Crossref]
  46. R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
    [Crossref]
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    [Crossref]
  48. J. W. Post, J. Veerman, H. V. M. Hamelers, G. J. W. Euverink, S. J. Metz, K. Nymeijer, C. J. N. Buisman, “Salinity-gradient power: evaluation of pressure-retarded osmosis and reverse electrodialysis,” J. Membr. Sci. 288, 218–230 (2007).
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    [Crossref]
  50. L. F. Range, J. C. Santamarina, D. O. Fratta, “Dynamic electrical–mechanical energy coupling in electrolyte–mineral systems,” Transp. Porous Media 50, 153–178 (2003).
    [Crossref]

2014 (3)

M. Moocarme, L. T. Vuong, “Ultralow-intensity magneto-optical and mechanical effects in metal nanocolloids,” Nano Lett. 14, 1178–1183 (2014).

S. Baral, A. Green, M. Y. Livshits, A. O. Govarov, H. H. Richardson, “Comparison of vapor formation of water at the solid/water interface to colloidal solutions using optically excited gold nanostructures,” ACS Nano 8, 1439–1448 (2014).
[Crossref]

M. Sedlak, D. Rak, “On the origin of mesoscale structures in aqueous solutions of tertiary butyl alcohol: the mystery resolved,” J. Phys. Chem. B 118, 2726–2737 (2014).
[Crossref]

2013 (10)

M. Sedlák, D. Rak, “Large-scale inhomogeneities in solutions of low molar mass compounds and mixtures of liquids: supramolecular structures or nanobubbles?” J. Phys. Chem. B 117, 2495–2504 (2013).
[Crossref]

E. Greenfield, J. Nemirovsky, R. El-Ganainy, N. Demetri, M. Segev, “Shockwave based nonlinear optical manipulation in densely scattering opaque suspensions,” Opt. Express 21, 2382–2384 (2013).
[Crossref]

R. Taylor, S. Coulombe, T. Otanicar, P. Phelan, A. Gunawan, W. Lv, G. Rosengarten, R. Prasher, H. Tyagi, “Small particles, big impacts: a review of the diverse applications of nanofluids,” J. Appl. Phys. 113, 011301 (2013).
[Crossref]

S. Mubeen, J. Lee, N. Singh, S. Krämer, G. D. Stucky, M. Moskovits, “An autonomous photosynthetic device in which all charge carriers derive from surface plasmons,” Nat. Nanotechnol. 8, 247–251 (2013).
[Crossref]

Z. Fang, Y.-R. Zhen, O. Neumann, A. Polman, F. J. García de Abajo, P. Nordlander, N. J. Halas, “Evolution of light-induced vapor generation at a liquid-immersed metallic nanoparticle,” Nano Lett. 13, 1736–1742 (2013).
[Crossref]

A. Bricard, J.-B. Caussin, N. Desreumaux, O. Dauchot, D. Bartolo, “Emergence of macroscopic directed motion in populations of motile colloids,” Nature 503, 95–98 (2013).
[Crossref]

H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
[Crossref]

E. Palleau, D. Morales, M. D. Dickey, O. D. Velev, “Reversible patterning and actuation of hydrogels by electrically assisted ionoprinting,” Nat. Commun. 4, 2257 (2013).
[Crossref]

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

G. Gouesbet, J. A. Lock, “List of problems for future research in generalized Lorenz–Mie theories and related topics, review and prospectus,” Appl. Opt. 52, 897–916 (2013).
[Crossref]

2012 (5)

N. Y. Yip, M. Elimelech, “Thermodynamic and energy efficiency analysis of power generation from natural salinity gradients by pressure retarded osmosis,” Environ. Sci. Technol. 46, 5230–5239 (2012).
[Crossref]

I. Gur, K. Sawyer, R. Prasher, “Searching for a better thermal battery,” Science 335, 1454–1455 (2012).
[Crossref]

N. D. Singh, M. Moocarme, B. Edelstein, N. Punnoose, L. T. Vuong, “Anomalously-large photo-induced magnetic response of metallic nanocolloids in aqueous solution using a solar simulator,” Opt. Express 20, 3054–3065 (2012).
[Crossref]

A. Pinke, P. Jedlovsky, “Modeling of mixing acetone and water: how can their full miscibility be reproduced in computer simulations?” J. Phys. Chem. B 116, 5977–5984 (2012).
[Crossref]

A. Mialdun, V. Yasnou, V. Shevtsova, A. Königer, W. Köhler, D. Alonso de Mezquia, M. M. Bou-Ali, “A comprehensive study of diffusion, thermodiffusion, and Soret coefficients of water–isopropanol mixtures,” J. Chem. Phys. 136, 244512 (2012).
[Crossref]

2011 (5)

Y. E. Geints, N. S. Panamarev, A. Zemlyanov, “Transient behavior of far-field diffraction patterns of a Gaussian laser beam due to the thermo-optical effect in metal nanocolloids,” J. Opt. 13, 055707 (2011).
[Crossref]

J. Fan, L. Wang, “Heat conduction in nanofluids: structure–property correlation,” Int. J. Heat Mass Transfer 54, 4349–4359 (2011).
[Crossref]

E. Greenfield, C. Rotschild, A. Szameit, J. Nemirovsky, R. El-Ganainy, D. N. Christodoulides, M. Saraf, E. Lifshitz, M. Segev, “Light-induced self-synchronizing flow patterns,” New J. Phys. 13, 053021 (2011).
[Crossref]

L. Wang, J. Fan, “Toward nanofluids of ultra-high thermal conductivity,” Nanoscale Res. Lett. 6, 153 (2011).
[Crossref]

B. L. Smorodin, I. N. Cherepanov, B. I. Myznikova, M. I. Shliomis, “Traveling-wave convection in colloids stratified by gravity,” Phys. Rev. E 84, 026305 (2011).
[Crossref]

2010 (5)

N. Shalkevich, W. Escher, T. Bürgi, B. Michel, L. Si-Ahmed, D. Poulikakos, “On the thermal conductivity of gold nanoparticle colloids,” Langmuir 26, 663–670 (2010).
[Crossref]

Y. Lamhot, A. Barak, O. Peleg, M. Segev, “Self-trapping of optical beams through thermophoresis,” Phys. Rev. Lett. 105, 163906 (2010).
[Crossref]

J. Gliński, A. Burakowski, “Compressibility of aqueous solutions of nonelectrolytes: an equilibrium model,” J. Chem. Phys. 132, 124507 (2010).
[Crossref]

A. Würger, “Thermal non-equilibrium transport in colloids,” Rep. Prog. Phys. 73, 126601 (2010).
[Crossref]

A. Häbich, W. Ducker, D. E. Dunstan, X. Zhang, “Do stable nanobubbles exist in mixtures of organic solvents and water?” J. Phys. Chem. B 114, 6962–6967 (2010).
[Crossref]

2009 (2)

M. Chaplin, “Theory vs experiment: what is the surface charge of water?” Water 1, 1–28 (2009).
[Crossref]

D. Brogioli, “Extracting renewable energy from a salinity difference using a capacitor,” Phys. Rev. Lett. 103, 058501 (2009).
[Crossref]

2008 (1)

M. Dienerowitz, M. Mazilu, K. Dholakia, “Optical manipulation of nanoparticles: a review,” J. Nanophoton. 2, 021875 (2008).
[Crossref]

2007 (3)

F. Jin, J. Ye, L. Hong, H. Lam, C. Wu, “Slow relaxation mode in mixtures of water and organic molecules: supramolecular structures or nanobubbles?” J. Phys. Chem. B 111, 2255–2261 (2007).
[Crossref]

I. M. Vellekoop, A. P. Mosk, “Focusing coherent light through opaque strongly scattering media,” Opt. Lett. 32, 2309–2311 (2007).
[Crossref]

J. W. Post, J. Veerman, H. V. M. Hamelers, G. J. W. Euverink, S. J. Metz, K. Nymeijer, C. J. N. Buisman, “Salinity-gradient power: evaluation of pressure-retarded osmosis and reverse electrodialysis,” J. Membr. Sci. 288, 218–230 (2007).
[Crossref]

2005 (1)

R. Prasher, P. Bhattacharya, P. Phelan, “Thermal conductivity of nanoscale colloidal solutions (nanofluids),” Phys. Rev. Lett. 94, 025901 (2005).
[Crossref]

2003 (1)

L. F. Range, J. C. Santamarina, D. O. Fratta, “Dynamic electrical–mechanical energy coupling in electrolyte–mineral systems,” Transp. Porous Media 50, 153–178 (2003).
[Crossref]

2002 (1)

S. Dixit, J. Crain, W. C. K. Poon, J. L. Finney, A. K. Soper, “Molecular segregation observed in a concentrated alcohol–water solution,” Nature 416, 829–832 (2002).
[Crossref]

2001 (2)

G. Gouesbet, C. Roze, “Instabilities by local heating below an interface,” J. Non-Equilib. Thermodyn. 25, 337–379 (2001).
[Crossref]

E. Ruckenstein, I. Shulgin, “Hydrophobic self-assembling in dilute aqueous solutions of alcohols and hydrocarbons,” Chem. Eng. Sci. 56, 5675–5680 (2001).
[Crossref]

2000 (2)

S. Dixit, W. C. K. Poon, J. Crain, “Hydration of methanol in aqueous solutions: a Raman spectroscopic study,” J. Phys. Condens. Matter 12, L323–L328 (2000).
[Crossref]

B. Ambravaneswaran, S. D. Phillips, O. Basaran, “Theoretical analysis of a dripping faucet,” Phys. Rev. Lett. 85, 5332–5335 (2000).
[Crossref]

1998 (3)

F. B. Hicks, C. Franck, “Low-power laser driving of a binary liquid,” Phys. Rev. E 58, 4582–4586 (1998).
[Crossref]

U. Buhvestov, F. Rived, C. Ra, E. Bosch, A. Rose, “Solute–solvent and solvent–solvent interactions in binary solvent mixtures. Part 7. Comparison of the enhancement of the water structure in alcohol–water mixtures measured by solvatochromic indicators,” J. Phys. Org. Chem. 11, 185–192 (1998).
[Crossref]

A. Bergeon, D. Henry, H. Benhadid, L. S. Tuckerman, “Marangoni convection in binary mixtures with Soret effect,” J. Fluid Mech. 375, 143–177 (1998).
[Crossref]

1997 (1)

Y. Takeuchi, T. Ida, K. Kimura, “Colloidal stability of gold nanoparticles in 2-propanol under laser irradiation,” J. Phys. Chem. B 101, 1322–1327 (1997).
[Crossref]

1994 (1)

1990 (1)

H. Hayashi, K. Nishikawa, T. Iijima, “Small-angle x-ray scattering study of fluctuations in 1-propanol–water and 2-propanol–water systems,” J. Phys. Chem. 94, 8334–8338 (1990).
[Crossref]

1989 (1)

V. Y. Bazhenov, M. V. Vasnetsov, M. S. Soskin, V. B. Tarenenko, “Self-oscillations of a liquid near a free interface during continuous local heating,” JETP Lett. 49, 376–379 (1989).

1980 (1)

G. Roux, D. Roberts, G. Perron, J. Desnoyers, “Microheterogeneity in aqueous-organic solutions: heat capacities, volumes and expansibilities of some alcohols, aminoalcohol and tertiary amines in water,” J. Solution Chem. 9, 629–647 (1980).
[Crossref]

1966 (1)

F. Franks, D. J. G. Ives, “The structural properties of alcohol–water mixtures,” Q. Rev. Chem. Soc. 20, 1–44 (1966).
[Crossref]

Alonso de Mezquia, D.

A. Mialdun, V. Yasnou, V. Shevtsova, A. Königer, W. Köhler, D. Alonso de Mezquia, M. M. Bou-Ali, “A comprehensive study of diffusion, thermodiffusion, and Soret coefficients of water–isopropanol mixtures,” J. Chem. Phys. 136, 244512 (2012).
[Crossref]

Ambravaneswaran, B.

B. Ambravaneswaran, S. D. Phillips, O. Basaran, “Theoretical analysis of a dripping faucet,” Phys. Rev. Lett. 85, 5332–5335 (2000).
[Crossref]

Amini, H.

H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
[Crossref]

Barak, A.

Y. Lamhot, A. Barak, O. Peleg, M. Segev, “Self-trapping of optical beams through thermophoresis,” Phys. Rev. Lett. 105, 163906 (2010).
[Crossref]

Baral, S.

S. Baral, A. Green, M. Y. Livshits, A. O. Govarov, H. H. Richardson, “Comparison of vapor formation of water at the solid/water interface to colloidal solutions using optically excited gold nanostructures,” ACS Nano 8, 1439–1448 (2014).
[Crossref]

Bartolo, D.

A. Bricard, J.-B. Caussin, N. Desreumaux, O. Dauchot, D. Bartolo, “Emergence of macroscopic directed motion in populations of motile colloids,” Nature 503, 95–98 (2013).
[Crossref]

Basaran, O.

B. Ambravaneswaran, S. D. Phillips, O. Basaran, “Theoretical analysis of a dripping faucet,” Phys. Rev. Lett. 85, 5332–5335 (2000).
[Crossref]

Bazhenov, V. Y.

V. Y. Bazhenov, M. V. Vasnetsov, M. S. Soskin, V. B. Tarenenko, “Self-oscillations of a liquid near a free interface during continuous local heating,” JETP Lett. 49, 376–379 (1989).

Benhadid, H.

A. Bergeon, D. Henry, H. Benhadid, L. S. Tuckerman, “Marangoni convection in binary mixtures with Soret effect,” J. Fluid Mech. 375, 143–177 (1998).
[Crossref]

Bergeon, A.

A. Bergeon, D. Henry, H. Benhadid, L. S. Tuckerman, “Marangoni convection in binary mixtures with Soret effect,” J. Fluid Mech. 375, 143–177 (1998).
[Crossref]

Bhattacharya, P.

R. Prasher, P. Bhattacharya, P. Phelan, “Thermal conductivity of nanoscale colloidal solutions (nanofluids),” Phys. Rev. Lett. 94, 025901 (2005).
[Crossref]

Block, S. M.

Bosch, E.

U. Buhvestov, F. Rived, C. Ra, E. Bosch, A. Rose, “Solute–solvent and solvent–solvent interactions in binary solvent mixtures. Part 7. Comparison of the enhancement of the water structure in alcohol–water mixtures measured by solvatochromic indicators,” J. Phys. Org. Chem. 11, 185–192 (1998).
[Crossref]

Bou-Ali, M. M.

A. Mialdun, V. Yasnou, V. Shevtsova, A. Königer, W. Köhler, D. Alonso de Mezquia, M. M. Bou-Ali, “A comprehensive study of diffusion, thermodiffusion, and Soret coefficients of water–isopropanol mixtures,” J. Chem. Phys. 136, 244512 (2012).
[Crossref]

Bricard, A.

A. Bricard, J.-B. Caussin, N. Desreumaux, O. Dauchot, D. Bartolo, “Emergence of macroscopic directed motion in populations of motile colloids,” Nature 503, 95–98 (2013).
[Crossref]

Brogioli, D.

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

D. Brogioli, “Extracting renewable energy from a salinity difference using a capacitor,” Phys. Rev. Lett. 103, 058501 (2009).
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U. Buhvestov, F. Rived, C. Ra, E. Bosch, A. Rose, “Solute–solvent and solvent–solvent interactions in binary solvent mixtures. Part 7. Comparison of the enhancement of the water structure in alcohol–water mixtures measured by solvatochromic indicators,” J. Phys. Org. Chem. 11, 185–192 (1998).
[Crossref]

Rak, D.

M. Sedlak, D. Rak, “On the origin of mesoscale structures in aqueous solutions of tertiary butyl alcohol: the mystery resolved,” J. Phys. Chem. B 118, 2726–2737 (2014).
[Crossref]

M. Sedlák, D. Rak, “Large-scale inhomogeneities in solutions of low molar mass compounds and mixtures of liquids: supramolecular structures or nanobubbles?” J. Phys. Chem. B 117, 2495–2504 (2013).
[Crossref]

Range, L. F.

L. F. Range, J. C. Santamarina, D. O. Fratta, “Dynamic electrical–mechanical energy coupling in electrolyte–mineral systems,” Transp. Porous Media 50, 153–178 (2003).
[Crossref]

Rica, R.

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

Richardson, H. H.

S. Baral, A. Green, M. Y. Livshits, A. O. Govarov, H. H. Richardson, “Comparison of vapor formation of water at the solid/water interface to colloidal solutions using optically excited gold nanostructures,” ACS Nano 8, 1439–1448 (2014).
[Crossref]

Rived, F.

U. Buhvestov, F. Rived, C. Ra, E. Bosch, A. Rose, “Solute–solvent and solvent–solvent interactions in binary solvent mixtures. Part 7. Comparison of the enhancement of the water structure in alcohol–water mixtures measured by solvatochromic indicators,” J. Phys. Org. Chem. 11, 185–192 (1998).
[Crossref]

Roberts, D.

G. Roux, D. Roberts, G. Perron, J. Desnoyers, “Microheterogeneity in aqueous-organic solutions: heat capacities, volumes and expansibilities of some alcohols, aminoalcohol and tertiary amines in water,” J. Solution Chem. 9, 629–647 (1980).
[Crossref]

Rose, A.

U. Buhvestov, F. Rived, C. Ra, E. Bosch, A. Rose, “Solute–solvent and solvent–solvent interactions in binary solvent mixtures. Part 7. Comparison of the enhancement of the water structure in alcohol–water mixtures measured by solvatochromic indicators,” J. Phys. Org. Chem. 11, 185–192 (1998).
[Crossref]

Rosengarten, G.

R. Taylor, S. Coulombe, T. Otanicar, P. Phelan, A. Gunawan, W. Lv, G. Rosengarten, R. Prasher, H. Tyagi, “Small particles, big impacts: a review of the diverse applications of nanofluids,” J. Appl. Phys. 113, 011301 (2013).
[Crossref]

Rotschild, C.

E. Greenfield, C. Rotschild, A. Szameit, J. Nemirovsky, R. El-Ganainy, D. N. Christodoulides, M. Saraf, E. Lifshitz, M. Segev, “Light-induced self-synchronizing flow patterns,” New J. Phys. 13, 053021 (2011).
[Crossref]

Roux, G.

G. Roux, D. Roberts, G. Perron, J. Desnoyers, “Microheterogeneity in aqueous-organic solutions: heat capacities, volumes and expansibilities of some alcohols, aminoalcohol and tertiary amines in water,” J. Solution Chem. 9, 629–647 (1980).
[Crossref]

Roze, C.

G. Gouesbet, C. Roze, “Instabilities by local heating below an interface,” J. Non-Equilib. Thermodyn. 25, 337–379 (2001).
[Crossref]

Ruckenstein, E.

E. Ruckenstein, I. Shulgin, “Hydrophobic self-assembling in dilute aqueous solutions of alcohols and hydrocarbons,” Chem. Eng. Sci. 56, 5675–5680 (2001).
[Crossref]

Salerno, D.

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

Santamarina, J. C.

L. F. Range, J. C. Santamarina, D. O. Fratta, “Dynamic electrical–mechanical energy coupling in electrolyte–mineral systems,” Transp. Porous Media 50, 153–178 (2003).
[Crossref]

Saraf, M.

E. Greenfield, C. Rotschild, A. Szameit, J. Nemirovsky, R. El-Ganainy, D. N. Christodoulides, M. Saraf, E. Lifshitz, M. Segev, “Light-induced self-synchronizing flow patterns,” New J. Phys. 13, 053021 (2011).
[Crossref]

Sawyer, K.

I. Gur, K. Sawyer, R. Prasher, “Searching for a better thermal battery,” Science 335, 1454–1455 (2012).
[Crossref]

Sedlak, M.

M. Sedlak, D. Rak, “On the origin of mesoscale structures in aqueous solutions of tertiary butyl alcohol: the mystery resolved,” J. Phys. Chem. B 118, 2726–2737 (2014).
[Crossref]

Sedlák, M.

M. Sedlák, D. Rak, “Large-scale inhomogeneities in solutions of low molar mass compounds and mixtures of liquids: supramolecular structures or nanobubbles?” J. Phys. Chem. B 117, 2495–2504 (2013).
[Crossref]

Segev, M.

E. Greenfield, J. Nemirovsky, R. El-Ganainy, N. Demetri, M. Segev, “Shockwave based nonlinear optical manipulation in densely scattering opaque suspensions,” Opt. Express 21, 2382–2384 (2013).
[Crossref]

E. Greenfield, C. Rotschild, A. Szameit, J. Nemirovsky, R. El-Ganainy, D. N. Christodoulides, M. Saraf, E. Lifshitz, M. Segev, “Light-induced self-synchronizing flow patterns,” New J. Phys. 13, 053021 (2011).
[Crossref]

Y. Lamhot, A. Barak, O. Peleg, M. Segev, “Self-trapping of optical beams through thermophoresis,” Phys. Rev. Lett. 105, 163906 (2010).
[Crossref]

Shalkevich, N.

N. Shalkevich, W. Escher, T. Bürgi, B. Michel, L. Si-Ahmed, D. Poulikakos, “On the thermal conductivity of gold nanoparticle colloids,” Langmuir 26, 663–670 (2010).
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A. Mialdun, V. Yasnou, V. Shevtsova, A. Königer, W. Köhler, D. Alonso de Mezquia, M. M. Bou-Ali, “A comprehensive study of diffusion, thermodiffusion, and Soret coefficients of water–isopropanol mixtures,” J. Chem. Phys. 136, 244512 (2012).
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B. L. Smorodin, I. N. Cherepanov, B. I. Myznikova, M. I. Shliomis, “Traveling-wave convection in colloids stratified by gravity,” Phys. Rev. E 84, 026305 (2011).
[Crossref]

Shulgin, I.

E. Ruckenstein, I. Shulgin, “Hydrophobic self-assembling in dilute aqueous solutions of alcohols and hydrocarbons,” Chem. Eng. Sci. 56, 5675–5680 (2001).
[Crossref]

Si-Ahmed, L.

N. Shalkevich, W. Escher, T. Bürgi, B. Michel, L. Si-Ahmed, D. Poulikakos, “On the thermal conductivity of gold nanoparticle colloids,” Langmuir 26, 663–670 (2010).
[Crossref]

Singh, N.

S. Mubeen, J. Lee, N. Singh, S. Krämer, G. D. Stucky, M. Moskovits, “An autonomous photosynthetic device in which all charge carriers derive from surface plasmons,” Nat. Nanotechnol. 8, 247–251 (2013).
[Crossref]

Singh, N. D.

N. D. Singh, M. Moocarme, B. Edelstein, N. Punnoose, L. T. Vuong, “Anomalously-large photo-induced magnetic response of metallic nanocolloids in aqueous solution using a solar simulator,” Opt. Express 20, 3054–3065 (2012).
[Crossref]

Smorodin, B. L.

B. L. Smorodin, I. N. Cherepanov, B. I. Myznikova, M. I. Shliomis, “Traveling-wave convection in colloids stratified by gravity,” Phys. Rev. E 84, 026305 (2011).
[Crossref]

Sollier, E.

H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
[Crossref]

Soper, A. K.

S. Dixit, J. Crain, W. C. K. Poon, J. L. Finney, A. K. Soper, “Molecular segregation observed in a concentrated alcohol–water solution,” Nature 416, 829–832 (2002).
[Crossref]

Soskin, M. S.

V. Y. Bazhenov, M. V. Vasnetsov, M. S. Soskin, V. B. Tarenenko, “Self-oscillations of a liquid near a free interface during continuous local heating,” JETP Lett. 49, 376–379 (1989).

Stone, H. A.

H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
[Crossref]

Stucky, G. D.

S. Mubeen, J. Lee, N. Singh, S. Krämer, G. D. Stucky, M. Moskovits, “An autonomous photosynthetic device in which all charge carriers derive from surface plasmons,” Nat. Nanotechnol. 8, 247–251 (2013).
[Crossref]

Svoboda, K.

Szameit, A.

E. Greenfield, C. Rotschild, A. Szameit, J. Nemirovsky, R. El-Ganainy, D. N. Christodoulides, M. Saraf, E. Lifshitz, M. Segev, “Light-induced self-synchronizing flow patterns,” New J. Phys. 13, 053021 (2011).
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Y. Takeuchi, T. Ida, K. Kimura, “Colloidal stability of gold nanoparticles in 2-propanol under laser irradiation,” J. Phys. Chem. B 101, 1322–1327 (1997).
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V. Y. Bazhenov, M. V. Vasnetsov, M. S. Soskin, V. B. Tarenenko, “Self-oscillations of a liquid near a free interface during continuous local heating,” JETP Lett. 49, 376–379 (1989).

Taylor, R.

R. Taylor, S. Coulombe, T. Otanicar, P. Phelan, A. Gunawan, W. Lv, G. Rosengarten, R. Prasher, H. Tyagi, “Small particles, big impacts: a review of the diverse applications of nanofluids,” J. Appl. Phys. 113, 011301 (2013).
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A. Bergeon, D. Henry, H. Benhadid, L. S. Tuckerman, “Marangoni convection in binary mixtures with Soret effect,” J. Fluid Mech. 375, 143–177 (1998).
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R. Taylor, S. Coulombe, T. Otanicar, P. Phelan, A. Gunawan, W. Lv, G. Rosengarten, R. Prasher, H. Tyagi, “Small particles, big impacts: a review of the diverse applications of nanofluids,” J. Appl. Phys. 113, 011301 (2013).
[Crossref]

van Roij, R.

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

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V. Y. Bazhenov, M. V. Vasnetsov, M. S. Soskin, V. B. Tarenenko, “Self-oscillations of a liquid near a free interface during continuous local heating,” JETP Lett. 49, 376–379 (1989).

Veerman, J.

J. W. Post, J. Veerman, H. V. M. Hamelers, G. J. W. Euverink, S. J. Metz, K. Nymeijer, C. J. N. Buisman, “Salinity-gradient power: evaluation of pressure-retarded osmosis and reverse electrodialysis,” J. Membr. Sci. 288, 218–230 (2007).
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E. Palleau, D. Morales, M. D. Dickey, O. D. Velev, “Reversible patterning and actuation of hydrogels by electrically assisted ionoprinting,” Nat. Commun. 4, 2257 (2013).
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Vuong, L. T.

M. Moocarme, L. T. Vuong, “Ultralow-intensity magneto-optical and mechanical effects in metal nanocolloids,” Nano Lett. 14, 1178–1183 (2014).

N. D. Singh, M. Moocarme, B. Edelstein, N. Punnoose, L. T. Vuong, “Anomalously-large photo-induced magnetic response of metallic nanocolloids in aqueous solution using a solar simulator,” Opt. Express 20, 3054–3065 (2012).
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J. Fan, L. Wang, “Heat conduction in nanofluids: structure–property correlation,” Int. J. Heat Mass Transfer 54, 4349–4359 (2011).
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L. Wang, J. Fan, “Toward nanofluids of ultra-high thermal conductivity,” Nanoscale Res. Lett. 6, 153 (2011).
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F. Jin, J. Ye, L. Hong, H. Lam, C. Wu, “Slow relaxation mode in mixtures of water and organic molecules: supramolecular structures or nanobubbles?” J. Phys. Chem. B 111, 2255–2261 (2007).
[Crossref]

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A. Würger, “Thermal non-equilibrium transport in colloids,” Rep. Prog. Phys. 73, 126601 (2010).
[Crossref]

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H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
[Crossref]

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A. Mialdun, V. Yasnou, V. Shevtsova, A. Königer, W. Köhler, D. Alonso de Mezquia, M. M. Bou-Ali, “A comprehensive study of diffusion, thermodiffusion, and Soret coefficients of water–isopropanol mixtures,” J. Chem. Phys. 136, 244512 (2012).
[Crossref]

Ye, J.

F. Jin, J. Ye, L. Hong, H. Lam, C. Wu, “Slow relaxation mode in mixtures of water and organic molecules: supramolecular structures or nanobubbles?” J. Phys. Chem. B 111, 2255–2261 (2007).
[Crossref]

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N. Y. Yip, M. Elimelech, “Thermodynamic and energy efficiency analysis of power generation from natural salinity gradients by pressure retarded osmosis,” Environ. Sci. Technol. 46, 5230–5239 (2012).
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Y. E. Geints, N. S. Panamarev, A. Zemlyanov, “Transient behavior of far-field diffraction patterns of a Gaussian laser beam due to the thermo-optical effect in metal nanocolloids,” J. Opt. 13, 055707 (2011).
[Crossref]

Zhang, X.

A. Häbich, W. Ducker, D. E. Dunstan, X. Zhang, “Do stable nanobubbles exist in mixtures of organic solvents and water?” J. Phys. Chem. B 114, 6962–6967 (2010).
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Zhen, Y.-R.

Z. Fang, Y.-R. Zhen, O. Neumann, A. Polman, F. J. García de Abajo, P. Nordlander, N. J. Halas, “Evolution of light-induced vapor generation at a liquid-immersed metallic nanoparticle,” Nano Lett. 13, 1736–1742 (2013).
[Crossref]

Ziano, R.

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

ACS Nano (1)

S. Baral, A. Green, M. Y. Livshits, A. O. Govarov, H. H. Richardson, “Comparison of vapor formation of water at the solid/water interface to colloidal solutions using optically excited gold nanostructures,” ACS Nano 8, 1439–1448 (2014).
[Crossref]

Appl. Opt. (1)

Chem. Eng. Sci. (1)

E. Ruckenstein, I. Shulgin, “Hydrophobic self-assembling in dilute aqueous solutions of alcohols and hydrocarbons,” Chem. Eng. Sci. 56, 5675–5680 (2001).
[Crossref]

Entropy (1)

R. Rica, R. Ziano, D. Salerno, F. Mantegazza, R. van Roij, D. Brogioli, “Capacitive mixing for harvesting the free energy of solutions at different concentrations,” Entropy 15, 1388–1407 (2013).
[Crossref]

Environ. Sci. Technol. (1)

N. Y. Yip, M. Elimelech, “Thermodynamic and energy efficiency analysis of power generation from natural salinity gradients by pressure retarded osmosis,” Environ. Sci. Technol. 46, 5230–5239 (2012).
[Crossref]

Int. J. Heat Mass Transfer (1)

J. Fan, L. Wang, “Heat conduction in nanofluids: structure–property correlation,” Int. J. Heat Mass Transfer 54, 4349–4359 (2011).
[Crossref]

J. Appl. Phys. (1)

R. Taylor, S. Coulombe, T. Otanicar, P. Phelan, A. Gunawan, W. Lv, G. Rosengarten, R. Prasher, H. Tyagi, “Small particles, big impacts: a review of the diverse applications of nanofluids,” J. Appl. Phys. 113, 011301 (2013).
[Crossref]

J. Chem. Phys. (2)

A. Mialdun, V. Yasnou, V. Shevtsova, A. Königer, W. Köhler, D. Alonso de Mezquia, M. M. Bou-Ali, “A comprehensive study of diffusion, thermodiffusion, and Soret coefficients of water–isopropanol mixtures,” J. Chem. Phys. 136, 244512 (2012).
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J. Gliński, A. Burakowski, “Compressibility of aqueous solutions of nonelectrolytes: an equilibrium model,” J. Chem. Phys. 132, 124507 (2010).
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J. Fluid Mech. (1)

A. Bergeon, D. Henry, H. Benhadid, L. S. Tuckerman, “Marangoni convection in binary mixtures with Soret effect,” J. Fluid Mech. 375, 143–177 (1998).
[Crossref]

J. Membr. Sci. (1)

J. W. Post, J. Veerman, H. V. M. Hamelers, G. J. W. Euverink, S. J. Metz, K. Nymeijer, C. J. N. Buisman, “Salinity-gradient power: evaluation of pressure-retarded osmosis and reverse electrodialysis,” J. Membr. Sci. 288, 218–230 (2007).
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M. Dienerowitz, M. Mazilu, K. Dholakia, “Optical manipulation of nanoparticles: a review,” J. Nanophoton. 2, 021875 (2008).
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J. Non-Equilib. Thermodyn. (1)

G. Gouesbet, C. Roze, “Instabilities by local heating below an interface,” J. Non-Equilib. Thermodyn. 25, 337–379 (2001).
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J. Opt. (1)

Y. E. Geints, N. S. Panamarev, A. Zemlyanov, “Transient behavior of far-field diffraction patterns of a Gaussian laser beam due to the thermo-optical effect in metal nanocolloids,” J. Opt. 13, 055707 (2011).
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J. Phys. Chem. (1)

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J. Phys. Chem. B (6)

Y. Takeuchi, T. Ida, K. Kimura, “Colloidal stability of gold nanoparticles in 2-propanol under laser irradiation,” J. Phys. Chem. B 101, 1322–1327 (1997).
[Crossref]

A. Häbich, W. Ducker, D. E. Dunstan, X. Zhang, “Do stable nanobubbles exist in mixtures of organic solvents and water?” J. Phys. Chem. B 114, 6962–6967 (2010).
[Crossref]

F. Jin, J. Ye, L. Hong, H. Lam, C. Wu, “Slow relaxation mode in mixtures of water and organic molecules: supramolecular structures or nanobubbles?” J. Phys. Chem. B 111, 2255–2261 (2007).
[Crossref]

M. Sedlák, D. Rak, “Large-scale inhomogeneities in solutions of low molar mass compounds and mixtures of liquids: supramolecular structures or nanobubbles?” J. Phys. Chem. B 117, 2495–2504 (2013).
[Crossref]

A. Pinke, P. Jedlovsky, “Modeling of mixing acetone and water: how can their full miscibility be reproduced in computer simulations?” J. Phys. Chem. B 116, 5977–5984 (2012).
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M. Sedlak, D. Rak, “On the origin of mesoscale structures in aqueous solutions of tertiary butyl alcohol: the mystery resolved,” J. Phys. Chem. B 118, 2726–2737 (2014).
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J. Phys. Condens. Matter (1)

S. Dixit, W. C. K. Poon, J. Crain, “Hydration of methanol in aqueous solutions: a Raman spectroscopic study,” J. Phys. Condens. Matter 12, L323–L328 (2000).
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J. Phys. Org. Chem. (1)

U. Buhvestov, F. Rived, C. Ra, E. Bosch, A. Rose, “Solute–solvent and solvent–solvent interactions in binary solvent mixtures. Part 7. Comparison of the enhancement of the water structure in alcohol–water mixtures measured by solvatochromic indicators,” J. Phys. Org. Chem. 11, 185–192 (1998).
[Crossref]

J. Solution Chem. (1)

G. Roux, D. Roberts, G. Perron, J. Desnoyers, “Microheterogeneity in aqueous-organic solutions: heat capacities, volumes and expansibilities of some alcohols, aminoalcohol and tertiary amines in water,” J. Solution Chem. 9, 629–647 (1980).
[Crossref]

JETP Lett. (1)

V. Y. Bazhenov, M. V. Vasnetsov, M. S. Soskin, V. B. Tarenenko, “Self-oscillations of a liquid near a free interface during continuous local heating,” JETP Lett. 49, 376–379 (1989).

Langmuir (1)

N. Shalkevich, W. Escher, T. Bürgi, B. Michel, L. Si-Ahmed, D. Poulikakos, “On the thermal conductivity of gold nanoparticle colloids,” Langmuir 26, 663–670 (2010).
[Crossref]

Nano Lett. (2)

M. Moocarme, L. T. Vuong, “Ultralow-intensity magneto-optical and mechanical effects in metal nanocolloids,” Nano Lett. 14, 1178–1183 (2014).

Z. Fang, Y.-R. Zhen, O. Neumann, A. Polman, F. J. García de Abajo, P. Nordlander, N. J. Halas, “Evolution of light-induced vapor generation at a liquid-immersed metallic nanoparticle,” Nano Lett. 13, 1736–1742 (2013).
[Crossref]

Nanoscale Res. Lett. (1)

L. Wang, J. Fan, “Toward nanofluids of ultra-high thermal conductivity,” Nanoscale Res. Lett. 6, 153 (2011).
[Crossref]

Nat. Commun. (2)

H. Amini, E. Sollier, M. Masaeli, Y. Xie, B. Ganapathysubramanian, H. A. Stone, D. Di Carlo, “Engineering fluid flow using sequenced microstructures,” Nat. Commun. 4, 1826 (2013).
[Crossref]

E. Palleau, D. Morales, M. D. Dickey, O. D. Velev, “Reversible patterning and actuation of hydrogels by electrically assisted ionoprinting,” Nat. Commun. 4, 2257 (2013).
[Crossref]

Nat. Nanotechnol. (1)

S. Mubeen, J. Lee, N. Singh, S. Krämer, G. D. Stucky, M. Moskovits, “An autonomous photosynthetic device in which all charge carriers derive from surface plasmons,” Nat. Nanotechnol. 8, 247–251 (2013).
[Crossref]

Nature (2)

S. Dixit, J. Crain, W. C. K. Poon, J. L. Finney, A. K. Soper, “Molecular segregation observed in a concentrated alcohol–water solution,” Nature 416, 829–832 (2002).
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New J. Phys. (1)

E. Greenfield, C. Rotschild, A. Szameit, J. Nemirovsky, R. El-Ganainy, D. N. Christodoulides, M. Saraf, E. Lifshitz, M. Segev, “Light-induced self-synchronizing flow patterns,” New J. Phys. 13, 053021 (2011).
[Crossref]

Opt. Express (2)

N. D. Singh, M. Moocarme, B. Edelstein, N. Punnoose, L. T. Vuong, “Anomalously-large photo-induced magnetic response of metallic nanocolloids in aqueous solution using a solar simulator,” Opt. Express 20, 3054–3065 (2012).
[Crossref]

E. Greenfield, J. Nemirovsky, R. El-Ganainy, N. Demetri, M. Segev, “Shockwave based nonlinear optical manipulation in densely scattering opaque suspensions,” Opt. Express 21, 2382–2384 (2013).
[Crossref]

Opt. Lett. (2)

Phys. Rev. E (2)

B. L. Smorodin, I. N. Cherepanov, B. I. Myznikova, M. I. Shliomis, “Traveling-wave convection in colloids stratified by gravity,” Phys. Rev. E 84, 026305 (2011).
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Y. Lamhot, A. Barak, O. Peleg, M. Segev, “Self-trapping of optical beams through thermophoresis,” Phys. Rev. Lett. 105, 163906 (2010).
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Rep. Prog. Phys. (1)

A. Würger, “Thermal non-equilibrium transport in colloids,” Rep. Prog. Phys. 73, 126601 (2010).
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Science (1)

I. Gur, K. Sawyer, R. Prasher, “Searching for a better thermal battery,” Science 335, 1454–1455 (2012).
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Transp. Porous Media (1)

L. F. Range, J. C. Santamarina, D. O. Fratta, “Dynamic electrical–mechanical energy coupling in electrolyte–mineral systems,” Transp. Porous Media 50, 153–178 (2003).
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M. Chaplin, “Theory vs experiment: what is the surface charge of water?” Water 1, 1–28 (2009).
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Figures (6)

Fig. 1.
Fig. 1. Illustration of a single oscillation period of the light-induced thermal cycle. Inset: schematic of the light propagation and experimental CCD images of the far-field transmitted patterns. Although absorption, dissipation, refraction, and convection are separately outlined, the processes occur simultaneously in varying degrees.
Fig. 2.
Fig. 2. (a) Side and (b) top views of the experimental setup. The half-wave plate (WP) and polarizer (P) control the beam power and polarization (fixed horizontally), respectively, while the vertical translation stage (MTS) varies the entrance depth of light into the nanofluid. The CCD camera records the imaged beam pattern as a function of time. (c) Side view images of the sample cuvette with 80 nm gold nanoparticles illustrating beam propagation and depth are shown where the two curved lines correspond to menisci with parasitic reflections formed by the residual light scattered. (d) Four images of the far-field pattern that are recorded during a single oscillation period. (e) Plots of the integrated CCD images as a function of time for five different depths.
Fig. 3.
Fig. 3. Logarithm of the Fourier decomposition of the transmitted light power as a function of depth in polar organic-aqueous mixtures containing 80 nm gold nanosphere stock solution. The three columns represent from left to right organic solvent/water/stock mixtures with ratios of 1 3 1 , 2 2 1 , and 3 1 1 , respectively. Sample data are shown with increasingly protic organic solvent from top to bottom: (a–c) acetone, (d–f) acetonitrile, (g–i) methanol, (j–l) ethanol, (m–o) isopropanol. The DC components of the Fourier transform are omitted.
Fig. 4.
Fig. 4. Transmission of low-intensity laser light ( λ = 532 nm , average power = 100 mW ) though isopropyl alcohol–water and acetone–water binary mixtures as a function of volume fraction. The isopropyl alcohol mixture features a sharp dip with 3 parts alcohol to 6 parts water.
Fig. 5.
Fig. 5. Numerically calculated far-field interference patterns I FF (above) associated with the temperature profiles of the nanofluid (below) for (a)  α = 1.7 e 2 / cm , C n v = 10 C T , (b)  α = 1.3 e 2 / cm , C n v = 1000 C T , (c)  α = 8 e 3 / cm , C n v = 3000 C T , and (d)  α = 0.5 e 3 / cm , C n v = C T .
Fig. 6.
Fig. 6. (a) Transmission spectra for isopropanol:water:stock nanoparticle sample in a ratio of 2 2 1 . (b) White-light-induced oscillations in the transmitted power through a silver nanofluid of the same ratio. (c) Logarithm of the Fourier decomposition of the oscillations (DC components removed), which shows a depth-dependent characteristic frequency.

Equations (3)

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I FF ( ξ , ν ) = e 2 α d | I inc ( x , y ) e i Δ ϕ ( x , y ) e i ( x ξ + y ν ) d x d y | 2 ,
Δ ϕ ( x , y ) = k d n T T ( x , y ) ,
d T d t = [ C T 2 x 2 + ( C n v + C T ) 2 y 2 ] T + α π P 0 ρ C ρ I 0 ,

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