Abstract

In this paper, novel Bi3+/Eu3+ co-doped white-emitting germanium-borate glasses were successfully prepared by the melt-quenching method. Their luminescent properties were evaluated using the transmission spectra, photoluminescence excitation, and emission spectra (with a temperature range of 298-573 K), and lifetime decay curves. Due to the efficient energy transfer from Bi3+ to Eu3+, tunable emitting color between the bluish-green and the orange-red region has been obtained by varying the content of Eu3+ (0-7%). Interestingly, a perfect white-light emission with CIE coordinates (X = 0.356, Y = 0.325) is realized upon the excitation at 345 nm light in the Bi3+/Eu3+ co-doped sample. More remarkably, the white-light emission glass maintains excellent color stability even at 423 K. Our results indicate that the Bi3+/Eu3+ co-doped germanium-borate glasses may be used as a potential single-phased white light-emitting matrix material for the UV converted organic-resin-free WLEDs in the future.

© 2016 Optical Society of America

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    [Crossref]
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    [Crossref]
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2016 (4)

Z. Xia, Z. Xu, M. Chen, and Q. Liu, “Recent developments in the new inorganic solid-state LED phosphors,” Dalton Trans. 45(28), 11214–11232 (2016).
[Crossref] [PubMed]

B. Wang, H. Lin, F. Huang, J. Xu, H. Chen, Z. B. Lin, and Y. S. Wang, “Non-rare-earth BaMgAl10-2xO17: xMn4+,xMg2+: a narrow-band red phosphor for high-power warm W-LED,” Chem. Mater. 28(10), 3515–3524 (2016).
[Crossref]

F. W. Kang, H. S. Zhang, L. Wondraczek, X. B. Yang, Y. Zhang, D. Y. Lei, and M. Y. Peng, “Band-Gap Modulation in Single Bi3+-Doped Yttrium-Scandium-Niobium Vanadates for Color Tuning over the Whole Visible Spectrum,” Chem. Mater. 28(8), 2692–2703 (2016).
[Crossref]

X. Y. Liu, H. Guo, Y. Liu, S. Ye, M. Y. Peng, and Q. Y. Zhang, “Thermal quenching and energy transfer in novel Bi3+/Mn2+co-doped white-emitting borosilicate glasses for UV LEDs,” J. Mater. Chem. C 4(13), 2506–2512 (2016).
[Crossref]

2015 (6)

K. Li, J. Fan, M. M. Shang, H. Z. Lian, and J. Lin, “Sr2Y8(SiO4)6O2:Bi3+/Eu3+: a single-component white-emitting phosphor via energy transfer for UV W-LEDs,” J. Mater. Chem. C 3(38), 9989–9998 (2015).
[Crossref]

L. J. Wang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “White luminescence and energy transfer process in Bi3+,Sm3+ co-doped Ca3Al2O6 phosphors,” Opt. Mater. 42, 233–236 (2015).
[Crossref]

F. Kang, Y. Zhang, and M. Peng, “Controlling the energy transfer via multi luminescent centers to achieve white light/tunable emissions in a single-phased X2-type Y2SiO5:Eu3+, Bi3+ phosphor for ultraviolet converted LEDs,” Inorg. Chem. 54(4), 1462–1473 (2015).
[Crossref] [PubMed]

W. B. Dai, S. Ye, E. L. Li, P. Z. Zhuo, and Q. Y. Zhang, “High quality LED lamps using color-tunable Ce3+-activated yellow-green oxyfluoride solid-solution and Eu3+-doped red borate phosphors,” J. Mater. Chem. C 3(31), 8132–8141 (2015).
[Crossref]

D. Q. Chen, W. D. Xiang, X. J. Liang, J. S. Zhong, H. Yu, M. Y. Ding, H. W. Lu, and Z. G. Ji, “Advances in transparent glass-ceramic phosphors for white light-emitting diodes–A review,” J. Eur. Ceram. Soc. 35(3), 859–869 (2015).
[Crossref]

Y. Shi, G. Zhu, M. Mikami, Y. Shimomura, and Y. Wang, “A novel Ce3+ activated Lu3MgAl3SiO12 garnet phosphor for blue chip light-emitting diodes with excellent performance,” Dalton Trans. 44(4), 1775–1781 (2015).
[Crossref] [PubMed]

2014 (7)

G. J. Gao and L. Wondraczek, “Heavily Eu3+-doped boroaluminosilicate glasses for UV/blue-to-red photoconversion with high quantum yield,” J. Mater. Chem. C 2(4), 691–695 (2014).
[Crossref]

X. Zhang, L. Huang, F. Pan, M. Wu, J. Wang, Y. Chen, and Q. Su, “Highly thermally stable single-component white-emitting silicate glass for organic-resin-free white-light-emitting diodes,” ACS Appl. Mater. Interfaces 6(4), 2709–2717 (2014).
[Crossref] [PubMed]

R. Zhang, H. Lin, Y. L. Yu, D. Q. Chen, J. Xu, and Y. S. Wang, “A new-generation color converter for high-power white LED: transparent Ce3+:YAG phosphor-in-glass,” Laser Photonics Rev. 8(1), 158–164 (2014).
[Crossref]

M. Shang, C. Li, and J. Lin, “How to produce white light in a single-phase host?” Chem. Soc. Rev. 43(5), 1372–1386 (2014).
[Crossref] [PubMed]

P. Kaur, S. Kaur, G. P. Singh, and D. P. Singh, “Cerium and samarium codoped lithium aluminoborate glasses for white light emitting devices,” J. Alloys Compd. 588(181), 394–398 (2014).
[Crossref]

J. W. Yang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “Luminescence and energy transfer process in Cu+,Sm3+ co-doped sodium silicate glasses,” Opt. Mater. Express 4(2), 315–320 (2014).
[Crossref]

F. W. Kang, X. B. Yang, M. Y. Peng, L. Wondraczek, Z. J. Ma, Q. Y. Zhang, and J. R. Qiu, “Red Photoluminescence from Bi3+ and the Influence of the Oxygen-Vacancy Perturbation in ScVO4:A Combined Experimental and Theoretical Study,” J. Phys. Chem. C 118(14), 7515–7522 (2014).
[Crossref]

2013 (2)

X. Y. Sun, D. G. Jiang, S. W. Chen, G. T. Zheng, S. M. Huang, M. Gu, Z. J. Zhang, and J. T. Zhao, “Eu3+-Activated Borogermanate Scintillating Glass with a High Gd2O3 Content,” J. Am. Ceram. Soc. 96(5), 1483–1489 (2013).
[Crossref]

C. C. Tsai, W. C. Cheng, J. K. Chang, L. Y. Chen, J. H. Chen, Y. C. Hsu, and W. H. Cheng, “Ultra-High Thermal-Stable Glass Phosphor Layer for Phosphor-Converted White Light-Emitting Diodes,” J. Disp. Technol. 9(6), 427–432 (2013).
[Crossref]

2012 (5)

J. J. Li, J. D. Chen, R. F. Wei, and H. Guo, “Combined White Luminescence from Eu3+, ML-Ag Particles and Ag+ in Ag/Eu3+ Co-Doped H3BO3-BaF2 Glasses,” J. Am. Ceram. Soc. 95(4), 1208–1211 (2012).
[Crossref]

X. L. Liang, Z. Y. Lin, Y. X. Yang, Z. W. Xing, and G. Chen, “Luminescence Properties of Tb-Eu Co-Doped Aluminosilicate and Zinc Silicate Glasses,” J. Am. Ceram. Soc. 95(1), 275–279 (2012).
[Crossref]

H. Guo, R. Wei, and X. Liu, “Tunable white luminescence and energy transfer in (Cu+)2, Eu3+ codoped sodium silicate glasses,” Opt. Lett. 37(10), 1670–1672 (2012).
[Crossref] [PubMed]

A. C. P. Rocha, L. H. C. Andrade, S. M. Lima, A. M. Farias, A. C. Bento, M. L. Baesso, Y. Guyot, and G. Boulon, “Tunable color temperature of Ce3+/Eu2+, 3+ co-doped low silica aluminosilicate glasses for white lighting,” Opt. Express 20(9), 10034–10041 (2012).
[Crossref] [PubMed]

H. Daicho, T. Iwasaki, K. Enomoto, Y. Sasaki, Y. Maeno, Y. Shinomiya, S. Aoyagi, E. Nishibori, M. Sakata, H. Sawa, S. Matsuishi, and H. Hosono, “A novel phosphor for glareless white light-emitting diodes,” Nat. Commun. 3(2138), 1132–1140 (2012).
[Crossref] [PubMed]

2011 (3)

Y. Liu, X. Zhang, Z. Hao, X. Wang, and J. Zhang, “Tunable full-color-emitting Ca3Sc2Si3O12:Ce3+, Mn2+ phosphor via charge compensation and energy transfer,” Chem. Commun. (Camb.) 47(38), 10677–10679 (2011).
[Crossref] [PubMed]

R. G. Ye, Z. G. Cui, Y. J. Hua, D. G. Deng, S. L. Zhao, C. X. Li, and S. Q. Xu, “Eu2+/Dy3+ co-doped white light emission glass ceramics under UV light excitation,” J. Non-Cryst. Solids 357(11–13), 2282–2285 (2011).
[Crossref]

G. F. Ju, Y. H. Hu, L. Chen, X. J. Wang, Z. F. Mu, H. Y. Wu, and F. W. Kang, “White-Light Generation and Energy Transfer in Y2O3:Bi,Eu Phosphor for Ultraviolet Light-Emitting Diodes,” J. Electrochem. Soc. 158(10), J294–J299 (2011).
[Crossref]

2010 (1)

S. Ye, F. Xiao, Y. X. Pan, Y. Y. Ma, and Q. Y. Zhang, “Phosphors in phosphor-converted white light-emitting diodes: Recent advances in materials, techniques and properties,” Mater. Sci. Eng. Rep. 71(1), 1–34 (2010).
[Crossref]

2009 (2)

S. Pimputkar, J. S. Speck, S. P. DenBaars, and S. J. Nakamura, “Prospects for LED lighting,” Nat. Photonics 3(4), 180–182 (2009).
[Crossref]

H. A. Höppe, “Recent developments in the field of inorganic phosphors,” Angew. Chem. Int. Ed. Engl. 48(20), 3572–3582 (2009).
[Crossref] [PubMed]

2008 (1)

D. Q. Chen, Y. S. Wang, Y. L. Yu, and P. Huang, “Structure and Optical Spectroscopy of Eu-Doped Glass Ceramics Containing GdF3,” J. Phys. Chem. C 112(48), 18943–18947 (2008).
[Crossref]

2005 (2)

E. F. Schubert and J. K. Kim, “Solid-State Light Sources Getting Smart,” Science 308(5726), 1274–1278 (2005).
[Crossref] [PubMed]

S. Fujita, S. Yoshihara, A. Sakamoto, S. Yamamoto, and S. Tanabe, “YAG glass-ceramic phosphor for white LED (I): background and development,” Proc. SPIE 5941, 186–192 (2005).
[Crossref]

2003 (1)

P. I. Paulosea, G. Josea, V. Thomasa, N. V. Unnikrishnana, and M. K. R. Warrier, “Sensitized fluorescence of Ce3+/Mn2+ system in phosphate glass,” J. Phys. Chem. Solids 64(5), 841–846 (2003).
[Crossref]

1988 (1)

S. Bhushan and M. V. Chukichev, “Temperature dependent studies of cathodoluminescence of green band of ZnO crystals,” J. Mater. Sci. Lett. 7(4), 319–321 (1988).
[Crossref]

1984 (1)

K. J. Laidler, “The Development of the Arrhenius Equation,” J. Chem. Educ. 61(6), 494–498 (1984).
[Crossref]

1980 (1)

G. Boulon, B. Moine, and J. C. Bourcet, “Spectroscopic properties of 3P1 and 3P0 excited states of Bi3+ ion in germanate glass,” Phys. Rev. B 22(3), 1163–1169 (1980).
[Crossref]

1979 (1)

G. Boulon, B. Moine, J. C. Bourcet, R. Reisefeld, and Y. Kalisky, “Time resolved spectroscopy about 3P1 and 3P0 levels in Bi3+ doped germanate glasses,” J. Lumin. 18(1), 924–928 (1979).
[Crossref]

1972 (1)

J. Tauc and A. Menth, “States in the gap,” J. Non-Cryst. Solids 8(10), 569–585 (1972).
[Crossref]

1965 (1)

M. Inokuti and F. Hirayama, “Influence of Energy Transfer by the Exchange Mechanism on Donor Luminescence,” J. Chem. Phys. 43(6), 1978–1989 (1965).
[Crossref]

1953 (1)

D. L. Dexter, “A Theory of Sensitized Luminescence in Solids,” J. Chem. Phys. 21(5), 836–850 (1953).
[Crossref]

Andrade, L. H. C.

Aoyagi, S.

H. Daicho, T. Iwasaki, K. Enomoto, Y. Sasaki, Y. Maeno, Y. Shinomiya, S. Aoyagi, E. Nishibori, M. Sakata, H. Sawa, S. Matsuishi, and H. Hosono, “A novel phosphor for glareless white light-emitting diodes,” Nat. Commun. 3(2138), 1132–1140 (2012).
[Crossref] [PubMed]

Baesso, M. L.

Bento, A. C.

Bhushan, S.

S. Bhushan and M. V. Chukichev, “Temperature dependent studies of cathodoluminescence of green band of ZnO crystals,” J. Mater. Sci. Lett. 7(4), 319–321 (1988).
[Crossref]

Boulon, G.

A. C. P. Rocha, L. H. C. Andrade, S. M. Lima, A. M. Farias, A. C. Bento, M. L. Baesso, Y. Guyot, and G. Boulon, “Tunable color temperature of Ce3+/Eu2+, 3+ co-doped low silica aluminosilicate glasses for white lighting,” Opt. Express 20(9), 10034–10041 (2012).
[Crossref] [PubMed]

G. Boulon, B. Moine, and J. C. Bourcet, “Spectroscopic properties of 3P1 and 3P0 excited states of Bi3+ ion in germanate glass,” Phys. Rev. B 22(3), 1163–1169 (1980).
[Crossref]

G. Boulon, B. Moine, J. C. Bourcet, R. Reisefeld, and Y. Kalisky, “Time resolved spectroscopy about 3P1 and 3P0 levels in Bi3+ doped germanate glasses,” J. Lumin. 18(1), 924–928 (1979).
[Crossref]

Bourcet, J. C.

G. Boulon, B. Moine, and J. C. Bourcet, “Spectroscopic properties of 3P1 and 3P0 excited states of Bi3+ ion in germanate glass,” Phys. Rev. B 22(3), 1163–1169 (1980).
[Crossref]

G. Boulon, B. Moine, J. C. Bourcet, R. Reisefeld, and Y. Kalisky, “Time resolved spectroscopy about 3P1 and 3P0 levels in Bi3+ doped germanate glasses,” J. Lumin. 18(1), 924–928 (1979).
[Crossref]

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Y. Shi, G. Zhu, M. Mikami, Y. Shimomura, and Y. Wang, “A novel Ce3+ activated Lu3MgAl3SiO12 garnet phosphor for blue chip light-emitting diodes with excellent performance,” Dalton Trans. 44(4), 1775–1781 (2015).
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G. Boulon, B. Moine, and J. C. Bourcet, “Spectroscopic properties of 3P1 and 3P0 excited states of Bi3+ ion in germanate glass,” Phys. Rev. B 22(3), 1163–1169 (1980).
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G. Boulon, B. Moine, J. C. Bourcet, R. Reisefeld, and Y. Kalisky, “Time resolved spectroscopy about 3P1 and 3P0 levels in Bi3+ doped germanate glasses,” J. Lumin. 18(1), 924–928 (1979).
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G. F. Ju, Y. H. Hu, L. Chen, X. J. Wang, Z. F. Mu, H. Y. Wu, and F. W. Kang, “White-Light Generation and Energy Transfer in Y2O3:Bi,Eu Phosphor for Ultraviolet Light-Emitting Diodes,” J. Electrochem. Soc. 158(10), J294–J299 (2011).
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Nakamura, S. J.

S. Pimputkar, J. S. Speck, S. P. DenBaars, and S. J. Nakamura, “Prospects for LED lighting,” Nat. Photonics 3(4), 180–182 (2009).
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H. Daicho, T. Iwasaki, K. Enomoto, Y. Sasaki, Y. Maeno, Y. Shinomiya, S. Aoyagi, E. Nishibori, M. Sakata, H. Sawa, S. Matsuishi, and H. Hosono, “A novel phosphor for glareless white light-emitting diodes,” Nat. Commun. 3(2138), 1132–1140 (2012).
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L. J. Wang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “White luminescence and energy transfer process in Bi3+,Sm3+ co-doped Ca3Al2O6 phosphors,” Opt. Mater. 42, 233–236 (2015).
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J. W. Yang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “Luminescence and energy transfer process in Cu+,Sm3+ co-doped sodium silicate glasses,” Opt. Mater. Express 4(2), 315–320 (2014).
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X. Zhang, L. Huang, F. Pan, M. Wu, J. Wang, Y. Chen, and Q. Su, “Highly thermally stable single-component white-emitting silicate glass for organic-resin-free white-light-emitting diodes,” ACS Appl. Mater. Interfaces 6(4), 2709–2717 (2014).
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Pan, Y. X.

S. Ye, F. Xiao, Y. X. Pan, Y. Y. Ma, and Q. Y. Zhang, “Phosphors in phosphor-converted white light-emitting diodes: Recent advances in materials, techniques and properties,” Mater. Sci. Eng. Rep. 71(1), 1–34 (2010).
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P. I. Paulosea, G. Josea, V. Thomasa, N. V. Unnikrishnana, and M. K. R. Warrier, “Sensitized fluorescence of Ce3+/Mn2+ system in phosphate glass,” J. Phys. Chem. Solids 64(5), 841–846 (2003).
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Peng, M.

F. Kang, Y. Zhang, and M. Peng, “Controlling the energy transfer via multi luminescent centers to achieve white light/tunable emissions in a single-phased X2-type Y2SiO5:Eu3+, Bi3+ phosphor for ultraviolet converted LEDs,” Inorg. Chem. 54(4), 1462–1473 (2015).
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Peng, M. Y.

F. W. Kang, H. S. Zhang, L. Wondraczek, X. B. Yang, Y. Zhang, D. Y. Lei, and M. Y. Peng, “Band-Gap Modulation in Single Bi3+-Doped Yttrium-Scandium-Niobium Vanadates for Color Tuning over the Whole Visible Spectrum,” Chem. Mater. 28(8), 2692–2703 (2016).
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X. Y. Liu, H. Guo, Y. Liu, S. Ye, M. Y. Peng, and Q. Y. Zhang, “Thermal quenching and energy transfer in novel Bi3+/Mn2+co-doped white-emitting borosilicate glasses for UV LEDs,” J. Mater. Chem. C 4(13), 2506–2512 (2016).
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F. W. Kang, X. B. Yang, M. Y. Peng, L. Wondraczek, Z. J. Ma, Q. Y. Zhang, and J. R. Qiu, “Red Photoluminescence from Bi3+ and the Influence of the Oxygen-Vacancy Perturbation in ScVO4:A Combined Experimental and Theoretical Study,” J. Phys. Chem. C 118(14), 7515–7522 (2014).
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S. Pimputkar, J. S. Speck, S. P. DenBaars, and S. J. Nakamura, “Prospects for LED lighting,” Nat. Photonics 3(4), 180–182 (2009).
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F. W. Kang, X. B. Yang, M. Y. Peng, L. Wondraczek, Z. J. Ma, Q. Y. Zhang, and J. R. Qiu, “Red Photoluminescence from Bi3+ and the Influence of the Oxygen-Vacancy Perturbation in ScVO4:A Combined Experimental and Theoretical Study,” J. Phys. Chem. C 118(14), 7515–7522 (2014).
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G. Boulon, B. Moine, J. C. Bourcet, R. Reisefeld, and Y. Kalisky, “Time resolved spectroscopy about 3P1 and 3P0 levels in Bi3+ doped germanate glasses,” J. Lumin. 18(1), 924–928 (1979).
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Sakamoto, A.

S. Fujita, S. Yoshihara, A. Sakamoto, S. Yamamoto, and S. Tanabe, “YAG glass-ceramic phosphor for white LED (I): background and development,” Proc. SPIE 5941, 186–192 (2005).
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H. Daicho, T. Iwasaki, K. Enomoto, Y. Sasaki, Y. Maeno, Y. Shinomiya, S. Aoyagi, E. Nishibori, M. Sakata, H. Sawa, S. Matsuishi, and H. Hosono, “A novel phosphor for glareless white light-emitting diodes,” Nat. Commun. 3(2138), 1132–1140 (2012).
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H. Daicho, T. Iwasaki, K. Enomoto, Y. Sasaki, Y. Maeno, Y. Shinomiya, S. Aoyagi, E. Nishibori, M. Sakata, H. Sawa, S. Matsuishi, and H. Hosono, “A novel phosphor for glareless white light-emitting diodes,” Nat. Commun. 3(2138), 1132–1140 (2012).
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Y. Shi, G. Zhu, M. Mikami, Y. Shimomura, and Y. Wang, “A novel Ce3+ activated Lu3MgAl3SiO12 garnet phosphor for blue chip light-emitting diodes with excellent performance,” Dalton Trans. 44(4), 1775–1781 (2015).
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Shimomura, Y.

Y. Shi, G. Zhu, M. Mikami, Y. Shimomura, and Y. Wang, “A novel Ce3+ activated Lu3MgAl3SiO12 garnet phosphor for blue chip light-emitting diodes with excellent performance,” Dalton Trans. 44(4), 1775–1781 (2015).
[Crossref] [PubMed]

Shinomiya, Y.

H. Daicho, T. Iwasaki, K. Enomoto, Y. Sasaki, Y. Maeno, Y. Shinomiya, S. Aoyagi, E. Nishibori, M. Sakata, H. Sawa, S. Matsuishi, and H. Hosono, “A novel phosphor for glareless white light-emitting diodes,” Nat. Commun. 3(2138), 1132–1140 (2012).
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P. Kaur, S. Kaur, G. P. Singh, and D. P. Singh, “Cerium and samarium codoped lithium aluminoborate glasses for white light emitting devices,” J. Alloys Compd. 588(181), 394–398 (2014).
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P. Kaur, S. Kaur, G. P. Singh, and D. P. Singh, “Cerium and samarium codoped lithium aluminoborate glasses for white light emitting devices,” J. Alloys Compd. 588(181), 394–398 (2014).
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S. Pimputkar, J. S. Speck, S. P. DenBaars, and S. J. Nakamura, “Prospects for LED lighting,” Nat. Photonics 3(4), 180–182 (2009).
[Crossref]

Su, Q.

X. Zhang, L. Huang, F. Pan, M. Wu, J. Wang, Y. Chen, and Q. Su, “Highly thermally stable single-component white-emitting silicate glass for organic-resin-free white-light-emitting diodes,” ACS Appl. Mater. Interfaces 6(4), 2709–2717 (2014).
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X. Y. Sun, D. G. Jiang, S. W. Chen, G. T. Zheng, S. M. Huang, M. Gu, Z. J. Zhang, and J. T. Zhao, “Eu3+-Activated Borogermanate Scintillating Glass with a High Gd2O3 Content,” J. Am. Ceram. Soc. 96(5), 1483–1489 (2013).
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S. Fujita, S. Yoshihara, A. Sakamoto, S. Yamamoto, and S. Tanabe, “YAG glass-ceramic phosphor for white LED (I): background and development,” Proc. SPIE 5941, 186–192 (2005).
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J. Tauc and A. Menth, “States in the gap,” J. Non-Cryst. Solids 8(10), 569–585 (1972).
[Crossref]

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P. I. Paulosea, G. Josea, V. Thomasa, N. V. Unnikrishnana, and M. K. R. Warrier, “Sensitized fluorescence of Ce3+/Mn2+ system in phosphate glass,” J. Phys. Chem. Solids 64(5), 841–846 (2003).
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P. I. Paulosea, G. Josea, V. Thomasa, N. V. Unnikrishnana, and M. K. R. Warrier, “Sensitized fluorescence of Ce3+/Mn2+ system in phosphate glass,” J. Phys. Chem. Solids 64(5), 841–846 (2003).
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B. Wang, H. Lin, F. Huang, J. Xu, H. Chen, Z. B. Lin, and Y. S. Wang, “Non-rare-earth BaMgAl10-2xO17: xMn4+,xMg2+: a narrow-band red phosphor for high-power warm W-LED,” Chem. Mater. 28(10), 3515–3524 (2016).
[Crossref]

Wang, J.

X. Zhang, L. Huang, F. Pan, M. Wu, J. Wang, Y. Chen, and Q. Su, “Highly thermally stable single-component white-emitting silicate glass for organic-resin-free white-light-emitting diodes,” ACS Appl. Mater. Interfaces 6(4), 2709–2717 (2014).
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L. J. Wang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “White luminescence and energy transfer process in Bi3+,Sm3+ co-doped Ca3Al2O6 phosphors,” Opt. Mater. 42, 233–236 (2015).
[Crossref]

Wang, X.

Y. Liu, X. Zhang, Z. Hao, X. Wang, and J. Zhang, “Tunable full-color-emitting Ca3Sc2Si3O12:Ce3+, Mn2+ phosphor via charge compensation and energy transfer,” Chem. Commun. (Camb.) 47(38), 10677–10679 (2011).
[Crossref] [PubMed]

Wang, X. J.

G. F. Ju, Y. H. Hu, L. Chen, X. J. Wang, Z. F. Mu, H. Y. Wu, and F. W. Kang, “White-Light Generation and Energy Transfer in Y2O3:Bi,Eu Phosphor for Ultraviolet Light-Emitting Diodes,” J. Electrochem. Soc. 158(10), J294–J299 (2011).
[Crossref]

Wang, Y.

Y. Shi, G. Zhu, M. Mikami, Y. Shimomura, and Y. Wang, “A novel Ce3+ activated Lu3MgAl3SiO12 garnet phosphor for blue chip light-emitting diodes with excellent performance,” Dalton Trans. 44(4), 1775–1781 (2015).
[Crossref] [PubMed]

Wang, Y. S.

B. Wang, H. Lin, F. Huang, J. Xu, H. Chen, Z. B. Lin, and Y. S. Wang, “Non-rare-earth BaMgAl10-2xO17: xMn4+,xMg2+: a narrow-band red phosphor for high-power warm W-LED,” Chem. Mater. 28(10), 3515–3524 (2016).
[Crossref]

R. Zhang, H. Lin, Y. L. Yu, D. Q. Chen, J. Xu, and Y. S. Wang, “A new-generation color converter for high-power white LED: transparent Ce3+:YAG phosphor-in-glass,” Laser Photonics Rev. 8(1), 158–164 (2014).
[Crossref]

D. Q. Chen, Y. S. Wang, Y. L. Yu, and P. Huang, “Structure and Optical Spectroscopy of Eu-Doped Glass Ceramics Containing GdF3,” J. Phys. Chem. C 112(48), 18943–18947 (2008).
[Crossref]

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P. I. Paulosea, G. Josea, V. Thomasa, N. V. Unnikrishnana, and M. K. R. Warrier, “Sensitized fluorescence of Ce3+/Mn2+ system in phosphate glass,” J. Phys. Chem. Solids 64(5), 841–846 (2003).
[Crossref]

Wei, R.

Wei, R. F.

J. J. Li, J. D. Chen, R. F. Wei, and H. Guo, “Combined White Luminescence from Eu3+, ML-Ag Particles and Ag+ in Ag/Eu3+ Co-Doped H3BO3-BaF2 Glasses,” J. Am. Ceram. Soc. 95(4), 1208–1211 (2012).
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Wei, Y. L.

L. J. Wang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “White luminescence and energy transfer process in Bi3+,Sm3+ co-doped Ca3Al2O6 phosphors,” Opt. Mater. 42, 233–236 (2015).
[Crossref]

J. W. Yang, H. Guo, Y. L. Wei, H. M. Noh, and J. H. Jeong, “Luminescence and energy transfer process in Cu+,Sm3+ co-doped sodium silicate glasses,” Opt. Mater. Express 4(2), 315–320 (2014).
[Crossref]

Wondraczek, L.

F. W. Kang, H. S. Zhang, L. Wondraczek, X. B. Yang, Y. Zhang, D. Y. Lei, and M. Y. Peng, “Band-Gap Modulation in Single Bi3+-Doped Yttrium-Scandium-Niobium Vanadates for Color Tuning over the Whole Visible Spectrum,” Chem. Mater. 28(8), 2692–2703 (2016).
[Crossref]

F. W. Kang, X. B. Yang, M. Y. Peng, L. Wondraczek, Z. J. Ma, Q. Y. Zhang, and J. R. Qiu, “Red Photoluminescence from Bi3+ and the Influence of the Oxygen-Vacancy Perturbation in ScVO4:A Combined Experimental and Theoretical Study,” J. Phys. Chem. C 118(14), 7515–7522 (2014).
[Crossref]

G. J. Gao and L. Wondraczek, “Heavily Eu3+-doped boroaluminosilicate glasses for UV/blue-to-red photoconversion with high quantum yield,” J. Mater. Chem. C 2(4), 691–695 (2014).
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Wu, H. Y.

G. F. Ju, Y. H. Hu, L. Chen, X. J. Wang, Z. F. Mu, H. Y. Wu, and F. W. Kang, “White-Light Generation and Energy Transfer in Y2O3:Bi,Eu Phosphor for Ultraviolet Light-Emitting Diodes,” J. Electrochem. Soc. 158(10), J294–J299 (2011).
[Crossref]

Wu, M.

X. Zhang, L. Huang, F. Pan, M. Wu, J. Wang, Y. Chen, and Q. Su, “Highly thermally stable single-component white-emitting silicate glass for organic-resin-free white-light-emitting diodes,” ACS Appl. Mater. Interfaces 6(4), 2709–2717 (2014).
[Crossref] [PubMed]

Xia, Z.

Z. Xia, Z. Xu, M. Chen, and Q. Liu, “Recent developments in the new inorganic solid-state LED phosphors,” Dalton Trans. 45(28), 11214–11232 (2016).
[Crossref] [PubMed]

Xiang, W. D.

D. Q. Chen, W. D. Xiang, X. J. Liang, J. S. Zhong, H. Yu, M. Y. Ding, H. W. Lu, and Z. G. Ji, “Advances in transparent glass-ceramic phosphors for white light-emitting diodes–A review,” J. Eur. Ceram. Soc. 35(3), 859–869 (2015).
[Crossref]

Xiao, F.

S. Ye, F. Xiao, Y. X. Pan, Y. Y. Ma, and Q. Y. Zhang, “Phosphors in phosphor-converted white light-emitting diodes: Recent advances in materials, techniques and properties,” Mater. Sci. Eng. Rep. 71(1), 1–34 (2010).
[Crossref]

Xing, Z. W.

X. L. Liang, Z. Y. Lin, Y. X. Yang, Z. W. Xing, and G. Chen, “Luminescence Properties of Tb-Eu Co-Doped Aluminosilicate and Zinc Silicate Glasses,” J. Am. Ceram. Soc. 95(1), 275–279 (2012).
[Crossref]

Xu, J.

B. Wang, H. Lin, F. Huang, J. Xu, H. Chen, Z. B. Lin, and Y. S. Wang, “Non-rare-earth BaMgAl10-2xO17: xMn4+,xMg2+: a narrow-band red phosphor for high-power warm W-LED,” Chem. Mater. 28(10), 3515–3524 (2016).
[Crossref]

R. Zhang, H. Lin, Y. L. Yu, D. Q. Chen, J. Xu, and Y. S. Wang, “A new-generation color converter for high-power white LED: transparent Ce3+:YAG phosphor-in-glass,” Laser Photonics Rev. 8(1), 158–164 (2014).
[Crossref]

Xu, S. Q.

R. G. Ye, Z. G. Cui, Y. J. Hua, D. G. Deng, S. L. Zhao, C. X. Li, and S. Q. Xu, “Eu2+/Dy3+ co-doped white light emission glass ceramics under UV light excitation,” J. Non-Cryst. Solids 357(11–13), 2282–2285 (2011).
[Crossref]

Xu, Z.

Z. Xia, Z. Xu, M. Chen, and Q. Liu, “Recent developments in the new inorganic solid-state LED phosphors,” Dalton Trans. 45(28), 11214–11232 (2016).
[Crossref] [PubMed]

Yamamoto, S.

S. Fujita, S. Yoshihara, A. Sakamoto, S. Yamamoto, and S. Tanabe, “YAG glass-ceramic phosphor for white LED (I): background and development,” Proc. SPIE 5941, 186–192 (2005).
[Crossref]

Yang, J. W.

Yang, X. B.

F. W. Kang, H. S. Zhang, L. Wondraczek, X. B. Yang, Y. Zhang, D. Y. Lei, and M. Y. Peng, “Band-Gap Modulation in Single Bi3+-Doped Yttrium-Scandium-Niobium Vanadates for Color Tuning over the Whole Visible Spectrum,” Chem. Mater. 28(8), 2692–2703 (2016).
[Crossref]

F. W. Kang, X. B. Yang, M. Y. Peng, L. Wondraczek, Z. J. Ma, Q. Y. Zhang, and J. R. Qiu, “Red Photoluminescence from Bi3+ and the Influence of the Oxygen-Vacancy Perturbation in ScVO4:A Combined Experimental and Theoretical Study,” J. Phys. Chem. C 118(14), 7515–7522 (2014).
[Crossref]

Yang, Y. X.

X. L. Liang, Z. Y. Lin, Y. X. Yang, Z. W. Xing, and G. Chen, “Luminescence Properties of Tb-Eu Co-Doped Aluminosilicate and Zinc Silicate Glasses,” J. Am. Ceram. Soc. 95(1), 275–279 (2012).
[Crossref]

Ye, R. G.

R. G. Ye, Z. G. Cui, Y. J. Hua, D. G. Deng, S. L. Zhao, C. X. Li, and S. Q. Xu, “Eu2+/Dy3+ co-doped white light emission glass ceramics under UV light excitation,” J. Non-Cryst. Solids 357(11–13), 2282–2285 (2011).
[Crossref]

Ye, S.

X. Y. Liu, H. Guo, Y. Liu, S. Ye, M. Y. Peng, and Q. Y. Zhang, “Thermal quenching and energy transfer in novel Bi3+/Mn2+co-doped white-emitting borosilicate glasses for UV LEDs,” J. Mater. Chem. C 4(13), 2506–2512 (2016).
[Crossref]

W. B. Dai, S. Ye, E. L. Li, P. Z. Zhuo, and Q. Y. Zhang, “High quality LED lamps using color-tunable Ce3+-activated yellow-green oxyfluoride solid-solution and Eu3+-doped red borate phosphors,” J. Mater. Chem. C 3(31), 8132–8141 (2015).
[Crossref]

S. Ye, F. Xiao, Y. X. Pan, Y. Y. Ma, and Q. Y. Zhang, “Phosphors in phosphor-converted white light-emitting diodes: Recent advances in materials, techniques and properties,” Mater. Sci. Eng. Rep. 71(1), 1–34 (2010).
[Crossref]

Yoshihara, S.

S. Fujita, S. Yoshihara, A. Sakamoto, S. Yamamoto, and S. Tanabe, “YAG glass-ceramic phosphor for white LED (I): background and development,” Proc. SPIE 5941, 186–192 (2005).
[Crossref]

Yu, H.

D. Q. Chen, W. D. Xiang, X. J. Liang, J. S. Zhong, H. Yu, M. Y. Ding, H. W. Lu, and Z. G. Ji, “Advances in transparent glass-ceramic phosphors for white light-emitting diodes–A review,” J. Eur. Ceram. Soc. 35(3), 859–869 (2015).
[Crossref]

Yu, Y. L.

R. Zhang, H. Lin, Y. L. Yu, D. Q. Chen, J. Xu, and Y. S. Wang, “A new-generation color converter for high-power white LED: transparent Ce3+:YAG phosphor-in-glass,” Laser Photonics Rev. 8(1), 158–164 (2014).
[Crossref]

D. Q. Chen, Y. S. Wang, Y. L. Yu, and P. Huang, “Structure and Optical Spectroscopy of Eu-Doped Glass Ceramics Containing GdF3,” J. Phys. Chem. C 112(48), 18943–18947 (2008).
[Crossref]

Zhang, H. S.

F. W. Kang, H. S. Zhang, L. Wondraczek, X. B. Yang, Y. Zhang, D. Y. Lei, and M. Y. Peng, “Band-Gap Modulation in Single Bi3+-Doped Yttrium-Scandium-Niobium Vanadates for Color Tuning over the Whole Visible Spectrum,” Chem. Mater. 28(8), 2692–2703 (2016).
[Crossref]

Zhang, J.

Y. Liu, X. Zhang, Z. Hao, X. Wang, and J. Zhang, “Tunable full-color-emitting Ca3Sc2Si3O12:Ce3+, Mn2+ phosphor via charge compensation and energy transfer,” Chem. Commun. (Camb.) 47(38), 10677–10679 (2011).
[Crossref] [PubMed]

Zhang, Q. Y.

X. Y. Liu, H. Guo, Y. Liu, S. Ye, M. Y. Peng, and Q. Y. Zhang, “Thermal quenching and energy transfer in novel Bi3+/Mn2+co-doped white-emitting borosilicate glasses for UV LEDs,” J. Mater. Chem. C 4(13), 2506–2512 (2016).
[Crossref]

W. B. Dai, S. Ye, E. L. Li, P. Z. Zhuo, and Q. Y. Zhang, “High quality LED lamps using color-tunable Ce3+-activated yellow-green oxyfluoride solid-solution and Eu3+-doped red borate phosphors,” J. Mater. Chem. C 3(31), 8132–8141 (2015).
[Crossref]

F. W. Kang, X. B. Yang, M. Y. Peng, L. Wondraczek, Z. J. Ma, Q. Y. Zhang, and J. R. Qiu, “Red Photoluminescence from Bi3+ and the Influence of the Oxygen-Vacancy Perturbation in ScVO4:A Combined Experimental and Theoretical Study,” J. Phys. Chem. C 118(14), 7515–7522 (2014).
[Crossref]

S. Ye, F. Xiao, Y. X. Pan, Y. Y. Ma, and Q. Y. Zhang, “Phosphors in phosphor-converted white light-emitting diodes: Recent advances in materials, techniques and properties,” Mater. Sci. Eng. Rep. 71(1), 1–34 (2010).
[Crossref]

Zhang, R.

R. Zhang, H. Lin, Y. L. Yu, D. Q. Chen, J. Xu, and Y. S. Wang, “A new-generation color converter for high-power white LED: transparent Ce3+:YAG phosphor-in-glass,” Laser Photonics Rev. 8(1), 158–164 (2014).
[Crossref]

Zhang, X.

X. Zhang, L. Huang, F. Pan, M. Wu, J. Wang, Y. Chen, and Q. Su, “Highly thermally stable single-component white-emitting silicate glass for organic-resin-free white-light-emitting diodes,” ACS Appl. Mater. Interfaces 6(4), 2709–2717 (2014).
[Crossref] [PubMed]

Y. Liu, X. Zhang, Z. Hao, X. Wang, and J. Zhang, “Tunable full-color-emitting Ca3Sc2Si3O12:Ce3+, Mn2+ phosphor via charge compensation and energy transfer,” Chem. Commun. (Camb.) 47(38), 10677–10679 (2011).
[Crossref] [PubMed]

Zhang, Y.

F. W. Kang, H. S. Zhang, L. Wondraczek, X. B. Yang, Y. Zhang, D. Y. Lei, and M. Y. Peng, “Band-Gap Modulation in Single Bi3+-Doped Yttrium-Scandium-Niobium Vanadates for Color Tuning over the Whole Visible Spectrum,” Chem. Mater. 28(8), 2692–2703 (2016).
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F. Kang, Y. Zhang, and M. Peng, “Controlling the energy transfer via multi luminescent centers to achieve white light/tunable emissions in a single-phased X2-type Y2SiO5:Eu3+, Bi3+ phosphor for ultraviolet converted LEDs,” Inorg. Chem. 54(4), 1462–1473 (2015).
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Figures (7)

Fig. 1
Fig. 1 UV-vis transmission spectra of the Host, GB1.0, GBEx (x = 0.3, 1.0) and GE0.3 samples.
Fig. 2
Fig. 2 Excitation and emission spectra of (a) GB1.0, (b) GE0.3 and GBE0.3 samples.
Fig. 3
Fig. 3 (a) Emission (λex = 345 nm), (b) Excitation (λem = 480 nm) spectra of the GB1.0 and GBEx (x = 0.1, 0.3, 0.5, 1.0, 2.0, 2.5, 3.5) samples. The inset of (b) shows the excitation spectra (λem = 612 nm). (c) Luminescence decay curves of GB1.0 and GBEx samples (λex = 345 nm, λem = 480 nm). (d) CIE chromaticity coordinates and luminescence photos corresponding to the emission of glass samples.
Fig. 4
Fig. 4 Dependence of ( I 0 /I ) values on (a) C6/3, (b) C8/3 and (c) C10/3 in GBEx (x = 0.3, 0.5, 1.0, 2.0, 2.5) samples. Correlation efficiencies are 99.66, 97.70 and 94.60% for the fittings to Eq. (5), respectively.
Fig. 5
Fig. 5 Energy level scheme of Bi3+ and Eu3+ ions as well as the possible ET process
Fig. 6
Fig. 6 (a) Temperature-dependent emission spectra of the GBE0.5 sample (λex = 345 nm). (b) Relative integrated emission intensity versus temperature upon excitation at 345 nm. (c) Plot of ln(I0/IT −1) versus 1/kT and the linear fit of the data through Eq. (6).
Fig. 7
Fig. 7 Chromaticity shift of the GBE0.5 sample (λex = 345 nm) as a function of temperature from 298 to 573 K. The inset shows the CIE chromaticity coordinates at different temperatures.

Tables (2)

Tables Icon

Table 1 Density, refractive index, and indirect optical band gap of glasses samples.

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Table 2 Lifetimes (λex = 345 nm, λem = 480 nm), ET efficiency η T , and CIE chromaticity coordinates of glasses samples.

Equations (7)

Equations on this page are rendered with MathJax. Learn more.

αhv=B (hν E g ) n
I(t)= A 1 exp(t/ τ 1 )+ A 2 exp(t/ τ 2 )
τ=( A 1 τ 1 2 + A 2 τ 2 2 )/( A 1 τ 1 + A 2 τ 2 )
η T =1 τ s / τ s0
η 0 η C n/3
I T = I 0 1+cexp( E a kT )
ΔE= ( u t u 0 ) 2 + ( v t v 0 ) 2 + ( w t w 0 ) 2

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