Abstract

We firstly obtained organic N-benzyl-2-methyl-4-nitroaniline (BNA) single crystals using solution growth method. The crystal quality obtained by solution growth method was much better than that of crystals grown by the Bridgman method. Furthermore, using difference frequency generation (DFG) in solution-grown BNA, we generated ultra-wideband tunable THz radiation.

© 2012 OSA

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    [CrossRef]
  21. K. Miyamoto, H. Minamide, M. Fujiwara, H. Hashimoto, and H. Ito, “Widely tunable terahertz-wave generation using an N-benzyl-2-methyl-4-nitroaniline crystal,” Opt. Lett.33(3), 252–254 (2008).
    [CrossRef] [PubMed]
  22. K. Miyamoto, S. Ohno, M. Fujiwara, H. Minamide, H. Hashimoto, and H. Ito, “Optimized terahertz-wave generation using BNA-DFG,” Opt. Express17(17), 14832–14838 (2009).
    [CrossRef] [PubMed]
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2010 (1)

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

2009 (3)

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

S. Ohno, A. Hamano, K. Miyamoto, C. Suzuki, and H. Ito, “Surface mapping of carrier density in a GaN wafer using a frequency-agile THz source,” J. Eur. Opt. Soc. Rapid Publ.4, 09012 (2009).
[CrossRef]

K. Miyamoto, S. Ohno, M. Fujiwara, H. Minamide, H. Hashimoto, and H. Ito, “Optimized terahertz-wave generation using BNA-DFG,” Opt. Express17(17), 14832–14838 (2009).
[CrossRef] [PubMed]

2008 (2)

K. Miyamoto, H. Minamide, M. Fujiwara, H. Hashimoto, and H. Ito, “Widely tunable terahertz-wave generation using an N-benzyl-2-methyl-4-nitroaniline crystal,” Opt. Lett.33(3), 252–254 (2008).
[CrossRef] [PubMed]

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

2007 (2)

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

2006 (2)

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

2004 (1)

B. S. Williams, S. Kumar, Q. Hu, and J. L. Reno, “Resonant-phonon terahertz quantum cascade laser at 2.1 THz (≃141 µm),” Electron. Lett.40(7), 431–433 (2004).
[CrossRef]

2001 (1)

K. Kawase, J. Shikata, and H. Ito, “Terahertz parametric source,” J. Phys. D Appl. Phys.34, R1–R14 (2001).

2000 (1)

T. Taniuchi, J. Shikata, and H. Ito, “Tunable terahertz-wave generation in DAST crystal with dual-wavelength KTP optical parametric oscillator,” Electron. Lett.36(16), 1414–1416 (2000).
[CrossRef]

1999 (1)

1997 (1)

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

1984 (1)

D. H. Auston, K. P. Cheung, and P. R. Smith, “Picosecond photoconducting Hertzian dipoles,” Appl. Phys. Lett.45(3), 284–286 (1984).
[CrossRef]

1969 (1)

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Agusu, L.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Aleshkin, V. Ya.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Antonov, A. A.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Aoshima, S.

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

Aoshima, S.-I.

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Auston, D. H.

D. H. Auston, K. P. Cheung, and P. R. Smith, “Picosecond photoconducting Hertzian dipoles,” Appl. Phys. Lett.45(3), 284–286 (1984).
[CrossRef]

Cheung, K. P.

D. H. Auston, K. P. Cheung, and P. R. Smith, “Picosecond photoconducting Hertzian dipoles,” Appl. Phys. Lett.45(3), 284–286 (1984).
[CrossRef]

Cogdell, R. J.

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

Dubinov, A. A.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Fujii, A.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Fujimura, H.

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Fujiwara, M.

K. Miyamoto, S. Ohno, M. Fujiwara, H. Minamide, H. Hashimoto, and H. Ito, “Optimized terahertz-wave generation using BNA-DFG,” Opt. Express17(17), 14832–14838 (2009).
[CrossRef] [PubMed]

K. Miyamoto, H. Minamide, M. Fujiwara, H. Hashimoto, and H. Ito, “Widely tunable terahertz-wave generation using an N-benzyl-2-methyl-4-nitroaniline crystal,” Opt. Lett.33(3), 252–254 (2008).
[CrossRef] [PubMed]

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Gall, A.

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Gaponov, S. V.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Hamano, A.

S. Ohno, A. Hamano, K. Miyamoto, C. Suzuki, and H. Ito, “Surface mapping of carrier density in a GaN wafer using a frequency-agile THz source,” J. Eur. Opt. Soc. Rapid Publ.4, 09012 (2009).
[CrossRef]

Hashimoto, H.

K. Miyamoto, S. Ohno, M. Fujiwara, H. Minamide, H. Hashimoto, and H. Ito, “Optimized terahertz-wave generation using BNA-DFG,” Opt. Express17(17), 14832–14838 (2009).
[CrossRef] [PubMed]

K. Miyamoto, H. Minamide, M. Fujiwara, H. Hashimoto, and H. Ito, “Widely tunable terahertz-wave generation using an N-benzyl-2-methyl-4-nitroaniline crystal,” Opt. Lett.33(3), 252–254 (2008).
[CrossRef] [PubMed]

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Hu, Q.

B. S. Williams, S. Kumar, Q. Hu, and J. L. Reno, “Resonant-phonon terahertz quantum cascade laser at 2.1 THz (≃141 µm),” Electron. Lett.40(7), 431–433 (2004).
[CrossRef]

Idehara, T.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Ito, H.

K. Miyamoto, S. Ohno, M. Fujiwara, H. Minamide, H. Hashimoto, and H. Ito, “Optimized terahertz-wave generation using BNA-DFG,” Opt. Express17(17), 14832–14838 (2009).
[CrossRef] [PubMed]

S. Ohno, A. Hamano, K. Miyamoto, C. Suzuki, and H. Ito, “Surface mapping of carrier density in a GaN wafer using a frequency-agile THz source,” J. Eur. Opt. Soc. Rapid Publ.4, 09012 (2009).
[CrossRef]

K. Miyamoto, H. Minamide, M. Fujiwara, H. Hashimoto, and H. Ito, “Widely tunable terahertz-wave generation using an N-benzyl-2-methyl-4-nitroaniline crystal,” Opt. Lett.33(3), 252–254 (2008).
[CrossRef] [PubMed]

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

K. Kawase, J. Shikata, and H. Ito, “Terahertz parametric source,” J. Phys. D Appl. Phys.34, R1–R14 (2001).

T. Taniuchi, J. Shikata, and H. Ito, “Tunable terahertz-wave generation in DAST crystal with dual-wavelength KTP optical parametric oscillator,” Electron. Lett.36(16), 1414–1416 (2000).
[CrossRef]

K. Kawase, M. Mizuno, S. Sohma, H. Takahashi, T. Taniuchi, Y. Urata, S. Wada, H. Tashiro, and H. Ito, “Difference-frequency terahertz-wave generation from 4-dimethylamino-N-methyl-4-stilbazolium-tosylate by use of an electronically tuned Ti:sapphire laser,” Opt. Lett.24(15), 1065–1067 (1999).
[CrossRef] [PubMed]

Johnson, B. C.

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Kawase, K.

Kawayama, I.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Kitaoka, Y.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Krasil’nik, Z. F.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Kudryavtsev, K. E.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Kumar, S.

B. S. Williams, S. Kumar, Q. Hu, and J. L. Reno, “Resonant-phonon terahertz quantum cascade laser at 2.1 THz (≃141 µm),” Electron. Lett.40(7), 431–433 (2004).
[CrossRef]

Kuroyanagi, K.

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Manuilov, V. N.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Maruyama, M.

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Matsukawa, T.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Matsushima, R.

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Minamide, H.

Miyamoto, K.

Mizuno, M.

Mori, Y.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Morioka, M.

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Nawahara, A.

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

Notake, T.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Ogasawara, S.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Ogawa, I.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Ohno, S.

K. Miyamoto, S. Ohno, M. Fujiwara, H. Minamide, H. Hashimoto, and H. Ito, “Optimized terahertz-wave generation using BNA-DFG,” Opt. Express17(17), 14832–14838 (2009).
[CrossRef] [PubMed]

S. Ohno, A. Hamano, K. Miyamoto, C. Suzuki, and H. Ito, “Surface mapping of carrier density in a GaN wafer using a frequency-agile THz source,” J. Eur. Opt. Soc. Rapid Publ.4, 09012 (2009).
[CrossRef]

Okada, S.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Okada, Y.

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Okamoto, N.

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Pantell, R. H.

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Purhoff, H. E.

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Reno, J. L.

B. S. Williams, S. Kumar, Q. Hu, and J. L. Reno, “Resonant-phonon terahertz quantum cascade laser at 2.1 THz (≃141 µm),” Electron. Lett.40(7), 431–433 (2004).
[CrossRef]

Saito, T.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Sasaki, T.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Sato, T.

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

Shikata, J.

K. Kawase, J. Shikata, and H. Ito, “Terahertz parametric source,” J. Phys. D Appl. Phys.34, R1–R14 (2001).

T. Taniuchi, J. Shikata, and H. Ito, “Tunable terahertz-wave generation in DAST crystal with dual-wavelength KTP optical parametric oscillator,” Electron. Lett.36(16), 1414–1416 (2000).
[CrossRef]

Smith, P. R.

D. H. Auston, K. P. Cheung, and P. R. Smith, “Picosecond photoconducting Hertzian dipoles,” Appl. Phys. Lett.45(3), 284–286 (1984).
[CrossRef]

Sohma, S.

Spivakov, A. G.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Sugihara, O.

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

Sugisaki, M.

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Suizu, K.

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

Sussman, S. S.

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Suzuki, C.

S. Ohno, A. Hamano, K. Miyamoto, C. Suzuki, and H. Ito, “Surface mapping of carrier density in a GaN wafer using a frequency-agile THz source,” J. Eur. Opt. Soc. Rapid Publ.4, 09012 (2009).
[CrossRef]

Takahashi, H.

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

K. Kawase, M. Mizuno, S. Sohma, H. Takahashi, T. Taniuchi, Y. Urata, S. Wada, H. Tashiro, and H. Ito, “Difference-frequency terahertz-wave generation from 4-dimethylamino-N-methyl-4-stilbazolium-tosylate by use of an electronically tuned Ti:sapphire laser,” Opt. Lett.24(15), 1065–1067 (1999).
[CrossRef] [PubMed]

Takahashi, Y.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Takemoto, Y.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Takeya, K.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Taniuchi, T.

Tashiro, H.

Tatematsu, Y.

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Tonouchi, M.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Tsuchiya, Y.

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

Urata, Y.

Wada, S.

Williams, B. S.

B. S. Williams, S. Kumar, Q. Hu, and J. L. Reno, “Resonant-phonon terahertz quantum cascade laser at 2.1 THz (≃141 µm),” Electron. Lett.40(7), 431–433 (2004).
[CrossRef]

Yablonskii, A. N.

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Yamashita, T.

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

Yanagi, K.

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

Yarborough, J. M.

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Yoshimura, M.

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Appl. Phys. Lett. (2)

D. H. Auston, K. P. Cheung, and P. R. Smith, “Picosecond photoconducting Hertzian dipoles,” Appl. Phys. Lett.45(3), 284–286 (1984).
[CrossRef]

J. M. Yarborough, S. S. Sussman, H. E. Purhoff, R. H. Pantell, and B. C. Johnson, “Efficient tunable optical emission from LiNbO3 without a resonator,” Appl. Phys. Lett.15(3), 102–105 (1969).
[CrossRef]

Electron. Lett. (2)

B. S. Williams, S. Kumar, Q. Hu, and J. L. Reno, “Resonant-phonon terahertz quantum cascade laser at 2.1 THz (≃141 µm),” Electron. Lett.40(7), 431–433 (2004).
[CrossRef]

T. Taniuchi, J. Shikata, and H. Ito, “Tunable terahertz-wave generation in DAST crystal with dual-wavelength KTP optical parametric oscillator,” Electron. Lett.36(16), 1414–1416 (2000).
[CrossRef]

J. Eur. Opt. Soc. Rapid Publ. (1)

S. Ohno, A. Hamano, K. Miyamoto, C. Suzuki, and H. Ito, “Surface mapping of carrier density in a GaN wafer using a frequency-agile THz source,” J. Eur. Opt. Soc. Rapid Publ.4, 09012 (2009).
[CrossRef]

J. Phys. D Appl. Phys. (1)

K. Kawase, J. Shikata, and H. Ito, “Terahertz parametric source,” J. Phys. D Appl. Phys.34, R1–R14 (2001).

JETP Lett. (1)

V. Ya. Aleshkin, A. A. Antonov, S. V. Gaponov, A. A. Dubinov, Z. F. Krasil’nik, K. E. Kudryavtsev, A. G. Spivakov, and A. N. Yablonskii, “Tunable Source of Terahertz Radiation Based on the Difference-Frequency Generation in a GaP Crystal,” JETP Lett.88(12), 787–789 (2008).
[CrossRef]

Jpn. J. Appl. Phys. (6)

H. Hashimoto, Y. Okada, H. Fujimura, M. Morioka, O. Sugihara, N. Okamoto, and R. Matsushima, “Second-Harmonic Generation from Single Crystal of N-substituted 4-Nitroanilines,” Jpn. J. Appl. Phys.36(Part 1, No. 11), 6754–6760 (1997).
[CrossRef]

H. Ito, K. Suizu, T. Yamashita, A. Nawahara, and T. Sato, “Random Frequency accessible broad tunable terahertz-wave source using phase-matched 4-Dimethylamino N-methyl 4-stibazolium tosylate crystal,” Jpn. J. Appl. Phys.46(11), 7321–7324 (2007).
[CrossRef]

K. Kuroyanagi, M. Fujiwara, H. Hashimoto, H. Takahashi, S. Aoshima, and Y. Tsuchiya, “Determination of refractive indices and absorption coefficients of highly purified N-benzyl-2-methyl-4-nitroaniline crystal in terahertz frequency region,” Jpn. J. Appl. Phys.45(29), L761–L764 (2006).
[CrossRef]

M. Fujiwara, K. Yanagi, M. Maruyama, M. Sugisaki, K. Kuroyanagi, H. Takahashi, S.-I. Aoshima, Y. Tsuchiya, A. Gall, and H. Hashimoto, “Second order nonlinear optical properties of the single crystal of N-Benzyl 2-methyl-4-nitroaniline: Anomalous enhancement of the d333 component and its possible origin,” Jpn. J. Appl. Phys.45(11), 8676–8685 (2006).
[CrossRef]

M. Fujiwara, M. Maruyama, M. Sugisaki, H. Takahashi, S. Aoshima, R. J. Cogdell, and H. Hashimoto, “Determination of the d-Tensor components of a single crystal of N-Benzyl-2-methyl-4-nitroaniline,” Jpn. J. Appl. Phys.46(4A), 1528–1530 (2007).
[CrossRef]

T. Matsukawa, M. Yoshimura, Y. Takahashi, Y. Takemoto, K. Takeya, I. Kawayama, S. Okada, M. Tonouchi, Y. Kitaoka, Y. Mori, and T. Sasaki, “Bulk Crystal Growth of Stilbazolium Derivatives for Terahertz Waves Generation,” Jpn. J. Appl. Phys.49(7), 075502 (2010).
[CrossRef]

Opt. Express (1)

Opt. Lett. (2)

Phys. Rev. Lett. (1)

T. Notake, T. Saito, Y. Tatematsu, A. Fujii, S. Ogasawara, L. Agusu, I. Ogawa, T. Idehara, and V. N. Manuilov, “Development of a novel high power sub-THz second harmonic gyrotron,” Phys. Rev. Lett.103(22), 225002 (2009).
[CrossRef] [PubMed]

Other (7)

H. Nakanishi, H. Matsuda, S. Okada, and M. Kato, “Organic and polymeric ion-complexes for nonlinear optics,” in Proc. MRS Int. Mtg. Adv. Mater. (1989), Vol. 1, pp. 97–104.

H. Ito, K. Miyamoto, and H. Minamide, “Ultra-broadband, frequency-agile THz-wave generator and its applications,” Advanced Solid-State Photonics, OSA Technical Digest Series, WD1 (2008).

X.-C. Zhang and J. Xu, Introduction to THz Wave Photonics (Springer, 2009).

http://www.ccdc.cam.ac.uk/products/csd/ .

B. E. Warren, X-ray Diffraction (Dover Publications, 1990).

K. Miyamoto, A. Nawahara, T. Yamashita, and H. Ito, “Phase-matched DAST DFG THz-wave generation using independently controllable dual wavelength light source,” Proc. of IRMMW-THz 2007 (2007), pp. 728–729.

H. E. Kartz, C. W. Dirk, M. L. Schilling, K. D. Singer, and J. E. Sohn, “Optimization of second-order nonlinear optical susceptibilities in organic materials,” Mat. Res. Soc. Symp. Proc. (1988), Vol. 109, p. 127.

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Figures (5)

Fig. 1
Fig. 1

(a) BNA polycrystal ingredients highly purified by several recrystallization process in ethanol, (b) BNA seed crystals for ethanol solution growth, (c) BNA crystals under the growth in ethanol solution, (d) typical BNA single crystal grown from ethanol solution.

Fig. 2
Fig. 2

(a) X-ray diffraction result of an ω-2θ measurement on (010) plane. (b) Experimentally assigned mirror index k as a function of (2/λ)sinθ. Data are well fitted with slope of b which indicates lattice parameter of b-axis 21.4 Å.

Fig. 3
Fig. 3

(a) Comparison of rocking curve of BNA grown from Brdigman and ethanol solution method. (b) Comparison of peak power density where crystal damage was observed.

Fig. 4
Fig. 4

Calculation result of prospective THz-wave intensity via BNA-DFG under the consideration of perfect phase matching and absorption effect.

Fig. 5
Fig. 5

THz-wave output spectrum via DFG from BNA grown from ethanol solution. Here, two pump wavelengths were independently controlled properly to generate highest power at each THz frequency.

Tables (1)

Tables Icon

Table 1 Comparison of Solubility of Several Organic Solvents at R.T. and 60°C for BNA Ingredient

Equations (1)

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k=b 2 λ sinθ.

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