Abstract

This article reviews the material properties that enable maximum optical response. We highlight theoretical results that enable shape-independent quantification of material “figures of merit,” ranging from classical sum rules to more recent single-frequency scattering bounds. A key delineation at optical frequencies is between polaritonic materials that support highly subwavelength resonances and dielectric materials that can have vanishingly small loss rates. We discuss the key metrics that enable comparisons both within these material classes and between them. We discuss analogous metrics for 2D materials, and point to applications for which rigorous comparison can be made between bulk- and 2D-material approaches. The various results highlight the synergy between materials discovery and theoretical nanophotonic bounds, and point to opportunities in achieving new extremes in light–matter interactions.

© 2020 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2019 (7)

T. Phan, D. Sell, E. W. Wang, S. Doshay, K. Edee, J. Yang, and J. A. Fan, “High-efficiency, large-area, topology-optimized metasurfaces,” Light: Sci. Appl. 8(1), 48 (2019).
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J. Michon, M. Benzaouia, W. Yao, O. D. Miller, and S. G. Johnson, “Limits to surface-enhanced Raman scattering near arbitrary-shape scatterers,” Opt. Express 27(24), 35189 (2019).
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J. B. Khurgin, “Relative merits of phononics vs. plasmonics: the energy balance approach,” Nanophotonics 7(1), 305–316 (2018).
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W. T. Hsieh, P. C. Wu, J. B. Khurgin, D. P. Tsai, N. Liu, and G. Sun, “Comparative Analysis of Metals and Alternative Infrared Plasmonic Materials,” ACS Photonics 5(7), 2541–2548 (2018).
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Y. Yang, A. Massuda, C. Roques-Carmes, S. E. Kooi, T. Christensen, S. G. Johnson, J. D. Joannopoulos, O. D. Miller, I. Kaminer, and M. Soljačić, “Maximal spontaneous photon emission and energy loss from free electrons,” Nat. Phys. 14(9), 894–899 (2018).
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A. Vaskin, J. Bohn, K. E. Chong, T. Bucher, M. Zilk, D.-Y. Choi, D. N. Neshev, Y. S. Kivshar, T. Pertsch, and I. Staude, “Directional and Spectral Shaping of Light Emission with Mie-Resonant Silicon Nanoantenna Arrays,” ACS Photonics 5(4), 1359–1364 (2018).
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M. Liu and D.-Y. Choi, “Extreme Huygens’ Metasurfaces Based on Quasi-Bound States in the Continuum,” Nano Lett. 18(12), 8062–8069 (2018).
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D. G. Baranov, D. A. Zuev, S. I. Lepeshov, O. V. Kotov, A. E. Krasnok, A. B. Evlyukhin, and B. N. Chichkov, “All-dielectric nanophotonics: the quest for better materials and fabrication techniques,” Optica 4(7), 814 (2017).
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H. Choi, M. Heuck, and D. Englund, “Self-Similar Nanocavity Design with Ultrasmall Mode Volume for Single-Photon Nonlinearities,” Phys. Rev. Lett. 118(22), 223605 (2017).
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C. Tan, X. Cao, X.-J. Wu, Q. He, J. Yang, X. Zhang, J. Chen, W. Zhao, S. Han, G.-H. Nam, M. Sindoro, and H. Zhang, “Recent advances in ultrathin two-dimensional nanomaterials,” Chem. Rev. 117(9), 6225–6331 (2017).
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T. Low, A. Chaves, J. D. Caldwell, A. Kumar, N. X. Fang, P. Avouris, T. F. Heinz, F. Guinea, L. Martin-Moreno, and F. Koppens, “Polaritons in layered two-dimensional materials,” Nat. Mater. 16(2), 182–194 (2017).
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O. D. Miller, O. Ilic, T. Christensen, M. T. Reid, H. A. Atwater, J. D. Joannopoulos, M. Soljačić, and S. G. Johnson, “Limits to the Optical Response of Graphene and Two-Dimensional Materials,” Nano Lett. 17(9), 5408–5415 (2017).
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Y. Yang, O. D. Miller, T. Christensen, J. D. Joannopoulos, and M. Soljačić, “Low-Loss Plasmonic Dielectric Nanoresonators,” Nano Lett. 17(5), 3238–3245 (2017).
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I. Liberal and N. Engheta, “Near-zero refractive index photonics,” Nat. Photonics 11(3), 149–158 (2017).
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2016 (12)

M. Z. Alam, I. De Leon, and R. W. Boyd, “Large optical nonlinearity of indium tin oxide in its epsilon-near-zero region,” Science 352(6287), 795–797 (2016).
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L. Caspani, R. P. M. Kaipurath, M. Clerici, M. Ferrera, T. Roger, J. Kim, N. Kinsey, M. Pietrzyk, A. Di Falco, V. M. Shalaev, A. Boltasseva, and D. Faccio, “Enhanced Nonlinear Refractive Index in ɛ-Near-Zero Materials,” Phys. Rev. Lett. 116(23), 233901 (2016).
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A. I. Kuznetsov, A. E. Miroshnichenko, M. L. Brongersma, Y. S. Kivshar, and B. Luk’yanchuk, “Optically resonant dielectric nanostructures,” Science 354(6314), aag2472 (2016).
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S. Jahani and Z. Jacob, “All-dielectric metamaterials,” Nat. Nanotechnol. 11(1), 23–36 (2016).
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S. Hu and S. M. Weiss, “Design of Photonic Crystal Cavities for Extreme Light Concentration,” ACS Photonics 3(9), 1647–1653 (2016).
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M. Khorasaninejad, A. Y. Zhu, C. Roques-Carmes, W. T. Chen, J. Oh, I. Mishra, R. C. Devlin, and F. Capasso, “Polarization-insensitive metalenses at visible wavelengths,” Nano Lett. 16(11), 7229–7234 (2016).
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E. Arbabi, A. Arbabi, S. M. Kamali, Y. Horie, and A. Faraon, “Multiwavelength metasurfaces through spatial multiplexing,” Sci. Rep. 6(1), 32803 (2016).
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2015 (30)

S. Tripathy, “Refractive indices of semiconductors from energy gaps,” Opt. Mater. 46, 240–246 (2015).
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F. Aieta, M. A. Kats, P. Genevet, and F. Capasso, “Multiwavelength achromatic metasurfaces by dispersive phase compensation,” Science 347(6228), 1342–1345 (2015).
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M. Khorasaninejad, F. Aieta, P. Kanhaiya, M. A. Kats, P. Genevet, D. Rousso, and F. Capasso, “Achromatic metasurface lens at telecommunication wavelengths,” Nano Lett. 15(8), 5358–5362 (2015).
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K. Luke, Y. Okawachi, M. R. E. Lamont, A. L. Gaeta, and M. Lipson, “Broadband mid-infrared frequency comb generation in a Si3N4 microresonator,” Opt. Lett. 40(21), 4823 (2015).
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Y. Yu, Y. Chen, H. Hu, W. Xue, K. Yvind, and J. Mork, “Nonreciprocal transmission in a nonlinear photonic-crystal Fano structure with broken symmetry,” Laser Photonics Rev. 9(2), 241–247 (2015).
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Y. Shi, Z. Yu, and S. Fan, “Limitations of nonlinear optical isolators due to dynamic reciprocity,” Nat. Photonics 9(6), 388–392 (2015).
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M. Decker, I. Staude, M. Falkner, J. Dominguez, D. N. Neshev, I. Brener, T. Pertsch, and Y. S. Kivshar, “High-Efficiency Dielectric Huygens’ Surfaces,” Adv. Opt. Mater. 3, 813–820 (2015).
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P. Moitra, B. A. Slovick, W. Li, I. I. Kravchencko, D. P. Briggs, S. Krishnamurthy, and J. Valentine, “Large-Scale All-Dielectric Metamaterial Perfect Reflectors,” ACS Photonics 2(6), 692–698 (2015).
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S. Raza, S. I. Bozhevolnyi, M. Wubs, and N. Asger Mortensen, “Nonlocal optical response in metallic nanostructures,” J. Phys.: Condens. Matter 27(18), 183204 (2015).
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D. Correas-Serrano, J. S. Gomez-Diaz, M. Tymchenko, and A. Alù, “Nonlocal response of hyperbolic metasurfaces,” Opt. Express 23(23), 29434 (2015).
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R. Faggiani, J. Yang, and P. Lalanne, “Quenching, plasmonic and radiative decays in nanogap emitting devices,” ACS Photonics 2(12), 1739–1744 (2015).
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V. Pacheco-Pe na, V. Torres, B. Orazbayev, M. Beruete, M. Navarro-Cía, M. Sorolla, and N. Engheta, “Mechanical 144 GHz beam steering with all-metallic epsilon-near-zero lens antenna,” Appl. Phys. Lett. 105(24), 243503 (2014).
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2013 (18)

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J. Kim, G. V. Naik, N. K. Emani, U. Guler, and A. Boltasseva, “Plasmonic Resonances in Nanostructured Transparent Conducting Oxide Films,” IEEE J. Sel. Top. Quantum Electron. 19(5), 1–7 (2013).
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2012 (19)

G. V. Naik, J. L. Schroeder, X. Ni, A. V. Kildishev, T. D. Sands, and A. Boltasseva, “Titanium nitride as a plasmonic material for visible and near-infrared wavelengths,” Opt. Mater. Express 2(4), 478 (2012).
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C. Ciraci, R. T. Hill, J. J. Mock, Y. Urzhumov, A. I. Fernandez-Dominguez, S. A. Maier, J. B. Pendry, A. Chilkoti, and D. R. Smith, “Probing the Ultimate Limits of Plasmonic Enhancement,” Science 337(6098), 1072–1074 (2012).
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K. X. Wang, Z. Yu, V. Liu, Y. Cui, and S. Fan, “Absorption Enhancement in Ultrathin Crystalline Silicon Solar Cells with Antireflection and Light-Trapping Nanocone Gratings,” Nano Lett. 12(3), 1616–1619 (2012).
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2011 (8)

J. A. Mason, S. Smith, and D. Wasserman, “Strong absorption and selective thermal emission from a midinfrared metamaterial,” Appl. Phys. Lett. 98(24), 241105 (2011).
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X. Liu, T. Tyler, T. Starr, A. F. Starr, N. M. Jokerst, and W. J. Padilla, “Taming the Blackbody with Infrared Metamaterials as Selective Thermal Emitters,” Phys. Rev. Lett. 107(4), 045901 (2011).
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A. Gonzalez-Tudela, D. Martin-Cano, E. Moreno, L. Martin-Moreno, C. Tejedor, and F. J. Garcia-Vidal, “Entanglement of Two Qubits Mediated by One-Dimensional Plasmonic Waveguides,” Phys. Rev. Lett. 106(2), 020501 (2011).
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2010 (19)

M. C. Gather, K. Meerholz, N. Danz, and K. Leosson, “Net optical gain in a plasmonic waveguide embedded in a fluorescent polymer,” Nat. Photonics 4(7), 457–461 (2010).
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R. Esteban, T. Teperik, and J.-J. Greffet, “Optical patch antennas for single photon emission using surface plasmon resonances,” Phys. Rev. Lett. 104(2), 026802 (2010).
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