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Spectral asymmetries in the resonance fluorescence of two-level systems under pulsed excitation

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Abstract

We present an open-system master equation study of the coherent and incoherent resonance fluorescence spectrum from a two-level quantum system under coherent pulsed excitation. Several pronounced features that differ from the fluorescence under a constant drive are highlighted, including a multi-peak structure and a pronounced off-resonant spectral asymmetry, in stark contrast to the conventional symmetrical Mollow triplet. We also study semiconductor quantum dot systems using a polaron master equation and show how the key features of dynamic resonance fluorescence change with electron–acoustic-phonon coupling.

© 2018 Optical Society of America

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