Abstract

We introduce an innovative high-sensitivity broadband pump-probe spectroscopy system, based on Fourier-transform detection, operating at 20-MHz modulation frequency. A common-mode interferometer employing birefringent wedges creates two phase-locked delayed replicas of the broadband probe pulse, interfering at a single photodetector. A single-channel lock-in amplifier demodulates the interferogram, whose Fourier transform provides the differential transmission spectrum. Our approach combines broad spectral coverage with high sensitivity, due to high-frequency modulation and detection. We demonstrate its performances by measuring two-dimensional differential transmission maps of a carbon nanotubes sample, simultaneously acquiring the signal over the entire 950–1350 nm range with 2.7·106  rms noise over 1.5 s integration time.

© 2016 Optical Society of America

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References

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  5. M. Bradler and E. Riedle, J. Opt. Soc. Am. B 31, 1465 (2014).
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    [Crossref]
  7. A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
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2016 (2)

C.-W. Luo, Y.-T. Wang, A. Yabushita, and T. Kobayashi, Optica 3, 82 (2016).
[Crossref]

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

2015 (2)

2014 (3)

2012 (1)

2011 (2)

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

2010 (1)

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

2009 (2)

U. Megerle, I. Pugliesi, C. Schriever, C. F. Sailer, and E. Riedle, Appl. Phys. B 96, 215 (2009).
[Crossref]

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

2007 (1)

D. Polli, L. Lüer, and G. Cerullo, Rev. Sci. Instrum. 78, 103108 (2007).
[Crossref]

2004 (2)

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

T. Polívka and V. Sundström, Chem. Rev. 104, 2021 (2004).
[Crossref]

2003 (3)

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

M. Raytchev, E. Pandurski, I. Buchvarov, C. Modrakowski, and T. Fiebig, J. Phys. Chem. A 107, 4592 (2003).
[Crossref]

S. Bourquin, R. P. Prasankumar, F. X. Kärtner, J. G. Fujimoto, T. Lasser, and R. P. Salathé, Opt. Lett. 28, 1588 (2003).
[Crossref]

2000 (1)

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Adachi, S.

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

Bachelier, G.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Baida, H.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Bourquin, S.

Bradler, M.

Brida, D.

Brixner, T.

Buchvarov, I.

M. Raytchev, E. Pandurski, I. Buchvarov, C. Modrakowski, and T. Fiebig, J. Phys. Chem. A 107, 4592 (2003).
[Crossref]

Capes, L.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Cassabois, G.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Cassinerio, M.

Cerullo, G.

Christofilos, D.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Ciardi, G.

Coluccelli, N.

Crisafi, F.

Crochet, J.

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

Crut, A.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Del Fatti, N.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Delalande, C.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Dobryakov, A. L.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Eck, R.

Eliash, T.

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

Ernsting, N. P.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Fiebig, T.

M. Raytchev, E. Pandurski, I. Buchvarov, C. Modrakowski, and T. Fiebig, J. Phys. Chem. A 107, 4592 (2003).
[Crossref]

Figueroa del Valle, D. G.

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

Fujimoto, J. G.

Galzerano, G.

Glanzmann, L. N.

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

Hertel, T.

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

Hoseinkhani, S.

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

Ishii, N.

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

Jost, O.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Jung, K.-H.

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

Kanal, F.

Karolczak, J.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Kärtner, F. X.

Keiber, S.

Kimura, T.

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

Kobayashi, T.

C.-W. Luo, Y.-T. Wang, A. Yabushita, and T. Kobayashi, Optica 3, 82 (2016).
[Crossref]

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

Kovalenko, S. A.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Kubicki, J.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Kukura, P.

F. M. Liebel, C. Schnedermann, T. Wende, and P. Kukura, J. Phys. Chem. 119, 9506 (2015).
[Crossref]

Kumar, V.

Lange, J.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Lanzani, G.

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

Lasser, T.

Lauret, J.-S.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Liebel, F. M.

F. M. Liebel, C. Schnedermann, T. Wende, and P. Kukura, J. Phys. Chem. 119, 9506 (2015).
[Crossref]

Lorenc, M.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Lüer, L.

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

D. Polli, L. Lüer, and G. Cerullo, Rev. Sci. Instrum. 78, 103108 (2007).
[Crossref]

Luo, C.-W.

Maciejewski, A.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Maioli, P.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Manzoni, C.

Marangoni, M.

Matsuda, H.

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

Matysiak, M.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Megerle, U.

U. Megerle, I. Pugliesi, C. Schriever, C. F. Sailer, and E. Riedle, Appl. Phys. B 96, 215 (2009).
[Crossref]

Modrakowski, C.

M. Raytchev, E. Pandurski, I. Buchvarov, C. Modrakowski, and T. Fiebig, J. Phys. Chem. A 107, 4592 (2003).
[Crossref]

Mongin, D.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Mowbray, D. J.

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

Mukamel, S.

S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University, 1995).

Müller, A.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Naskrecki, R.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Oriana, A.

A. Oriana, J. Réhault, F. Preda, D. Polli, and G. Cerullo, J. Opt. Soc. Am. A (submitted).

Pandurski, E.

M. Raytchev, E. Pandurski, I. Buchvarov, C. Modrakowski, and T. Fiebig, J. Phys. Chem. A 107, 4592 (2003).
[Crossref]

Pérez-Lustres, J. L.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Polívka, T.

T. Polívka and V. Sundström, Chem. Rev. 104, 2021 (2004).
[Crossref]

Polli, D.

J. Réhault, F. Crisafi, V. Kumar, G. Ciardi, M. Marangoni, G. Cerullo, and D. Polli, Opt. Express 23, 25235 (2015).
[Crossref]

L. Lüer, S. Hoseinkhani, D. Polli, J. Crochet, T. Hertel, and G. Lanzani, Nat. Phys. 5, 54 (2009).
[Crossref]

D. Polli, L. Lüer, and G. Cerullo, Rev. Sci. Instrum. 78, 103108 (2007).
[Crossref]

A. Oriana, J. Réhault, F. Preda, D. Polli, and G. Cerullo, J. Opt. Soc. Am. A (submitted).

Prasankumar, R. P.

Preda, F.

A. Oriana, J. Réhault, F. Preda, D. Polli, and G. Cerullo, J. Opt. Soc. Am. A (submitted).

Pugliesi, I.

U. Megerle, I. Pugliesi, C. Schriever, C. F. Sailer, and E. Riedle, Appl. Phys. B 96, 215 (2009).
[Crossref]

Raytchev, M.

M. Raytchev, E. Pandurski, I. Buchvarov, C. Modrakowski, and T. Fiebig, J. Phys. Chem. A 107, 4592 (2003).
[Crossref]

Réhault, J.

J. Réhault, F. Crisafi, V. Kumar, G. Ciardi, M. Marangoni, G. Cerullo, and D. Polli, Opt. Express 23, 25235 (2015).
[Crossref]

A. Oriana, J. Réhault, F. Preda, D. Polli, and G. Cerullo, J. Opt. Soc. Am. A (submitted).

Riedle, E.

M. Bradler and E. Riedle, J. Opt. Soc. Am. B 31, 1465 (2014).
[Crossref]

U. Megerle, I. Pugliesi, C. Schriever, C. F. Sailer, and E. Riedle, Appl. Phys. B 96, 215 (2009).
[Crossref]

Roussignol, Ph.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Rozin, R.

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

Rubio, A.

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

Ruhman, S.

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

Sailer, C. F.

U. Megerle, I. Pugliesi, C. Schriever, C. F. Sailer, and E. Riedle, Appl. Phys. B 96, 215 (2009).
[Crossref]

Salathé, R. P.

Schnedermann, C.

F. M. Liebel, C. Schnedermann, T. Wende, and P. Kukura, J. Phys. Chem. 119, 9506 (2015).
[Crossref]

Schriever, C.

U. Megerle, I. Pugliesi, C. Schriever, C. F. Sailer, and E. Riedle, Appl. Phys. B 96, 215 (2009).
[Crossref]

Scotognella, F.

L. N. Glanzmann, D. J. Mowbray, D. G. Figueroa del Valle, F. Scotognella, G. Lanzani, and A. Rubio, J. Phys. Chem. C 120, 1926 (2016).
[Crossref]

Sheves, M.

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

Smith, B. C.

B. C. Smith, Fundamentals of Fourier Transform Infrared Spectroscopy (CRC Press, 2011).

Sundström, V.

T. Polívka and V. Sundström, Chem. Rev. 104, 2021 (2004).
[Crossref]

Szymanski, M.

A. Maciejewski, R. Naskrecki, M. Lorenc, M. Ziolek, J. Karolczak, J. Kubicki, M. Matysiak, and M. Szymanski, J. Mol. Struct. 555, 1 (2000).
[Crossref]

Tokunaga, E.

N. Ishii, E. Tokunaga, S. Adachi, T. Kimura, H. Matsuda, and T. Kobayashi, Phys. Rev. A 70, 023811 (2004).
[Crossref]

Vallée, F.

H. Baida, D. Mongin, D. Christofilos, G. Bachelier, A. Crut, P. Maioli, N. Del Fatti, and F. Vallée, Phys. Rev. Lett. 107, 057402 (2011).
[Crossref]

Voisin, C.

J.-S. Lauret, C. Voisin, G. Cassabois, C. Delalande, Ph. Roussignol, O. Jost, and L. Capes, Phys. Rev. Lett. 90, 057404 (2003).
[Crossref]

Wand, A.

A. Wand, R. Rozin, T. Eliash, K.-H. Jung, M. Sheves, and S. Ruhman, J. Am. Chem. Soc. 133, 20922 (2011).
[Crossref]

Wang, Y.-T.

Weigel, A.

A. L. Dobryakov, S. A. Kovalenko, A. Weigel, J. L. Pérez-Lustres, J. Lange, A. Müller, and N. P. Ernsting, Rev. Sci. Instrum. 81, 113106 (2010).
[Crossref]

Wende, T.

F. M. Liebel, C. Schnedermann, T. Wende, and P. Kukura, J. Phys. Chem. 119, 9506 (2015).
[Crossref]

Yabushita, A.

Ziolek, M.

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Figures (3)

Fig. 1.
Fig. 1. Schematic drawing of the setup. WP, Wollaston prism; BPD, balanced photodiode; ADC, analog-to-digital conversion board. The directions of the optical axis of the birefringent materials in TWINS are indicated in yellow. The blue and black arrows indicate the direction of movement of translating stages.
Fig. 2.
Fig. 2. Comparison of Δ T / T spectra collected on a β -carotene sample in solution at the same 1-ps delay using a standard OMA based on a CCD camera (squares) and the FT procedure introduced here (solid red line). Hashed area: probe spectrum.
Fig. 3.
Fig. 3. (a) Apodized linear (black line) and differential (blue line) interferograms at 100 fs delay, together with the apodization window used. (b) Two-dimensional Δ T / T ( λ pr , τ ) map for a SWNT sample. (c) Solid lines, Δ T / T spectra at selected probe delays as indicated; hashed area, probe spectrum. (d)  Δ T / T dynamics (solid lines) and corresponding fits (circles) at selected probe wavelengths (red: λ = 1065    nm ; black: λ = 1215    nm ). Inset: close-up of the signal at λ = 1215    nm for negative delays.

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