Abstract

The efficiency of third-harmonic generation in cuprous oxide was measured. Intensities followed a noncubic power law that indicates nonperturbative behavior. Polarization anisotropy of the harmonic generation was demonstrated and related to the third-order susceptibility. The results will influence the understanding of harmonic generation in centrosymmetric materials and are potentially relevant to device design and the interpretation of exciton behavior.

© 2014 Optical Society of America

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A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
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K. Yoshioka and M. Kuwata-Gonokami, New J. Phys. 14, 055024 (2012).
[CrossRef]

R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
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2011

M. Fu, H. Long, K. Wang, G. Yang, and P. Lu, Thin Solid Films 519, 6557 (2011).
[CrossRef]

2010

S. Mani, J. Jang, and J. B. Ketterson, Phys. Rev. B 82, 113203 (2010).
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S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
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T. Ideguchi, K. Yoshioka, A. Mysyrowicz, and M. Kuwata-Gonokami, Phys. Rev. Lett. 100, 233001 (2008).
[CrossRef]

2006

K. Yoshioka and M. Kuwata-Gonokami, Phys. Rev. B 73, 081202 (2006).
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Y. Sun, G. K. L. Wong, and J. B. Ketterson, Phys. Rev. B 63, 125323 (2001).
[CrossRef]

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T. Ito, H. Yamaguchi, K. Okabe, and T. Masumi, J. Mater. Sci. 33, 3555 (1998).
[CrossRef]

1997

1996

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

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J. Macklin, J. Kmetec, and C. Gordon, Phys. Rev. Lett. 70, 766 (1993).
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A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

1991

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

1990

D. Moss, E. Ghahramani, J. Sipe, and H. Van Driel, Phys. Rev. B 41, 1542 (1990).
[CrossRef]

1987

J. Sipe, D. Moss, and H. Van Driel, Phys. Rev. B 35, 1129 (1987).
[CrossRef]

1986

D. Trauernicht, J. Wolfe, and A. Mysyrowicz, Phys. Rev. B 34, 2561 (1986).
[CrossRef]

1981

G. Meredith, Phys. Rev. B 24, 5522 (1981).
[CrossRef]

1974

R. Schmidt-Whitley, M. Martinez-Clemente, and A. Revcolevschi, J. Cryst. Growth 23, 113 (1974).
[CrossRef]

1971

G. Boyd, H. Kasper, and J. McFee, IEEE J. Quantum Electron. 7, 563 (1971).
[CrossRef]

1961

P. Baumeister, Phys. Rev. 121, 359 (1961).
[CrossRef]

Agostini, P.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

Auerbach, J.

Balcou, P.

A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

Barker, C.

Baumeister, P.

P. Baumeister, Phys. Rev. 121, 359 (1961).
[CrossRef]

Blaga, C.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

Boyd, G.

G. Boyd, H. Kasper, and J. McFee, IEEE J. Quantum Electron. 7, 563 (1971).
[CrossRef]

Candel, S.

A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

Chang, K.

K. Chang, L. Frazer, J. Schwartz, J. B. Ketterson, and K. Poeppelmeier, Cryst. Growth Des. 13, 4914 (2013).
[CrossRef]

DiChiara, A.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

DiMauro, L.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

Eimerl, D.

Frazer, L.

K. Chang, L. Frazer, J. Schwartz, J. B. Ketterson, and K. Poeppelmeier, Cryst. Growth Des. 13, 4914 (2013).
[CrossRef]

L. Frazer, R. Schaller, and J. B. Ketterson, Solid State Commun. 170, 34 (2013).
[CrossRef]

Fröhlich, D.

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

Fu, M.

M. Fu, H. Long, K. Wang, G. Yang, and P. Lu, Thin Solid Films 519, 6557 (2011).
[CrossRef]

Ghahramani, E.

D. Moss, E. Ghahramani, J. Sipe, and H. Van Driel, Phys. Rev. B 41, 1542 (1990).
[CrossRef]

Ghimire, S.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

Gordon, C.

J. Macklin, J. Kmetec, and C. Gordon, Phys. Rev. Lett. 70, 766 (1993).
[CrossRef]

Goto, T.

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

Ideguchi, T.

T. Ideguchi, K. Yoshioka, A. Mysyrowicz, and M. Kuwata-Gonokami, Phys. Rev. Lett. 100, 233001 (2008).
[CrossRef]

Ito, T.

T. Ito, H. Yamaguchi, K. Okabe, and T. Masumi, J. Mater. Sci. 33, 3555 (1998).
[CrossRef]

Jang, J.

S. Mani, J. Jang, and J. B. Ketterson, Phys. Rev. B 82, 113203 (2010).
[CrossRef]

S. Mani, J. Jang, and J. B. Ketterson, Opt. Lett. 34, 2817 (2009).
[CrossRef]

Kasper, H.

G. Boyd, H. Kasper, and J. McFee, IEEE J. Quantum Electron. 7, 563 (1971).
[CrossRef]

Ketterson, J. B.

L. Frazer, R. Schaller, and J. B. Ketterson, Solid State Commun. 170, 34 (2013).
[CrossRef]

K. Chang, L. Frazer, J. Schwartz, J. B. Ketterson, and K. Poeppelmeier, Cryst. Growth Des. 13, 4914 (2013).
[CrossRef]

S. Mani, J. Jang, and J. B. Ketterson, Phys. Rev. B 82, 113203 (2010).
[CrossRef]

S. Mani, J. Jang, and J. B. Ketterson, Opt. Lett. 34, 2817 (2009).
[CrossRef]

Y. Sun, G. K. L. Wong, and J. B. Ketterson, Phys. Rev. B 63, 125323 (2001).
[CrossRef]

Kieseling, F.

R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
[CrossRef]

Kmetec, J.

J. Macklin, J. Kmetec, and C. Gordon, Phys. Rev. Lett. 70, 766 (1993).
[CrossRef]

Koyama, S.

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

Kulander, K.

A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

Kulik, A.

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

Kuroda, N.

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

Kuwata-Gonokami, M.

K. Yoshioka and M. Kuwata-Gonokami, New J. Phys. 14, 055024 (2012).
[CrossRef]

T. Ideguchi, K. Yoshioka, A. Mysyrowicz, and M. Kuwata-Gonokami, Phys. Rev. Lett. 100, 233001 (2008).
[CrossRef]

K. Yoshioka and M. Kuwata-Gonokami, Phys. Rev. B 73, 081202 (2006).
[CrossRef]

L’Huillier, A.

A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

Langer, V.

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

Liu, Y.

Y. Liu, “Excitons at high density in cuprous oxide and coupled quantum wells,” Ph.D. thesis (University of Pittsburgh, 2004).

Long, H.

M. Fu, H. Long, K. Wang, G. Yang, and P. Lu, Thin Solid Films 519, 6557 (2011).
[CrossRef]

Lu, P.

M. Fu, H. Long, K. Wang, G. Yang, and P. Lu, Thin Solid Films 519, 6557 (2011).
[CrossRef]

Macklin, J.

J. Macklin, J. Kmetec, and C. Gordon, Phys. Rev. Lett. 70, 766 (1993).
[CrossRef]

Mani, S.

S. Mani, J. Jang, and J. B. Ketterson, Phys. Rev. B 82, 113203 (2010).
[CrossRef]

S. Mani, J. Jang, and J. B. Ketterson, Opt. Lett. 34, 2817 (2009).
[CrossRef]

March, A.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

Martinez-Clemente, M.

R. Schmidt-Whitley, M. Martinez-Clemente, and A. Revcolevschi, J. Cryst. Growth 23, 113 (1974).
[CrossRef]

Masumi, T.

T. Ito, H. Yamaguchi, K. Okabe, and T. Masumi, J. Mater. Sci. 33, 3555 (1998).
[CrossRef]

McFee, J.

G. Boyd, H. Kasper, and J. McFee, IEEE J. Quantum Electron. 7, 563 (1971).
[CrossRef]

Meredith, G.

G. Meredith, Phys. Rev. B 24, 5522 (1981).
[CrossRef]

Milam, D.

Miller, T.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

Milonni, P.

Moss, D.

D. Moss, E. Ghahramani, J. Sipe, and H. Van Driel, Phys. Rev. B 41, 1542 (1990).
[CrossRef]

J. Sipe, D. Moss, and H. Van Driel, Phys. Rev. B 35, 1129 (1987).
[CrossRef]

Mysyrowicz, A.

T. Ideguchi, K. Yoshioka, A. Mysyrowicz, and M. Kuwata-Gonokami, Phys. Rev. Lett. 100, 233001 (2008).
[CrossRef]

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

D. Trauernicht, J. Wolfe, and A. Mysyrowicz, Phys. Rev. B 34, 2561 (1986).
[CrossRef]

Naka, N.

R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
[CrossRef]

Okabe, K.

T. Ito, H. Yamaguchi, K. Okabe, and T. Masumi, J. Mater. Sci. 33, 3555 (1998).
[CrossRef]

Poeppelmeier, K.

K. Chang, L. Frazer, J. Schwartz, J. B. Ketterson, and K. Poeppelmeier, Cryst. Growth Des. 13, 4914 (2013).
[CrossRef]

Power, E.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

Reis, D.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

Revcolevschi, A.

R. Schmidt-Whitley, M. Martinez-Clemente, and A. Revcolevschi, J. Cryst. Growth 23, 113 (1974).
[CrossRef]

Saito, M.

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

Schafer, K.

A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

Schaller, R.

L. Frazer, R. Schaller, and J. B. Ketterson, Solid State Commun. 170, 34 (2013).
[CrossRef]

Schmidt-Whitley, R.

R. Schmidt-Whitley, M. Martinez-Clemente, and A. Revcolevschi, J. Cryst. Growth 23, 113 (1974).
[CrossRef]

Schwartz, J.

K. Chang, L. Frazer, J. Schwartz, J. B. Ketterson, and K. Poeppelmeier, Cryst. Growth Des. 13, 4914 (2013).
[CrossRef]

Schwartz, R.

R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
[CrossRef]

Shen, M.

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

Sipe, J.

D. Moss, E. Ghahramani, J. Sipe, and H. Van Driel, Phys. Rev. B 41, 1542 (1990).
[CrossRef]

J. Sipe, D. Moss, and H. Van Driel, Phys. Rev. B 35, 1129 (1987).
[CrossRef]

Sistrunk, E.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

Stolz, H.

R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
[CrossRef]

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

Sun, Y.

Y. Sun, G. K. L. Wong, and J. B. Ketterson, Phys. Rev. B 63, 125323 (2001).
[CrossRef]

Trauernicht, D.

D. Trauernicht, J. Wolfe, and A. Mysyrowicz, Phys. Rev. B 34, 2561 (1986).
[CrossRef]

Uebbing, B.

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

Van Driel, H.

D. Moss, E. Ghahramani, J. Sipe, and H. Van Driel, Phys. Rev. B 41, 1542 (1990).
[CrossRef]

J. Sipe, D. Moss, and H. Van Driel, Phys. Rev. B 35, 1129 (1987).
[CrossRef]

von der Osten, W.

D. Fröhlich, A. Kulik, B. Uebbing, A. Mysyrowicz, V. Langer, H. Stolz, and W. von der Osten, Phys. Rev. Lett. 67, 2343 (1991).
[CrossRef]

Wang, K.

M. Fu, H. Long, K. Wang, G. Yang, and P. Lu, Thin Solid Films 519, 6557 (2011).
[CrossRef]

Wolfe, J.

D. Trauernicht, J. Wolfe, and A. Mysyrowicz, Phys. Rev. B 34, 2561 (1986).
[CrossRef]

Wong, G. K. L.

Y. Sun, G. K. L. Wong, and J. B. Ketterson, Phys. Rev. B 63, 125323 (2001).
[CrossRef]

Yamaguchi, H.

T. Ito, H. Yamaguchi, K. Okabe, and T. Masumi, J. Mater. Sci. 33, 3555 (1998).
[CrossRef]

Yang, G.

M. Fu, H. Long, K. Wang, G. Yang, and P. Lu, Thin Solid Films 519, 6557 (2011).
[CrossRef]

Yoshioka, K.

K. Yoshioka and M. Kuwata-Gonokami, New J. Phys. 14, 055024 (2012).
[CrossRef]

T. Ideguchi, K. Yoshioka, A. Mysyrowicz, and M. Kuwata-Gonokami, Phys. Rev. Lett. 100, 233001 (2008).
[CrossRef]

K. Yoshioka and M. Kuwata-Gonokami, Phys. Rev. B 73, 081202 (2006).
[CrossRef]

Cryst. Growth Des.

K. Chang, L. Frazer, J. Schwartz, J. B. Ketterson, and K. Poeppelmeier, Cryst. Growth Des. 13, 4914 (2013).
[CrossRef]

IEEE J. Quantum Electron.

G. Boyd, H. Kasper, and J. McFee, IEEE J. Quantum Electron. 7, 563 (1971).
[CrossRef]

IEEE J. Sel. Top. Quantum Electron.

A. DiChiara, S. Ghimire, C. Blaga, E. Sistrunk, E. Power, A. March, T. Miller, D. Reis, P. Agostini, and L. DiMauro, IEEE J. Sel. Top. Quantum Electron. 18, 419 (2012).
[CrossRef]

J. Cryst. Growth

R. Schmidt-Whitley, M. Martinez-Clemente, and A. Revcolevschi, J. Cryst. Growth 23, 113 (1974).
[CrossRef]

J. Mater. Sci.

T. Ito, H. Yamaguchi, K. Okabe, and T. Masumi, J. Mater. Sci. 33, 3555 (1998).
[CrossRef]

Nat. Phys.

S. Ghimire, A. DiChiara, E. Sistrunk, P. Agostini, L. DiMauro, and D. Reis, Nat. Phys. 7, 138 (2010).
[CrossRef]

New J. Phys.

K. Yoshioka and M. Kuwata-Gonokami, New J. Phys. 14, 055024 (2012).
[CrossRef]

R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
[CrossRef]

Opt. Lett.

Phys. Rev.

P. Baumeister, Phys. Rev. 121, 359 (1961).
[CrossRef]

Phys. Rev. A

A. L’Huillier, P. Balcou, S. Candel, K. Schafer, and K. Kulander, Phys. Rev. A 46, 2778 (1992).
[CrossRef]

Phys. Rev. B

M. Shen, S. Koyama, M. Saito, T. Goto, and N. Kuroda, Phys. Rev. B 53, 13477 (1996).
[CrossRef]

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