Abstract

We present a method that allows one to measure the real and imaginary parts of the third-order susceptibility in a wide-field coherent anti-Stokes Raman scattering setup using a quadriwave lateral shearing interferometer. This permits the retrieval of the undistorted Raman spectrum and the removal of a nonresonant signal from the surrounding solvent, which otherwise may overwhelm weak resonances.

© 2013 Optical Society of America

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2012 (1)

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

2011 (2)

W. Min, C. W. Freudiger, S. Lu, and X. S. Xie, Annu. Rev. Phys. Chem. 62, 507 (2011).
[CrossRef]

A. Jesacher, C. Roider, S. Khan, G. Thalhammer, S. Bernet, and M. Ritsch-Marte, Opt. Lett. 36, 2245(2011).
[CrossRef]

2010 (1)

D. Gachet, S. Brustlein, and H. Rigneault, Phys. Rev. Lett. 104, 213905 (2010).
[CrossRef]

2009 (3)

2007 (1)

2006 (2)

E. O. Potma, C. L. Evans, and X. S. Xie, Opt. Lett. 31, 241 (2006).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, New J. Phys. 8, 36 (2006).
[CrossRef]

2004 (1)

C. Heinrich, S. Bernet, and M. Ritsch-Marte, Appl. Phys. Lett. 84, 816 (2004).
[CrossRef]

2002 (2)

A. Volkmer, L. D. Book, and X. S. Xie, Appl. Phys. Lett. 80, 1505 (2002).
[CrossRef]

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef]

2001 (1)

1999 (1)

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

1995 (1)

1982 (1)

1979 (2)

J.-L. Oudar, R. W. Smith, and Y. R. Shen, Appl. Phys. Lett. 34, 758 (1979).
[CrossRef]

R. Hellwarth, Prog. Quantum Electron. 5, 1 (1979).
[CrossRef]

Bernet, S.

A. Jesacher, C. Roider, S. Khan, G. Thalhammer, S. Bernet, and M. Ritsch-Marte, Opt. Lett. 36, 2245(2011).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, New J. Phys. 8, 36 (2006).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, Appl. Phys. Lett. 84, 816 (2004).
[CrossRef]

Berto, P.

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

Bon, P.

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

P. Bon, G. Maucort, B. Wattellier, and S. Monneret, Opt. Express 17, 13080 (2009).
[CrossRef]

Book, L. D.

A. Volkmer, L. D. Book, and X. S. Xie, Appl. Phys. Lett. 80, 1505 (2002).
[CrossRef]

J.-X. Cheng, L. D. Book, and X. S. Xie, Opt. Lett. 26, 1341 (2001).
[CrossRef]

Brustlein, S.

D. Gachet, S. Brustlein, and H. Rigneault, Phys. Rev. Lett. 104, 213905 (2010).
[CrossRef]

Cheng, J.-X.

Cohn, K.

Dudovich, N.

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef]

Duncan, M. D.

Evans, C. L.

Freudiger, C. W.

W. Min, C. W. Freudiger, S. Lu, and X. S. Xie, Annu. Rev. Phys. Chem. 62, 507 (2011).
[CrossRef]

Gachet, D.

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

D. Gachet, S. Brustlein, and H. Rigneault, Phys. Rev. Lett. 104, 213905 (2010).
[CrossRef]

Heinrich, C.

C. Heinrich, S. Bernet, and M. Ritsch-Marte, New J. Phys. 8, 36 (2006).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, Appl. Phys. Lett. 84, 816 (2004).
[CrossRef]

Hellwarth, R.

R. Hellwarth, Prog. Quantum Electron. 5, 1 (1979).
[CrossRef]

Herek, J. L.

M. Jurna, J. P. Korterik, C. Otto, J. L. Herek, and H. L. Offerhaus, Phys. Rev. Lett. 103, 043905 (2009).
[CrossRef]

Holtom, G. R.

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Jesacher, A.

Jurna, M.

M. Jurna, J. P. Korterik, C. Otto, J. L. Herek, and H. L. Offerhaus, Phys. Rev. Lett. 103, 043905 (2009).
[CrossRef]

Khan, S.

Korterik, J. P.

M. Jurna, J. P. Korterik, C. Otto, J. L. Herek, and H. L. Offerhaus, Phys. Rev. Lett. 103, 043905 (2009).
[CrossRef]

Lu, S.

W. Min, C. W. Freudiger, S. Lu, and X. S. Xie, Annu. Rev. Phys. Chem. 62, 507 (2011).
[CrossRef]

Manuccia, T. J.

Maucort, G.

Min, W.

W. Min, C. W. Freudiger, S. Lu, and X. S. Xie, Annu. Rev. Phys. Chem. 62, 507 (2011).
[CrossRef]

Monneret, S.

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

P. Bon, G. Maucort, B. Wattellier, and S. Monneret, Opt. Express 17, 13080 (2009).
[CrossRef]

Offerhaus, H. L.

M. Jurna, J. P. Korterik, C. Otto, J. L. Herek, and H. L. Offerhaus, Phys. Rev. Lett. 103, 043905 (2009).
[CrossRef]

Oron, D.

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef]

Otto, C.

M. Jurna, J. P. Korterik, C. Otto, J. L. Herek, and H. L. Offerhaus, Phys. Rev. Lett. 103, 043905 (2009).
[CrossRef]

Oudar, J.-L.

J.-L. Oudar, R. W. Smith, and Y. R. Shen, Appl. Phys. Lett. 34, 758 (1979).
[CrossRef]

Palanker, D.

Potma, E. O.

Primot, J.

Reintjes, J.

Rigneault, H.

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

D. Gachet, S. Brustlein, and H. Rigneault, Phys. Rev. Lett. 104, 213905 (2010).
[CrossRef]

Ritsch-Marte, M.

A. Jesacher, C. Roider, S. Khan, G. Thalhammer, S. Bernet, and M. Ritsch-Marte, Opt. Lett. 36, 2245(2011).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, New J. Phys. 8, 36 (2006).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, Appl. Phys. Lett. 84, 816 (2004).
[CrossRef]

Roider, C.

Shen, Y. R.

J.-L. Oudar, R. W. Smith, and Y. R. Shen, Appl. Phys. Lett. 34, 758 (1979).
[CrossRef]

Silberberg, Y.

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef]

Simanovskii, D.

Smith, R. W.

J.-L. Oudar, R. W. Smith, and Y. R. Shen, Appl. Phys. Lett. 34, 758 (1979).
[CrossRef]

Smith, T.

Sogno, L.

Thalhammer, G.

Toytman, I.

Volkmer, A.

A. Volkmer, L. D. Book, and X. S. Xie, Appl. Phys. Lett. 80, 1505 (2002).
[CrossRef]

Wattellier, B.

Xie, X. S.

W. Min, C. W. Freudiger, S. Lu, and X. S. Xie, Annu. Rev. Phys. Chem. 62, 507 (2011).
[CrossRef]

E. O. Potma, C. L. Evans, and X. S. Xie, Opt. Lett. 31, 241 (2006).
[CrossRef]

A. Volkmer, L. D. Book, and X. S. Xie, Appl. Phys. Lett. 80, 1505 (2002).
[CrossRef]

J.-X. Cheng, L. D. Book, and X. S. Xie, Opt. Lett. 26, 1341 (2001).
[CrossRef]

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Zumbusch, A.

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Annu. Rev. Phys. Chem. (1)

W. Min, C. W. Freudiger, S. Lu, and X. S. Xie, Annu. Rev. Phys. Chem. 62, 507 (2011).
[CrossRef]

Appl. Phys. Lett. (3)

J.-L. Oudar, R. W. Smith, and Y. R. Shen, Appl. Phys. Lett. 34, 758 (1979).
[CrossRef]

A. Volkmer, L. D. Book, and X. S. Xie, Appl. Phys. Lett. 80, 1505 (2002).
[CrossRef]

C. Heinrich, S. Bernet, and M. Ritsch-Marte, Appl. Phys. Lett. 84, 816 (2004).
[CrossRef]

J. Opt. Soc. Am. A (1)

Nature (1)

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef]

New J. Phys. (1)

C. Heinrich, S. Bernet, and M. Ritsch-Marte, New J. Phys. 8, 36 (2006).
[CrossRef]

Opt. Express (2)

Opt. Lett. (5)

Phys. Rev. Lett. (4)

P. Berto, D. Gachet, P. Bon, S. Monneret, and H. Rigneault, Phys. Rev. Lett. 109, 093902 (2012).
[CrossRef]

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

M. Jurna, J. P. Korterik, C. Otto, J. L. Herek, and H. L. Offerhaus, Phys. Rev. Lett. 103, 043905 (2009).
[CrossRef]

D. Gachet, S. Brustlein, and H. Rigneault, Phys. Rev. Lett. 104, 213905 (2010).
[CrossRef]

Prog. Quantum Electron. (1)

R. Hellwarth, Prog. Quantum Electron. 5, 1 (1979).
[CrossRef]

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Figures (3)

Fig. 1.
Fig. 1.

(a) Extremely folded box-CARS beam geometry. (b) Experimental setup: D, dichroic mirror; MHM, modified Hartmann mask. (c) Sample cell.

Fig. 2.
Fig. 2.

CARS measurements on a 4.5 μm polystyrene bead by QWLSI. (a) Phase and intensity images on resonance (Ω=3050cm1) and off resonance (Ω=3200cm1). (b) Comparison of the phase profile on resonance (red triangles) and off resonance (blue circles). On resonance, an extra phase shift φCARS=64° corresponding to the vibrational phase is visible.

Fig. 3.
Fig. 3.

CARS spectra of a polystyrene bead measured by QWLSI. (a) CARS phase spectrum, (b) CARS intensity spectrum, and (c) comparison of the retrieved Raman spectrum (red solid line) with the spontaneous Raman spectrum (blue dashed line).

Equations (2)

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IRamanIm(χ(3)).
IRamanIm(ECARS)ICARS·sin(φCARS).

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