Abstract

We report, for the first time to our knowledge, femtosecond pulse generation from a graphene mode-locked Cr:ZnSe laser at 2500 nm. To minimize the insertion losses at the lasing wavelength, high-quality monolayer graphene transferred on a CaF2 substrate was used in the experiments. Once mode-locking was initiated, the laser generated a stable train of 226 fs pulses with a time–bandwidth product of 0.39. The mode-locked laser operated at a pulse repetition rate of 77 MHz and produced 80 mW output power with an incident pump power of 1.6 W. To our knowledge, this is the longest laser wavelength at which graphene-based passive mode-locking has been demonstrated to date.

© 2013 Optical Society of America

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2012

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Z. Sun, T. Hasan, and A. C. Ferrari, Physica E 44, 1082 (2012).
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A. Schliesser, N. Picque, and T. W. Hansch, Nat. Photonics 6, 440 (2012).
[CrossRef]

A. Schmidt, P. Koopmann, G. Huber, P. Fuhrberg, S. Y. Choi, D.-I. Yeom, F. Rotermund, V. Petrov, and U. Griebner, Opt. Express 20, 5313 (2012).
[CrossRef]

J. Ma, G. Q. Xie, P. Lv, W. L. Gao, P. Yuan, L. J. Qian, H. H. Yu, H. J. Zhang, J. Y. Wang, and D. Y. Tang, Opt. Lett. 37, 2085 (2012).
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2011

2010

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, Nat. Photonics 4, 611 (2010).
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2009

2008

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
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2006

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

U. Demirbas and A. Sennaroglu, Opt. Lett. 31, 2293 (2006).
[CrossRef]

2004

S. Y. Set, H. Yaguchi, Y. Tanaka, and M. Jablonski, IEEE J. Sel. Top. Quantum Electron. 10, 137 (2004).
[CrossRef]

2000

1996

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Agnesi, A.

Ahn, Y. H.

I. H. Baek, H. W. Lee, S. Bae, B. H. Hong, Y. H. Ahn, D.-I. Yeom, and F. Rotermund, Appl. Phys. Express 5, 032701 (2012).
[CrossRef]

Aus der Au, J.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Bae, S.

I. H. Baek, H. W. Lee, S. Bae, B. H. Hong, Y. H. Ahn, D.-I. Yeom, and F. Rotermund, Appl. Phys. Express 5, 032701 (2012).
[CrossRef]

W. B. Cho, J. W. Kim, H. W. Lee, S. Bae, B. H. Hong, S. Y. Choi, I. H. Baek, K. Kim, D.-I. Yeom, and F. Rotermund, Opt. Lett. 36, 4089 (2011).
[CrossRef]

Baek, I. H.

Bonaccorso, F.

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, Nat. Photonics 4, 611 (2010).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Braun, B.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
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Brown, C. L.

B. V. Cunning, C. L. Brown, and D. Kielpinski, Appl. Phys. Lett. 99, 261109 (2011).
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Bulovic, V.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
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Cankaya, H.

Carrig, T.

I. T. Sorokina, E. Sorokin, and T. Carrig, in Conference on Lasers and Electro-Optics (CLEO) (Optical Society of America, 2006), paper CMQ2.

Carrig, T. J.

Casiraghi, C.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Chen, J.

Cheng, Y.

Cho, W. B.

Choi, S. Y.

Chu, W.

Cizmeciyan, M. N.

Cunning, B. V.

B. V. Cunning, C. L. Brown, and D. Kielpinski, Appl. Phys. Lett. 99, 261109 (2011).
[CrossRef]

Demirbas, U.

Dresselhaus, M. S.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
[CrossRef]

Fedorov, V. V.

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

Ferrari, A. C.

Z. Sun, T. Hasan, and A. C. Ferrari, Physica E 44, 1082 (2012).
[CrossRef]

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, Nat. Photonics 4, 611 (2010).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Fluck, R.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Fu, Y.

Fuhrberg, P.

Gao, W. L.

Geim, A. K.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
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Griebner, U.

Hansch, T. W.

A. Schliesser, N. Picque, and T. W. Hansch, Nat. Photonics 6, 440 (2012).
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Hasan, T.

Z. Sun, T. Hasan, and A. C. Ferrari, Physica E 44, 1082 (2012).
[CrossRef]

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, Nat. Photonics 4, 611 (2010).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Ho, J.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
[CrossRef]

Hong, B. H.

I. H. Baek, H. W. Lee, S. Bae, B. H. Hong, Y. H. Ahn, D.-I. Yeom, and F. Rotermund, Appl. Phys. Express 5, 032701 (2012).
[CrossRef]

W. B. Cho, J. W. Kim, H. W. Lee, S. Bae, B. H. Hong, S. Y. Choi, I. H. Baek, K. Kim, D.-I. Yeom, and F. Rotermund, Opt. Lett. 36, 4089 (2011).
[CrossRef]

Hönninger, C.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Huber, G.

Jablonski, M.

S. Y. Set, H. Yaguchi, Y. Tanaka, and M. Jablonski, IEEE J. Sel. Top. Quantum Electron. 10, 137 (2004).
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Jeong, J. Y.

Jia, X.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
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Jiang, D.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Jung, I. D.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Kartner, F. X.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Keller, U.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Kielpinski, D.

B. V. Cunning, C. L. Brown, and D. Kielpinski, Appl. Phys. Lett. 99, 261109 (2011).
[CrossRef]

Kim, J. W.

Kim, K.

Kong, J.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
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Koopmann, P.

Kopf, D.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Kurt, A.

Lazzeri, M.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Lee, H. W.

Liu, X.

Lv, P.

Ma, J.

Matuschek, N.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Mauri, F.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
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Meyer, J. C.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
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Midorikawa, K.

Mirov, M. S.

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

Mirov, S. B.

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

Moskalev, I. S.

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

Nezich, D.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
[CrossRef]

Novoselov, K. S.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Pasiskevicius, V.

Petrov, V.

Picque, N.

A. Schliesser, N. Picque, and T. W. Hansch, Nat. Photonics 6, 440 (2012).
[CrossRef]

Piscanec, S.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Pollock, C. R.

Qian, L. J.

Reina, A.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
[CrossRef]

Rotermund, F.

Roth, S.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Rozhin, A. G.

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Scardaci, V.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Schliesser, A.

A. Schliesser, N. Picque, and T. W. Hansch, Nat. Photonics 6, 440 (2012).
[CrossRef]

Schmidt, A.

Sennaroglu, A.

Set, S. Y.

S. Y. Set, H. Yaguchi, Y. Tanaka, and M. Jablonski, IEEE J. Sel. Top. Quantum Electron. 10, 137 (2004).
[CrossRef]

Son, H.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
[CrossRef]

Sorokin, E.

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

I. T. Sorokina, E. Sorokin, and T. Carrig, in Conference on Lasers and Electro-Optics (CLEO) (Optical Society of America, 2006), paper CMQ2.

Sorokina, I. T.

I. T. Sorokina, E. Sorokin, and T. Carrig, in Conference on Lasers and Electro-Optics (CLEO) (Optical Society of America, 2006), paper CMQ2.

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

Sun, Z.

Z. Sun, T. Hasan, and A. C. Ferrari, Physica E 44, 1082 (2012).
[CrossRef]

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, Nat. Photonics 4, 611 (2010).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Takahashi, E. J.

Tan, P. H.

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Tanaka, Y.

S. Y. Set, H. Yaguchi, Y. Tanaka, and M. Jablonski, IEEE J. Sel. Top. Quantum Electron. 10, 137 (2004).
[CrossRef]

Tang, D. Y.

Wagner, G. J.

Wang, F.

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Wang, J. Y.

Weingarten, K. J.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

Xie, G. Q.

Xiong, H.

Xu, H.

Xu, Z.

Yaguchi, H.

S. Y. Set, H. Yaguchi, Y. Tanaka, and M. Jablonski, IEEE J. Sel. Top. Quantum Electron. 10, 137 (2004).
[CrossRef]

Yao, J.

Yeom, D. I.

Yeom, D.-I.

Yu, H. H.

Yuan, P.

Zeng, B.

Zhang, H. J.

Adv. Mater.

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, Adv. Mater. 21, 3874 (2009).
[CrossRef]

Appl. Phys. Express

I. H. Baek, H. W. Lee, S. Bae, B. H. Hong, Y. H. Ahn, D.-I. Yeom, and F. Rotermund, Appl. Phys. Express 5, 032701 (2012).
[CrossRef]

Appl. Phys. Lett.

B. V. Cunning, C. L. Brown, and D. Kielpinski, Appl. Phys. Lett. 99, 261109 (2011).
[CrossRef]

IEEE J. Sel. Top. Quantum Electron.

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, R. Fluck, C. Hönninger, N. Matuschek, and J. Aus der Au, IEEE J. Sel. Top. Quantum Electron. 2, 435 (1996).
[CrossRef]

S. Y. Set, H. Yaguchi, Y. Tanaka, and M. Jablonski, IEEE J. Sel. Top. Quantum Electron. 10, 137 (2004).
[CrossRef]

Nano Lett.

A. Reina, X. Jia, J. Ho, D. Nezich, H. Son, V. Bulovic, M. S. Dresselhaus, and J. Kong, Nano Lett. 9, 30 (2008).
[CrossRef]

Nat. Photonics

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, Nat. Photonics 4, 611 (2010).
[CrossRef]

A. Schliesser, N. Picque, and T. W. Hansch, Nat. Photonics 6, 440 (2012).
[CrossRef]

Opt. Express

Opt. Lett.

Phys. Rev. Lett.

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, Phys. Rev. Lett. 97, 187401(2006).
[CrossRef]

Physica E

Z. Sun, T. Hasan, and A. C. Ferrari, Physica E 44, 1082 (2012).
[CrossRef]

Other

E. Sorokin, I. T. Sorokina, M. S. Mirov, V. V. Fedorov, I. S. Moskalev, and S. B. Mirov, in Advanced Solid-State Photonics (Optical Society of America, 2010), paper AMC2.

I. T. Sorokina, E. Sorokin, and T. Carrig, in Conference on Lasers and Electro-Optics (CLEO) (Optical Society of America, 2006), paper CMQ2.

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Figures (5)

Fig. 1.
Fig. 1.

Optical transmission of the high-quality monolayer graphene transferred onto CaF2.

Fig. 2.
Fig. 2.

Measured Raman spectrum of the monolayer graphene on CaF2.

Fig. 3.
Fig. 3.

Experimental setup of the GSA mode-locked Cr:ZnSe laser. M1, M2, M3, and M4 are highly reflecting concave mirrors (ROC=100mm). L is the pump focusing lens (f=7.5cm). P1 and P2 are the CaF2 dispersion compensation prisms.

Fig. 4.
Fig. 4.

Efficiency curves of the Cr:ZnSe laser in different configurations.

Fig. 5.
Fig. 5.

(a) Measured laser spectrum and (b) measured interferometric autocorrelation trace of the pulses near 2500 nm.

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