Abstract

We investigated the interaction of an intense laser radiation with colloidal solutions containing CdSe/ZnS core shell quantum dots (QDs; mean size 3.4 nm), fullerene C60, and Perylene. These materials would give rise to the photoinduced electron transfer and charge separation on the QDs and thus the optical limiting effect. Results confirm the intended aim, obtained by means of intermediate metastable products of reversible photochemical reactions, i.e., ion radicals of hybrid systems containing semiconductor nanoparticles.

© 2012 Optical Society of America

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  1. J. D. Swalen and F. Kajzar, Nonlinear Opt. 105, 2981 (2001).
  2. M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
    [CrossRef]
  3. M. V. Gryaznova, V. V. Danilov, and T. A. Shakhverdov, Opt. Spectrosc. 105, 874 (2008).
    [CrossRef]
  4. A. P. Brown and P. V. Kamat, J. Am. Chem. Soc. 130, 8890 (2008).
    [CrossRef]
  5. R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
    [CrossRef]
  6. V. V. Danilov, Opt. Zh. 74, 65 (2008).
  7. D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
    [CrossRef]
  8. T. A. Shahverdov, Opt. Spectrosc. 29, 315 (1970).
  9. A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
    [CrossRef]
  10. S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).
  11. J. A. Barltrop and J. D. Coyle, Excited States in Organic Chemistry (Wiley, 1978).

2010 (2)

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

2008 (3)

V. V. Danilov, Opt. Zh. 74, 65 (2008).

M. V. Gryaznova, V. V. Danilov, and T. A. Shakhverdov, Opt. Spectrosc. 105, 874 (2008).
[CrossRef]

A. P. Brown and P. V. Kamat, J. Am. Chem. Soc. 130, 8890 (2008).
[CrossRef]

2007 (1)

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

2004 (1)

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

2001 (1)

J. D. Swalen and F. Kajzar, Nonlinear Opt. 105, 2981 (2001).

1999 (1)

D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
[CrossRef]

1970 (1)

T. A. Shahverdov, Opt. Spectrosc. 29, 315 (1970).

Andrianov, V. E.

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

Armstrong, N. R.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Artemyev, M. V.

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

Baranov, A. V.

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

Barltrop, J. A.

J. A. Barltrop and J. D. Coyle, Excited States in Organic Chemistry (Wiley, 1978).

Brown, A. P.

A. P. Brown and P. V. Kamat, J. Am. Chem. Soc. 130, 8890 (2008).
[CrossRef]

Coyle, J. D.

J. A. Barltrop and J. D. Coyle, Excited States in Organic Chemistry (Wiley, 1978).

D’Ambruoso, G. D.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Danilov, V. V.

M. V. Gryaznova, V. V. Danilov, and T. A. Shakhverdov, Opt. Spectrosc. 105, 874 (2008).
[CrossRef]

V. V. Danilov, Opt. Zh. 74, 65 (2008).

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

Dneprovsky, S.

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

Drichko, N. V.

D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
[CrossRef]

Graja, A.

D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
[CrossRef]

Gryaznova, M. V.

M. V. Gryaznova, V. V. Danilov, and T. A. Shakhverdov, Opt. Spectrosc. 105, 874 (2008).
[CrossRef]

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

Hall, H. K.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Hieu, D. S.

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

Kajzar, F.

J. D. Swalen and F. Kajzar, Nonlinear Opt. 105, 2981 (2001).

Kamat, P. V.

A. P. Brown and P. V. Kamat, J. Am. Chem. Soc. 130, 8890 (2008).
[CrossRef]

Khapova, O. V.

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

Khrebtov, A. I.

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

Konarev, D. V.

D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
[CrossRef]

Korth, B. D.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Kozlova, M. V.

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

Maslov, V. G.

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

Orlova, A. O.

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

Parfenov, P. S.

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

Pyun, J.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Semkin, V. N.

D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
[CrossRef]

Shahverdov, T. A.

T. A. Shahverdov, Opt. Spectrosc. 29, 315 (1970).

Shakhverdov, T. A.

M. V. Gryaznova, V. V. Danilov, and T. A. Shakhverdov, Opt. Spectrosc. 105, 874 (2008).
[CrossRef]

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

Shallcross, R. C.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Swalen, J. D.

J. D. Swalen and F. Kajzar, Nonlinear Opt. 105, 2981 (2001).

Wumaier, T.

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

Zheng, Z.

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Zhukov, E. A.

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

J. Am. Chem. Soc. (2)

A. P. Brown and P. V. Kamat, J. Am. Chem. Soc. 130, 8890 (2008).
[CrossRef]

R. C. Shallcross, G. D. D’Ambruoso, B. D. Korth, H. K. Hall, Z. Zheng, J. Pyun, and N. R. Armstrong, J. Am. Chem. Soc. 129, 11310 (2007).
[CrossRef]

Nonlinear Opt. (1)

J. D. Swalen and F. Kajzar, Nonlinear Opt. 105, 2981 (2001).

Opt. Spectrosc. (3)

M. V. Gryaznova, V. V. Danilov, and T. A. Shakhverdov, Opt. Spectrosc. 105, 874 (2008).
[CrossRef]

T. A. Shahverdov, Opt. Spectrosc. 29, 315 (1970).

A. O. Orlova, V. E. Andrianov, V. G. Maslov, P. S. Parfenov, and A. V. Baranov, Opt. Spectrosc. 108, 807 (2010).
[CrossRef]

Opt. Zh. (1)

V. V. Danilov, Opt. Zh. 74, 65 (2008).

Quantum Electron. (1)

M. V. Gryaznova, V. V. Danilov, O. V. Khapova, A. I. Khrebtov, and T. A. Shakhverdov, Quantum Electron. 34, 407 (2004).
[CrossRef]

Solid State Phys. (1)

S. Dneprovsky, E. A. Zhukov, M. V. Kozlova, T. Wumaier, D. S. Hieu, and M. V. Artemyev, Solid State Phys. 52, 1809 (2010).

Synth. Met. (1)

D. V. Konarev, N. V. Drichko, V. N. Semkin, and A. Graja, Synth. Met. 103, 2384 (1999).
[CrossRef]

Other (1)

J. A. Barltrop and J. D. Coyle, Excited States in Organic Chemistry (Wiley, 1978).

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Figures (4)

Fig. 1.
Fig. 1.

Absorption spectra of tested solutions. Curve 1: CdSe/ZnS QDs; curve 2: fullerene C60; and curve 3: Perylene. In all cases, the solvent is toluene.

Fig. 2.
Fig. 2.

Dependence of the solution transmittance on the energy of the incident radiation Ein[J] λexit=532nm. 1: CdSe/ZnS QDs; 2: 0.75C60+0.25QDs; 3: C60; 4: 0.75C60+0.25QDs+Per(1.1mM). The initial transmittance of all solutions is 45%.

Fig. 3.
Fig. 3.

Graphical representation of the photochemical processes occurring in the semiconductor nanophotoreactor under intense light exposure.

Fig. 4.
Fig. 4.

Dependence of the transmittance of solution 4 (0.75C60+0.25QDs+Per1.1mM), under different illumination conditions. Curve 1: only λ=1064nm. Curve 2: combined action of λ=532nm and λ=1064nm light sources.

Equations (1)

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[QDs;C60]+hν[C60,QDs+][C60,QDs++Per][C60+QDs+Per+]

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