Abstract

The fluorescence behavior of a chiral polybinaphthyl excited with 100fs 800nm laser pulses was investigated in tetrahydrofuran solution. The peak fluorescence intensity versus the input irradiance was measured to meet a square dependence, giving evidence for two-photon excited fluorescence (TPF). The variations of the TPF intensity were found to be strongly modulated by the different polarized incident lights and tightly depend on the linearly polarized component of the incident light. Furthermore, combining with the characteristics of chiral molecules, the two-photon polarization ratio was studied to reveal the symmetry of the involved excited states.

© 2011 Optical Society of America

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2011 (1)

J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

2010 (8)

A. Nag and D. Goswami, J. Chem. Phys. 132, 154508 (2010).
[CrossRef] [PubMed]

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

Y. Hu, Z. Zhang, Y. Chen, Q. Zhang, and W. Huang, Opt. Lett. 35, 46 (2010).
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X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
[CrossRef]

Z. Wu, W. B. Chen, D. C. Abeysinghe, R. L. Nelson, and Q. W. Zhan, Opt. Lett. 35, 1755 (2010).
[CrossRef] [PubMed]

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
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C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
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2009 (2)

A. Nag, A. K. De, and D. Goswami, J. Phys. B 42, 065103(2009).
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L. M. Haupert and G. J. Simpson, Annu. Rev. Phys. Chem. 60, 345 (2009).
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2008 (2)

2006 (1)

C. C. Corredor, Z. L. Huang, and K. D. Belfield, Adv. Mater. 18, 2910 (2006).
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2004 (1)

L. Pu, Chem. Rev. 104, 1687 (2004).
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2002 (1)

A. Zoumi, A. Yeh, and B. J. Tromberg, Proc. Natl. Acad. Sci. USA 99, 11014 (2002).
[CrossRef] [PubMed]

2001 (2)

P. K. Frederiksen, M. Jørgensen, and P. R. Ogilby, J. Am. Chem. Soc. 123, 1215 (2001).
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Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
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2000 (1)

M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
[CrossRef]

1999 (2)

E. J. Sanchez, L. Novotny, and X. S. Xie, Phys. Rev. Lett. 82, 4014 (1999).
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H. B. Sun, S. Matsuo, and H. Misawa, Appl. Phys. Lett. 74, 786 (1999).
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1983 (1)

M. A. C. Nascimento, Chem. Phys. 74, 51 (1983).
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Abeysinghe, D. C.

Andraud, C.

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
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Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
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D. Wanapun, R. D. Wampler, N. J. Begue, and G. J. Simpson, Chem. Phys. Lett. 455, 6 (2008).
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C. C. Corredor, Z. L. Huang, and K. D. Belfield, Adv. Mater. 18, 2910 (2006).
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X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
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H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
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Chen, W. B.

Chen, Y.

Cheng, Y.

X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
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C. C. Corredor, Z. L. Huang, and K. D. Belfield, Adv. Mater. 18, 2910 (2006).
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De, A. K.

A. Nag, A. K. De, and D. Goswami, J. Phys. B 42, 065103(2009).
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C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
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Ding, R.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Donegan, J. F.

Dong, Y.

X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
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Fang, H. H.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Feng, J.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
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Flood, E.

Frederiksen, P. K.

P. K. Frederiksen, M. Jørgensen, and P. R. Ogilby, J. Am. Chem. Soc. 123, 1215 (2001).
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Fuchs, H.

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
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M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
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X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
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A. Nag and D. Goswami, J. Chem. Phys. 132, 154508 (2010).
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A. Nag, A. K. De, and D. Goswami, J. Phys. B 42, 065103(2009).
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M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
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Guo, W. H.

Haupert, L. M.

L. M. Haupert and G. J. Simpson, Annu. Rev. Phys. Chem. 60, 345 (2009).
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J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

Hehlen, M. P.

M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
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C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
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Hu, Y.

Huang, W.

Huang, X.

X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
[CrossRef]

Huang, Z. L.

C. C. Corredor, Z. L. Huang, and K. D. Belfield, Adv. Mater. 18, 2910 (2006).
[CrossRef]

Inoue, Y.

Y. Inoue, Chiral Photochemistry (CRC Press, 2004).
[CrossRef]

Irimia, A.

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
[CrossRef]

Jia, T. Q.

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
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P. K. Frederiksen, M. Jørgensen, and P. R. Ogilby, J. Am. Chem. Soc. 123, 1215 (2001).
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Kervella, Y.

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
[CrossRef]

Lin, N.

C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
[CrossRef] [PubMed]

Lu, C. H.

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

Lüthi, S. R.

M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
[CrossRef]

Lynch, M.

Ma, Y. G.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Matsuo, S.

H. B. Sun, S. Matsuo, and H. Misawa, Appl. Phys. Lett. 74, 786 (1999).
[CrossRef]

Meng, J.

X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
[CrossRef]

Misawa, H.

H. B. Sun, S. Matsuo, and H. Misawa, Appl. Phys. Lett. 74, 786 (1999).
[CrossRef]

Morel, Y.

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
[CrossRef]

Nag, A.

A. Nag and D. Goswami, J. Chem. Phys. 132, 154508 (2010).
[CrossRef] [PubMed]

A. Nag, A. K. De, and D. Goswami, J. Phys. B 42, 065103(2009).
[CrossRef]

Najechalski, P.

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
[CrossRef]

Nascimento, M. A. C.

M. A. C. Nascimento, Chem. Phys. 74, 51 (1983).
[CrossRef]

Nelson, R. L.

Novotny, L.

E. J. Sanchez, L. Novotny, and X. S. Xie, Phys. Rev. Lett. 82, 4014 (1999).
[CrossRef]

O’Dowd, J.

Ogilby, P. R.

P. K. Frederiksen, M. Jørgensen, and P. R. Ogilby, J. Am. Chem. Soc. 123, 1215 (2001).
[CrossRef] [PubMed]

Pollnau, M.

M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
[CrossRef]

Pu, L.

L. Pu, Chem. Rev. 104, 1687 (2004).
[CrossRef] [PubMed]

Rizzo, A.

C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
[CrossRef] [PubMed]

Sanchez, E. J.

E. J. Sanchez, L. Novotny, and X. S. Xie, Phys. Rev. Lett. 82, 4014 (1999).
[CrossRef]

Santoro, F.

C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
[CrossRef] [PubMed]

Simpson, G. J.

L. M. Haupert and G. J. Simpson, Annu. Rev. Phys. Chem. 60, 345 (2009).
[CrossRef]

D. Wanapun, R. D. Wampler, N. J. Begue, and G. J. Simpson, Chem. Phys. Lett. 455, 6 (2008).
[CrossRef]

Stephan, O.

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
[CrossRef]

Su, B.

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
[CrossRef]

Sun, H. B.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

H. B. Sun, S. Matsuo, and H. Misawa, Appl. Phys. Lett. 74, 786 (1999).
[CrossRef]

Sun, T.

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
[CrossRef]

Sun, Z. R.

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

Toro, C.

C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
[CrossRef] [PubMed]

Tromberg, B. J.

A. Zoumi, A. Yeh, and B. J. Tromberg, Proc. Natl. Acad. Sci. USA 99, 11014 (2002).
[CrossRef] [PubMed]

Vestweber, D.

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
[CrossRef]

Wampler, R. D.

D. Wanapun, R. D. Wampler, N. J. Begue, and G. J. Simpson, Chem. Phys. Lett. 455, 6 (2008).
[CrossRef]

Wanapun, D.

D. Wanapun, R. D. Wampler, N. J. Begue, and G. J. Simpson, Chem. Phys. Lett. 455, 6 (2008).
[CrossRef]

Wang, C. S.

J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

Wang, L.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Wang, X.

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
[CrossRef]

Wang, Z. G.

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

Wu, Z.

Xia, H.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Xie, X. S.

E. J. Sanchez, L. Novotny, and X. S. Xie, Phys. Rev. Lett. 82, 4014 (1999).
[CrossRef]

Yang, J.

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Yeh, A.

A. Zoumi, A. Yeh, and B. J. Tromberg, Proc. Natl. Acad. Sci. USA 99, 11014 (2002).
[CrossRef] [PubMed]

Zeng, Y.

J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

Zhan, Q. W.

Zhang, H.

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

Zhang, J. W.

J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

Zhang, Q.

Zhang, S. A.

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

Zhang, X. Q.

J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

Zhang, Z.

Zhu, C.

X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
[CrossRef]

Zoumi, A.

A. Zoumi, A. Yeh, and B. J. Tromberg, Proc. Natl. Acad. Sci. USA 99, 11014 (2002).
[CrossRef] [PubMed]

Adv. Mater. (1)

C. C. Corredor, Z. L. Huang, and K. D. Belfield, Adv. Mater. 18, 2910 (2006).
[CrossRef]

Annu. Rev. Phys. Chem. (1)

L. M. Haupert and G. J. Simpson, Annu. Rev. Phys. Chem. 60, 345 (2009).
[CrossRef]

Appl. Phys. Lett. (2)

H. B. Sun, S. Matsuo, and H. Misawa, Appl. Phys. Lett. 74, 786 (1999).
[CrossRef]

H. H. Fang, J. Yang, R. Ding, Q. D. Chen, L. Wang, H. Xia, J. Feng, Y. G. Ma, and H. B. Sun, Appl. Phys. Lett. 97, 101101(2010).
[CrossRef]

Chem. Eur. J. (1)

C. Toro, L. De Boni, N. Lin, F. Santoro, A. Rizzo, and F. E. Hernandez, Chem. Eur. J. 16, 3504 (2010).
[CrossRef] [PubMed]

Chem. Phys. (1)

M. A. C. Nascimento, Chem. Phys. 74, 51 (1983).
[CrossRef]

Chem. Phys. Lett. (1)

D. Wanapun, R. D. Wampler, N. J. Begue, and G. J. Simpson, Chem. Phys. Lett. 455, 6 (2008).
[CrossRef]

Chem. Rev. (1)

L. Pu, Chem. Rev. 104, 1687 (2004).
[CrossRef] [PubMed]

J. Am. Chem. Soc. (1)

P. K. Frederiksen, M. Jørgensen, and P. R. Ogilby, J. Am. Chem. Soc. 123, 1215 (2001).
[CrossRef] [PubMed]

J. Chem. Phys. (3)

Y. Morel, A. Irimia, P. Najechalski, Y. Kervella, O. Stephan, P. L. Baldeck, and C. Andraud, J. Chem. Phys. 114, 5391(2001).
[CrossRef]

A. Nag and D. Goswami, J. Chem. Phys. 132, 154508 (2010).
[CrossRef] [PubMed]

S. A. Zhang, H. Zhang, C. H. Lu, T. Q. Jia, Z. G. Wang, and Z. R. Sun, J. Chem. Phys. 133, 214504 (2010).
[CrossRef] [PubMed]

J. Phys. B (1)

A. Nag, A. K. De, and D. Goswami, J. Phys. B 42, 065103(2009).
[CrossRef]

J. Polym. Sci. A (1)

X. Huang, J. Meng, Y. Dong, Y. Cheng, and C. Zhu, J. Polym. Sci. A 48, 997 (2010).
[CrossRef]

Opt. Express (1)

Opt. Laser Technol. (1)

J. W. Zhang, T. He, C. S. Wang, X. Q. Zhang, and Y. Zeng, Opt. Laser Technol. 43, 974 (2011).
[CrossRef]

Opt. Lett. (2)

Phys. Rev. B (1)

M. Pollnau, D. R. Gamelin, S. R. Lüthi, H. U. Güdel, and M. P. Hehlen, Phys. Rev. B 61, 3337 (2000).
[CrossRef]

Phys. Rev. Lett. (1)

E. J. Sanchez, L. Novotny, and X. S. Xie, Phys. Rev. Lett. 82, 4014 (1999).
[CrossRef]

Proc. Natl. Acad. Sci. USA (1)

A. Zoumi, A. Yeh, and B. J. Tromberg, Proc. Natl. Acad. Sci. USA 99, 11014 (2002).
[CrossRef] [PubMed]

Soft Mater. (1)

X. Wang, H. Gan, T. Sun, B. Su, H. Fuchs, D. Vestweber, and S. Butz, Soft Mater. 6, 3851 (2010).
[CrossRef]

Other (1)

Y. Inoue, Chiral Photochemistry (CRC Press, 2004).
[CrossRef]

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Figures (4)

Fig. 1
Fig. 1

Linear absorption spectra (left) and the SPF spectra (right) of the chiral polymer in tetrahydrofuran; inset: the molecular structure of the chiral polymer.

Fig. 2
Fig. 2

(a) Fluorescence spectra excited at fs 800 nm under several excitation levels. (b) Corresponding peak fluorescence intensity as a function of P 0 (dots). The solid curve is a square fit to the data.

Fig. 3
Fig. 3

Variation in normalized SPF and TPF intensity of the chiral polymer and the normalized intensity of the linear component of the polarized incident light passed through a Glan- Laser polarizer (analyzer) with the rotation of a λ / 4 wave plate (dots); solid curves are the fitting curves of the dots with the function a cos 2 ( π ω β / 180 + b ) + c .

Fig. 4
Fig. 4

TPF spectra of the chiral polymer excited by the linearly polarized and CP light, respectively.

Tables (1)

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Table 1 Intensity Dependence of Polarization Ratio Ω L and Ω R

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