Abstract

We introduce fully noncollinear coherent two-dimensional (2D) spectroscopy in the UV domain with an all-reflective and miniaturized setup design. Phase stability is achieved via pairwise beam manipulation, and the concept can be transferred to all wavelength regimes. Here we present results from an implementation that has been optimized for wavelengths between 250 and 375nm. Interferometric measurements prove phase stability over several hours. We obtained 2D spectra of the nonpolar UV chromophore p-terphenyl in ethanol, excited with 50fs pulses at 287nm.

© 2010 Optical Society of America

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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef]
  7. A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
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2010 (1)

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

2009 (4)

2008 (5)

U. Selig, F. Langhojer, F. Dimler, T. Löhrig, C. Schwarz, B. Gieseking, and T. Brixner, Opt. Lett. 33, 2851 (2008).
[CrossRef] [PubMed]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

M. Cho, Chem. Rev. 108, 1331 (2008).
[CrossRef] [PubMed]

K. Hyeon-Deuk, Y. Tanimura, and M. Cho, J. Chem. Phys. 128, 135102 (2008).
[CrossRef] [PubMed]

2007 (2)

2006 (1)

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

2005 (3)

T. Zhang, C. Borca, X. Li, and S. Cundiff, Opt. Express 13, 7432 (2005).
[CrossRef] [PubMed]

V. Volkov, R. Schanz, and P. Hamm, Opt. Lett. 30, 2010(2005).
[CrossRef] [PubMed]

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

2004 (2)

T. Brixner, T. Mančal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[CrossRef] [PubMed]

M. L. Cowan, J. P. Ogilvie, and R. J. D. Miller, Chem. Phys. Lett. 386, 184 (2004).
[CrossRef]

2003 (2)

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, Science 300, 1553 (2003).
[CrossRef] [PubMed]

D. M. Jonas, Annu. Rev. Phys. Chem. 54, 425 (2003).
[CrossRef] [PubMed]

2002 (1)

Q. Xu, Y. Ma, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 116, 9333 (2002).
[CrossRef]

2000 (1)

S. Mukamel, Annu. Rev. Phys. Chem. 51, 691 (2000).
[CrossRef] [PubMed]

1997 (1)

D. Zimdars, R. S. Francis, C. Ferrante, and M. D. Fayer, J. Chem. Phys. 106, 7498 (1997).
[CrossRef]

Avlasevich, Y.

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Bazan, G. C.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Borca, C.

Bräm, O.

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

Brixner, T.

Bruner, B. D.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Cannizzo, A.

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

Chergui, M.

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

Cho, M.

M. Cho, Chem. Rev. 108, 1331 (2008).
[CrossRef] [PubMed]

K. Hyeon-Deuk, Y. Tanimura, and M. Cho, J. Chem. Phys. 128, 135102 (2008).
[CrossRef] [PubMed]

Christensson, N.

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Chugh, B.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Cowan, M. L.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

M. L. Cowan, J. P. Ogilvie, and R. J. D. Miller, Chem. Phys. Lett. 386, 184 (2004).
[CrossRef]

Cundiff, S.

Damrauer, N. H.

Dimler, F.

Dwyer, J. R.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Elsaesser, T.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Fayer, M. D.

D. Zimdars, R. S. Francis, C. Ferrante, and M. D. Fayer, J. Chem. Phys. 106, 7498 (1997).
[CrossRef]

Ferrante, C.

D. Zimdars, R. S. Francis, C. Ferrante, and M. D. Fayer, J. Chem. Phys. 106, 7498 (1997).
[CrossRef]

Fleming, G. R.

T. Brixner, T. Mančal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[CrossRef] [PubMed]

Q. Xu, Y. Ma, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 116, 9333 (2002).
[CrossRef]

Francis, R. S.

D. Zimdars, R. S. Francis, C. Ferrante, and M. D. Fayer, J. Chem. Phys. 106, 7498 (1997).
[CrossRef]

Gieseking, B.

Grumstrup, E. M.

Gundogdu, K.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, Chem. Phys. 341, 89 (2007).
[CrossRef]

Halpin, A.

Hamm, P.

Hauer, J.

Hong, J. W.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Huse, N.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Hyeon-Deuk, K.

K. Hyeon-Deuk, Y. Tanimura, and M. Cho, J. Chem. Phys. 128, 135102 (2008).
[CrossRef] [PubMed]

Jonas, D. M.

D. M. Jonas, Annu. Rev. Phys. Chem. 54, 425 (2003).
[CrossRef] [PubMed]

Kauffmann, H. F.

Keusters, D.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, Science 300, 1553 (2003).
[CrossRef] [PubMed]

Kim, J.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Langhojer, F.

Li, X.

Löhrig, T.

Ma, Y.

Q. Xu, Y. Ma, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 116, 9333 (2002).
[CrossRef]

Maddox, J. B.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Mancal, T.

T. Brixner, T. Mančal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[CrossRef] [PubMed]

Matsika, S.

Miller, R. J. D.

V. I. Prokhorenko, A. Halpin, and R. J. D. Miller, Opt. Express 17, 9764 (2009).
[CrossRef] [PubMed]

R. J. D. Miller, A. Paarmann, and V. I. Prokhorenko, Acc. Chem. Res. 42, 1442 (2009).
[CrossRef] [PubMed]

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

M. L. Cowan, J. P. Ogilvie, and R. J. D. Miller, Chem. Phys. Lett. 386, 184 (2004).
[CrossRef]

Milota, F.

Montgomery, M. A.

Moran, A. M.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Mukamel, S.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

S. Mukamel, Annu. Rev. Phys. Chem. 51, 691 (2000).
[CrossRef] [PubMed]

Müllen, K.

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Nelson, K. A.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, Chem. Phys. 341, 89 (2007).
[CrossRef]

Nemeth, A.

Nibbering, E. T. J.

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Nome, R. A.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Ogilvie, J. P.

M. L. Cowan, J. P. Ogilvie, and R. J. D. Miller, Chem. Phys. Lett. 386, 184 (2004).
[CrossRef]

Oskouei, A. A.

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

Paarmann, A.

R. J. D. Miller, A. Paarmann, and V. I. Prokhorenko, Acc. Chem. Res. 42, 1442 (2009).
[CrossRef] [PubMed]

Pascher, T.

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Prokhorenko, V. I.

V. I. Prokhorenko, A. Halpin, and R. J. D. Miller, Opt. Express 17, 9764 (2009).
[CrossRef] [PubMed]

R. J. D. Miller, A. Paarmann, and V. I. Prokhorenko, Acc. Chem. Res. 42, 1442 (2009).
[CrossRef] [PubMed]

Pullerits, T.

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Schanz, R.

Scherer, N. F.

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

Schwarz, C.

Selig, U.

Shim, S.

Sperling, J.

Stiopkin, I. V.

T. Brixner, T. Mančal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[CrossRef] [PubMed]

Q. Xu, Y. Ma, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 116, 9333 (2002).
[CrossRef]

Stone, K. W.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, Chem. Phys. 341, 89 (2007).
[CrossRef]

Suzaki, Y.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, Science 300, 1553 (2003).
[CrossRef] [PubMed]

Tanimura, Y.

K. Hyeon-Deuk, Y. Tanimura, and M. Cho, J. Chem. Phys. 128, 135102 (2008).
[CrossRef] [PubMed]

Tian, P.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, Science 300, 1553 (2003).
[CrossRef] [PubMed]

Tortschanoff, A.

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

Tseng, C.-H.

Turner, D. B.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, Chem. Phys. 341, 89 (2007).
[CrossRef]

van Mourik, F.

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

Volkov, V.

Warren, W. S.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, Science 300, 1553 (2003).
[CrossRef] [PubMed]

Weinacht, T. C.

Xu, Q.

Q. Xu, Y. Ma, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 116, 9333 (2002).
[CrossRef]

Yartsev, A.

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Zanni, M. T.

Zhang, T.

Zimdars, D.

D. Zimdars, R. S. Francis, C. Ferrante, and M. D. Fayer, J. Chem. Phys. 106, 7498 (1997).
[CrossRef]

Acc. Chem. Res. (1)

R. J. D. Miller, A. Paarmann, and V. I. Prokhorenko, Acc. Chem. Res. 42, 1442 (2009).
[CrossRef] [PubMed]

Annu. Rev. Phys. Chem. (2)

S. Mukamel, Annu. Rev. Phys. Chem. 51, 691 (2000).
[CrossRef] [PubMed]

D. M. Jonas, Annu. Rev. Phys. Chem. 54, 425 (2003).
[CrossRef] [PubMed]

Chem. Phys. (2)

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, Chem. Phys. 350, 104 (2008).
[CrossRef]

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, Chem. Phys. 341, 89 (2007).
[CrossRef]

Chem. Phys. Lett. (1)

M. L. Cowan, J. P. Ogilvie, and R. J. D. Miller, Chem. Phys. Lett. 386, 184 (2004).
[CrossRef]

Chem. Rev. (1)

M. Cho, Chem. Rev. 108, 1331 (2008).
[CrossRef] [PubMed]

J. Chem. Phys. (6)

K. Hyeon-Deuk, Y. Tanimura, and M. Cho, J. Chem. Phys. 128, 135102 (2008).
[CrossRef] [PubMed]

D. Zimdars, R. S. Francis, C. Ferrante, and M. D. Fayer, J. Chem. Phys. 106, 7498 (1997).
[CrossRef]

A. M. Moran, J. B. Maddox, J. W. Hong, J. Kim, R. A. Nome, G. C. Bazan, S. Mukamel, and N. F. Scherer, J. Chem. Phys. 124, 194904 (2006).
[CrossRef] [PubMed]

N. Christensson, Y. Avlasevich, A. Yartsev, K. Müllen, T. Pascher, and T. Pullerits, J. Chem. Phys. 132, 174508(2010).
[CrossRef] [PubMed]

Q. Xu, Y. Ma, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 116, 9333 (2002).
[CrossRef]

T. Brixner, T. Mančal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[CrossRef] [PubMed]

J. Mol. Liq. (1)

A. A. Oskouei, O. Bräm, A. Cannizzo, F. van Mourik, A. Tortschanoff, and M. Chergui, J. Mol. Liq. 141, 118 (2008).
[CrossRef]

Nature (1)

M. L. Cowan, B. D. Bruner, N. Huse, J. R. Dwyer, B. Chugh, E. T. J. Nibbering, T. Elsaesser, and R. J. D. Miller, Nature 434, 199 (2005).
[CrossRef] [PubMed]

Opt. Express (4)

Opt. Lett. (3)

Science (1)

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, Science 300, 1553 (2003).
[CrossRef] [PubMed]

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Figures (2)

Fig. 1
Fig. 1

Experimental setup. Four beams in box geometry diffracted off a crossed grating (CG) are parallelized with a first off-axis parabolic mirror (OAP 1). Two delay stages (DS 1 and DS 2) introduce time delays between the excitation pulses. OAP 2 then focuses the beams onto the sample. The footprint of the setup is 20 cm × 30 cm .

Fig. 2
Fig. 2

Results. (a) Transient grating data of PTP in ethanol (black) and ethanol only (gray). Absorptive 2D spectra of PTP in ethanol at (b) T = 300 fs and (c) T = 1300 fs . Contour lines from 10% to 90% of the maximum of the T = 300 fs data are drawn in steps of 10%. (d) Phase stability data of the PTP in ethanol (gray) and fused silica (black, offset by π 20 for clarity) with a long-term standard deviation of λ 65 and λ 85 , respectively.

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