Abstract

A mapping technique is developed to spatially resolve random laser-emission spectra from disordered solid media with an optical gain above the threshold excitation intensity for lasing; the technique is applied to π-conjugated polymer 1ms. By mapping the spatial extent of emission peaks in the random laser spectrum, bright areas that correspond to naturally formed lasing microcavities are unraveled. The size of the obtained microcavities matches the size extracted from the Fourier transform analysis of the laser-emission spectrum. Mapping at increased excitation intensities shows multiple resonant microcavities that lase at increasing threshold intensities.

© 2010 Optical Society of America

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    [CrossRef]
  2. C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
    [CrossRef]
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    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef]

2010 (2)

A. Tulek, R. C. Polson, and Z. V. Vardeny, Nature Phys. 6, 303 (2010).
[CrossRef]

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

2009 (1)

J. Fallert, R. J. B. Dietz, J. Sartor, D. Schneider, and C. K. H. Kalt, Nat. Photon. 3, 279 (2009).
[CrossRef]

2008 (1)

D. S. Wiersma, Nat. Phys. 4, 359 (2008).
[CrossRef]

2007 (4)

A. Tulek and Z. V. Vardeny, Appl. Phys. Lett. 91, 121102 (2007).
[CrossRef]

K. L. van der Molen, R. W. Tjerkstra, A. P. Mosk, and A. Lagendijk, Phys. Rev. Lett. 98, 143901 (2007).
[CrossRef] [PubMed]

C. Vanneste, P. Sebbah, and H. Cao, Phys. Rev. Lett. 98, 143902 (2007).
[CrossRef] [PubMed]

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

2006 (2)

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

G. Strangi, S. Ferjani, V. Barna, A. De Luca, C. Versace, N. Scaramuzza, and R. Bartolino, Opt. Express 14, 7737 (2006).
[CrossRef] [PubMed]

2005 (2)

R. C. Polson and Z. V. Vardeny, Phys. Rev. B 71, 045205 (2005).
[CrossRef]

V. Milner and A. Z. Genack, Phys. Rev. Lett. 94, 073901 (2005).
[CrossRef] [PubMed]

2004 (2)

S. Mujumdar, M. Ricci, R. Torre, and D. S. Wiersma, Phys. Rev. Lett. 93, 053903 (2004).
[CrossRef] [PubMed]

V. M. Apalkov, M. E. Raikh, and B. Shapiro, J. Opt. Soc. Am. B 21, 132 (2004).
[CrossRef]

2003 (2)

A. A. Chabanov, Z. Q. Zhang, and A. Z. Genack, Phys. Rev. Lett. 90, 203903 (2003).
[CrossRef] [PubMed]

R. Polson, M. Raikh, and Z. Vardeny, IEEE J. Sel. Top. Quantum Electron. 9, 120 (2003).
[CrossRef]

2002 (2)

R. C. Polson, Z. V. Vardeny, and D. A. Chinn, Appl. Phys. Lett. 81, 1561 (2002).
[CrossRef]

V. M. Apalkov, M. E. Raikh, and B. Shapiro, Phys. Rev. Lett. 89, 016802 (2002).
[CrossRef] [PubMed]

2000 (1)

R. C. Polson, G. Levina, and Z. V. Vardeny, Appl. Phys. Lett. 76, 3858 (2000).
[CrossRef]

1999 (3)

S. V. Frolov, Z. V. Vardeny, K. Yoshino, A. Zakhidov, and R. H. Baughman, Phys. Rev. B 59, R5284 (1999).
[CrossRef]

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

S. Frolov, Z. Vardeny, A. Zakhidov, and R. Baughman, Opt. Commun. 162, 241 (1999).
[CrossRef]

1994 (1)

N. Lawandry, B. R. M. A. Gomes, and E. Sauvain, Nature 368, 436 (1994).
[CrossRef]

1993 (1)

C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
[CrossRef]

Ania-Castañón, J.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

Apalkov, V. M.

V. M. Apalkov, M. E. Raikh, and B. Shapiro, J. Opt. Soc. Am. B 21, 132 (2004).
[CrossRef]

V. M. Apalkov, M. E. Raikh, and B. Shapiro, Phys. Rev. Lett. 89, 016802 (2002).
[CrossRef] [PubMed]

Auzel, F.

C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
[CrossRef]

Babin, S.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

Barna, V.

Bartolino, R.

Baughman, R.

S. Frolov, Z. Vardeny, A. Zakhidov, and R. Baughman, Opt. Commun. 162, 241 (1999).
[CrossRef]

Baughman, R. H.

S. V. Frolov, Z. V. Vardeny, K. Yoshino, A. Zakhidov, and R. H. Baughman, Phys. Rev. B 59, R5284 (1999).
[CrossRef]

Brito-Silva, A. M.

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

Cao, H.

C. Vanneste, P. Sebbah, and H. Cao, Phys. Rev. Lett. 98, 143902 (2007).
[CrossRef] [PubMed]

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

Chabanov, A. A.

A. A. Chabanov, Z. Q. Zhang, and A. Z. Genack, Phys. Rev. Lett. 90, 203903 (2003).
[CrossRef] [PubMed]

Chang, R. P. H.

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

Chen, X.

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

Chinn, D. A.

R. C. Polson, Z. V. Vardeny, and D. A. Chinn, Appl. Phys. Lett. 81, 1561 (2002).
[CrossRef]

Churkin, D.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

de Araújo, C. B.

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

De Luca, A.

de Matos, C. J. S.

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

Dietz, R. J. B.

J. Fallert, R. J. B. Dietz, J. Sartor, D. Schneider, and C. K. H. Kalt, Nat. Photon. 3, 279 (2009).
[CrossRef]

Ellingham, T.

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

El-Taher, A.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

Fallert, J.

J. Fallert, R. J. B. Dietz, J. Sartor, D. Schneider, and C. K. H. Kalt, Nat. Photon. 3, 279 (2009).
[CrossRef]

Ferjani, S.

Frolov, S.

S. Frolov, Z. Vardeny, A. Zakhidov, and R. Baughman, Opt. Commun. 162, 241 (1999).
[CrossRef]

Frolov, S. V.

S. V. Frolov, Z. V. Vardeny, K. Yoshino, A. Zakhidov, and R. H. Baughman, Phys. Rev. B 59, R5284 (1999).
[CrossRef]

Genack, A. Z.

V. Milner and A. Z. Genack, Phys. Rev. Lett. 94, 073901 (2005).
[CrossRef] [PubMed]

A. A. Chabanov, Z. Q. Zhang, and A. Z. Genack, Phys. Rev. Lett. 90, 203903 (2003).
[CrossRef] [PubMed]

Gomes, A. S. L.

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

Gomes, B. R. M. A.

N. Lawandry, B. R. M. A. Gomes, and E. Sauvain, Nature 368, 436 (1994).
[CrossRef]

Gouedard, C.

C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
[CrossRef]

Harper, P.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

Ho, S. T.

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

Husson, D.

C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
[CrossRef]

Ibbotson, R.

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

Kablukov, S.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

Kalt, C. K. H.

J. Fallert, R. J. B. Dietz, J. Sartor, D. Schneider, and C. K. H. Kalt, Nat. Photon. 3, 279 (2009).
[CrossRef]

Karalekas, V.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

Lagendijk, A.

K. L. van der Molen, R. W. Tjerkstra, A. P. Mosk, and A. Lagendijk, Phys. Rev. Lett. 98, 143901 (2007).
[CrossRef] [PubMed]

Lawandry, N.

N. Lawandry, B. R. M. A. Gomes, and E. Sauvain, Nature 368, 436 (1994).
[CrossRef]

Levina, G.

R. C. Polson, G. Levina, and Z. V. Vardeny, Appl. Phys. Lett. 76, 3858 (2000).
[CrossRef]

Martinez Gámez, M. A.

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

Menezes, L. de S.

C. J. S. de Matos, L. de S. Menezes, A. M. Brito-Silva, M. A. Martinez Gámez, A. S. L. Gomes, and C. B. de Araújo, Phys. Rev. Lett. 99, 153903 (2007).
[CrossRef] [PubMed]

Migus, A.

C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
[CrossRef]

Milner, V.

V. Milner and A. Z. Genack, Phys. Rev. Lett. 94, 073901 (2005).
[CrossRef] [PubMed]

Mosk, A. P.

K. L. van der Molen, R. W. Tjerkstra, A. P. Mosk, and A. Lagendijk, Phys. Rev. Lett. 98, 143901 (2007).
[CrossRef] [PubMed]

Mujumdar, S.

S. Mujumdar, M. Ricci, R. Torre, and D. S. Wiersma, Phys. Rev. Lett. 93, 053903 (2004).
[CrossRef] [PubMed]

Podivilov, E.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

Polson, R.

R. Polson, M. Raikh, and Z. Vardeny, IEEE J. Sel. Top. Quantum Electron. 9, 120 (2003).
[CrossRef]

Polson, R. C.

A. Tulek, R. C. Polson, and Z. V. Vardeny, Nature Phys. 6, 303 (2010).
[CrossRef]

R. C. Polson and Z. V. Vardeny, Phys. Rev. B 71, 045205 (2005).
[CrossRef]

R. C. Polson, Z. V. Vardeny, and D. A. Chinn, Appl. Phys. Lett. 81, 1561 (2002).
[CrossRef]

R. C. Polson, G. Levina, and Z. V. Vardeny, Appl. Phys. Lett. 76, 3858 (2000).
[CrossRef]

Raikh, M.

R. Polson, M. Raikh, and Z. Vardeny, IEEE J. Sel. Top. Quantum Electron. 9, 120 (2003).
[CrossRef]

Raikh, M. E.

V. M. Apalkov, M. E. Raikh, and B. Shapiro, J. Opt. Soc. Am. B 21, 132 (2004).
[CrossRef]

V. M. Apalkov, M. E. Raikh, and B. Shapiro, Phys. Rev. Lett. 89, 016802 (2002).
[CrossRef] [PubMed]

Ricci, M.

S. Mujumdar, M. Ricci, R. Torre, and D. S. Wiersma, Phys. Rev. Lett. 93, 053903 (2004).
[CrossRef] [PubMed]

Sartor, J.

J. Fallert, R. J. B. Dietz, J. Sartor, D. Schneider, and C. K. H. Kalt, Nat. Photon. 3, 279 (2009).
[CrossRef]

Sauteret, C.

C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, J. Opt. Soc. Am. B. 10, 2358 (1993).
[CrossRef]

Sauvain, E.

N. Lawandry, B. R. M. A. Gomes, and E. Sauvain, Nature 368, 436 (1994).
[CrossRef]

Scaramuzza, N.

Schneider, D.

J. Fallert, R. J. B. Dietz, J. Sartor, D. Schneider, and C. K. H. Kalt, Nat. Photon. 3, 279 (2009).
[CrossRef]

Sebbah, P.

C. Vanneste, P. Sebbah, and H. Cao, Phys. Rev. Lett. 98, 143902 (2007).
[CrossRef] [PubMed]

Seelig, E. W.

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

Shapiro, B.

V. M. Apalkov, M. E. Raikh, and B. Shapiro, J. Opt. Soc. Am. B 21, 132 (2004).
[CrossRef]

V. M. Apalkov, M. E. Raikh, and B. Shapiro, Phys. Rev. Lett. 89, 016802 (2002).
[CrossRef] [PubMed]

Strangi, G.

Tjerkstra, R. W.

K. L. van der Molen, R. W. Tjerkstra, A. P. Mosk, and A. Lagendijk, Phys. Rev. Lett. 98, 143901 (2007).
[CrossRef] [PubMed]

Torre, R.

S. Mujumdar, M. Ricci, R. Torre, and D. S. Wiersma, Phys. Rev. Lett. 93, 053903 (2004).
[CrossRef] [PubMed]

Tulek, A.

A. Tulek, R. C. Polson, and Z. V. Vardeny, Nature Phys. 6, 303 (2010).
[CrossRef]

A. Tulek and Z. V. Vardeny, Appl. Phys. Lett. 91, 121102 (2007).
[CrossRef]

Turitsyn, S.

S. Turitsyn, S. Babin, A. El-Taher, P. Harper, D. Churkin, S. Kablukov, J. Ania-Castañón, V. Karalekas, and E. Podivilov, Nat. Photon. 4, 231 (2010).
[CrossRef]

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

van der Molen, K. L.

K. L. van der Molen, R. W. Tjerkstra, A. P. Mosk, and A. Lagendijk, Phys. Rev. Lett. 98, 143901 (2007).
[CrossRef] [PubMed]

Vanneste, C.

C. Vanneste, P. Sebbah, and H. Cao, Phys. Rev. Lett. 98, 143902 (2007).
[CrossRef] [PubMed]

Vardeny, Z.

R. Polson, M. Raikh, and Z. Vardeny, IEEE J. Sel. Top. Quantum Electron. 9, 120 (2003).
[CrossRef]

S. Frolov, Z. Vardeny, A. Zakhidov, and R. Baughman, Opt. Commun. 162, 241 (1999).
[CrossRef]

Vardeny, Z. V.

A. Tulek, R. C. Polson, and Z. V. Vardeny, Nature Phys. 6, 303 (2010).
[CrossRef]

A. Tulek and Z. V. Vardeny, Appl. Phys. Lett. 91, 121102 (2007).
[CrossRef]

R. C. Polson and Z. V. Vardeny, Phys. Rev. B 71, 045205 (2005).
[CrossRef]

R. C. Polson, Z. V. Vardeny, and D. A. Chinn, Appl. Phys. Lett. 81, 1561 (2002).
[CrossRef]

R. C. Polson, G. Levina, and Z. V. Vardeny, Appl. Phys. Lett. 76, 3858 (2000).
[CrossRef]

S. V. Frolov, Z. V. Vardeny, K. Yoshino, A. Zakhidov, and R. H. Baughman, Phys. Rev. B 59, R5284 (1999).
[CrossRef]

Versace, C.

Wang, Q. H.

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

Wiersma, D. S.

D. S. Wiersma, Nat. Phys. 4, 359 (2008).
[CrossRef]

S. Mujumdar, M. Ricci, R. Torre, and D. S. Wiersma, Phys. Rev. Lett. 93, 053903 (2004).
[CrossRef] [PubMed]

Yoshino, K.

S. V. Frolov, Z. V. Vardeny, K. Yoshino, A. Zakhidov, and R. H. Baughman, Phys. Rev. B 59, R5284 (1999).
[CrossRef]

Zakhidov, A.

S. V. Frolov, Z. V. Vardeny, K. Yoshino, A. Zakhidov, and R. H. Baughman, Phys. Rev. B 59, R5284 (1999).
[CrossRef]

S. Frolov, Z. Vardeny, A. Zakhidov, and R. Baughman, Opt. Commun. 162, 241 (1999).
[CrossRef]

Zhang, L.

J. Ania-Castañón, T. Ellingham, R. Ibbotson, X. Chen, L. Zhang, and S. Turitsyn, Phys. Rev. Lett. 96, 023902(2006).
[CrossRef] [PubMed]

Zhang, Z. Q.

A. A. Chabanov, Z. Q. Zhang, and A. Z. Genack, Phys. Rev. Lett. 90, 203903 (2003).
[CrossRef] [PubMed]

Zhao, Y. G.

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys. Rev. Lett. 82, 2278 (1999).
[CrossRef]

Appl. Phys. Lett. (3)

R. C. Polson, G. Levina, and Z. V. Vardeny, Appl. Phys. Lett. 76, 3858 (2000).
[CrossRef]

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Figures (3)

Fig. 1
Fig. 1

(a) Schematic of the experimental setup for imaging RL: L1–L3, lenses; S, sample film; Sp, spectrometer; CCD, CCD camera. (b) Integrated emission spectrum from X = 50 μm . The red diamonds are calculated wavelengths based on an assumption of an underlying circular microcavity having diameter D = 59 m (see text). (c) Power Fourier transform of the emission in (b).

Fig. 2
Fig. 2

(a) RL spectra from positions 50 μm and 175 μm with excitation intensity I = I th = 0.6 μJ / pulse . (b) Mapping intensity of the 633.5 nm mode as indicated by the gray band in (a).

Fig. 3
Fig. 3

Same as in Fig. 2 but for I = 2.5 I th .

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