Abstract

We report on the observation of optically detected magnetic resonance (ODMR) in bismuth-doped silica glass. To explain the results of the experiment we adopted the intramolecular charge transfer model for Bi5+On2 molecules in the frame of a semiempirical molecular orbitals approach. The results of our calculations are in good agreement with observed features of luminescence and ODMR experiments.

© 2009 Optical Society of America

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    [CrossRef]
  2. E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
    [CrossRef]
  3. E. Dianov, A. Shubin, M. Melkumov, O. Medvedkov, and I. Bufetov, J. Opt. Soc. Am. B 24, 1749 (2007).
    [CrossRef]
  4. I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
    [CrossRef]
  5. H.-P. Xia and X.-J. Wang, Appl. Phys. Lett. 89, 051917 (2006).
    [CrossRef]
  6. V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.
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    [CrossRef] [PubMed]
  8. M. Peng, J. Qiu, D. Chen, X. Meng, and C. Zhu, Opt. Lett. 30, 2433 (2005).
    [CrossRef] [PubMed]
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    [CrossRef]
  10. V. O. Sokolov, V. G. Plotnichenko, and E. M. Dianov, Opt. Lett. 33, 1488 (2008).
    [CrossRef] [PubMed]
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    [CrossRef]
  12. B. Henderson and G. F. Imbusch, Optical Spectroscopy of Inorganic Solids (Oxford University, 2006).
  13. L. D. Landau and E. M. Lifshits, Quantum Mechanics. Nonrelativistic Theory, 3rd ed. (Nauka, 1974).
  14. J. E. Mack and M. Fromer, Phys. Rev. 48, 357 (1935).
    [CrossRef]
  15. R. Winkler, Spin-Orbit Coupling Effects in Two-Dimensional Electron and Hole Systems (Springer, 2003).
    [CrossRef]
  16. E. F. Kustov, L. I. Bulatov, V. V. Dvoyrin, and V. M. Mashinsky, Opt. Lett. 34, 1549 (2009).
    [CrossRef] [PubMed]

2009 (1)

2008 (2)

V. O. Sokolov, V. G. Plotnichenko, and E. M. Dianov, Opt. Lett. 33, 1488 (2008).
[CrossRef] [PubMed]

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

2007 (2)

E. Dianov, A. Shubin, M. Melkumov, O. Medvedkov, and I. Bufetov, J. Opt. Soc. Am. B 24, 1749 (2007).
[CrossRef]

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

2006 (2)

H.-P. Xia and X.-J. Wang, Appl. Phys. Lett. 89, 051917 (2006).
[CrossRef]

J. Ren, L. Yang, J. Qiu, D. Chen, X. Jiang, and C. Zhu, Solid State Commun. 140, 38 (2006).
[CrossRef]

2005 (3)

2001 (1)

Y. Fujimoto and M. Nakatsuka, Jpn. J. Appl. Phys. 40, L279 (2001).
[CrossRef]

1935 (1)

J. E. Mack and M. Fromer, Phys. Rev. 48, 357 (1935).
[CrossRef]

Bigot, L.

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

Bowmans, G.

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

Bufetov, I.

Bulatov, L. I.

Chen, D.

Dianov, E.

Dianov, E. M.

V. O. Sokolov, V. G. Plotnichenko, and E. M. Dianov, Opt. Lett. 33, 1488 (2008).
[CrossRef] [PubMed]

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

Douay, M.

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

Dvoyrin, V. V.

E. F. Kustov, L. I. Bulatov, V. V. Dvoyrin, and V. M. Mashinsky, Opt. Lett. 34, 1549 (2009).
[CrossRef] [PubMed]

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

Favre, A.

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

Fromer, M.

J. E. Mack and M. Fromer, Phys. Rev. 48, 357 (1935).
[CrossRef]

Fujimoto, Y.

Y. Fujimoto and M. Nakatsuka, Jpn. J. Appl. Phys. 40, L279 (2001).
[CrossRef]

Guryanov, A. N.

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

Gur'yanov, A. N.

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

Henderson, B.

B. Henderson and G. F. Imbusch, Optical Spectroscopy of Inorganic Solids (Oxford University, 2006).

Imbusch, G. F.

B. Henderson and G. F. Imbusch, Optical Spectroscopy of Inorganic Solids (Oxford University, 2006).

Jiang, X.

J. Ren, L. Yang, J. Qiu, D. Chen, X. Jiang, and C. Zhu, Solid State Commun. 140, 38 (2006).
[CrossRef]

X. Meng, J. Qiu, M. Peng, D. Chen, Q. Zhao, X. Jiang, and C. Zhu, Opt. Express 13, 1628 (2005).
[CrossRef] [PubMed]

Kustov, E. F.

Landau, L. D.

L. D. Landau and E. M. Lifshits, Quantum Mechanics. Nonrelativistic Theory, 3rd ed. (Nauka, 1974).

Lerouge, A.

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

Lifshits, E. M.

L. D. Landau and E. M. Lifshits, Quantum Mechanics. Nonrelativistic Theory, 3rd ed. (Nauka, 1974).

Mack, J. E.

J. E. Mack and M. Fromer, Phys. Rev. 48, 357 (1935).
[CrossRef]

Mashinsky, V. M.

E. F. Kustov, L. I. Bulatov, V. V. Dvoyrin, and V. M. Mashinsky, Opt. Lett. 34, 1549 (2009).
[CrossRef] [PubMed]

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

Medvedkov, O.

Melkumov, M.

Meng, X.

Nakatsuka, M.

Y. Fujimoto and M. Nakatsuka, Jpn. J. Appl. Phys. 40, L279 (2001).
[CrossRef]

Peng, M.

Plotnichenko, V. G.

Pureur, V.

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

Qiu, J.

Razdobreev, I.

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

Ren, J.

J. Ren, L. Yang, J. Qiu, D. Chen, X. Jiang, and C. Zhu, Solid State Commun. 140, 38 (2006).
[CrossRef]

Shubin, A.

Sokolov, V. O.

Truong, V. G.

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

Umnikov, A. A.

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

Wang, X.-J.

H.-P. Xia and X.-J. Wang, Appl. Phys. Lett. 89, 051917 (2006).
[CrossRef]

Winkler, R.

R. Winkler, Spin-Orbit Coupling Effects in Two-Dimensional Electron and Hole Systems (Springer, 2003).
[CrossRef]

Xia, H.-P.

H.-P. Xia and X.-J. Wang, Appl. Phys. Lett. 89, 051917 (2006).
[CrossRef]

Yang, L.

J. Ren, L. Yang, J. Qiu, D. Chen, X. Jiang, and C. Zhu, Solid State Commun. 140, 38 (2006).
[CrossRef]

Yashkov, M. V.

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

Zhao, Q.

Zhu, C.

Appl. Phys. Lett. (3)

I. Razdobreev, L. Bigot, V. Pureur, A. Favre, G. Bowmans, and M. Douay, Appl. Phys. Lett. 90, 031103 (2007).
[CrossRef]

H.-P. Xia and X.-J. Wang, Appl. Phys. Lett. 89, 051917 (2006).
[CrossRef]

V. G. Truong, L. Bigot, A. Lerouge, M. Douay, and I. Razdobreev, Appl. Phys. Lett. 92, 041908 (2008).
[CrossRef]

J. Opt. Soc. Am. B (1)

Jpn. J. Appl. Phys. (1)

Y. Fujimoto and M. Nakatsuka, Jpn. J. Appl. Phys. 40, L279 (2001).
[CrossRef]

Opt. Express (1)

Opt. Lett. (3)

Phys. Rev. (1)

J. E. Mack and M. Fromer, Phys. Rev. 48, 357 (1935).
[CrossRef]

Solid State Commun. (1)

J. Ren, L. Yang, J. Qiu, D. Chen, X. Jiang, and C. Zhu, Solid State Commun. 140, 38 (2006).
[CrossRef]

Sov. J. Quantum Electron. (1)

E. M. Dianov, V. V. Dvoyrin, V. M. Mashinsky, A. A. Umnikov, M. V. Yashkov, and A. N. Gur'yanov, Sov. J. Quantum Electron. 35, 1083 (2005).
[CrossRef]

Other (4)

V. V. Dvoyrin, V. M. Mashinsky, E. M. Dianov, A. A. Umnikov, M. V. Yashkov, and A. N. Guryanov, in 31st European Conference on Optical Communication (IEEE, 2005), Vol. 4, p. 949.

R. Winkler, Spin-Orbit Coupling Effects in Two-Dimensional Electron and Hole Systems (Springer, 2003).
[CrossRef]

B. Henderson and G. F. Imbusch, Optical Spectroscopy of Inorganic Solids (Oxford University, 2006).

L. D. Landau and E. M. Lifshits, Quantum Mechanics. Nonrelativistic Theory, 3rd ed. (Nauka, 1974).

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Figures (5)

Fig. 1
Fig. 1

PL signal of SAY:Bi sample: open circles, experiment; dashed lines, Gaussian decomposition.

Fig. 2
Fig. 2

ODMR signal from SAY:Bi sample in the wavelength region of 1100 1300 nm , where μ and B are Bohr magneton and MF, respectively.

Fig. 3
Fig. 3

CF P 1 3 and P 2 3 energy levels of Bi + ion.

Fig. 4
Fig. 4

(a) Structure of electronic transitions between GS and mixed unfilled MO configurations. On the right: e h radiative recombination between filled MO configurations t 1 6 [ h 0 ] , e 4 [ h 0 ] , t 2 6 [ h 0 ] , and hole t 2 5 [ h 1 ] , where [ h 1 ] is a hole. (b) Detailed energy diagram of e h transition between t 1 6 [ h 0 ] ES and t 1 5 [ h 1 ] GS. The interactions responsible for the splitting of energy levels are indicated at the top of the figure.

Fig. 5
Fig. 5

Dependence of g factors of t 1 ES and Γ 4 GS as a function of ratio A 20 ξ p , where A 20 and ξ p are the CF potential of trigonal distortion ( C 3 V ) and the constant of SO interaction of p electrons, respectively.

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