Measurement of the second hyperpolarizability of linear conjugated polymer based on attenuated-total-reflection technique

Xiang Zheng; Xiaoxu Deng; Zhuangqi Cao; Qishun Shen; Honggen Li; Wei Wei; Feng Liu

doi:10.1364/OL.33.000887

Measurement of the second hyperpolarizability of linear conjugated polymer based on attenuated-total-reflection technique

Xiang Zheng, Xiaoxu Deng, Zhuangqi Cao, Qishun Shen, Honggen Li, Wei Wei, and Feng Liu

Optics Letters
Vol. 33,
Issue 8,
pp. 887-889
(2008)
•https://doi.org/10.1364/OL.33.000887

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Xiang Zheng, Xiaoxu Deng, Zhuangqi Cao, Qishun Shen, Honggen Li, Wei Wei, and Feng Liu, "Measurement of the second hyperpolarizability of linear conjugated polymer based on attenuated-total-reflection technique," Opt. Lett. 33, 887-889 (2008)

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Related Topics
Table of Contents Category
- Materials
Optics & Photonics Topics
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The topics in this list come from the OSA Optics and Photonics Topics applied to this article.
Previously assigned OCIS codes
- Nonlinear optical materials (160.4330)
- Polymers (160.5470)
- Optical nonlinearities in organic materials (190.4710)
- Guided waves (310.2790)

About this Article
History
- Original Manuscript: January 30, 2008
- Revised Manuscript: March 9, 2008
- Manuscript Accepted: March 11, 2008
- Published: April 14, 2008

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Abstract

Based on the attenuated-total-reflection technique, a new method has been proposed to determine the second hyperpolarizability $γ (- ω_{4}; ω_{3}, ω_{2}, ω_{1})$ of the linear conjugated polymer in the off-resonant region by means of quadratic electro-optic effect. An important feature of this method is the absence of a high-power pulse laser, resulting in more convenience and cost effectivity than other techniques.

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Wavelength (nm)	$n (ω)$	$γ (- ω; 0, 0, ω)$ $(\times 10^{- 44} m^{5} ∕ V^{2})$
532	1.614	$1.81 \pm 0.08$
650	1.588	$1.04 \pm 0.05$
780	1.576	$0.801 \pm 0.026$
832	1.571	$0.768 \pm 0.023$
980	1.566	$0.687 \pm 0.032$
1064	1.562	$0.653 \pm 0.051$
1310	1.558	$0.603 \pm 0.032$
1550	1.554	$0.578 \pm 0.041$

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