Abstract

Based on the attenuated-total-reflection technique, a new method has been proposed to determine the second hyperpolarizability γ(ω4;ω3,ω2,ω1) of the linear conjugated polymer in the off-resonant region by means of quadratic electro-optic effect. An important feature of this method is the absence of a high-power pulse laser, resulting in more convenience and cost effectivity than other techniques.

© 2008 Optical Society of America

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