Abstract

A new scheme for single attosecond pulse generation from asymmetric molecules with a multicycle laser pulse is proposed. It is shown that both even and odd harmonics are generated from the asymmetric molecules, and the attosecond pulses are produced every full cycle of the driving laser field rather than each half-cycle. By filtering the harmonics in the cutoff of the spectrum, a single attosecond pulse can be obtained with a multicycle laser pulse with a duration of 2 times longer than the few-cycle pulse conventionally used.

© 2007 Optical Society of America

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  1. P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  3. M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef]

2006 (2)

T. Pfeifer, L. Gallmann, M. J. Abel, D. M. Neumark, and S. R. Leone, Opt. Lett. 31, 975 (2006).
[CrossRef] [PubMed]

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

2005 (2)

G. L. Kamta and A. D. Bandrauk, Phys. Rev. Lett. 94, 203003 (2005).
[CrossRef] [PubMed]

P. F. Lan, P. X. Lu, W. Cao, and X. L. Wang, Phys. Rev. E 72, 066501 (2005).
[CrossRef]

2004 (2)

2003 (2)

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

H. Stapelfeldt and T. Seideman, Rev. Mod. Phys. 75, 543 (2003).
[CrossRef]

2002 (1)

A. E. Kaplan and P. L. Shkolnikov, Phys. Rev. Lett. 88, 074801 (2002).
[CrossRef] [PubMed]

2001 (2)

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

1998 (1)

S. E. Harris and A. V. Sokolov, Phys. Rev. Lett. 81, 2894 (1998).
[CrossRef]

1997 (1)

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, Phys. Rev. Lett. 78, 1251 (1997).
[CrossRef]

1996 (1)

P. Antoine, A. L'Huillier, and M. Lewenstein, Phys. Rev. Lett. 77, 1234 (1996).
[CrossRef] [PubMed]

1995 (1)

M. Ivanov, P. B. Corkum, T. Zuo, and A. Bandrauk, Phys. Rev. Lett. 74, 2933 (1995).
[CrossRef] [PubMed]

1994 (2)

1993 (2)

I. Ben-Itzhak, I. Gerther, O. Heber, and B. Rosner, Phys. Rev. Lett. 71, 1347 (1993).
[CrossRef] [PubMed]

P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993).
[CrossRef] [PubMed]

1991 (1)

B. Friedrich and D. R. Herschbach, Nature 353, 412 (1991).
[CrossRef]

Abel, M. J.

Agostini, P.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Antoine, P.

P. Antoine, A. L'Huillier, and M. Lewenstein, Phys. Rev. Lett. 77, 1234 (1996).
[CrossRef] [PubMed]

Augé, F.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Balcou, P.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Baltuska, A.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Bandrauk, A.

M. Ivanov, P. B. Corkum, T. Zuo, and A. Bandrauk, Phys. Rev. Lett. 74, 2933 (1995).
[CrossRef] [PubMed]

Bandrauk, A. D.

G. L. Kamta and A. D. Bandrauk, Phys. Rev. Lett. 94, 203003 (2005).
[CrossRef] [PubMed]

Ben-Itzhak, I.

I. Ben-Itzhak, I. Gerther, O. Heber, and B. Rosner, Phys. Rev. Lett. 71, 1347 (1993).
[CrossRef] [PubMed]

Brabec, T.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Breer, P.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Burnett, N. H.

Cao, W.

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

P. F. Lan, P. X. Lu, W. Cao, and X. L. Wang, Phys. Rev. E 72, 066501 (2005).
[CrossRef]

Christov, I. P.

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, Phys. Rev. Lett. 78, 1251 (1997).
[CrossRef]

Corkum, P.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Corkum, P. B.

M. Ivanov, P. B. Corkum, T. Zuo, and A. Bandrauk, Phys. Rev. Lett. 74, 2933 (1995).
[CrossRef] [PubMed]

P. B. Corkum, N. H. Burnett, and M. Y. Ivanov, Opt. Lett. 19, 1870 (1994).
[CrossRef] [PubMed]

P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993).
[CrossRef] [PubMed]

Drescher, M.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Friedrich, B.

B. Friedrich and D. R. Herschbach, Nature 353, 412 (1991).
[CrossRef]

Gallmann, L.

Gerther, I.

I. Ben-Itzhak, I. Gerther, O. Heber, and B. Rosner, Phys. Rev. Lett. 71, 1347 (1993).
[CrossRef] [PubMed]

Gohle, Ch.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Goulielmakis, E.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Hänsch, T. W.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Harris, S. E.

S. E. Harris and A. V. Sokolov, Phys. Rev. Lett. 81, 2894 (1998).
[CrossRef]

Heber, O.

I. Ben-Itzhak, I. Gerther, O. Heber, and B. Rosner, Phys. Rev. Lett. 71, 1347 (1993).
[CrossRef] [PubMed]

Heinzmann, U.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Hentschel, M.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Herschbach, D. R.

B. Friedrich and D. R. Herschbach, Nature 353, 412 (1991).
[CrossRef]

Holzwarth, R.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Hou, B.

Ivanov, M.

M. Ivanov, P. B. Corkum, T. Zuo, and A. Bandrauk, Phys. Rev. Lett. 74, 2933 (1995).
[CrossRef] [PubMed]

Ivanov, M. Y.

Kamta, G. L.

G. L. Kamta and A. D. Bandrauk, Phys. Rev. Lett. 94, 203003 (2005).
[CrossRef] [PubMed]

Kanai, T.

T. Sekikawa, A. Kosuge, T. Kanai, and S. Watanabe, Nature 432, 605 (2004).
[CrossRef] [PubMed]

Kaplan, A. E.

A. E. Kaplan and P. L. Shkolnikov, Phys. Rev. Lett. 88, 074801 (2002).
[CrossRef] [PubMed]

A. E. Kaplan, Phys. Rev. Lett. 73, 1243 (1994).
[CrossRef] [PubMed]

Kapteyn, H. C.

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, Phys. Rev. Lett. 78, 1251 (1997).
[CrossRef]

Kienberger, R.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Kosuge, A.

T. Sekikawa, A. Kosuge, T. Kanai, and S. Watanabe, Nature 432, 605 (2004).
[CrossRef] [PubMed]

Krausz, F.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Lan, P F.

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

Lan, P. F.

P. F. Lan, P. X. Lu, W. Cao, and X. L. Wang, Phys. Rev. E 72, 066501 (2005).
[CrossRef]

Leone, S. R.

Lewenstein, M.

P. Antoine, A. L'Huillier, and M. Lewenstein, Phys. Rev. Lett. 77, 1234 (1996).
[CrossRef] [PubMed]

L'Huillier, A.

P. Antoine, A. L'Huillier, and M. Lewenstein, Phys. Rev. Lett. 77, 1234 (1996).
[CrossRef] [PubMed]

Lu, P. X.

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

P. F. Lan, P. X. Lu, W. Cao, and X. L. Wang, Phys. Rev. E 72, 066501 (2005).
[CrossRef]

Milosevic, N.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Mourou, G. A.

Muller, H. G.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Mullot, G.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Murnane, M. M.

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, Phys. Rev. Lett. 78, 1251 (1997).
[CrossRef]

Naumova, N. M.

Nees, J. A.

Neumark, D. M.

Paul, P. M.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Pfeifer, T.

Reider, G. A.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Rosner, B.

I. Ben-Itzhak, I. Gerther, O. Heber, and B. Rosner, Phys. Rev. Lett. 71, 1347 (1993).
[CrossRef] [PubMed]

Seideman, T.

H. Stapelfeldt and T. Seideman, Rev. Mod. Phys. 75, 543 (2003).
[CrossRef]

Sekikawa, T.

T. Sekikawa, A. Kosuge, T. Kanai, and S. Watanabe, Nature 432, 605 (2004).
[CrossRef] [PubMed]

Shkolnikov, P. L.

A. E. Kaplan and P. L. Shkolnikov, Phys. Rev. Lett. 88, 074801 (2002).
[CrossRef] [PubMed]

Sokolov, A. V.

S. E. Harris and A. V. Sokolov, Phys. Rev. Lett. 81, 2894 (1998).
[CrossRef]

Sokolov, I. V.

Spielmann, C.

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

Srinzi, A.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Stapelfeldt, H.

H. Stapelfeldt and T. Seideman, Rev. Mod. Phys. 75, 543 (2003).
[CrossRef]

Toma, E. S.

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

Udem, Th.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Uiberacker, M.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Wang, X. L.

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

P. F. Lan, P. X. Lu, W. Cao, and X. L. Wang, Phys. Rev. E 72, 066501 (2005).
[CrossRef]

Watanabe, S.

T. Sekikawa, A. Kosuge, T. Kanai, and S. Watanabe, Nature 432, 605 (2004).
[CrossRef] [PubMed]

Yakovlev, V. S.

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

Yang, G.

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

Zuo, T.

M. Ivanov, P. B. Corkum, T. Zuo, and A. Bandrauk, Phys. Rev. Lett. 74, 2933 (1995).
[CrossRef] [PubMed]

Nature (4)

M. Hentschel, R. Kienberger, C. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, Nature 414, 509 (2001).
[CrossRef] [PubMed]

A. Baltuska, Th. Udem, M. Uiberacker, M. Hentschel, E. Goulielmakis, Ch. Gohle, R. Holzwarth, V. S. Yakovlev, A. Srinzi, T. W. Hänsch, and F. Krausz, Nature 421, 611 (2003).
[CrossRef] [PubMed]

T. Sekikawa, A. Kosuge, T. Kanai, and S. Watanabe, Nature 432, 605 (2004).
[CrossRef] [PubMed]

B. Friedrich and D. R. Herschbach, Nature 353, 412 (1991).
[CrossRef]

Opt. Lett. (3)

Phys. Rev. A (1)

P F. Lan, P. X. Lu, W. Cao, X. L. Wang, and G. Yang, Phys. Rev. A 74, 063411 (2006).
[CrossRef]

Phys. Rev. E (1)

P. F. Lan, P. X. Lu, W. Cao, and X. L. Wang, Phys. Rev. E 72, 066501 (2005).
[CrossRef]

Phys. Rev. Lett. (9)

M. Ivanov, P. B. Corkum, T. Zuo, and A. Bandrauk, Phys. Rev. Lett. 74, 2933 (1995).
[CrossRef] [PubMed]

P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993).
[CrossRef] [PubMed]

I. Ben-Itzhak, I. Gerther, O. Heber, and B. Rosner, Phys. Rev. Lett. 71, 1347 (1993).
[CrossRef] [PubMed]

G. L. Kamta and A. D. Bandrauk, Phys. Rev. Lett. 94, 203003 (2005).
[CrossRef] [PubMed]

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, Phys. Rev. Lett. 78, 1251 (1997).
[CrossRef]

P. Antoine, A. L'Huillier, and M. Lewenstein, Phys. Rev. Lett. 77, 1234 (1996).
[CrossRef] [PubMed]

A. E. Kaplan, Phys. Rev. Lett. 73, 1243 (1994).
[CrossRef] [PubMed]

S. E. Harris and A. V. Sokolov, Phys. Rev. Lett. 81, 2894 (1998).
[CrossRef]

A. E. Kaplan and P. L. Shkolnikov, Phys. Rev. Lett. 88, 074801 (2002).
[CrossRef] [PubMed]

Rev. Mod. Phys. (1)

H. Stapelfeldt and T. Seideman, Rev. Mod. Phys. 75, 543 (2003).
[CrossRef]

Science (1)

P. M. Paul, E. S. Toma, P. Breer, G. Mullot, F. Augé, P. Balcou, H. G. Muller, and P. Agostini, Science 292, 1689 (2001).
[CrossRef] [PubMed]

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Figures (3)

Fig. 1
Fig. 1

(a) Harmonic spectrum of HeH 2 + in the plane laser field. (b) Temporal profiles of the attosecond pulses by superposing the harmonics in the cutoff from 270th to 280th.

Fig. 2
Fig. 2

Combined Coulomb and driving field potential V ( z ) + E z for HeH 2 + along the molecular axis. The arrows are drawn at the energy level of the dressed initial state of HeH 2 + .

Fig. 3
Fig. 3

Temporal profiles of the attosecond pulses in the interaction of HeH 2 + with (a) a 12 fs cosine laser pulse, (b) a 12 fs sine laser pulse.

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