Abstract

The combination of broadband pulses from a photonic crystal fiber (PCF) pumped by a standard 100 fs oscillator and pulse shaping is successfully employed for coherently controlled nonlinear spectroscopy. The pulse shaper manages not only to compress the PCF supercontinuum in a closed-loop optimization scheme but also to manipulate the phase at the same time for quantum control applications. This approach is demonstrated by single-beam coherent anti-Stokes Raman microspectroscopy and should be, due to its simplicity, well suited for general applications in nonlinear microscopy.

© 2006 Optical Society of America

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  1. P. St. J. Russell, Science 299, 358 (2003).
    [CrossRef] [PubMed]
  2. V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
    [CrossRef]
  3. H. N. Paulsen, K. M. Hilligsoe, J. Thogersen, S. R. Keiding, and J. J. Larsen, Opt. Lett. 28, 1123 (2003).
    [CrossRef] [PubMed]
  4. H. Kano and H. Hamaguchi, Appl. Phys. Lett. 85, 4298 (2004).
    [CrossRef]
  5. T. W. Kee and M. T. Cicerone, Opt. Lett. 29, 2701 (2004).
    [CrossRef] [PubMed]
  6. S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
    [CrossRef]
  7. J. M. Dudley, X. Gu, L. Xu, M. Kimmel, E. Zeek, P. O'Shea, R. Trebino, S. Coen, and R. S. Windeler, Opt. Express 10, 1215 (2002).
    [PubMed]
  8. S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
    [CrossRef]
  9. M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
    [CrossRef]
  10. B. Schenkel, R. Paschotta, and U. Keller, J. Opt. Soc. Am. B 22, 687 (2005).
    [CrossRef]
  11. A. M. Weiner, Rev. Sci. Instrum. 71, 1929 (2000).
    [CrossRef]
  12. H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
    [CrossRef] [PubMed]
  13. I. Pastirk, J. M. Dela Cruz, K. A. Walowicz, V. V. Lozovoy, and M. Dantus, Opt. Express 11, 1695 (2003).
    [CrossRef] [PubMed]
  14. D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
    [CrossRef]
  15. N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
    [CrossRef] [PubMed]
  16. N. Dudovich, D. Oron, and Y. Silberberg, J. Chem. Phys. 118, 9208 (2003).
    [CrossRef]
  17. B. von Vacano, W. Wohlleben, and M. Motzkus, "Single-beam CARS spectroscopy applied to low-wavenumber vibrational modes," J. Raman Spectrosc. (to be published). [DOI10.1002/jrs1457]
  18. A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
    [CrossRef]
  19. J. X. Cheng and X. S. Xie, J. Phys. Chem. B 108, 827 (2004).
    [CrossRef]
  20. E. O. Potma, D. J. Jones, J. X. Cheng, X. S. Xie, and J. Ye, Opt. Lett. 27, 1168 (2002).
    [CrossRef]
  21. M. Hashimoto and T. Araki, Opt. Lett. 25, 1768 (2000).
    [CrossRef]
  22. A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
    [CrossRef] [PubMed]
  23. R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
    [CrossRef]
  24. T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
    [CrossRef]
  25. D. Yelin, D. Meshulach, and Y. Silberberg, Opt. Lett. 22, 1793 (1997).
    [CrossRef]
  26. D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
    [CrossRef]

2005 (1)

2004 (5)

J. X. Cheng and X. S. Xie, J. Phys. Chem. B 108, 827 (2004).
[CrossRef]

H. Kano and H. Hamaguchi, Appl. Phys. Lett. 85, 4298 (2004).
[CrossRef]

T. W. Kee and M. T. Cicerone, Opt. Lett. 29, 2701 (2004).
[CrossRef] [PubMed]

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
[CrossRef]

2003 (5)

N. Dudovich, D. Oron, and Y. Silberberg, J. Chem. Phys. 118, 9208 (2003).
[CrossRef]

P. St. J. Russell, Science 299, 358 (2003).
[CrossRef] [PubMed]

H. N. Paulsen, K. M. Hilligsoe, J. Thogersen, S. R. Keiding, and J. J. Larsen, Opt. Lett. 28, 1123 (2003).
[CrossRef] [PubMed]

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

I. Pastirk, J. M. Dela Cruz, K. A. Walowicz, V. V. Lozovoy, and M. Dantus, Opt. Express 11, 1695 (2003).
[CrossRef] [PubMed]

2002 (5)

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef] [PubMed]

E. O. Potma, D. J. Jones, J. X. Cheng, X. S. Xie, and J. Ye, Opt. Lett. 27, 1168 (2002).
[CrossRef]

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

J. M. Dudley, X. Gu, L. Xu, M. Kimmel, E. Zeek, P. O'Shea, R. Trebino, S. Coen, and R. S. Windeler, Opt. Express 10, 1215 (2002).
[PubMed]

2001 (1)

D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
[CrossRef]

2000 (3)

M. Hashimoto and T. Araki, Opt. Lett. 25, 1768 (2000).
[CrossRef]

A. M. Weiner, Rev. Sci. Instrum. 71, 1929 (2000).
[CrossRef]

H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
[CrossRef] [PubMed]

1999 (1)

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

1997 (3)

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

D. Yelin, D. Meshulach, and Y. Silberberg, Opt. Lett. 22, 1793 (1997).
[CrossRef]

1990 (1)

A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
[CrossRef] [PubMed]

Adachi, M.

M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
[CrossRef]

Akimov, D. A.

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

Alfimov, M. V.

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

Apai, P.

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

Araki, T.

Balazs, J.

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

Baumert, T.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

Brixner, T.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

Busch, F.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

Chen, T.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

Cheng, J. X.

Cicerone, M. T.

Coen, S.

Cruz, J. M.

Dantus, M.

de Vivie-Riedle, R.

H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
[CrossRef] [PubMed]

DeLong, K. W.

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

Dudley, J. M.

Dudovich, N.

N. Dudovich, D. Oron, and Y. Silberberg, J. Chem. Phys. 118, 9208 (2003).
[CrossRef]

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef] [PubMed]

Fittinghoff, D. N.

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

Frey, S.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
[CrossRef]

Gerber, G.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

Gu, X.

Hamaguchi, H.

H. Kano and H. Hamaguchi, Appl. Phys. Lett. 85, 4298 (2004).
[CrossRef]

Hashimoto, M.

Hilligsoe, K. M.

Holtom, G. R.

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Ivanov, A. A.

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

Johnson, E.

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

Jones, D. J.

Kane, D. J.

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

Kano, H.

H. Kano and H. Hamaguchi, Appl. Phys. Lett. 85, 4298 (2004).
[CrossRef]

Kee, T. W.

Keiding, S. R.

Keller, U.

Kiefer, W.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

Kimmel, M.

Kompa, K. L.

D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
[CrossRef]

Kompa, K.-L.

H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
[CrossRef] [PubMed]

Konorov, S. O.

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

Krumbugel, M. A.

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

Lako, S.

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

Larsen, J. J.

Leaird, D. E.

A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
[CrossRef] [PubMed]

Lozovoy, V. V.

Materny, A.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

Meshulach, D.

Morita, R.

M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
[CrossRef]

Motzkus, M.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
[CrossRef]

H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
[CrossRef] [PubMed]

B. von Vacano, W. Wohlleben, and M. Motzkus, "Single-beam CARS spectroscopy applied to low-wavenumber vibrational modes," J. Raman Spectrosc. (to be published). [DOI10.1002/jrs1457]

Nagarajan, V.

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

Nelson, K. A.

A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
[CrossRef] [PubMed]

Oron, D.

N. Dudovich, D. Oron, and Y. Silberberg, J. Chem. Phys. 118, 9208 (2003).
[CrossRef]

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef] [PubMed]

O'Shea, P.

Parson, W.

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

Paschotta, R.

Pastirk, I.

Paulsen, H. N.

Potma, E. O.

Rabitz, H.

H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
[CrossRef] [PubMed]

Richman, B. A.

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

Russell, P. St.

P. St. J. Russell, Science 299, 358 (2003).
[CrossRef] [PubMed]

Schellenberg, P.

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

Schenkel, B.

Seres, J.

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

Seyfried, V.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

Silberberg, Y.

N. Dudovich, D. Oron, and Y. Silberberg, J. Chem. Phys. 118, 9208 (2003).
[CrossRef]

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef] [PubMed]

D. Yelin, D. Meshulach, and Y. Silberberg, Opt. Lett. 22, 1793 (1997).
[CrossRef]

Strehle, M.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

Sweetser, J. N.

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

Szipocs, R.

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

Thogersen, J.

Trebino, R.

J. M. Dudley, X. Gu, L. Xu, M. Kimmel, E. Zeek, P. O'Shea, R. Trebino, S. Coen, and R. S. Windeler, Opt. Express 10, 1215 (2002).
[PubMed]

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

von Vacano, B.

B. von Vacano, W. Wohlleben, and M. Motzkus, "Single-beam CARS spectroscopy applied to low-wavenumber vibrational modes," J. Raman Spectrosc. (to be published). [DOI10.1002/jrs1457]

Walowicz, K. A.

Weiner, A. M.

A. M. Weiner, Rev. Sci. Instrum. 71, 1929 (2000).
[CrossRef]

A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
[CrossRef] [PubMed]

Wiederrecht, G. P.

A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
[CrossRef] [PubMed]

Windeler, R.

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

Windeler, R. S.

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

J. M. Dudley, X. Gu, L. Xu, M. Kimmel, E. Zeek, P. O'Shea, R. Trebino, S. Coen, and R. S. Windeler, Opt. Express 10, 1215 (2002).
[PubMed]

Wohlleben, W.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

B. von Vacano, W. Wohlleben, and M. Motzkus, "Single-beam CARS spectroscopy applied to low-wavenumber vibrational modes," J. Raman Spectrosc. (to be published). [DOI10.1002/jrs1457]

Xie, X. S.

J. X. Cheng and X. S. Xie, J. Phys. Chem. B 108, 827 (2004).
[CrossRef]

E. O. Potma, D. J. Jones, J. X. Cheng, X. S. Xie, and J. Ye, Opt. Lett. 27, 1168 (2002).
[CrossRef]

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Xu, L.

Yamane, K.

M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
[CrossRef]

Yamashita, M.

M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
[CrossRef]

Ye, J.

Yelin, D.

Zeek, E.

Zeidler, D.

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
[CrossRef]

Zheltikov, A. M.

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

Zumbusch, A.

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Appl. Phys. B (3)

S. Lako, J. Seres, P. Apai, J. Balazs, R. S. Windeler, and R. Szipocs, Appl. Phys. B 76, 267 (2003).
[CrossRef]

S. O. Konorov, D. A. Akimov, A. A. Ivanov, M. V. Alfimov, and A. M. Zheltikov, Appl. Phys. B 78, 565 (2004).
[CrossRef]

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl. Phys. B 65, 779 (1997).
[CrossRef]

Appl. Phys. Lett. (1)

H. Kano and H. Hamaguchi, Appl. Phys. Lett. 85, 4298 (2004).
[CrossRef]

IEEE Photon. Technol. Lett. (1)

M. Adachi, K. Yamane, R. Morita, and M. Yamashita, IEEE Photon. Technol. Lett. 16, 1951 (2004).
[CrossRef]

J. Chem. Phys. (2)

D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, and A. Materny, J. Chem. Phys. 116, 5231 (2002).
[CrossRef]

N. Dudovich, D. Oron, and Y. Silberberg, J. Chem. Phys. 118, 9208 (2003).
[CrossRef]

J. Opt. Soc. Am. B (1)

J. Phys. Chem. B (1)

J. X. Cheng and X. S. Xie, J. Phys. Chem. B 108, 827 (2004).
[CrossRef]

Nature (1)

N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002).
[CrossRef] [PubMed]

Opt. Express (2)

Opt. Lett. (5)

Phys. Rev. A (1)

D. Zeidler, S. Frey, K. L. Kompa, and M. Motzkus, Phys. Rev. A 64, 023420 (2001).
[CrossRef]

Phys. Rev. Lett. (1)

A. Zumbusch, G. R. Holtom, and X. S. Xie, Phys. Rev. Lett. 82, 4142 (1999).
[CrossRef]

Rev. Sci. Instrum. (3)

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbugel, B. A. Richman, and D. J. Kane, Rev. Sci. Instrum. 68, 3277 (1997).
[CrossRef]

V. Nagarajan, E. Johnson, P. Schellenberg, W. Parson, and R. Windeler, Rev. Sci. Instrum. 73, 4145 (2002).
[CrossRef]

A. M. Weiner, Rev. Sci. Instrum. 71, 1929 (2000).
[CrossRef]

Science (3)

H. Rabitz, R. de Vivie-Riedle, M. Motzkus, and K.-L. Kompa, Science 288, 824 (2000).
[CrossRef] [PubMed]

P. St. J. Russell, Science 299, 358 (2003).
[CrossRef] [PubMed]

A. M. Weiner, D. E. Leaird, G. P. Wiederrecht, and K. A. Nelson, Science 247, 1317 (1990).
[CrossRef] [PubMed]

Other (1)

B. von Vacano, W. Wohlleben, and M. Motzkus, "Single-beam CARS spectroscopy applied to low-wavenumber vibrational modes," J. Raman Spectrosc. (to be published). [DOI10.1002/jrs1457]

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Figures (3)

Fig. 1
Fig. 1

Experimental setup consisting of (a) supercontinuum generation, (b) pulse shaper, and (c) microspectroscopy experiment. FI, Faraday isolator; XYZ, piezo stage; BS, beam splitter; G1–2, gratings; SM1–2, spherical mirrors; SLM, spatial light modulator; KE, knife edge in the Fourier plane; FM, flipping mirror; MO1, MO2, microscope objectives; IF, interference short-pass filter; FL, focusing lens.

Fig. 2
Fig. 2

(Color online) Characterization of shaped supercontinuum pulses. Top row, experimental FROG traces; bottom row, supercontinuum spectrum (gray) with spectral phases retrieved from FROG (dashed curves) and phase functions applied to the SLM (solid curves). (a) and (d) uncompressed supercontinuum; (b) and (e) compressed supercontinuum; (c) and (f) compressed pulse shaped into multipulse.

Fig. 3
Fig. 3

Single-beam CARS results on toluene. (a) τ m -scan data with oscillations. Inset: a zoom into the decay of nonresonant signal (shaded area), with the experimental data (circles) and simulation (gray solid curve). (b) Fourier transform. The literature positions of the three strongest fingerprint modes are indicated as gray bars.

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