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Resonant optical activity induced in gases by collisions with right–left nonsymmetrical molecules

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Abstract

Frequency-dependent collision-induced circular dichroism and optical rotation are predicted for gases in the visible and infrared regions near resonance. For the appearance of those effects, the gas should contain right–left non-symmetrical molecules, and the pressure should correspond to the condition (l/λ) ~ 1, where l is the free-path length. Possible right–left nonsymmetrical effects in nonlinear spectroscopy of gases at l ≫ λ are mentioned.

© 1978 Optical Society of America

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