Frequency detuning as a result of self-phase modulation that exceeds by four times the primary laser frequency is demonstrated. The white light, ranging from the IR to 150 nm, was generated by a self-trapped femtosecond Ti:Al2O3 laser pulse in atmospheric-pressure rare gases. Spectral intensities in the UV and the visible regions are 100 MW/nm and 1 GW/nm, respectively. The beam divergence was measured to be 1 mrad.
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