Abstract

The theory of enhanced energy transfer within an aerosol particle based on donor coupling to morphological dependent resonances is tested for the first time to our knowledge. The correspondence between theory and experiment is good and allows one to obtain the photon lifetime within the longest-lived resonances. A comparison between this lifetime and the lifetime as obtained by Mie theory is discussed.

© 1989 Optical Society of America

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  1. L. M. Folan, S. Arnold, S. D. Druger, Chem. Phys. Lett. 118, 322 (1986).
    [Crossref]
  2. R. G. Pinnick, A. Biswas, P. Chylek, R. G. Armstrong, H. Latifi, E. Creegan, V. Srivastava, M. Jarzembski, G. Fernandez, Opt. Lett. 13, 494 (1988).
    [Crossref] [PubMed]
  3. J.-Z. Zhang, D. L. Leach, R. K. Chang, Opt. Lett. 13, 270 (1988).
    [Crossref] [PubMed]
  4. S. D. Druger, S. Arnold, L. M. Folan, J. Chem. Phys. 87, 2649 (1987).
    [Crossref]
  5. P. T. Leung, K. Young, J. Chem. Phys. 89, 2894 (1988).
    [Crossref]
  6. S. Arnold, L. M. Folan, Rev. Sci. Instrum. 57, 2250 (1986).
    [Crossref]
  7. R. Thurn, W. Kiefer, Appl. Opt. 24, 1515 (1985).
    [Crossref] [PubMed]
  8. F. Urbach, Phys. Rev. 92, 1324 (1953).
    [Crossref]
  9. A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
    [Crossref] [PubMed]
  10. L. M. Folan, S. Arnold, Opt. Lett. 13, 1 (1988).
    [Crossref] [PubMed]
  11. S. Arnold, L. M. Folan, Rev. Sci. Instrum. 58, 1732 (1987).
    [Crossref]
  12. S. Arnold, in Optical Effects Associated with Small Particles, P. W. Barber, R. K. Chang, eds. (World Scientific, Singapore, 1988), Chap. 2.

1988 (4)

1987 (2)

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 58, 1732 (1987).
[Crossref]

S. D. Druger, S. Arnold, L. M. Folan, J. Chem. Phys. 87, 2649 (1987).
[Crossref]

1986 (2)

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 57, 2250 (1986).
[Crossref]

L. M. Folan, S. Arnold, S. D. Druger, Chem. Phys. Lett. 118, 322 (1986).
[Crossref]

1985 (2)

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

R. Thurn, W. Kiefer, Appl. Opt. 24, 1515 (1985).
[Crossref] [PubMed]

1953 (1)

F. Urbach, Phys. Rev. 92, 1324 (1953).
[Crossref]

Als-Nielsen, J.

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Armstrong, R. G.

Arnold, S.

L. M. Folan, S. Arnold, Opt. Lett. 13, 1 (1988).
[Crossref] [PubMed]

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 58, 1732 (1987).
[Crossref]

S. D. Druger, S. Arnold, L. M. Folan, J. Chem. Phys. 87, 2649 (1987).
[Crossref]

L. M. Folan, S. Arnold, S. D. Druger, Chem. Phys. Lett. 118, 322 (1986).
[Crossref]

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 57, 2250 (1986).
[Crossref]

S. Arnold, in Optical Effects Associated with Small Particles, P. W. Barber, R. K. Chang, eds. (World Scientific, Singapore, 1988), Chap. 2.

Biswas, A.

Bohr, J.

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Braslau, A.

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Chang, R. K.

Chylek, P.

Creegan, E.

Deutsch, M.

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Druger, S. D.

S. D. Druger, S. Arnold, L. M. Folan, J. Chem. Phys. 87, 2649 (1987).
[Crossref]

L. M. Folan, S. Arnold, S. D. Druger, Chem. Phys. Lett. 118, 322 (1986).
[Crossref]

Fernandez, G.

Folan, L. M.

L. M. Folan, S. Arnold, Opt. Lett. 13, 1 (1988).
[Crossref] [PubMed]

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 58, 1732 (1987).
[Crossref]

S. D. Druger, S. Arnold, L. M. Folan, J. Chem. Phys. 87, 2649 (1987).
[Crossref]

L. M. Folan, S. Arnold, S. D. Druger, Chem. Phys. Lett. 118, 322 (1986).
[Crossref]

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 57, 2250 (1986).
[Crossref]

Jarzembski, M.

Kiefer, W.

Latifi, H.

Leach, D. L.

Leung, P. T.

P. T. Leung, K. Young, J. Chem. Phys. 89, 2894 (1988).
[Crossref]

Pershan, P. S.

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Pinnick, R. G.

Srivastava, V.

Thurn, R.

Urbach, F.

F. Urbach, Phys. Rev. 92, 1324 (1953).
[Crossref]

Weiss, A. H.

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Young, K.

P. T. Leung, K. Young, J. Chem. Phys. 89, 2894 (1988).
[Crossref]

Zhang, J.-Z.

Appl. Opt. (1)

Chem. Phys. Lett. (1)

L. M. Folan, S. Arnold, S. D. Druger, Chem. Phys. Lett. 118, 322 (1986).
[Crossref]

J. Chem. Phys. (2)

S. D. Druger, S. Arnold, L. M. Folan, J. Chem. Phys. 87, 2649 (1987).
[Crossref]

P. T. Leung, K. Young, J. Chem. Phys. 89, 2894 (1988).
[Crossref]

Opt. Lett. (3)

Phys. Rev. (1)

F. Urbach, Phys. Rev. 92, 1324 (1953).
[Crossref]

Phys. Rev. Lett. (1)

A. Braslau, M. Deutsch, P. S. Pershan, A. H. Weiss, J. Als-Nielsen, J. Bohr, Phys. Rev. Lett. 54, 114 (1985).
[Crossref] [PubMed]

Rev. Sci. Instrum. (2)

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 58, 1732 (1987).
[Crossref]

S. Arnold, L. M. Folan, Rev. Sci. Instrum. 57, 2250 (1986).
[Crossref]

Other (1)

S. Arnold, in Optical Effects Associated with Small Particles, P. W. Barber, R. K. Chang, eds. (World Scientific, Singapore, 1988), Chap. 2.

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Figures (3)

Fig. 1
Fig. 1

Measured peak ratios of acceptor-to-donor fluorescence for the 9-Aminoacridine/Rhodamine 6G (triangles) and Coumarin 1/Rhodamine 6G (circles) systems in individual aerosol particles. The straight line represents a Forster theory fit to bulk measurements in the Coumarin 1/Rhodamine 6G system.1

Fig. 2
Fig. 2

A fit of all data in Fig. 1 to the concentration dependence predicted by the Leung–Young model (solid curve) of energy transfer in an aerosol particle. Squares, 9-Aminoacridine/Rhodamine 6G system; triangles, Coumarin 1/Rhodamine 6G system. The only adjustable parameter, γ, was found to be 7.7 × 108 sec−1.

Fig. 3
Fig. 3

Measured decadic attenuation in glycerol. The midband of the overlap region for both energy-transfer systems is 530 nm.

Equations (2)

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Γ tr = [ π 2 c 3 D τ V n 3 ϕ ( ω 0 ) ω 0 2 ] ( c / n ) σ a ρ a γ + ( c / n ) σ a ρ a ,
P = ( c / n ) σ a ρ a γ + ( c / n ) σ a ρ a ,

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