Abstract

Theoretical explanations of the kinetics of scalar and vector holographic gratings are developed, and experimental results are obtained in amorphous As2S3 thin films. The large nonlinear-optical susceptibilities are evaluated from experimental data in the vicinity of the fundamental absorption edge, and it is found that χ1111(3)3.2×102esu and χ1122(3)/χ1111(3)0.98.

© 1988 Optical Society of America

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