Abstract

We report the first observation to our knowledge of the saturation effect in a Raman transition of a liquid, liquid N2. Using cw coherent anti-Stokes Raman spectroscopy, Raman line broadening by a factor of ≃2 is observed. This corresponds to vibrational excitation of up to 30% of the N2 molecules in the interaction volume.

© 1986 Optical Society of America

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