Abstract

We present a compact passively phase-stabilized ultra-broadband 2D Fourier transform setup. A gas (argon)-filled hollow core fiber pumped by an amplified Ti:Al2O3 laser is used as a light source providing spectral range spanning from 420 to 900 nm. Sub-10-fs pulses were obtained using a deformable mirror-based pulse shaper. We probe the nonlinear response of Rhodamine 101 using 90 nm bandwidth and resolve vibrational coherences of 150 fs period in the ground state.

© 2015 Optical Society of America

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References

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    [Crossref]
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    [Crossref]
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2014 (1)

2012 (3)

G. Aubock, C. Consani, F. van Mourik, and M. Chergui, Opt. Lett. 37, 2337 (2012).
[Crossref]

B. A. West and A. M. Moran, J. Phys. Chem. Lett. 3, 2575 (2012).
[Crossref]

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

2010 (2)

2009 (1)

2008 (2)

2006 (1)

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

2004 (2)

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

T. Brixner, T. Mancal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[Crossref]

2003 (1)

D. M. Jonas, Annu. Rev. Phys. Chem. 54, 425 (2003).
[Crossref]

2000 (2)

S. Mukamel, Annu. Rev. Phys. Chem. 51, 691 (2000).
[Crossref]

S. Woutersen and P. Hamm, J. Phys. Chem. B 104, 11316 (2000).
[Crossref]

1999 (1)

1998 (2)

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, Chem. Phys. Lett. 297, 307 (1998).
[Crossref]

P. Hamm, M. Lim, and R. M. Hochstrasser, J. Phys. Chem. B 102, 6123 (1998).
[Crossref]

1997 (1)

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Albrecht, A. W.

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, Chem. Phys. Lett. 297, 307 (1998).
[Crossref]

Aubock, G.

Auböck, G.

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Backus, S.

Baumert, T.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Béjot, P.

Biegert, J.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Brixner, T.

U. Selig, C. F. Schleussner, M. Foerster, F. Langhojer, P. Nuernberger, and T. Brixner, Opt. Lett. 35, 4178 (2010).
[Crossref]

U. Selig, F. Langhojer, F. Dimler, T. Lohrig, C. Schwarz, B. Gieseking, and T. Brixner, Opt. Lett. 33, 2851 (2008).
[Crossref]

T. Brixner, T. Mancal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[Crossref]

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Cannizzo, A.

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Caram, J. R.

Chergui, M.

G. Aubock, C. Consani, F. van Mourik, and M. Chergui, Opt. Lett. 37, 2337 (2012).
[Crossref]

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Cho, M.

M. Cho, Chem. Rev. 108, 1331 (2008).
[Crossref]

Consani, C.

G. Aubock, C. Consani, F. van Mourik, and M. Chergui, Opt. Lett. 37, 2337 (2012).
[Crossref]

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Couairon, A.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Dahlberg, P. D.

Dimler, F.

Dolzhnikov, D. S.

Dudley, J. M.

Engel, G. S.

Fleming, G. R.

T. Brixner, T. Mancal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[Crossref]

Foerster, M.

Gallagher Faeder, S. M.

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, Chem. Phys. Lett. 297, 307 (1998).
[Crossref]

Gerber, G.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Gieseking, B.

Hamm, P.

S. Woutersen and P. Hamm, J. Phys. Chem. B 104, 11316 (2000).
[Crossref]

P. Hamm, M. Lim, and R. M. Hochstrasser, J. Phys. Chem. B 102, 6123 (1998).
[Crossref]

Hauri, C. P.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Haworth, C. A.

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

Heinrich, A.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Helbing, F. W.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Hochstrasser, R. M.

P. Hamm, M. Lim, and R. M. Hochstrasser, J. Phys. Chem. B 102, 6123 (1998).
[Crossref]

Hybl, J. D.

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, Chem. Phys. Lett. 297, 307 (1998).
[Crossref]

Jonas, D. M.

D. M. Jonas, Annu. Rev. Phys. Chem. 54, 425 (2003).
[Crossref]

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, Chem. Phys. Lett. 297, 307 (1998).
[Crossref]

Kapteyn, H.

Kasparian, J.

Keller, U.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Khadivi, A.

Kida, Y.

Kobayashi, T.

Kornelis, W.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Langhojer, F.

Lim, M.

P. Hamm, M. Lim, and R. M. Hochstrasser, J. Phys. Chem. B 102, 6123 (1998).
[Crossref]

Liu, J.

Lohrig, T.

Maginnis, K.

Mancal, T.

T. Brixner, T. Mancal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[Crossref]

Marangos, J. P.

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

Monni, R.

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Moran, A. M.

B. A. West and A. M. Moran, J. Phys. Chem. Lett. 3, 2575 (2012).
[Crossref]

Mourou, G.

Mukamel, S.

S. Mukamel, Annu. Rev. Phys. Chem. 51, 691 (2000).
[Crossref]

Murnane, M.

Mysyrowicz, A.

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Nuernberger, P.

Okamura, K.

Robinson, J. S.

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

Rolczynski, B. S.

Russek, U.

Schleussner, C. F.

Schwarz, C.

Selig, U.

Seyfried, V.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Smith, R. A.

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

Stiopkin, I. V.

T. Brixner, T. Mancal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[Crossref]

Strehle, M.

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Talapin, D. V.

Teng, H.

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

Teramoto, T.

Tisch, J. W. G.

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

van Mourik, F.

G. Aubock, C. Consani, F. van Mourik, and M. Chergui, Opt. Lett. 37, 2337 (2012).
[Crossref]

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Vdovin, G.

Viswanathan, S.

West, B. A.

B. A. West and A. M. Moran, J. Phys. Chem. Lett. 3, 2575 (2012).
[Crossref]

Wolf, J.-P.

Woutersen, S.

S. Woutersen and P. Hamm, J. Phys. Chem. B 104, 11316 (2000).
[Crossref]

Zeek, E.

Zheng, H. B.

Annu. Rev. Phys. Chem. (2)

S. Mukamel, Annu. Rev. Phys. Chem. 51, 691 (2000).
[Crossref]

D. M. Jonas, Annu. Rev. Phys. Chem. 54, 425 (2003).
[Crossref]

Appl Phys B (1)

T. Baumert, T. Brixner, V. Seyfried, M. Strehle, and G. Gerber, Appl Phys B 65, 779 (1997).
[Crossref]

Appl. Opt. (1)

Appl. Phys. B (1)

C. P. Hauri, W. Kornelis, F. W. Helbing, A. Heinrich, A. Couairon, A. Mysyrowicz, J. Biegert, and U. Keller, Appl. Phys. B 79, 673 (2004).
[Crossref]

Appl. Phys. B Lasers Opt. (1)

J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, J. P. Marangos, and J. W. G. Tisch, Appl. Phys. B Lasers Opt. 85, 525 (2006).
[Crossref]

Chem. Phys. Lett. (1)

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, Chem. Phys. Lett. 297, 307 (1998).
[Crossref]

Chem. Rev. (1)

M. Cho, Chem. Rev. 108, 1331 (2008).
[Crossref]

J. Chem. Phys. (1)

T. Brixner, T. Mancal, I. V. Stiopkin, and G. R. Fleming, J. Chem. Phys. 121, 4221 (2004).
[Crossref]

J. Phys. Chem. B (2)

P. Hamm, M. Lim, and R. M. Hochstrasser, J. Phys. Chem. B 102, 6123 (1998).
[Crossref]

S. Woutersen and P. Hamm, J. Phys. Chem. B 104, 11316 (2000).
[Crossref]

J. Phys. Chem. Lett. (1)

B. A. West and A. M. Moran, J. Phys. Chem. Lett. 3, 2575 (2012).
[Crossref]

Opt. Express (2)

Opt. Lett. (4)

Rev. Sci. Instrum. (1)

G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. van Mourik, and M. Chergui, Rev. Sci. Instrum. 83, 093105 (2012).

Other (1)

D. Beasley and J. Heitköter, The Hitch-Hiker’s Guide to Evolutionary Computation, http://aiinfinance.com/gafaq.pdf .

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Figures (5)

Fig. 1.
Fig. 1. Accessible spectrum of the hollow core fiber pumped 0.5-mJ, 55-fs pulses centered at 790 nm. (b) shows a TG-FROG autocorrelation trace of the selected spectrum from 480 to 685 nm with a flat spectral phase.
Fig. 2.
Fig. 2. Schematic drawing of the setup. (a) Side view showing the metallic holders and the spitting of the pulses. (b) Pulse shaper schematic showing the grating, deformable mirror DM, and a 27 cm spherical mirror SM. (c) Top view of the setup showing the stages and the path of the 4 (black) beams through the sample and into the spectrometer. (d) Generated pulse sequence.
Fig. 3.
Fig. 3. Phase stability measurements. (a) Phase deviation calculated from the spectral interference between third-order nonlinear signal generated by a thin glass plate and the local oscillator was recorded every second over 12 h. (b) Cuts from different 2D spectra take over multiple 2D scans (6 h apart) showing stability of the fringes and reproducibility of the general shape.
Fig. 4.
Fig. 4. (a) Absolute 2D spectrum of Rhodamine 101 at 100 fs showing the diagonal peaks. (b) Contour plot of the phase showing a stable phase along the diagonal peaks.
Fig. 5.
Fig. 5. Oscillations detected in the pump probe data and 2D spectra showing 150 fs period.

Equations (2)

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φ si = φ Lo φ s = φ Lo i ω 0 ( t 1 + t 2 + t 3 ) .
ω 0 ( Δ t 1 Δ t 3 + Δ t 2 Δ t 4 ) = 0 ,

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