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Wide-field vibrational phase imaging in an extremely folded box-CARS geometry

Pascal Berto, Alexander Jesacher, Clemens Roider, Serge Monneret, Hervé Rigneault, and Monika Ritsch-Marte

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Abstract

We present a method that allows one to measure the real and imaginary parts of the third-order susceptibility in a wide-field coherent anti-Stokes Raman scattering setup using a quadriwave lateral shearing interferometer. This permits the retrieval of the undistorted Raman spectrum and the removal of a nonresonant signal from the surrounding solvent, which otherwise may overwhelm weak resonances.

© 2013 Optical Society of America

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