Second-harmonic generation with magnetic-field controllability

Sheng Ju; Tian-Yi Cai; Chi-I Wei; Guang-Yu Guo

doi:10.1364/OL.34.003860

Optics Letters
Vol. 34,
Issue 24,
pp. 3860-3862
(2009)
•https://doi.org/10.1364/OL.34.003860

Second-harmonic generation with magnetic-field controllability

Sheng Ju, Tian-Yi Cai, Chi-I Wei, and Guang-Yu Guo

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Sheng Ju, Tian-Yi Cai, Chi-I Wei, and Guang-Yu Guo, "Second-harmonic generation with magnetic-field controllability," Opt. Lett. 34, 3860-3862 (2009)

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Abstract

Based on density functional theory with the generalized gradient approximation plus on-site Coulomb repulsion method, we study the magnetic-ordering dependence of second-harmonic generation (SHG) in a polar magnet $Bi Co O_{3}$ . The large second-order optical susceptibility, which can reach $3.7 \times 10^{- 7} esu$ , exhibits a strong magnetic-ordering dependence, giving rise to magnetic-field controllable SHG response in polar magnets.

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	C-Type AFM	G-Type AFM	A-Type AFM	FM
$ϵ_{x x}$	6.55	6.54	6.38	6.24
$ϵ_{z z}$	6.93	6.76	7.05	6.79
$χ_{x x z}^{(2)}$	6.9	9.05	0.29	2.57
$χ_{z x x}^{(2)}$	2.19	4.56	$- 7.36$	$- 5.65$
$χ_{z z z}^{(2)}$	$- 36.86$	$- 22.59$	$- 39.69$	$- 36.24$

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Optics Letters