Abstract

Si3N4 waveguides, pumped at 1550 nm, can provide spectrally smooth, broadband light for gas spectroscopy in the important 2 μm to 2.5 μm atmospheric water window, which is only partially accessible with silica-fiber based systems. By combining Er+ fiber frequency combs and supercontinuum generation in tailored Si3N4 waveguides, high signal-to-noise dual-comb spectroscopy spanning 2 μm to 2.5 μm is demonstrated. Acquired broadband dual-comb spectra of CO and CO2 agree well with database line shape models and have a spectral-signal-to-noise as high as 48/√s, showing that the high coherence between the two combs is retained in the Si3N4 supercontinuum generation. The dual-comb spectroscopy figure of merit is 6 × 106/√s, equivalent to that of all-fiber dual-comb spectroscopy systems in the 1.6 μm band. based on these results, future dual-comb spectroscopy can combine fiber comb technology with Si3N4 waveguides to access new spectral windows in a robust non-laboratory platform.

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  40. The use of tradenames in this manuscript is necessary to specify experimental results and does not imply endorsement by the National Institute of Standards and Technology.

2018 (9)

A. V. Muraviev, V. O. Smolski, Z. E. Loparo, and K. L. Vodopyanov, “Massively parallel sensing of trace molecules and their isotopologues with broadband subharmonic mid-infrared frequency combs,” Nat. Photonics 12(4), 209–214 (2018).
[Crossref]

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

H. Guo, C. Herkommer, A. Billat, D. Grassani, C. Zhang, M. H. P. Pfeiffer, W. Weng, C.-S. Brès, and T. J. Kippenberg, “Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides,” Nat. Photonics 12(6), 330–335 (2018).
[Crossref]

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
[Crossref]

G. Ycas, F. R. Giorgetta, E. Baumann, I. Coddington, D. Herman, S. A. Diddams, and N. R. Newbury, “High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm,” Nat. Photonics 12(4), 202–208 (2018).
[Crossref]

S. Coburn, C. B. Alden, R. Wright, K. Cossel, E. Baumann, G.-W. Truong, F. Giorgetta, C. Sweeney, N. R. Newbury, K. Prasad, I. Coddington, and G. B. Rieker, “Regional trace-gas source attribution using a field-deployed dual frequency comb spectrometer,” Optica 5(4), 320–327 (2018).
[Crossref]

R. Liao, Y. Song, W. Liu, H. Shi, L. Chai, and M. Hu, “Dual-comb spectroscopy with a single free-running thulium-doped fiber laser,” Opt. Express 26(8), 11046–11054 (2018).
[Crossref] [PubMed]

D. T. H. Tan, K. J. A. Ooi, and D. K. T. Ng, “Nonlinear optics on silicon-rich nitride—a high nonlinear figure of merit CMOS platform [Invited],” Photon. Res. 6(5), B50–B66 (2018).
[Crossref]

M. I. Kayes, N. Abdukerim, A. Rekik, and M. Rochette, “Free-running mode-locked laser based dual-comb spectroscopy,” Opt. Lett. 43(23), 5809–5812 (2018).
[Crossref] [PubMed]

2017 (8)

K. C. Cossel, E. M. Waxman, I. A. Finneran, G. A. Blake, J. Ye, and N. R. Newbury, “Gas-phase broadband spectroscopy using active sources: progress, status, and applications,” J. Opt. Soc. Am. B 34(1), 104–129 (2017).
[Crossref] [PubMed]

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

T. Ideguchi, “Dual-Comb Spectroscopy,” Opt. Photonics News 28(1), 32–39 (2017).
[Crossref]

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
[Crossref]

D. Yoon Oh, K. Y. Yang, C. Fredrick, G. Ycas, S. A. Diddams, and K. J. Vahala, “Coherent ultra-violet to near-infrared generation in silica ridge waveguides,” Nat. Commun. 8, 13922 (2017).
[Crossref] [PubMed]

M. A. G. Porcel, F. Schepers, J. P. Epping, T. Hellwig, M. Hoekman, R. G. Heideman, P. J. M. van der Slot, C. J. Lee, R. Schmidt, R. Bratschitsch, C. Fallnich, and K.-J. Boller, “Two-octave spanning supercontinuum generation in stoichiometric silicon nitride waveguides pumped at telecom wavelengths,” Opt. Express 25(2), 1542–1554 (2017).
[Crossref] [PubMed]

D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
[Crossref] [PubMed]

S. Wang, S. Droste, L. C. Sinclair, I. Coddington, N. R. Newbury, T. F. Carruthers, and C. R. Menyuk, “Wake mode sidebands and instability in mode-locked lasers with slow saturable absorbers,” Opt. Lett. 42(12), 2362–2365 (2017).
[Crossref] [PubMed]

2016 (5)

2015 (5)

L. C. Sinclair, J.-D. Deschênes, L. Sonderhouse, W. C. Swann, I. H. Khader, E. Baumann, N. R. Newbury, and I. Coddington, “Invited Article: A compact optically coherent fiber frequency comb,” Rev. Sci. Instrum. 86(8), 081301 (2015).
[Crossref] [PubMed]

N. Singh, D. D. Hudson, Y. Yu, C. Grillet, S. D. Jackson, A. Casas-Bedoya, A. Read, P. Atanackovic, S. G. Duvall, S. Palomba, B. Luther-Davies, S. Madden, D. J. Moss, and B. J. Eggleton, “Midinfrared supercontinuum generation from 2 to 6 μm in a silicon nanowire,” Optica 2(9), 797–802 (2015).
[Crossref]

A. R. Johnson, A. S. Mayer, A. Klenner, K. Luke, E. S. Lamb, M. R. E. Lamont, C. Joshi, Y. Okawachi, F. W. Wise, M. Lipson, U. Keller, and A. L. Gaeta, “Octave-spanning coherent supercontinuum generation in a silicon nitride waveguide,” Opt. Lett. 40(21), 5117–5120 (2015).
[Crossref] [PubMed]

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
[Crossref] [PubMed]

S. Okubo, K. Iwakuni, H. Inaba, K. Hosaka, A. Onae, H. Sasada, and F.-L. Hong, “Ultra-broadband dual-comb spectroscopy across 1.0–1.9 µm,” Appl. Phys. Express 8(8), 082402 (2015).
[Crossref]

2014 (1)

2012 (1)

A. Schliesser, N. Picqué, and T. W. Hänsch, “Mid-infrared frequency combs,” Nat. Photonics 6(7), 440–449 (2012).
[Crossref]

2011 (1)

T. J. Kippenberg, R. Holzwarth, and S. A. Diddams, “Microresonator-based optical frequency combs,” Science 332(6029), 555–559 (2011).
[Crossref] [PubMed]

2010 (3)

B. Bernhardt, E. Sorokin, P. Jacquet, R. Thon, T. Becker, I. T. Sorokina, N. Picqué, and T. W. Hänsch, “Mid-infrared dual-comb spectroscopy with 2.4 μm Cr2+:ZnSe femtosecond lasers,” Appl. Phys. B 100(1), 3–8 (2010).
[Crossref]

F. Adler, M. J. Thorpe, K. C. Cossel, and J. Ye, “Cavity-enhanced direct frequency comb spectroscopy: technology and applications,” Annu. Rev. Anal. Chem. (Palo Alto, Calif.) 3(1), 175–205 (2010).
[Crossref] [PubMed]

N. R. Newbury, I. Coddington, and W. Swann, “Sensitivity of coherent dual-comb spectroscopy,” Opt. Express 18(8), 7929–7945 (2010).
[Crossref] [PubMed]

2008 (2)

M. A. Foster, A. C. Turner, M. Lipson, and A. L. Gaeta, “Nonlinear optics in photonic nanowires,” Opt. Express 16(2), 1300–1320 (2008).
[Crossref] [PubMed]

G. Ehret, C. Kiemle, M. Wirth, A. Amediek, A. Fix, and S. Houweling, “Space-borne remote sensing of CO2, CH4, and N2O by integrated path differential absorption lidar: a sensitivity analysis,” Appl. Phys. B 90(3-4), 593–608 (2008).
[Crossref]

2007 (1)

C. D. Boone, K. A. Walker, and P. F. Bernath, “Speed-dependent Voigt profile for water vapor in infrared remote sensing applications,” J. Quant. Spectrosc. Radiat. Transf. 105(3), 525–532 (2007).
[Crossref]

1999 (1)

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
[Crossref]

Abdukerim, N.

Adler, F.

F. Adler, M. J. Thorpe, K. C. Cossel, and J. Ye, “Cavity-enhanced direct frequency comb spectroscopy: technology and applications,” Annu. Rev. Anal. Chem. (Palo Alto, Calif.) 3(1), 175–205 (2010).
[Crossref] [PubMed]

Alden, C. B.

Amediek, A.

G. Ehret, C. Kiemle, M. Wirth, A. Amediek, A. Fix, and S. Houweling, “Space-borne remote sensing of CO2, CH4, and N2O by integrated path differential absorption lidar: a sensitivity analysis,” Appl. Phys. B 90(3-4), 593–608 (2008).
[Crossref]

Atanackovic, P.

Auwera, J. V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Baets, R.

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
[Crossref] [PubMed]

Barbe, A.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Baumann, E.

S. Coburn, C. B. Alden, R. Wright, K. Cossel, E. Baumann, G.-W. Truong, F. Giorgetta, C. Sweeney, N. R. Newbury, K. Prasad, I. Coddington, and G. B. Rieker, “Regional trace-gas source attribution using a field-deployed dual frequency comb spectrometer,” Optica 5(4), 320–327 (2018).
[Crossref]

G. Ycas, F. R. Giorgetta, E. Baumann, I. Coddington, D. Herman, S. A. Diddams, and N. R. Newbury, “High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm,” Nat. Photonics 12(4), 202–208 (2018).
[Crossref]

G.-W. Truong, E. M. Waxman, K. C. Cossel, E. Baumann, A. Klose, F. R. Giorgetta, W. C. Swann, N. R. Newbury, and I. Coddington, “Accurate frequency referencing for fieldable dual-comb spectroscopy,” Opt. Express 24(26), 30495–30504 (2016).
[Crossref] [PubMed]

L. C. Sinclair, J.-D. Deschênes, L. Sonderhouse, W. C. Swann, I. H. Khader, E. Baumann, N. R. Newbury, and I. Coddington, “Invited Article: A compact optically coherent fiber frequency comb,” Rev. Sci. Instrum. 86(8), 081301 (2015).
[Crossref] [PubMed]

Becker, T.

B. Bernhardt, E. Sorokin, P. Jacquet, R. Thon, T. Becker, I. T. Sorokina, N. Picqué, and T. W. Hänsch, “Mid-infrared dual-comb spectroscopy with 2.4 μm Cr2+:ZnSe femtosecond lasers,” Appl. Phys. B 100(1), 3–8 (2010).
[Crossref]

Bernath, P. F.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

C. D. Boone, K. A. Walker, and P. F. Bernath, “Speed-dependent Voigt profile for water vapor in infrared remote sensing applications,” J. Quant. Spectrosc. Radiat. Transf. 105(3), 525–532 (2007).
[Crossref]

Bernhardt, B.

B. Bernhardt, E. Sorokin, P. Jacquet, R. Thon, T. Becker, I. T. Sorokina, N. Picqué, and T. W. Hänsch, “Mid-infrared dual-comb spectroscopy with 2.4 μm Cr2+:ZnSe femtosecond lasers,” Appl. Phys. B 100(1), 3–8 (2010).
[Crossref]

Billat, A.

H. Guo, C. Herkommer, A. Billat, D. Grassani, C. Zhang, M. H. P. Pfeiffer, W. Weng, C.-S. Brès, and T. J. Kippenberg, “Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides,” Nat. Photonics 12(6), 330–335 (2018).
[Crossref]

Birk, M.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Blake, G. A.

Boller, K.-J.

Boone, C. D.

C. D. Boone, K. A. Walker, and P. F. Bernath, “Speed-dependent Voigt profile for water vapor in infrared remote sensing applications,” J. Quant. Spectrosc. Radiat. Transf. 105(3), 525–532 (2007).
[Crossref]

Boudon, V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Bovensmann, H.

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
[Crossref]

Brasch, V.

Bratschitsch, R.

Brès, C.-S.

H. Guo, C. Herkommer, A. Billat, D. Grassani, C. Zhang, M. H. P. Pfeiffer, W. Weng, C.-S. Brès, and T. J. Kippenberg, “Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides,” Nat. Photonics 12(6), 330–335 (2018).
[Crossref]

Buchwitz, M.

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
[Crossref]

Burrows, J. P.

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
[Crossref]

Campargue, A.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Carlson, D. R.

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
[Crossref]

D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
[Crossref] [PubMed]

Carruthers, T. F.

Casas-Bedoya, A.

Chai, L.

Chance, K. V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
[Crossref]

Chen, G. F. R.

J. W. Choi, G. F. R. Chen, D. K. T. Ng, K. J. A. Ooi, and D. T. H. Tan, “Wideband nonlinear spectral broadening in ultra-short ultra - silicon rich nitride waveguides,” Sci. Rep. 6(1), 27120 (2016).
[Crossref] [PubMed]

Chiles, J.

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
[Crossref]

Choi, J. W.

J. W. Choi, G. F. R. Chen, D. K. T. Ng, K. J. A. Ooi, and D. T. H. Tan, “Wideband nonlinear spectral broadening in ultra-short ultra - silicon rich nitride waveguides,” Sci. Rep. 6(1), 27120 (2016).
[Crossref] [PubMed]

Coburn, S.

Coddington, I.

S. Coburn, C. B. Alden, R. Wright, K. Cossel, E. Baumann, G.-W. Truong, F. Giorgetta, C. Sweeney, N. R. Newbury, K. Prasad, I. Coddington, and G. B. Rieker, “Regional trace-gas source attribution using a field-deployed dual frequency comb spectrometer,” Optica 5(4), 320–327 (2018).
[Crossref]

G. Ycas, F. R. Giorgetta, E. Baumann, I. Coddington, D. Herman, S. A. Diddams, and N. R. Newbury, “High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm,” Nat. Photonics 12(4), 202–208 (2018).
[Crossref]

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
[Crossref]

S. Wang, S. Droste, L. C. Sinclair, I. Coddington, N. R. Newbury, T. F. Carruthers, and C. R. Menyuk, “Wake mode sidebands and instability in mode-locked lasers with slow saturable absorbers,” Opt. Lett. 42(12), 2362–2365 (2017).
[Crossref] [PubMed]

D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
[Crossref] [PubMed]

I. Coddington, N. Newbury, and W. Swann, “Dual-comb spectroscopy,” Optica 3(4), 414–426 (2016).
[Crossref]

G.-W. Truong, E. M. Waxman, K. C. Cossel, E. Baumann, A. Klose, F. R. Giorgetta, W. C. Swann, N. R. Newbury, and I. Coddington, “Accurate frequency referencing for fieldable dual-comb spectroscopy,” Opt. Express 24(26), 30495–30504 (2016).
[Crossref] [PubMed]

L. C. Sinclair, J.-D. Deschênes, L. Sonderhouse, W. C. Swann, I. H. Khader, E. Baumann, N. R. Newbury, and I. Coddington, “Invited Article: A compact optically coherent fiber frequency comb,” Rev. Sci. Instrum. 86(8), 081301 (2015).
[Crossref] [PubMed]

N. R. Newbury, I. Coddington, and W. Swann, “Sensitivity of coherent dual-comb spectroscopy,” Opt. Express 18(8), 7929–7945 (2010).
[Crossref] [PubMed]

Coen, S.

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
[Crossref] [PubMed]

Cole, D. C.

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
[Crossref]

Cossel, K.

Cossel, K. C.

Cruz, F. C.

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
[Crossref]

Császár, A. G.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Deschênes, J.-D.

L. C. Sinclair, J.-D. Deschênes, L. Sonderhouse, W. C. Swann, I. H. Khader, E. Baumann, N. R. Newbury, and I. Coddington, “Invited Article: A compact optically coherent fiber frequency comb,” Rev. Sci. Instrum. 86(8), 081301 (2015).
[Crossref] [PubMed]

Devi, V. M.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
[Crossref]

Diddams, S.

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
[Crossref]

Diddams, S. A.

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

G. Ycas, F. R. Giorgetta, E. Baumann, I. Coddington, D. Herman, S. A. Diddams, and N. R. Newbury, “High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm,” Nat. Photonics 12(4), 202–208 (2018).
[Crossref]

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
[Crossref]

D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
[Crossref] [PubMed]

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A. Klose, G. Ycas, D. L. Maser, and S. A. Diddams, “Tunable, stable source of femtosecond pulses near 2 μm via supercontinuum of an Erbium mode-locked laser,” Opt. Express 22(23), 28400–28411 (2014).
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T. J. Kippenberg, R. Holzwarth, and S. A. Diddams, “Microresonator-based optical frequency combs,” Science 332(6029), 555–559 (2011).
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Droste, S.

D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
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S. Wang, S. Droste, L. C. Sinclair, I. Coddington, N. R. Newbury, T. F. Carruthers, and C. R. Menyuk, “Wake mode sidebands and instability in mode-locked lasers with slow saturable absorbers,” Opt. Lett. 42(12), 2362–2365 (2017).
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D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Eggleton, B. J.

Ehret, G.

G. Ehret, C. Kiemle, M. Wirth, A. Amediek, A. Fix, and S. Houweling, “Space-borne remote sensing of CO2, CH4, and N2O by integrated path differential absorption lidar: a sensitivity analysis,” Appl. Phys. B 90(3-4), 593–608 (2008).
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Fallnich, C.

Finneran, I. A.

Fix, A.

G. Ehret, C. Kiemle, M. Wirth, A. Amediek, A. Fix, and S. Houweling, “Space-borne remote sensing of CO2, CH4, and N2O by integrated path differential absorption lidar: a sensitivity analysis,” Appl. Phys. B 90(3-4), 593–608 (2008).
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Fredrick, C.

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D. Yoon Oh, K. Y. Yang, C. Fredrick, G. Ycas, S. A. Diddams, and K. J. Vahala, “Coherent ultra-violet to near-infrared generation in silica ridge waveguides,” Nat. Commun. 8, 13922 (2017).
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D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
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Frerick, J.

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Gamache, R. R.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Geiselmann, M.

Giorgetta, F.

Giorgetta, F. R.

G. Ycas, F. R. Giorgetta, E. Baumann, I. Coddington, D. Herman, S. A. Diddams, and N. R. Newbury, “High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm,” Nat. Photonics 12(4), 202–208 (2018).
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Goede, A. P. H.

H. Bovensmann, J. P. Burrows, M. Buchwitz, J. Frerick, S. Noël, V. V. Rozanov, K. V. Chance, and A. P. H. Goede, “SCIAMACHY: mission objectives and measurement modes,” J. Atmos. Sci. 56(2), 127–150 (1999).
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Gordon, I. E.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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H. Guo, C. Herkommer, A. Billat, D. Grassani, C. Zhang, M. H. P. Pfeiffer, W. Weng, C.-S. Brès, and T. J. Kippenberg, “Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides,” Nat. Photonics 12(6), 330–335 (2018).
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Guo, H.

H. Guo, C. Herkommer, A. Billat, D. Grassani, C. Zhang, M. H. P. Pfeiffer, W. Weng, C.-S. Brès, and T. J. Kippenberg, “Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides,” Nat. Photonics 12(6), 330–335 (2018).
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Hänsch, T. W.

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
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A. Schliesser, N. Picqué, and T. W. Hänsch, “Mid-infrared frequency combs,” Nat. Photonics 6(7), 440–449 (2012).
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B. Bernhardt, E. Sorokin, P. Jacquet, R. Thon, T. Becker, I. T. Sorokina, N. Picqué, and T. W. Hänsch, “Mid-infrared dual-comb spectroscopy with 2.4 μm Cr2+:ZnSe femtosecond lasers,” Appl. Phys. B 100(1), 3–8 (2010).
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Harrison, J. J.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Hellwig, T.

Herkommer, C.

H. Guo, C. Herkommer, A. Billat, D. Grassani, C. Zhang, M. H. P. Pfeiffer, W. Weng, C.-S. Brès, and T. J. Kippenberg, “Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides,” Nat. Photonics 12(6), 330–335 (2018).
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Herman, D.

G. Ycas, F. R. Giorgetta, E. Baumann, I. Coddington, D. Herman, S. A. Diddams, and N. R. Newbury, “High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm,” Nat. Photonics 12(4), 202–208 (2018).
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A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
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D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
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Hill, C.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Holzner, S.

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
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Holzwarth, R.

T. J. Kippenberg, R. Holzwarth, and S. A. Diddams, “Microresonator-based optical frequency combs,” Science 332(6029), 555–559 (2011).
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Hong, F.-L.

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S. Okubo, K. Iwakuni, H. Inaba, K. Hosaka, A. Onae, H. Sasada, and F.-L. Hong, “Ultra-broadband dual-comb spectroscopy across 1.0–1.9 µm,” Appl. Phys. Express 8(8), 082402 (2015).
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G. Ehret, C. Kiemle, M. Wirth, A. Amediek, A. Fix, and S. Houweling, “Space-borne remote sensing of CO2, CH4, and N2O by integrated path differential absorption lidar: a sensitivity analysis,” Appl. Phys. B 90(3-4), 593–608 (2008).
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S. Okubo, K. Iwakuni, H. Inaba, K. Hosaka, A. Onae, H. Sasada, and F.-L. Hong, “Ultra-broadband dual-comb spectroscopy across 1.0–1.9 µm,” Appl. Phys. Express 8(8), 082402 (2015).
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S. Okubo, K. Iwakuni, H. Inaba, K. Hosaka, A. Onae, H. Sasada, and F.-L. Hong, “Ultra-broadband dual-comb spectroscopy across 1.0–1.9 µm,” Appl. Phys. Express 8(8), 082402 (2015).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Jacquet, P.

B. Bernhardt, E. Sorokin, P. Jacquet, R. Thon, T. Becker, I. T. Sorokina, N. Picqué, and T. W. Hänsch, “Mid-infrared dual-comb spectroscopy with 2.4 μm Cr2+:ZnSe femtosecond lasers,” Appl. Phys. B 100(1), 3–8 (2010).
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Johnson, A. R.

Johnson, T. J.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Jost, J. D.

Jung, H.

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Klose, A.

Kochanov, R. V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Kordts, A.

Kowligy, A.

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D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
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Kowligy, A. S.

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

Kuyken, B.

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
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Kyuberis, A. A.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Lamb, E. S.

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
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A. R. Johnson, A. S. Mayer, A. Klenner, K. Luke, E. S. Lamb, M. R. E. Lamont, C. Joshi, Y. Okawachi, F. W. Wise, M. Lipson, U. Keller, and A. L. Gaeta, “Octave-spanning coherent supercontinuum generation in a silicon nitride waveguide,” Opt. Lett. 40(21), 5117–5120 (2015).
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Lamont, M. R. E.

Lee, C. J.

Leo, F.

B. Kuyken, T. Ideguchi, S. Holzner, M. Yan, T. W. Hänsch, J. Van Campenhout, P. Verheyen, S. Coen, F. Leo, R. Baets, G. Roelkens, and N. Picqué, “An octave-spanning mid-infrared frequency comb generated in a silicon nanophotonic wire waveguide,” Nat. Commun. 6(1), 6310 (2015).
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Liao, R.

Lind, A.

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

D. D. Hickstein, H. Jung, D. R. Carlson, A. Lind, I. Coddington, K. Srinivasan, G. G. Ycas, D. C. Cole, A. Kowligy, C. Fredrick, S. Droste, E. S. Lamb, N. R. Newbury, H. X. Tang, S. A. Diddams, and S. B. Papp, “Ultrabroadband supercontinuum generation and frequency-comb stabilization using on-chip waveguides with both cubic and quadratic nonlinearities,” Phys. Rev. Appl. 8(1), 014025 (2017).
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D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
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Lipson, M.

Liu, W.

Loos, J.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Loparo, Z. E.

A. V. Muraviev, V. O. Smolski, Z. E. Loparo, and K. L. Vodopyanov, “Massively parallel sensing of trace molecules and their isotopologues with broadband subharmonic mid-infrared frequency combs,” Nat. Photonics 12(4), 209–214 (2018).
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Luke, K.

Luther-Davies, B.

Lyulin, O. M.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Madden, S.

Maser, D. L.

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
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A. Klose, G. Ycas, D. L. Maser, and S. A. Diddams, “Tunable, stable source of femtosecond pulses near 2 μm via supercontinuum of an Erbium mode-locked laser,” Opt. Express 22(23), 28400–28411 (2014).
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Massie, S. T.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Mayer, A. S.

Menyuk, C. R.

Mikhailenko, S. N.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Mirin, R. P.

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
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Moazzen-Ahmadi, N.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Moss, D. J.

Müller, H. S. P.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. V. Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transf. 203, 3–69 (2017).
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Muraviev, A. V.

A. V. Muraviev, V. O. Smolski, Z. E. Loparo, and K. L. Vodopyanov, “Massively parallel sensing of trace molecules and their isotopologues with broadband subharmonic mid-infrared frequency combs,” Nat. Photonics 12(4), 209–214 (2018).
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Nader, N.

A. S. Kowligy, A. Lind, D. D. Hickstein, D. R. Carlson, H. Timmers, N. Nader, F. C. Cruz, G. Ycas, S. B. Papp, and S. A. Diddams, “Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides,” Optics Letters 43(8) 1678-1681 (2018).

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
[Crossref]

D. R. Carlson, D. D. Hickstein, A. Lind, S. Droste, D. Westly, N. Nader, I. Coddington, N. R. Newbury, K. Srinivasan, S. A. Diddams, and S. B. Papp, “Self-referenced frequency combs using high-efficiency silicon-nitride waveguides,” Opt. Lett. 42(12), 2314–2317 (2017).
[Crossref] [PubMed]

Nam, S. W.

N. Nader, D. L. Maser, F. C. Cruz, A. Kowligy, H. Timmers, J. Chiles, C. Fredrick, D. A. Westly, S. W. Nam, R. P. Mirin, J. M. Shainline, and S. Diddams, “Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy,” APL Photonics 3(3), 036102 (2018).
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Other (3)

The use of tradenames in this manuscript is necessary to specify experimental results and does not imply endorsement by the National Institute of Standards and Technology.

T. J. Kippenberg, A. L. Gaeta, M. Lipson, and M. L. Gorodetsky, “Dissipative Kerr solitons in optical microresonators,” Science 361, eaan8083 (2018).
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D. Grassani, E. Tagkoudi, H. Guo, C. Herkommer, T. J. Kippenberg, and C.-S. Brès, “Highly efficient 4 micron light generation through fs-fiber laser driven supercontinuum in Si3N4 waveguides,” ArXiv180606633 Phys. (2018).

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Figures (4)

Fig. 1
Fig. 1 Overview. a) Experimental setup. Two mutually coherent, self-referenced fiber laser frequency combs are amplified in an Er+-doped fiber amplifier (EDFA) and then focused into the waveguides with aspheric lenses. The supercontinuum output is collimated by an off-axis parabolic mirror (OPM), combined on a CaF2 beam splitter (BS), directed through a 1.8 μm optical long-pass filter, spatially filtered with a 10 μm diameter pinhole, and finally transmitted through a 0.75 m gas cell filled with CO2 and CO. A reference background spectrum is acquired over the labelled reference path sequentially after bypassing the cell via flip-mirrors. b) Scanning electron microscopy cross section of a non-tapered waveguide facet suspended in SiO2 showing the waveguide dimensions. In the experiment, tapered waveguides are used for increased coupling efficiency. c) Calculated waveguide dispersion for a waveguide with a width of 2000 nm and a thickness of 770 nm. d) SiN generated supercontinuum (pink) and the input spectrum (blue), measured with an FTIR, as well as modelled transmission across a 2 m open-air path at 0.5% water (grey).
Fig. 2
Fig. 2 Dual-comb spectroscopy spectra (1-minute long measurements, 160 MHz resolution). a) Without pinhole (green) and with pinhole preventing multimode interference (blue). The spectral coverage between the measurements varies due to different input power and input coupling. The narrow absorption features arise from CO2 and water. The inset shows part of the spectrum where the signal-to-noise ratio (SNR) for the two measurements was comparable. b) Dual-comb spectroscopy spectra after spatial filtering with a pinhole (blue trace) and after additional normalization with the reference spectrum (black trace). CO2 and CO absorption features from the gas cell are clearly visible. c) Detail of the normalized spectrum around the CO band. Both the fully resolved spectrum (grey trace, 160 MHz resolution) and a smoothed spectrum (black trace, 1.3 GHz resolution) show no baseline structure.
Fig. 3
Fig. 3 Comparison between measurement and model at the combs’ native 160 MHz resolution: a) Molecular absorbance from a 1-minute long dual-comb spectroscopy measurement (black) and from a fitted model based on Hitran 2016 (red) offset for clarity, along with their difference (grey). Expanded view of b) one CO absorption line at ν0 = 128.559400 THz and c) one CO2 line at ν1 = 148.830794 THz.
Fig. 4
Fig. 4 Relative intensity noise (RIN) measurements of the amplified comb light (green) and the SiN-waveguide broadened supercontinuum after the 1.8 μm filter (blue). The noise peak at 13 MHz arises from the non-linear amplification of a wake-mode instability specific to this oscillator design [39]. b) Averaged spectral SNR for a 60-second-long measurement as a function of optical power on the detector (squares). The dashed line is the calculated detector-noise limited SNR for a 12 pW /  Hz noise-equivalent-power (NEP), the solid line is the RIN limited SNR (calculated for −140 dBc/Hz), and the dotted line is the calculated shot-noise limited SNR. Note that at an optical power of 300 μW, the shot-noise is equivalent to a noise level of 9 pW /  Hz , below the 12 pW /  Hz NEP of the detector.

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