Abstract

We report on multidimensional spectroscopy in the mid-infrared, performed using a calomel-based acousto-optic programmable dispersive filter. Although the associated spectral resolution is currently not as good as what has been previously reported using time-domain interferometers or other pulse-shaping technologies, the extreme compactness of the calomel crystal allows a straightforward implementation in a pre-existing pump-probe setup. Furthermore, the frequency-domain approach allows easy measurement of 2D slices of the multidimensional spectrum associated with a given pump frequency. We demonstrate our method with the measurement of the mid-infrared spectrum of carboxy-hemoglobin in three spectro-temporal dimensions.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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References

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    [Crossref]
  4. V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
    [Crossref] [PubMed]
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    [Crossref] [PubMed]
  6. S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” P. Natl. Acad. Sci. U.S.A. 104, 14197–14202 (2007).
    [Crossref]
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  14. P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
    [Crossref] [PubMed]
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    [Crossref]
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    [Crossref] [PubMed]
  24. M. Lim, P. Hamm, and R. M. Hochstrasser, “Protein fluctuations are sensed by stimulated infrared echoes of the vibrations of carbon monoxide and azide probes,” P. Natl. Acad. Sci. U.S.A. 95, 15315–15320 (1998).
    [Crossref]

2016 (1)

V. Kemlin, A. Bonvalet, L. Daniault, and M. Joffre, “Transient two-dimensional infrared spectroscopy in a vibrational ladder,” J. Phys. Chem. Lett. 7, 3377–3382 (2016).
[Crossref] [PubMed]

2015 (1)

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

2014 (1)

2013 (1)

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

2010 (3)

2009 (2)

K. F. Lee, P. Nuernberger, A. Bonvalet, and M. Joffre, “Removing cross-phase modulation from midinfrared chirped-pulse upconversion spectra,” Opt. Express 17, 18738–18744 (2009).
[Crossref]

S. H. Shim and M. T. Zanni, “How to turn your pump-probe instrument into a multidimensional spectrometer: 2D IR and Vis spectroscopies via pulse shaping,” Phys. Chem. Chem. Phys. 11, 748–761 (2009).
[Crossref] [PubMed]

2008 (2)

P. Tournois, “Design of acousto-optic programmable filters in mercury halides for mid-infrared laser pulse shaping,” Opt. Comm. 281, 4054–4056 (2008).
[Crossref]

J. A. Myers, K. L. M. Lewis, P. F. Tekavec, and J. P. Ogilvie, “Two-color two-dimensional Fourier transform electronic spectroscopy with a pulse-shaper,” Opt. Express 16, 17420–17428 (2008).
[Crossref]

2007 (3)

L. P. DeFlores, R. A. Nicodemus, and A. Tokmakoff, “Two dimensonal Fourier transform spectroscopy in the pump-probe geometry,” Opt. Lett. 32, 2966–2968 (2007).
[Crossref] [PubMed]

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” P. Natl. Acad. Sci. U.S.A. 104, 14197–14202 (2007).
[Crossref]

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, “Multidimensional coherent spectroscopy made easy,” Chem. Phys. 341, 89–94 (2007).
[Crossref]

2006 (1)

2004 (1)

V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
[Crossref] [PubMed]

2000 (2)

1999 (1)

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: Theory and model calculations,” J. Phys. Chem. A 103, 10489–10505 (1999).
[Crossref]

1998 (2)

P. Hamm, M. H. Lim, and R. M. Hochstrasser, “Structure of the amide I band of peptides measured by femtosecond nonlinear-infrared spectroscopy,” J. Phys. Chem. B 102, 6123–6138 (1998).
[Crossref]

M. Lim, P. Hamm, and R. M. Hochstrasser, “Protein fluctuations are sensed by stimulated infrared echoes of the vibrations of carbon monoxide and azide probes,” P. Natl. Acad. Sci. U.S.A. 95, 15315–15320 (1998).
[Crossref]

1997 (1)

1996 (1)

Anna, J. M.

Baiz, C. R.

Barta, C.

Bloem, R.

Bonora, S.

Bonvalet, A.

V. Kemlin, A. Bonvalet, L. Daniault, and M. Joffre, “Transient two-dimensional infrared spectroscopy in a vibrational ladder,” J. Phys. Chem. Lett. 7, 3377–3382 (2016).
[Crossref] [PubMed]

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

R. Maksimenka, P. Nuernberger, K. F. Lee, A. Bonvalet, J. Milkiewicz, C. Barta, M. Klima, T. Oksenhendler, P. Tournois, D. Kaplan, and M. Joffre, “Direct mid-infrared femtosecond pulse shaping with a calomel acousto-optic programmable dispersive filter,” Opt. Lett. 35, 3565–3567 (2010).
[Crossref] [PubMed]

K. F. Lee, P. Nuernberger, A. Bonvalet, and M. Joffre, “Removing cross-phase modulation from midinfrared chirped-pulse upconversion spectra,” Opt. Express 17, 18738–18744 (2009).
[Crossref]

Bredenbeck, J.

V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
[Crossref] [PubMed]

Cartella, A.

Cavalleri, A.

Cerullo, G.

Cervetto, V.

V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
[Crossref] [PubMed]

Cheng, Z.

Crozatier, V.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Daniault, L.

V. Kemlin, A. Bonvalet, L. Daniault, and M. Joffre, “Transient two-dimensional infrared spectroscopy in a vibrational ladder,” J. Phys. Chem. Lett. 7, 3377–3382 (2016).
[Crossref] [PubMed]

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

DeFlores, L. P.

Donaldson, P.

Dugan, M. A.

Falvo, C.

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

Forget, N.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Forst, M.

Fulmer, E. C.

Gallagher Faeder, S. M.

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: Theory and model calculations,” J. Phys. Chem. A 103, 10489–10505 (1999).
[Crossref]

Garrett-roe, S.

Gundogdu, K.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, “Multidimensional coherent spectroscopy made easy,” Chem. Phys. 341, 89–94 (2007).
[Crossref]

Hamm, P.

R. Bloem, S. Garrett-roe, H. Strzalka, P. Hamm, and P. Donaldson, “Enhancing signal detection and completely eliminating scattering using quasi-phase-cycling in 2D IR experiments,” Opt. Express 18, 27067–27078 (2010).
[Crossref]

V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
[Crossref] [PubMed]

P. Hamm, M. H. Lim, and R. M. Hochstrasser, “Structure of the amide I band of peptides measured by femtosecond nonlinear-infrared spectroscopy,” J. Phys. Chem. B 102, 6123–6138 (1998).
[Crossref]

M. Lim, P. Hamm, and R. M. Hochstrasser, “Protein fluctuations are sensed by stimulated infrared echoes of the vibrations of carbon monoxide and azide probes,” P. Natl. Acad. Sci. U.S.A. 95, 15315–15320 (1998).
[Crossref]

P. Hamm and M. Zanni, Concepts and Methods of 2D Infrared Spectroscopy (Cambridge University, 2011).
[Crossref]

Helbing, J.

V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
[Crossref] [PubMed]

Hochstrasser, R. M.

P. Hamm, M. H. Lim, and R. M. Hochstrasser, “Structure of the amide I band of peptides measured by femtosecond nonlinear-infrared spectroscopy,” J. Phys. Chem. B 102, 6123–6138 (1998).
[Crossref]

M. Lim, P. Hamm, and R. M. Hochstrasser, “Protein fluctuations are sensed by stimulated infrared echoes of the vibrations of carbon monoxide and azide probes,” P. Natl. Acad. Sci. U.S.A. 95, 15315–15320 (1998).
[Crossref]

Joffre, M.

Jonas, D. M.

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: Theory and model calculations,” J. Phys. Chem. A 103, 10489–10505 (1999).
[Crossref]

Kabir, A.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Kambhampati, P.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Kaplan, D.

Kemlin, V.

V. Kemlin, A. Bonvalet, L. Daniault, and M. Joffre, “Transient two-dimensional infrared spectroscopy in a vibrational ladder,” J. Phys. Chem. Lett. 7, 3377–3382 (2016).
[Crossref] [PubMed]

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

Klima, M.

Kubarych, K. J.

Lambry, J. C.

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

Laude, V.

Lee, K. F.

Lepetit, L.

Lewis, K. L. M.

Lim, M.

M. Lim, P. Hamm, and R. M. Hochstrasser, “Protein fluctuations are sensed by stimulated infrared echoes of the vibrations of carbon monoxide and azide probes,” P. Natl. Acad. Sci. U.S.A. 95, 15315–15320 (1998).
[Crossref]

Lim, M. H.

P. Hamm, M. H. Lim, and R. M. Hochstrasser, “Structure of the amide I band of peptides measured by femtosecond nonlinear-infrared spectroscopy,” J. Phys. Chem. B 102, 6123–6138 (1998).
[Crossref]

Ling, Y. L.

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” P. Natl. Acad. Sci. U.S.A. 104, 14197–14202 (2007).
[Crossref]

Maksimenka, R.

Manzoni, C.

McCanne, R.

Meier, C.

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

Milkiewicz, J.

Myers, J. A.

Nee, M. J.

Nelson, K. A.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, “Multidimensional coherent spectroscopy made easy,” Chem. Phys. 341, 89–94 (2007).
[Crossref]

Nicodemus, R. A.

Nuernberger, P.

Ogilvie, J. P.

Oksenhendler, T.

Saari, J. I.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Shim, S. H.

S. H. Shim and M. T. Zanni, “How to turn your pump-probe instrument into a multidimensional spectrometer: 2D IR and Vis spectroscopies via pulse shaping,” Phys. Chem. Chem. Phys. 11, 748–761 (2009).
[Crossref] [PubMed]

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” P. Natl. Acad. Sci. U.S.A. 104, 14197–14202 (2007).
[Crossref]

Shim, S.-H.

Spielmann, C.

Stone, K. W.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, “Multidimensional coherent spectroscopy made easy,” Chem. Phys. 341, 89–94 (2007).
[Crossref]

Strasfeld, D. B.

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” P. Natl. Acad. Sci. U.S.A. 104, 14197–14202 (2007).
[Crossref]

S.-H. Shim, D. B. Strasfeld, E. C. Fulmer, and M. T. Zanni, “Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation,” Opt. Lett. 31, 838–840 (2006).
[Crossref] [PubMed]

Strzalka, H.

Tekavec, P. F.

Tokmakoff, A.

Tournois, P.

Tull, J. X.

Turner, D. B.

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, “Multidimensional coherent spectroscopy made easy,” Chem. Phys. 341, 89–94 (2007).
[Crossref]

Tyagi, P.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Verluise, F.

Vieille, T.

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

Vos, M. H.

C. Falvo, L. Daniault, T. Vieille, V. Kemlin, J. C. Lambry, C. Meier, M. H. Vos, A. Bonvalet, and M. Joffre, “Ultrafast dynamics of carboxy-hemoglobin: Two-dimensional infrared spectroscopy experiments and simulations,” J. Phys. Chem. Lett. 6, 2216–2222 (2015).
[Crossref] [PubMed]

Walsh, B.

P. Tyagi, J. I. Saari, B. Walsh, A. Kabir, V. Crozatier, N. Forget, and P. Kambhampati, “Two-color two-dimensional electronic spectroscopy using dual acousto-optic pulse shapers for complete amplitude, phase, and polarization control of femtosecond laser pulses,” J. Phys. Chem. A 117, 6264–6269 (2013).
[Crossref] [PubMed]

Warren, W. S.

Weiner, A. M.

A. M. Weiner, “Femtosecond pulse shaping using spatial light modulators,” Rev. Sci. Instr. 71, 1929–1960 (2000).
[Crossref]

Zanni, M.

P. Hamm and M. Zanni, Concepts and Methods of 2D Infrared Spectroscopy (Cambridge University, 2011).
[Crossref]

Zanni, M. T.

S. H. Shim and M. T. Zanni, “How to turn your pump-probe instrument into a multidimensional spectrometer: 2D IR and Vis spectroscopies via pulse shaping,” Phys. Chem. Chem. Phys. 11, 748–761 (2009).
[Crossref] [PubMed]

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” P. Natl. Acad. Sci. U.S.A. 104, 14197–14202 (2007).
[Crossref]

S.-H. Shim, D. B. Strasfeld, E. C. Fulmer, and M. T. Zanni, “Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation,” Opt. Lett. 31, 838–840 (2006).
[Crossref] [PubMed]

Chem. Phys. (1)

K. Gundogdu, K. W. Stone, D. B. Turner, and K. A. Nelson, “Multidimensional coherent spectroscopy made easy,” Chem. Phys. 341, 89–94 (2007).
[Crossref]

J. Chem. Phys. (1)

V. Cervetto, J. Helbing, J. Bredenbeck, and P. Hamm, “Double-resonance versus pulsed Fourier transform two-dimensional infrared spectroscopy: An experimental and theoretical comparison,” J. Chem. Phys. 121, 5935–5942 (2004).
[Crossref] [PubMed]

J. Opt. Soc. Am. B (2)

J. Phys. Chem. A (2)

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: Theory and model calculations,” J. Phys. Chem. A 103, 10489–10505 (1999).
[Crossref]

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Supplementary Material (2)

NameDescription
» Visualization 1       Series of 2DIR spectra measured in carboxy-hemoglobin using a calomel pulse shaper.
» Visualization 2       Series of 2DIR spectra measured in carboxy-hemoglobin using a calomel pulse shaper.

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Figures (4)

Fig. 1
Fig. 1 Experimental setup for 2DIR spectroscopy using an Acousto-Optic Programmable Dispersive Filter (AOPDF). (BS) Beam splitter, (HWP) Half-Wave Plate, (L) lens, (M) Mirror mounted on a motorized rotation stage around the vertical axis and on a translation stage along the direction of the reflected beam. Dotted lines 1 and 2 show alternate paths used during the alignment procedure (see text).
Fig. 2
Fig. 2 Schematic view of the 4N pulse sequence used in the 2DIR measurement, where N is the number of different pump frequencies.
Fig. 3
Fig. 3 Set of 2DIR spectra measured for the specified values of the waiting time T. The color scale is common to all plots and shows the relative change in differential transmission (in percents) of non-interpolated data. The dotted-line curves superimposed on the last 2DIR spectrum show two examples of scattered pump spectra, centered respectively at 1941 and 1962 cm−1. ( Visualization 1) Full 3D set with waiting time T varying between −3 and +48 ps. ( Visualization 2) Full 3D set with linear interpolation on pump wavenumber and waiting time axes.
Fig. 4
Fig. 4 (a) Dependence of the pump-probe signal as a function of time delay, for a pump frequency tuned to 1951 cm−1. (b) Time dependence of induced bleaching (blue disks) and induced absorption (red diamonds, inverted scale) peak amplitude. The solid line shows an exponential fit, yielding a vibrational time constant T1 ≈ 22.3 ps.

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