Abstract

A spectroscopic method free from systematic errors is desired for many challenging applications of gas detection. Although existing cavity-enhanced techniques exhibit very high precision, their accuracy strongly depends on propagation of the light amplitude through an optical system and its detection. Here, we demonstrate that the frequency-based molecular dispersion spectroscopy, involving sub-Hz-level precision in frequency measurements of optical cavity resonances, leads to sub-per-mille accuracy and a wide dynamic range, both previously unattainable by any other spectroscopic technique. The method offers great sensitivity of 5×10−11 cm−1, high speed, limited only by the fundamental response time of the cavity, and traceability of both axes of the spectrum to the primary frequency standard. All these features are necessary for convenient realization of comprehensive molecular spectroscopy from Doppler up to collisional regime without changing the spectroscopic method and modification of the experimental setup. Moreover, the presented approach does not require linear, high-bandwidth nor phase-sensitive detectors and can be directly implemented in existing cavity-enhanced spectrometers utilizing either continuous-wave or coherent broadband radiation. We experimentally prove the predominance of frequency-based spectroscopy over intensity-based one. Our results motivate replacement of intensity-based absorption spectroscopy with a pure frequency-based dispersion one in applications where the highest accuracy is required.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2019 (1)

G. Kowzan, D. Charczun, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband optical cavity mode measurements at Hz-level precision with a comb-based VIPA spectrometer,” Sci. Rep. 9(1), 8206 (2019).
[Crossref]

2018 (6)

L.-G. Tao, A.-W. Liu, K. Pachucki, J. Komasa, Y. R. Sun, J. Wang, and S.-M. Hu, “Toward a determination of the proton-electron mass ratio from the Lamb-dip measurement of HD,” Phys. Rev. Lett. 120(15), 153001 (2018).
[Crossref]

F. M. J. Cozijn, P. Dupre, E. J. Salumbides, K. S. E. Eikema, and W. Ubachs, “Sub-Doppler frequency metrology in HD for tests of fundamental physics,” Phys. Rev. Lett. 120(15), 153002 (2018).
[Crossref]

A. C. Johansson, L. Rutkowski, A. Filipsson, T. Hausmaninger, G. Zhao, O. Axner, and A. Foltynowicz, “Broadband calibration-free cavity-enhanced complex refractive index spectroscopy using a frequency comb,” Opt. Express 26(16), 20633 (2018).
[Crossref]

D. Charczun, G. Kowzan, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband and high resolution measurements of cavity loss and dispersion,” Photonics Lett. Pol. 10(2), 48 (2018).
[Crossref]

S. Koulikov, S. Assonov, A. Fajgelj, and P. Tans, “Potential improvements aimed at high precision δ13C isotopic ratio determinations in CO2 mixtures using optical absorption spectrometry,” Talanta 184, 73–86 (2018).
[Crossref]

S. Wójtewicz, A. Cygan, J. Domysławska, K. Bielska, P. Morzyński, P. Masłowski, R. Ciuryło, and D. Lisak, “Response of an optical cavity to phase-controlled incomplete power switching of nearly resonant incident light,” Opt. Express 26(5), 5644 (2018).
[Crossref]

2017 (3)

L. Rutkowski, A. C. Johansson, G. Zhao, T. Hausmaninger, A. Khodabakhsh, O. Axner, and A. Foltynowicz, “Sensitive and broadband measurement of dispersion in a cavity using a Fourier transform spectrometer with kHz resolution,” Opt. Express 25(18), 21711 (2017).
[Crossref]

M. Zaborowski, P. Wcisło, F. Thibault, S. Wójtewicz, A. Cygan, G. Kowzan, P. Masłowski, D. Lisak, and R. Ciuryło, “Ultra accurate measurements and ab initio calculations of collisional effects in pure D2,” J. Phys.: Conf. Ser. 810, 012042 (2017).
[Crossref]

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

2016 (2)

A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
[Crossref]

A. Cygan, S. Wójtewicz, M. Zaborowski, P. Wcisło, R. Guo, R. Ciuryło, and D. Lisak, “One-dimensional cavity mode-dispersion spectroscopy for validation of CRDS technique,” Meas. Sci. Technol. 27(4), 045501 (2016).
[Crossref]

2015 (6)

A. Cygan, P. Wcisło, S. Wójtewicz, P. Masłowski, J. T. Hodges, R. Ciuryło, and D. Lisak, “One-dimensional frequency-based spectroscopy,” Opt. Express 23(11), 14472 (2015).
[Crossref]

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
[Crossref]

S. Seager and W. Bains, “The search for signs of life on exoplanets at the interface of chemistry and planetary science,” Sci. Adv. 1(2), e1500047 (2015).
[Crossref]

O. L. Polyansky, K. Bielska, M. Ghysels, L. Lodi, N. F. Zobov, J. T. Hodges, and J. Tennyson, “High-accuracy CO2 line intensities determined from theory and experiment,” Phys. Rev. Lett. 114(24), 243001 (2015).
[Crossref]

D. Lisak, A. Cygan, D. Bermejo, J. L. Domenech, J. T. Hodges, and H. Tran, “Application of the Hartmann-Tran profile to analysis of H2O spectra,” J. Quant. Spectrosc. Radiat. Transfer 164, 221–230 (2015).
[Crossref]

D. Mondelain, T. Sala, S. Kassi, D. Romanini, M. Marangoni, and A. Campargue, “Broadband and highly sensitive comb-assisted cavity ring down spectroscopy of CO near 1.57 µm with sub-MHz frequency accuracy,” J. Quant. Spectrosc. Radiat. Transfer 154, 35–43 (2015).
[Crossref]

2014 (6)

J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
[Crossref]

A. S. Burrows, “Highlights in the study of exoplanet atmospheres,” Nature 513(7518), 345–352 (2014).
[Crossref]

P. F. Bernath, “Molecular opacities for exoplanets,” Phil. Trans. R. Soc. A 372(2014), 20130087 (2014).
[Crossref]

D. A. Long, G.-W. Truong, R. D. van Zee, D. F. Plusquellic, and J. T. Hodges, “Frequency-agile, rapid scanning spectroscopy: absorption sensitivity of 2×10−12 cm−1Hz−1/2 with a tunable diode laser,” Appl. Phys. B: Lasers Opt. 114(4), 489–495 (2014).
[Crossref]

S. Wójtewicz, A. Cygan, P. Masłowski, J. Domysławska, D. Lisak, R. S. Trawiński, and R. Ciuryło, “Spectral line shapes of self-broadened P-branch transitions of oxygen B band,” J. Quant. Spectrosc. Radiat. Transfer 144, 36–48 (2014).
[Crossref]

J. Wang, P. Ehlers, I. Silander, and O. Axner, “On the accuracy of the assessment of molecular concentration and spectroscopic parameters by frequency modulation spectrometry and NICE-OHMS,” J. Quant. Spectrosc. Radiat. Transfer 136, 28–44 (2014).
[Crossref]

2013 (4)

G.-W. Truong, K. O. Douglass, S. E. Maxwell, R. D. van Zee, D. F. Plusquellic, J. T. Hodges, and D. A. Long, “Frequency-agile, rapid scanning spectroscopy,” Nat. Photonics 7(7), 532–534 (2013).
[Crossref]

J. Burkart, D. Romanini, and S. Kassi, “Optical feedback stabilized laser tuned by single-sideband modulation,” Opt. Lett. 38(12), 2062 (2013).
[Crossref]

A. Cygan, D. Lisak, P. Morzyński, M. Bober, M. Zawada, E. Pazderski, and R. Ciuryło, “Cavity mode-width spectroscopy with widely tunable ultra-narrow laser,” Opt. Express 21(24), 29744 (2013).
[Crossref]

E. J. Salumbides, J. C. J. Koelemeij, J. Komasa, K. Pachucki, K. S. E. Eikema, and W. Ubachs, “Bounds on fifth forces from precision measurements on molecules,” Phys. Rev. D 87(11), 112008 (2013).
[Crossref]

2012 (3)

D. R. Thompson, D. C. Benner, L. R. Brown, D. Crisp, V. Malathy Devi, Y. Jiang, V. Natraj, F. Oyafuso, K. Sung, D. Wunch, R. Castaño, and C. E. Miller, “Atmospheric validation of high accuracy CO2 absorption coefficients for the OCO-2 mission,” J. Quant. Spectrosc. Radiat. Transfer 113(17), 2265–2276 (2012).
[Crossref]

S. Yu, C. E. Miller, B. J. Drouin, and H. S. Müller, “High resolution spectral analysis of oxygen. I. Isotopically invariant Dunham fit for the X3Σg-, a1Δg, b1Σg+ states,” J. Chem. Phys. 137(2), 024304 (2012).
[Crossref]

A. Cygan, D. Lisak, S. Wójtewicz, J. Domysławska, J. T. Hodges, R. S. Trawiński, and R. Ciuryło, “High signal-to-noise ratio laser technique for accurate measurements of spectral line parameters,” Phys. Rev. A 85(2), 022508 (2012).
[Crossref]

2011 (4)

A. Cygan, D. Lisak, S. Wójtewicz, J. Domysławska, R. S. Trawiński, and R. Ciuryło, “Active control of the Pound-Drever-Hall error signal offset in high-repetition-rate cavity ring-down spectroscopy,” Meas. Sci. Technol. 22(11), 115303 (2011).
[Crossref]

I. Galli, S. Bartalini, S. Borri, P. Cancio, D. Mazzotti, P. De Natale, and G. Giusfredi, “Molecular gas sensing below parts per trillion: radiocarbon-dioxide optical detection,” Phys. Rev. Lett. 107(27), 270802 (2011).
[Crossref]

E. J. Salumbides, G. D. Dickenson, T. I. Ivanov, and W. Ubachs, “QED Effects in Molecules: Test on Rotational Quantum States of H2,” Phys. Rev. Lett. 107(4), 043005 (2011).
[Crossref]

S. Wójtewicz, D. Lisak, A. Cygan, J. Domysławska, R. Trawiński, and R. Ciuryło, “Line-shape study of self-broadened O2 transitions measured by Pound-Drever-Hall-locked frequency-stabilized cavity ring-down spectroscopy,” Phys. Rev. A 84(3), 032511 (2011).
[Crossref]

2010 (1)

F. M. Schmidt, W. Ma, A. Foltynowicz, and O. Axner, “Highly sensitive dispersion spectroscopy by probing the free spectral range of an optical cavity using dual-frequency modulation,” Appl. Phys. B: Lasers Opt. 101(3), 497–509 (2010).
[Crossref]

2009 (1)

H. Huang and K. K. Lehmann, “Noise caused by a finite extinction ratio of the light modulator in CW cavity ring-down spectroscopy,” Appl. Phys. B: Lasers Opt. 94(2), 355–366 (2009).
[Crossref]

2004 (1)

K. Sung and P. Varanasi, “Intensities, collision-broadened half-widths, and collision-induced line shifts in the second overtone band of 12C16O,” J. Quant. Spectrosc. Radiat. Transfer 83(3-4), 445–458 (2004).
[Crossref]

2002 (1)

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
[Crossref]

2001 (1)

A. S. Pine and R. Ciuryło, “Multispectrum fits of Ar-broadened HF with a generalized asymmetric lineshape: effects of correlation, hardness, speed dependence, and collision duration,” J. Mol. Spectrosc. 208(2), 180–187 (2001).
[Crossref]

1999 (1)

A. S. Pine, “Asymmetries and correlations in speed-dependent Dicke-narrowed line shapes of argon-broadened HF,” J. Quant. Spectrosc. Radiat. Transfer 62(4), 397–423 (1999).
[Crossref]

1998 (1)

1997 (1)

R. Ciuryło and J. Szudy, “Speed-dependent pressure broadening and shift in the soft collision approximation,” J. Quant. Spectrosc. Radiat. Transfer 57(3), 411–423 (1997).
[Crossref]

1996 (1)

J. T. Hodges, J. P. Looney, and R. D. van Zee, “Response of a ring-down cavity to an arbitrary excitation,” J. Chem. Phys. 105(23), 10278–10288 (1996).
[Crossref]

1995 (1)

D. C. Benner, C. P. Rinsland, V. M. Devi, M. A. H. Smith, and D. Atkins, “A multispectrum nonlinear least squares fitting technique,” J. Quant. Spectrosc. Radiat. Transfer 53(6), 705–721 (1995).
[Crossref]

1994 (1)

K. Nakagawa, T. Katsuda, A. S. Shelkovnikov, M. de Labachelerie, and M. Ohtsu, “Highly sensitive detection of molecular absorption using a high finesse optical cavity,” Opt. Commun. 107(5-6), 369–372 (1994).
[Crossref]

1985 (1)

1972 (1)

P. R. Berman, “Speed-dependent collisional width and shift parameters in spectral profiles,” J. Quant. Spectrosc. Radiat. Transfer 12(9), 1331–1342 (1972).
[Crossref]

1953 (1)

R. H. Dicke, “The effect of collisions upon the Doppler width of spectral lines,” Phys. Rev. 89(2), 472–473 (1953).
[Crossref]

Adkins, E. M.

A. J. Fleisher, E. M. Adkins, Z. D. Reed, H. Yi, D. A. Long, H. M. Fleurbaey, and J. T. Hodges, “Twenty-five-fold reduction in measurement uncertainty for a molecular line intensity,” Phys. Rev. Lett. (accepted for publication).

Assonov, S.

S. Koulikov, S. Assonov, A. Fajgelj, and P. Tans, “Potential improvements aimed at high precision δ13C isotopic ratio determinations in CO2 mixtures using optical absorption spectrometry,” Talanta 184, 73–86 (2018).
[Crossref]

Atkins, D.

D. C. Benner, C. P. Rinsland, V. M. Devi, M. A. H. Smith, and D. Atkins, “A multispectrum nonlinear least squares fitting technique,” J. Quant. Spectrosc. Radiat. Transfer 53(6), 705–721 (1995).
[Crossref]

Axner, O.

A. C. Johansson, L. Rutkowski, A. Filipsson, T. Hausmaninger, G. Zhao, O. Axner, and A. Foltynowicz, “Broadband calibration-free cavity-enhanced complex refractive index spectroscopy using a frequency comb,” Opt. Express 26(16), 20633 (2018).
[Crossref]

L. Rutkowski, A. C. Johansson, G. Zhao, T. Hausmaninger, A. Khodabakhsh, O. Axner, and A. Foltynowicz, “Sensitive and broadband measurement of dispersion in a cavity using a Fourier transform spectrometer with kHz resolution,” Opt. Express 25(18), 21711 (2017).
[Crossref]

J. Wang, P. Ehlers, I. Silander, and O. Axner, “On the accuracy of the assessment of molecular concentration and spectroscopic parameters by frequency modulation spectrometry and NICE-OHMS,” J. Quant. Spectrosc. Radiat. Transfer 136, 28–44 (2014).
[Crossref]

F. M. Schmidt, W. Ma, A. Foltynowicz, and O. Axner, “Highly sensitive dispersion spectroscopy by probing the free spectral range of an optical cavity using dual-frequency modulation,” Appl. Phys. B: Lasers Opt. 101(3), 497–509 (2010).
[Crossref]

Bains, W.

S. Seager and W. Bains, “The search for signs of life on exoplanets at the interface of chemistry and planetary science,” Sci. Adv. 1(2), e1500047 (2015).
[Crossref]

Baker, D.

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
[Crossref]

Barbe, A.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

Bartalini, S.

I. Galli, S. Bartalini, S. Borri, P. Cancio, D. Mazzotti, P. De Natale, and G. Giusfredi, “Molecular gas sensing below parts per trillion: radiocarbon-dioxide optical detection,” Phys. Rev. Lett. 107(27), 270802 (2011).
[Crossref]

Bartoszek-Bober, D.

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
[Crossref]

Benner, D. C.

D. R. Thompson, D. C. Benner, L. R. Brown, D. Crisp, V. Malathy Devi, Y. Jiang, V. Natraj, F. Oyafuso, K. Sung, D. Wunch, R. Castaño, and C. E. Miller, “Atmospheric validation of high accuracy CO2 absorption coefficients for the OCO-2 mission,” J. Quant. Spectrosc. Radiat. Transfer 113(17), 2265–2276 (2012).
[Crossref]

D. C. Benner, C. P. Rinsland, V. M. Devi, M. A. H. Smith, and D. Atkins, “A multispectrum nonlinear least squares fitting technique,” J. Quant. Spectrosc. Radiat. Transfer 53(6), 705–721 (1995).
[Crossref]

Berman, P. R.

P. R. Berman, “Speed-dependent collisional width and shift parameters in spectral profiles,” J. Quant. Spectrosc. Radiat. Transfer 12(9), 1331–1342 (1972).
[Crossref]

Bermejo, D.

D. Lisak, A. Cygan, D. Bermejo, J. L. Domenech, J. T. Hodges, and H. Tran, “Application of the Hartmann-Tran profile to analysis of H2O spectra,” J. Quant. Spectrosc. Radiat. Transfer 164, 221–230 (2015).
[Crossref]

Bernath, P. F.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
[Crossref]

P. F. Bernath, “Molecular opacities for exoplanets,” Phil. Trans. R. Soc. A 372(2014), 20130087 (2014).
[Crossref]

Bielska, K.

S. Wójtewicz, A. Cygan, J. Domysławska, K. Bielska, P. Morzyński, P. Masłowski, R. Ciuryło, and D. Lisak, “Response of an optical cavity to phase-controlled incomplete power switching of nearly resonant incident light,” Opt. Express 26(5), 5644 (2018).
[Crossref]

O. L. Polyansky, K. Bielska, M. Ghysels, L. Lodi, N. F. Zobov, J. T. Hodges, and J. Tennyson, “High-accuracy CO2 line intensities determined from theory and experiment,” Phys. Rev. Lett. 114(24), 243001 (2015).
[Crossref]

Birk, M.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

Bober, M.

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
[Crossref]

A. Cygan, D. Lisak, P. Morzyński, M. Bober, M. Zawada, E. Pazderski, and R. Ciuryło, “Cavity mode-width spectroscopy with widely tunable ultra-narrow laser,” Opt. Express 21(24), 29744 (2013).
[Crossref]

Boone, C. D.

J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
[Crossref]

Borri, S.

I. Galli, S. Bartalini, S. Borri, P. Cancio, D. Mazzotti, P. De Natale, and G. Giusfredi, “Molecular gas sensing below parts per trillion: radiocarbon-dioxide optical detection,” Phys. Rev. Lett. 107(27), 270802 (2011).
[Crossref]

Boudon, V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

Bousquet, P.

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
[Crossref]

Brown, L. R.

D. R. Thompson, D. C. Benner, L. R. Brown, D. Crisp, V. Malathy Devi, Y. Jiang, V. Natraj, F. Oyafuso, K. Sung, D. Wunch, R. Castaño, and C. E. Miller, “Atmospheric validation of high accuracy CO2 absorption coefficients for the OCO-2 mission,” J. Quant. Spectrosc. Radiat. Transfer 113(17), 2265–2276 (2012).
[Crossref]

Bruhwiler, L.

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
[Crossref]

Buldyreva, J.

J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
[Crossref]

Burkart, J.

Burrows, A. S.

A. S. Burrows, “Highlights in the study of exoplanet atmospheres,” Nature 513(7518), 345–352 (2014).
[Crossref]

Campargue, A.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

D. Mondelain, T. Sala, S. Kassi, D. Romanini, M. Marangoni, and A. Campargue, “Broadband and highly sensitive comb-assisted cavity ring down spectroscopy of CO near 1.57 µm with sub-MHz frequency accuracy,” J. Quant. Spectrosc. Radiat. Transfer 154, 35–43 (2015).
[Crossref]

J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
[Crossref]

Cancio, P.

I. Galli, S. Bartalini, S. Borri, P. Cancio, D. Mazzotti, P. De Natale, and G. Giusfredi, “Molecular gas sensing below parts per trillion: radiocarbon-dioxide optical detection,” Phys. Rev. Lett. 107(27), 270802 (2011).
[Crossref]

Castaño, R.

D. R. Thompson, D. C. Benner, L. R. Brown, D. Crisp, V. Malathy Devi, Y. Jiang, V. Natraj, F. Oyafuso, K. Sung, D. Wunch, R. Castaño, and C. E. Miller, “Atmospheric validation of high accuracy CO2 absorption coefficients for the OCO-2 mission,” J. Quant. Spectrosc. Radiat. Transfer 113(17), 2265–2276 (2012).
[Crossref]

Chance, K. V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

Charczun, D.

G. Kowzan, D. Charczun, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband optical cavity mode measurements at Hz-level precision with a comb-based VIPA spectrometer,” Sci. Rep. 9(1), 8206 (2019).
[Crossref]

D. Charczun, G. Kowzan, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband and high resolution measurements of cavity loss and dispersion,” Photonics Lett. Pol. 10(2), 48 (2018).
[Crossref]

Chen, Y.-H.

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
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Ciais, P.

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Flaud, J.-M.

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Ghysels, M.

O. L. Polyansky, K. Bielska, M. Ghysels, L. Lodi, N. F. Zobov, J. T. Hodges, and J. Tennyson, “High-accuracy CO2 line intensities determined from theory and experiment,” Phys. Rev. Lett. 114(24), 243001 (2015).
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J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
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Hall, J. L.

Harrison, J. J.

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J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
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Heimann, M.

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A. Cygan, D. Lisak, S. Wójtewicz, J. Domysławska, J. T. Hodges, R. S. Trawiński, and R. Ciuryło, “High signal-to-noise ratio laser technique for accurate measurements of spectral line parameters,” Phys. Rev. A 85(2), 022508 (2012).
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Hu, S.-M.

L.-G. Tao, A.-W. Liu, K. Pachucki, J. Komasa, Y. R. Sun, J. Wang, and S.-M. Hu, “Toward a determination of the proton-electron mass ratio from the Lamb-dip measurement of HD,” Phys. Rev. Lett. 120(15), 153001 (2018).
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John, J.

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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
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Khodabakhsh, A.

Kleiner, I.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

Kochanov, R. V.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
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Koelemeij, J. C. J.

E. J. Salumbides, J. C. J. Koelemeij, J. Komasa, K. Pachucki, K. S. E. Eikema, and W. Ubachs, “Bounds on fifth forces from precision measurements on molecules,” Phys. Rev. D 87(11), 112008 (2013).
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Komasa, J.

L.-G. Tao, A.-W. Liu, K. Pachucki, J. Komasa, Y. R. Sun, J. Wang, and S.-M. Hu, “Toward a determination of the proton-electron mass ratio from the Lamb-dip measurement of HD,” Phys. Rev. Lett. 120(15), 153001 (2018).
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E. J. Salumbides, J. C. J. Koelemeij, J. Komasa, K. Pachucki, K. S. E. Eikema, and W. Ubachs, “Bounds on fifth forces from precision measurements on molecules,” Phys. Rev. D 87(11), 112008 (2013).
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Koulikov, S.

S. Koulikov, S. Assonov, A. Fajgelj, and P. Tans, “Potential improvements aimed at high precision δ13C isotopic ratio determinations in CO2 mixtures using optical absorption spectrometry,” Talanta 184, 73–86 (2018).
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Kowzan, G.

G. Kowzan, D. Charczun, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband optical cavity mode measurements at Hz-level precision with a comb-based VIPA spectrometer,” Sci. Rep. 9(1), 8206 (2019).
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D. Charczun, G. Kowzan, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband and high resolution measurements of cavity loss and dispersion,” Photonics Lett. Pol. 10(2), 48 (2018).
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M. Zaborowski, P. Wcisło, F. Thibault, S. Wójtewicz, A. Cygan, G. Kowzan, P. Masłowski, D. Lisak, and R. Ciuryło, “Ultra accurate measurements and ab initio calculations of collisional effects in pure D2,” J. Phys.: Conf. Ser. 810, 012042 (2017).
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A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
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Krehlik, P.

A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
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P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
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Lehmann, K. K.

H. Huang and K. K. Lehmann, “Noise caused by a finite extinction ratio of the light modulator in CW cavity ring-down spectroscopy,” Appl. Phys. B: Lasers Opt. 94(2), 355–366 (2009).
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Lipinski, M.

A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
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P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
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Lisak, D.

G. Kowzan, D. Charczun, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband optical cavity mode measurements at Hz-level precision with a comb-based VIPA spectrometer,” Sci. Rep. 9(1), 8206 (2019).
[Crossref]

D. Charczun, G. Kowzan, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband and high resolution measurements of cavity loss and dispersion,” Photonics Lett. Pol. 10(2), 48 (2018).
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S. Wójtewicz, A. Cygan, J. Domysławska, K. Bielska, P. Morzyński, P. Masłowski, R. Ciuryło, and D. Lisak, “Response of an optical cavity to phase-controlled incomplete power switching of nearly resonant incident light,” Opt. Express 26(5), 5644 (2018).
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M. Zaborowski, P. Wcisło, F. Thibault, S. Wójtewicz, A. Cygan, G. Kowzan, P. Masłowski, D. Lisak, and R. Ciuryło, “Ultra accurate measurements and ab initio calculations of collisional effects in pure D2,” J. Phys.: Conf. Ser. 810, 012042 (2017).
[Crossref]

A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
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A. Cygan, S. Wójtewicz, M. Zaborowski, P. Wcisło, R. Guo, R. Ciuryło, and D. Lisak, “One-dimensional cavity mode-dispersion spectroscopy for validation of CRDS technique,” Meas. Sci. Technol. 27(4), 045501 (2016).
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P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
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D. Lisak, A. Cygan, D. Bermejo, J. L. Domenech, J. T. Hodges, and H. Tran, “Application of the Hartmann-Tran profile to analysis of H2O spectra,” J. Quant. Spectrosc. Radiat. Transfer 164, 221–230 (2015).
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A. Cygan, P. Wcisło, S. Wójtewicz, P. Masłowski, J. T. Hodges, R. Ciuryło, and D. Lisak, “One-dimensional frequency-based spectroscopy,” Opt. Express 23(11), 14472 (2015).
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J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
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S. Wójtewicz, A. Cygan, P. Masłowski, J. Domysławska, D. Lisak, R. S. Trawiński, and R. Ciuryło, “Spectral line shapes of self-broadened P-branch transitions of oxygen B band,” J. Quant. Spectrosc. Radiat. Transfer 144, 36–48 (2014).
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A. Cygan, D. Lisak, P. Morzyński, M. Bober, M. Zawada, E. Pazderski, and R. Ciuryło, “Cavity mode-width spectroscopy with widely tunable ultra-narrow laser,” Opt. Express 21(24), 29744 (2013).
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A. Cygan, D. Lisak, S. Wójtewicz, J. Domysławska, J. T. Hodges, R. S. Trawiński, and R. Ciuryło, “High signal-to-noise ratio laser technique for accurate measurements of spectral line parameters,” Phys. Rev. A 85(2), 022508 (2012).
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S. Wójtewicz, D. Lisak, A. Cygan, J. Domysławska, R. Trawiński, and R. Ciuryło, “Line-shape study of self-broadened O2 transitions measured by Pound-Drever-Hall-locked frequency-stabilized cavity ring-down spectroscopy,” Phys. Rev. A 84(3), 032511 (2011).
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A. Cygan, D. Lisak, S. Wójtewicz, J. Domysławska, R. S. Trawiński, and R. Ciuryło, “Active control of the Pound-Drever-Hall error signal offset in high-repetition-rate cavity ring-down spectroscopy,” Meas. Sci. Technol. 22(11), 115303 (2011).
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Liu, A.-W.

L.-G. Tao, A.-W. Liu, K. Pachucki, J. Komasa, Y. R. Sun, J. Wang, and S.-M. Hu, “Toward a determination of the proton-electron mass ratio from the Lamb-dip measurement of HD,” Phys. Rev. Lett. 120(15), 153001 (2018).
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Lodi, L.

O. L. Polyansky, K. Bielska, M. Ghysels, L. Lodi, N. F. Zobov, J. T. Hodges, and J. Tennyson, “High-accuracy CO2 line intensities determined from theory and experiment,” Phys. Rev. Lett. 114(24), 243001 (2015).
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Long, D. A.

D. A. Long, G.-W. Truong, R. D. van Zee, D. F. Plusquellic, and J. T. Hodges, “Frequency-agile, rapid scanning spectroscopy: absorption sensitivity of 2×10−12 cm−1Hz−1/2 with a tunable diode laser,” Appl. Phys. B: Lasers Opt. 114(4), 489–495 (2014).
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G.-W. Truong, K. O. Douglass, S. E. Maxwell, R. D. van Zee, D. F. Plusquellic, J. T. Hodges, and D. A. Long, “Frequency-agile, rapid scanning spectroscopy,” Nat. Photonics 7(7), 532–534 (2013).
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A. J. Fleisher, E. M. Adkins, Z. D. Reed, H. Yi, D. A. Long, H. M. Fleurbaey, and J. T. Hodges, “Twenty-five-fold reduction in measurement uncertainty for a molecular line intensity,” Phys. Rev. Lett. (accepted for publication).

Looney, J. P.

J. T. Hodges, J. P. Looney, and R. D. van Zee, “Response of a ring-down cavity to an arbitrary excitation,” J. Chem. Phys. 105(23), 10278–10288 (1996).
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Loos, J.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
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Ma, L.-S.

Ma, W.

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Maksyutov, S.

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
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Malathy Devi, V.

D. R. Thompson, D. C. Benner, L. R. Brown, D. Crisp, V. Malathy Devi, Y. Jiang, V. Natraj, F. Oyafuso, K. Sung, D. Wunch, R. Castaño, and C. E. Miller, “Atmospheric validation of high accuracy CO2 absorption coefficients for the OCO-2 mission,” J. Quant. Spectrosc. Radiat. Transfer 113(17), 2265–2276 (2012).
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Marangoni, M.

D. Mondelain, T. Sala, S. Kassi, D. Romanini, M. Marangoni, and A. Campargue, “Broadband and highly sensitive comb-assisted cavity ring down spectroscopy of CO near 1.57 µm with sub-MHz frequency accuracy,” J. Quant. Spectrosc. Radiat. Transfer 154, 35–43 (2015).
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Masarie, K.

K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
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Maslowski, P.

G. Kowzan, D. Charczun, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband optical cavity mode measurements at Hz-level precision with a comb-based VIPA spectrometer,” Sci. Rep. 9(1), 8206 (2019).
[Crossref]

D. Charczun, G. Kowzan, A. Cygan, R. S. Trawiński, D. Lisak, and P. Masłowski, “Broadband and high resolution measurements of cavity loss and dispersion,” Photonics Lett. Pol. 10(2), 48 (2018).
[Crossref]

S. Wójtewicz, A. Cygan, J. Domysławska, K. Bielska, P. Morzyński, P. Masłowski, R. Ciuryło, and D. Lisak, “Response of an optical cavity to phase-controlled incomplete power switching of nearly resonant incident light,” Opt. Express 26(5), 5644 (2018).
[Crossref]

M. Zaborowski, P. Wcisło, F. Thibault, S. Wójtewicz, A. Cygan, G. Kowzan, P. Masłowski, D. Lisak, and R. Ciuryło, “Ultra accurate measurements and ab initio calculations of collisional effects in pure D2,” J. Phys.: Conf. Ser. 810, 012042 (2017).
[Crossref]

A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
[Crossref]

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, Ł. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the 1S0 − 3P0 clock transition in neutral 88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5(1), 17495 (2015).
[Crossref]

A. Cygan, P. Wcisło, S. Wójtewicz, P. Masłowski, J. T. Hodges, R. Ciuryło, and D. Lisak, “One-dimensional frequency-based spectroscopy,” Opt. Express 23(11), 14472 (2015).
[Crossref]

S. Wójtewicz, A. Cygan, P. Masłowski, J. Domysławska, D. Lisak, R. S. Trawiński, and R. Ciuryło, “Spectral line shapes of self-broadened P-branch transitions of oxygen B band,” J. Quant. Spectrosc. Radiat. Transfer 144, 36–48 (2014).
[Crossref]

Massie, S. T.

I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
[Crossref]

Maxwell, S. E.

G.-W. Truong, K. O. Douglass, S. E. Maxwell, R. D. van Zee, D. F. Plusquellic, J. T. Hodges, and D. A. Long, “Frequency-agile, rapid scanning spectroscopy,” Nat. Photonics 7(7), 532–534 (2013).
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J. Tennyson, P. F. Bernath, A. Campargue, A. G. Csaszar, L. Daumont, R. R. Gamache, J. T. Hodges, D. Lisak, O. V. Naumenko, L. S. Rothman, H. Tran, N. F. Zobov, J. Buldyreva, C. D. Boone, M. D. De Vizia, L. Gianfrani, J.-M. Hartmann, R. McPheat, D. Weidmann, J. Murray, N. H. Ngo, and O. L. Polyanski, “Recommended isolated-line profile for representing high-resolution spectroscopic transitions (IUPAC Technical Report),” Pure Appl. Chem. 86(12), 1931–1943 (2014).
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I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, V. I. Perevalov, A. Perrin, K. P. Shine, M.-A. H. Smith, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, A. Barbe, A. G. Császár, V. M. Devi, T. Furtenbacher, J. J. Harrison, J.-M. Hartmann, A. Jolly, T. J. Johnson, T. Karman, I. Kleiner, A. A. Kyuberis, J. Loos, O. M. Lyulin, S. T. Massie, S. N. Mikhailenko, N. Moazzen-Ahmadi, H. S. P. Müller, O. V. Naumenko, A. V. Nikitin, O. L. Polyansky, M. Rey, M. Rotger, S. W. Sharpe, K. Sung, E. Starikova, S. A. Tashkun, J. Vander Auwera, G. Wagner, J. Wilzewski, P. Wcisło, S. Yu, and E. J. Zak, “The HITRAN2016 molecular spectroscopic database,” J. Quant. Spectrosc. Radiat. Transfer 203, 3–69 (2017).
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Perevalov, V. I.

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K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
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K. R. Gurney, R. M. Law, A. S. Denning, P. J. Rayner, D. Baker, P. Bousquet, L. Bruhwiler, Y.-H. Chen, P. Ciais, S. Fan, I. Y. Fung, M. Gloor, M. Heimann, K. Higuchi, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Peylin, M. Prather, B. C. Pak, J. Randerson, J. Sarmiento, S. Taguchi, T. Takahashi, and C.-W. Yuen, “Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models,” Nature 415(6872), 626–630 (2002).
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A. Cygan, D. Lisak, S. Wójtewicz, J. Domysławska, R. S. Trawiński, and R. Ciuryło, “Active control of the Pound-Drever-Hall error signal offset in high-repetition-rate cavity ring-down spectroscopy,” Meas. Sci. Technol. 22(11), 115303 (2011).
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A. Cygan, S. Wójtewicz, M. Zaborowski, P. Wcisło, R. Guo, R. Ciuryło, and D. Lisak, “One-dimensional cavity mode-dispersion spectroscopy for validation of CRDS technique,” Meas. Sci. Technol. 27(4), 045501 (2016).
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A. Cygan, P. Wcisło, S. Wójtewicz, P. Masłowski, J. T. Hodges, R. Ciuryło, and D. Lisak, “One-dimensional frequency-based spectroscopy,” Opt. Express 23(11), 14472 (2015).
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S. Yu, C. E. Miller, B. J. Drouin, and H. S. Müller, “High resolution spectral analysis of oxygen. I. Isotopically invariant Dunham fit for the X3Σg-, a1Δg, b1Σg+ states,” J. Chem. Phys. 137(2), 024304 (2012).
[Crossref]

A. Cygan, S. Wójtewicz, G. Kowzan, M. Zaborowski, P. Wcisło, J. Nawrocki, P. Krehlik, Ł Śliwczyński, M. Lipiński, P. Masłowski, R. Ciuryło, and D. Lisak, “Absolute molecular transitions frequencies measured by three cavity-enhanced spectroscopy techniques,” J. Chem. Phys. 144(21), 214202 (2016).
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J. Quant. Spectrosc. Radiat. Transfer (11)

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Figures (4)

Fig. 1.
Fig. 1. Diagram of universal experimental setup for implementation of methods: CRDS, CMWS and CMDS. (a) A beam of laser 1 with frequency νL is divided into three parts. The first one is sent to the optical frequency comb (OFC) in order to monitor the frequency stability of the laser and to provide an absolute frequency axis for measurements. The second one, vertically polarized, is used to tightly phase-lock the laser to the optical cavity resonance. The third one, horizontally polarized, is first modulated by the high-bandwidth electrooptical modulator (EOM) with the radiofrequency νRF and next frequency shifted by the acoustooptic modulator driven by the radiofrequency δ. The single sideband of the EOM is used as a probe beam for measuring cavity mode shapes in case of CMWS and CMDS methods. The AOM is used both to prevent pumping the cavity with carrier frequency and other EOM sidebands, as well as to initiate ring-down decays in the CRDS. The experimental conditions are chosen so that at any given moment, only one cavity mode was excited. The OFC, EOM and AOM are frequency referenced to a primary atomic standard. The comb of cavity modes is actively stabilized to the frequency νC of laser 2. (b) Allan deviation of measured mode positions of empty cavity in frequency and absorption units (n – number of measurements). Time interval between measurements was 3 ms. The plot minimum corresponds to detection limit of 5×10−11 cm−1. (c) High-speed measurement procedure of dispersive spectrum. Each spectrum scan is a series of equidistant in time processes of cavity pumping corresponding to various EOM radiofrequencies νRF grouped around consecutive cavity mode centers. A gray decay shows the process of cavity emptying from the light for previous radiofrequency νRF which starts just after the EOM frequency change.
Fig. 2.
Fig. 2. Absorption and dispersion cavity-enhanced spectroscopy. The shown R23 transition in the second overtone of CO was measured at the room temperature and indicated pressures by three cavity-enhanced spectroscopy methods: CRDS, CMWS and CMDS. (a) Top: simulation of cavity transmission in direct cavity-enhanced absorption spectroscopy (CEAS). Middle: absorption spectra measured by CRDS and CMWS. For clarity, the CRDS data were moved up slightly. Bottom: dispersion spectra measured by CMDS. Every spectrum in the pressure range 0.1-2 kPa is the average of 10 scans. Spectra for pressures 13 kPa and 54 kPa are the average of 20 scans. (b) Upper: comparison of CRDS and CMWS residuals obtained from the single-spectrum fit analysis. Lower: comparison of CMDS and CMWS residuals obtained from the multi-spectrum fit analysis. Standard deviation of CMDS low-pressure residuals corresponds to absorption of 5×10 10 cm−1. The Hartmann-Tran profile with collisional line mixing was used to model spectra for all investigated methods. In the single-spectrum analysis, spectra were fitted individually for every pressure, whereas in the multi-spectrum analysis all spectra were fitted together with forced linear pressure dependence of chosen line-shape parameters. CRDS results are limited to low pressures. Above the pressure of 2 kPa, ring-downs are too short for accurate measurement, which leads to the large structure in residuals from the fit. CMWS and CMDS spectra expose the wide dynamic range of absorption and dispersion measurements, respectively. The small instrumental asymmetry affecting CMWS spectra, well masked in the case of the single-spectrum analysis, can be detected by the multi-spectrum fit technique. Among the three studied methods, CMDS represents the highest standard in providing ultra-accurate laboratory spectra. For quantitative comparison of CMWS and CMDS results, the quality of the fit factors (QF) from the multi-spectrum fit analysis are given. Horizontal axes and pressures are common for each column of plots (a) and (b).
Fig. 3.
Fig. 3. Line intensity of R23 CO transition. Line intensities obtained from CMWS and CMDS spectra are shown. Full circles and diamonds: Intensities provided by the multi-spectrum analysis with use of the recommended Hartmann-Tran profile with collisional line mixing. The results for CMWS and CMDS agree up to 0.04% for low pressures and systematically disagree by 0.2% to 0.8% above pressures of 2 kPa, due to instrumental errors affecting the CMWS method. CMDS shows an excellent constancy of the line intensity with pressure. Open circles and diamonds: Intensities provided by the single spectrum analysis with the use of the ordinary Voigt profile. The results present strong nonphysical dependence on pressure and inaccuracies of up to 3% caused by use of a too-simplified line-shape model. Plotted intensities are normalized to the mean value with the lowest uncertainty obtained in CMDS. Error bars on graph correspond to combined standard uncertainties. The uncertainty budget of the line intensity, including type A (statistical) and type B (other) components, achieved from the multi-spectrum analysis of CMDS spectra is shown.
Fig. 4.
Fig. 4. Line position and collisional shift of R23 CO transition. Unperturbed line positions and shifts obtained from CMDS, CMWS and CRDS spectra are shown for various methods of data analysis employed to two ranges of pressures. In the case of the single spectrum analysis (triangles), the results were determined from the linear regression. In the first multi-spectrum analysis (squares), one value of the line position and pressure shift coefficient was fitted for all pressures. In the second multi-spectrum analysis (diamonds), the pressure shift coefficient was constrained to the best value determined from the first high-pressure range multi-spectrum analysis of CMDS spectra. Experimental spectra were fitted by the Hartman-Tran profile. The results for CMDS agree within their standard fit uncertainties with each other for all pressures. The results for CMWS are scattered due to the systematic errors of this method. CRDS results are limited to low pressures and agree with CMWS low-pressure results. Correlations between line positions and line shifts occur at low pressures for all investigated methods, but CMDS shows the greatest resistance to it. Error bars on graph correspond to combined standard uncertainties. The uncertainty budget of the line position and collisional shift, including type A (statistical) and type B (other) components, achieved from the multi-spectrum analysis of CMDS spectra is shown.

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