Abstract

We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency-shifting loop seeded with a continuous-wave (CW) monochromatic laser. The comb lines are generated by successive passes of the CW laser through an acousto-optic frequency shifter. We report the generation of frequency combs with more than 1500 mutually coherent lines, without resorting to non-linear broadening phenomena or external electronic modulation. The comb line spacing is easily reconfigurable from tens of MHz down to the kHz region. We first use a single acousto-optic frequency comb to conduct self-heterodyne interferometry with a high frequency resolution (500 kHz). By increasing the line spacing to 80 MHz, we demonstrate molecular spectroscopy on the sub-millisecond time scale. In order to reduce the detection bandwidth, we subsequently implement an acousto-optic dual-comb spectrometer with the aid of two mutually coherent frequency shifting loops. In each architecture, the potentiality of acousto-optic frequency combs for spectroscopy is validated by spectral measurements of hydrogen cyanide in the near-infrared region.

© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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References

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    [Crossref]
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    [Crossref]

2018 (4)

2017 (6)

2016 (10)

P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
[Crossref]

M.-G. Suh, Q.-F. Yang, K. Y. Yang, X. Yi, and K. J. Vahala, “Microresonator soliton dual-comb spectroscopy,” Science 354(6312), 600–603 (2016).
[Crossref] [PubMed]

A. J. Fleisher, D. A. Long, Z. D. Reed, J. T. Hodges, and D. F. Plusquellic, “Coherent cavity-enhanced dual-comb spectroscopy,” Opt. Express 24(10), 10424–10434 (2016).
[Crossref] [PubMed]

V. Durán, P. A. Andrekson, and V. Torres-Company, “Electro-optic dual-comb interferometry over 40 nm bandwidth,” Opt. Lett. 41(18), 4190–4193 (2016).
[Crossref] [PubMed]

G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
[Crossref]

B. Jerez, P. Martín-Mateos, E. Prior, C. de Dios, and P. Acedo, “Gain-switching injection-locked dual optical frequency combs: characterization and optimization,” Opt. Lett. 41(18), 4293–4296 (2016).
[Crossref] [PubMed]

B. Jerez, P. Martín-Mateos, E. Prior, C. de Dios, and P. Acedo, “Dual optical frequency comb architecture with capabilities from visible to mid-infrared,” Opt. Express 24(13), 14986–14994 (2016).
[Crossref] [PubMed]

N. B. Hébert, V. Michaud-Belleau, C. Perella, G-W. Truog, J. D. Anstie, T. M. Stace, J. Genest, and A. N. Luiteu, “Real-Time Dynamic Atomic Spectroscopy Using Electro-Optic Frequency Combs,” Phys. Rev. Appl. 6(4), 044012 (2016).
[Crossref]

H. Guillet de Chatellus, L. R. Cortés, and J. Azaña, “Optical real-time Fourier transformation with kilohertz resolutions,” Optica 3(1), 1–7 (2016).
[Crossref]

I. Coddington, N. R. Newbury, and W. C. Swann, “Dual-comb spectroscopy,” Optica 3(4), 414–426 (2016).
[Crossref]

2015 (4)

2014 (4)

2013 (4)

2011 (2)

2009 (2)

F. Ferdous, D. E. Leaird, C.-B. Huang, and A. M. Weiner, “Dual-comb electric-field cross-correlation technique for optical arbitrary waveform characterization,” Opt. Lett. 34(24), 3875–3877 (2009).
[Crossref] [PubMed]

I. Coddington, W. C. Swann, L. Nenadovic, and N. R. Newbury, “Rapid and precise absolute distance measurements at long range,” Nat. Photonics 3(6), 351–356 (2009).
[Crossref]

2008 (3)

C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
[Crossref] [PubMed]

I. Coddington, W. C. Swann, and N. R. Newbury, “Coherent multiheterodyne spectroscopy using stabilized optical frequency combs,” Phys. Rev. Lett. 100(1), 013902 (2008).
[Crossref] [PubMed]

E. J. Moyer, D. S. Sayres, G. S. Engel, J. M. St Clair, F. N. Keutsch, N. T. Allen, J. H. Kroll, and J. G. Anderson, “Design considerations in high-sensitivity off-axis integrated cavity output spectroscopy,” Appl. Phys. B 92, 467–474 (2008).
[Crossref]

2006 (1)

2002 (1)

T. Udem, R. Holzwarth, and T. W. Hänsch, “Optical frequency metrology,” Nature 416(6877), 233–237 (2002).
[Crossref] [PubMed]

2000 (1)

D. J. Jones, S. A. Diddams, J. K. Ranka, A. Stentz, R. S. Windeler, J. L. Hall, and S. T. Cundiff, “Carrier-Envelope Phase Control of Femtosecond Mode-Locked Lasers and Direct Optical Frequency Synthesis,” Science 288(5466), 635–640 (2000).
[Crossref] [PubMed]

Abe, M.

Acedo, P.

Allen, N. T.

E. J. Moyer, D. S. Sayres, G. S. Engel, J. M. St Clair, F. N. Keutsch, N. T. Allen, J. H. Kroll, and J. G. Anderson, “Design considerations in high-sensitivity off-axis integrated cavity output spectroscopy,” Appl. Phys. B 92, 467–474 (2008).
[Crossref]

Anderson, J. G.

E. J. Moyer, D. S. Sayres, G. S. Engel, J. M. St Clair, F. N. Keutsch, N. T. Allen, J. H. Kroll, and J. G. Anderson, “Design considerations in high-sensitivity off-axis integrated cavity output spectroscopy,” Appl. Phys. B 92, 467–474 (2008).
[Crossref]

Anderson, M. H.

P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
[Crossref] [PubMed]

Andrekson, P. A.

Anstie, J. D.

N. B. Hébert, V. Michaud-Belleau, C. Perella, G-W. Truog, J. D. Anstie, T. M. Stace, J. Genest, and A. N. Luiteu, “Real-Time Dynamic Atomic Spectroscopy Using Electro-Optic Frequency Combs,” Phys. Rev. Appl. 6(4), 044012 (2016).
[Crossref]

N. B. Hébert, V. Michaud-Belleau, J. D. Anstie, J.-D. Deschênes, A. N. Luiten, and J. Genest, “Self-heterodyne interference spectroscopy using a comb generated by pseudo-random modulation,” Opt. Express 23(21), 27806–27818 (2015).
[Crossref] [PubMed]

Azaña, J.

Beha, K.

K. Beha, D. C. Cole, P. Del’Haye, A. Coillet, S. A. Diddams, and S. B. Papp, “Electronic synthesis of light,” Optica 4(4), 406–411 (2017).
[Crossref]

P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
[Crossref]

Bendahmane, A.

G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
[Crossref]

Benedick, A. J.

C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
[Crossref] [PubMed]

Bernhardt, B.

T. Ideguchi, S. Holzner, B. Bernhardt, G. Guelachvili, N. Picqué, and T. W. Hänsch, “Coherent Raman spectro-imaging with laser frequency combs,” Nature 502(7471), 355–358 (2013).
[Crossref] [PubMed]

Bielska, K.

Bosse, H.

Boudreau, S.

Brasch, V.

P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
[Crossref] [PubMed]

Chi, N.

Coddington, I.

I. Coddington, N. R. Newbury, and W. C. Swann, “Dual-comb spectroscopy,” Optica 3(4), 414–426 (2016).
[Crossref]

I. Coddington, W. C. Swann, L. Nenadovic, and N. R. Newbury, “Rapid and precise absolute distance measurements at long range,” Nat. Photonics 3(6), 351–356 (2009).
[Crossref]

I. Coddington, W. C. Swann, and N. R. Newbury, “Coherent multiheterodyne spectroscopy using stabilized optical frequency combs,” Phys. Rev. Lett. 100(1), 013902 (2008).
[Crossref] [PubMed]

Coillet, A.

K. Beha, D. C. Cole, P. Del’Haye, A. Coillet, S. A. Diddams, and S. B. Papp, “Electronic synthesis of light,” Optica 4(4), 406–411 (2017).
[Crossref]

P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
[Crossref]

Cole, D. C.

K. Beha, D. C. Cole, P. Del’Haye, A. Coillet, S. A. Diddams, and S. B. Papp, “Electronic synthesis of light,” Optica 4(4), 406–411 (2017).
[Crossref]

P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
[Crossref]

Cortés, L. R.

Cundiff, S. T.

D. J. Jones, S. A. Diddams, J. K. Ranka, A. Stentz, R. S. Windeler, J. L. Hall, and S. T. Cundiff, “Carrier-Envelope Phase Control of Femtosecond Mode-Locked Lasers and Direct Optical Frequency Synthesis,” Science 288(5466), 635–640 (2000).
[Crossref] [PubMed]

de Dios, C.

Del’Haye, P.

K. Beha, D. C. Cole, P. Del’Haye, A. Coillet, S. A. Diddams, and S. B. Papp, “Electronic synthesis of light,” Optica 4(4), 406–411 (2017).
[Crossref]

P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
[Crossref]

Deschênes, J.-D.

Diddams, S. A.

K. Beha, D. C. Cole, P. Del’Haye, A. Coillet, S. A. Diddams, and S. B. Papp, “Electronic synthesis of light,” Optica 4(4), 406–411 (2017).
[Crossref]

P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
[Crossref]

T. J. Kippenberg, R. Holzwarth, and S. A. Diddams, “Microresonator-Based Optical Frequency Combs,” Science 332(6029), 555–559 (2011).
[Crossref] [PubMed]

D. J. Jones, S. A. Diddams, J. K. Ranka, A. Stentz, R. S. Windeler, J. L. Hall, and S. T. Cundiff, “Carrier-Envelope Phase Control of Femtosecond Mode-Locked Lasers and Direct Optical Frequency Synthesis,” Science 288(5466), 635–640 (2000).
[Crossref] [PubMed]

Dong, Z.

Douglass, K. O.

Durán, V.

Eliyahu, D.

W. Liang, D. Eliyahu, V. S. Ilchenko, A. A. Savchenkov, A. B. Matsko, D. Seidel, and L. Maleki, “High spectral purity Kerr frequency comb radio frequency photonic oscillator,” Nat. Commun. 6(1), 7957 (2015).
[Crossref] [PubMed]

Engel, G. S.

E. J. Moyer, D. S. Sayres, G. S. Engel, J. M. St Clair, F. N. Keutsch, N. T. Allen, J. H. Kroll, and J. G. Anderson, “Design considerations in high-sensitivity off-axis integrated cavity output spectroscopy,” Appl. Phys. B 92, 467–474 (2008).
[Crossref]

Eriksson, T. A.

Fan, X.

Fendel, P.

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Fleisher, A. J.

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Glastre, W.

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G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
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T. Udem, R. Holzwarth, and T. W. Hänsch, “Optical frequency metrology,” Nature 416(6877), 233–237 (2002).
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G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
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C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
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W. Liang, D. Eliyahu, V. S. Ilchenko, A. A. Savchenkov, A. B. Matsko, D. Seidel, and L. Maleki, “High spectral purity Kerr frequency comb radio frequency photonic oscillator,” Nat. Commun. 6(1), 7957 (2015).
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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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Martín-Mateos, P.

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W. Liang, D. Eliyahu, V. S. Ilchenko, A. A. Savchenkov, A. B. Matsko, D. Seidel, and L. Maleki, “High spectral purity Kerr frequency comb radio frequency photonic oscillator,” Nat. Commun. 6(1), 7957 (2015).
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N. B. Hébert, V. Michaud-Belleau, J. D. Anstie, J.-D. Deschênes, A. N. Luiten, and J. Genest, “Self-heterodyne interference spectroscopy using a comb generated by pseudo-random modulation,” Opt. Express 23(21), 27806–27818 (2015).
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G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
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Moyer, E. J.

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P. Del’Haye, A. Coillet, T. Fortier, K. Beha, D. C. Cole, K. Y. Yang, H. Lee, K. J. Vahala, S. B. Papp, and S. A. Diddams, “Phase-coherent microwave-to-optical link with a self-referenced microcomb,” Nat. Photonics 10(8), 516–520 (2016).
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N. B. Hébert, V. Michaud-Belleau, C. Perella, G-W. Truog, J. D. Anstie, T. M. Stace, J. Genest, and A. N. Luiteu, “Real-Time Dynamic Atomic Spectroscopy Using Electro-Optic Frequency Combs,” Phys. Rev. Appl. 6(4), 044012 (2016).
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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
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G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
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T. Ideguchi, S. Holzner, B. Bernhardt, G. Guelachvili, N. Picqué, and T. W. Hänsch, “Coherent Raman spectro-imaging with laser frequency combs,” Nature 502(7471), 355–358 (2013).
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G. Millot, S. Pitois, M. Yan, T. Hovannysyan, A. Bendahmane, T. W. Hänsch, and N. Picqué, “Frequency-agile dual-comb spectroscopy,” Nat. Photonics 10(1), 27–30 (2016).
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Rosenberger, R.

P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
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W. Liang, D. Eliyahu, V. S. Ilchenko, A. A. Savchenkov, A. B. Matsko, D. Seidel, and L. Maleki, “High spectral purity Kerr frequency comb radio frequency photonic oscillator,” Nat. Commun. 6(1), 7957 (2015).
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E. J. Moyer, D. S. Sayres, G. S. Engel, J. M. St Clair, F. N. Keutsch, N. T. Allen, J. H. Kroll, and J. G. Anderson, “Design considerations in high-sensitivity off-axis integrated cavity output spectroscopy,” Appl. Phys. B 92, 467–474 (2008).
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Seidel, D.

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St Clair, J. M.

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D. J. Jones, S. A. Diddams, J. K. Ranka, A. Stentz, R. S. Windeler, J. L. Hall, and S. T. Cundiff, “Carrier-Envelope Phase Control of Femtosecond Mode-Locked Lasers and Direct Optical Frequency Synthesis,” Science 288(5466), 635–640 (2000).
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I. Coddington, N. R. Newbury, and W. C. Swann, “Dual-comb spectroscopy,” Optica 3(4), 414–426 (2016).
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I. Coddington, W. C. Swann, L. Nenadovic, and N. R. Newbury, “Rapid and precise absolute distance measurements at long range,” Nat. Photonics 3(6), 351–356 (2009).
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I. Coddington, W. C. Swann, and N. R. Newbury, “Coherent multiheterodyne spectroscopy using stabilized optical frequency combs,” Phys. Rev. Lett. 100(1), 013902 (2008).
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C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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N. B. Hébert, V. Michaud-Belleau, C. Perella, G-W. Truog, J. D. Anstie, T. M. Stace, J. Genest, and A. N. Luiteu, “Real-Time Dynamic Atomic Spectroscopy Using Electro-Optic Frequency Combs,” Phys. Rev. Appl. 6(4), 044012 (2016).
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T. Udem, R. Holzwarth, and T. W. Hänsch, “Optical frequency metrology,” Nature 416(6877), 233–237 (2002).
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Vahala, K. J.

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P. Marin-Palomo, J. N. Kemal, M. Karpov, A. Kordts, J. Pfeifle, M. H. P. Pfeiffer, P. Trocha, S. Wolf, V. Brasch, M. H. Anderson, R. Rosenberger, K. Vijayan, W. Freude, T. J. Kippenberg, and C. Koos, “Microresonator-based solitons for massively parallel coherent optical communications,” Nature 546(7657), 274–279 (2017).
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C.-H. Li, A. J. Benedick, P. Fendel, A. G. Glenday, F. X. Kärtner, D. F. Phillips, D. Sasselov, A. Szentgyorgyi, and R. L. Walsworth, “A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s-1.,” Nature 452(7187), 610–612 (2008).
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Xu, B.

Xuan, Y.

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Yang, Q.-F.

M.-G. Suh, Q.-F. Yang, K. Y. Yang, X. Yi, and K. J. Vahala, “Microresonator soliton dual-comb spectroscopy,” Science 354(6312), 600–603 (2016).
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Yang, R.

Yi, X.

M.-G. Suh, Q.-F. Yang, K. Y. Yang, X. Yi, and K. J. Vahala, “Microresonator soliton dual-comb spectroscopy,” Science 354(6312), 600–603 (2016).
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Yu, J.

Zhang, J.

Zhang, X.

Zou, X.

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Figures (4)

Fig. 1
Fig. 1 (a) Sketch of the experimental setup used to generate and resolve the individual lines of an acousto-optic frequency comb by self-heterodyne interferometry. The inset shows a 1-µs fraction of a complete recorded trace. (b) RF spectrum obtained by self-heterodyning showing 1800 lines within 10 dB. The right inset is a zoom-in view of the central part of the spectrum, showing 100 lines separated from each other by 1 MHz.
Fig. 2
Fig. 2 Left. Dark blue: transmission spectrum of the Fabry-Pérot cavity (FSR = 1.6 GHz). Light blue: reference spectrum (no cavity inserted). The line spacing is 5 MHz. Center: Complex amplitude of a single transmission peak. The phase curve shows the expected π-jump. Right: Zoom-in view of the transmission peak (green area in the central plot) when the line spacing is reduced to 500 kHz.
Fig. 3
Fig. 3 (a) Sketch of the experimental setup used to perform self-heterodyne molecular spectroscopy of HCN. (b) Transmission and phase corresponding to the 11th line of the HCN P-branch. In the transmission curve, the red line is the Voigt profile that fits the experimental data (in blue) and the green squares plotted below are the corresponding residuals. In the phase plot, the red curve corresponds to the theoretical function derived from the Voigt profile.
Fig. 4
Fig. 4 (a) Sketch of the optical setup used to perform dual-comb spectroscopy. RFA: RF amplifier; LPF: low-pass filter. Lower inset: RF spectrum obtained by directly mixing the output of the two FSLs with and without the stabilization loop (blue and red spectra, respectively). A zoom-in view of a single line is also included. The PID regulator allows obtaining around 240 lines within 10 dB. (b) Transmission and phase corresponding to the 11th line of the HCN P-branch. In the transmission curve, the red line is the Voigt profile that fits the experimental data (in blue) and the green squares plotted below are the corresponding residuals. In the phase plot, the red curve corresponds to the theoretical function derived from the Voigt profile.

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