Abstract

Plasmonic nanoantennas and metamaterials concentrate optical energy into nanometric volumes strongly enhancing the light-matter interaction. This makes them promising platforms for optical sensing, nonlinear effects and quantum optics. However, absorption losses and radiative damping result in broad, low quality factor (Q) resonances of plasmonic systems that significantly limit their performance. Here, we develop a hybrid plasmonic/dielectric metasurface that can simultaneously achieve high Q and large field enhancement values in the near infrared by forming a hybridized mode between the nanoantennas’ plasmonic mode and the photonic waveguide mode of Si device layer. The tunability of the modes and quality factors of our platform allows us to study the effect of the geometric parameters on the optical properties of the metasurface. We demonstrate that the strongest near field enhancement and nonlinear signal generation can be achieved by balancing the high Q factors and in-coupling efficiency in hybrid resonators.

© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2017 (3)

F. Wang, A. B. F. Martinson, and H. Harutyunyan, “Efficient nonlinear metasurface based on non-planar plasmonic nanocavities,” ACS Photonics 4(5), 1188–1194 (2017).
[Crossref]

Y. Yin, Y. Chen, E. Saei Ghareh Naz, X. Lu, S. Li, V. Engemaier, L. Ma, and O. G. Schmidt, “Silver nanocap enabled conversion and tuning of hybrid photon-plasmon modes in microtubular cavities,” ACS Photonics 4(4), 736–740 (2017).
[Crossref]

T. Shibanuma, G. Grinblat, P. Albella, and S. A. Maier, “Efficient third harmonic generation from metal-dielectric hybrid nanoantennas,” Nano Lett. 17(4), 2647–2651 (2017).
[Crossref] [PubMed]

2016 (8)

M. Mesch, B. Metzger, M. Hentschel, and H. Giessen, “Nonlinear plasmonic sensing,” Nano Lett. 16(5), 3155–3159 (2016).
[Crossref] [PubMed]

H. M. Doeleman, E. Verhagen, and A. F. Koenderink, “Antenna-cavity hybrids: Matching polar opposites for Purcell enhancements at any linewidth,” ACS Photonics 3(10), 1943–1951 (2016).
[Crossref]

V. F. Gili, L. Carletti, A. Locatelli, D. Rocco, M. Finazzi, L. Ghirardini, I. Favero, C. Gomez, A. Lemaître, M. Celebrano, C. De Angelis, and G. Leo, “Monolithic AlGaAs second-harmonic nanoantennas,” Opt. Express 24(14), 15965–15971 (2016).
[Crossref] [PubMed]

W. Tong, C. Gong, X. Liu, S. Yuan, Q. Huang, J. Xia, and Y. Wang, “Enhanced third harmonic generation in a silicon metasurface using trapped mode,” Opt. Express 24(17), 19661–19670 (2016).
[Crossref] [PubMed]

S. D. Gennaro, M. Rahmani, V. Giannini, H. Aouani, T. P. H. Sidiropoulos, M. Navarro-Cía, S. A. Maier, and R. F. Oulton, “The Interplay of Symmetry and Scattering Phase in Second Harmonic Generation from Gold Nanoantennas,” Nano Lett. 16(8), 5278–5285 (2016).
[Crossref] [PubMed]

Y. Yang, B. Zhen, C. W. Hsu, O. D. Miller, J. D. Joannopoulos, and M. Soljačić, “Optically thin metallic films for high radiative-efficiency plasmonics,” Nano Lett. 16(7), 4110–4117 (2016).
[Crossref] [PubMed]

G. Grinblat, Y. Li, M. P. Nielsen, R. F. Oulton, and S. A. Maier, “Enhanced Third Harmonic Generation in Single Germanium Nanodisks Excited at the Anapole Mode,” Nano Lett. 16(7), 4635–4640 (2016).
[Crossref] [PubMed]

S. Liu, M. B. Sinclair, S. Saravi, G. A. Keeler, Y. Yang, J. Reno, G. M. Peake, F. Setzpfandt, I. Staude, T. Pertsch, and I. Brener, “Resonantly Enhanced Second-Harmonic Generation Using III-V Semiconductor All-Dielectric Metasurfaces,” Nano Lett. 16(9), 5426–5432 (2016).
[Crossref] [PubMed]

2015 (5)

Y. Yang, W. Wang, A. Boulesbaa, I. I. Kravchenko, D. P. Briggs, A. Puretzky, D. Geohegan, and J. Valentine, “Nonlinear fano-resonant dielectric metasurfaces,” Nano Lett. 15(11), 7388–7393 (2015).
[Crossref] [PubMed]

H. Harutyunyan, A. B. F. Martinson, D. Rosenmann, L. K. Khorashad, L. V. Besteiro, A. O. Govorov, and G. P. Wiederrecht, “Anomalous ultrafast dynamics of hot plasmonic electrons in nanostructures with hot spots,” Nat. Nanotechnol. 10(9), 770–774 (2015).
[Crossref] [PubMed]

M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
[Crossref] [PubMed]

M. Pelton, “Modified spontaneous emission in nanophotonic structures,” Nat. Photonics 9(7), 427–435 (2015).
[Crossref]

J. He, P. Ding, J. Wang, C. Fan, and E. Liang, “Ultra-narrow band perfect absorbers based on plasmonic analog of electromagnetically induced absorption,” Opt. Express 23(5), 6083–6091 (2015).
[Crossref] [PubMed]

2014 (8)

G. M. Akselrod, C. Argyropoulos, T. B. Hoang, C. Ciracì, C. Fang, J. Huang, D. R. Smith, and M. H. Mikkelsen, “Probing the mechanisms of large purcell enhancement in plasmonic nanoantennas,” Nat. Photonics 8(11), 835–840 (2014).
[Crossref]

Y. Zhan, D. Y. Lei, X. Li, and S. A. Maier, “Plasmonic fano resonances in nanohole quadrumers for ultra-sensitive refractive index sensing,” Nanoscale 6(9), 4705–4715 (2014).
[Crossref] [PubMed]

J. B. Lassiter, X. Chen, X. Liu, C. Ciraci, T. Hoang, S. Larouche, S.-H. Oh, M. H. Mikkelsen, and D. Smith, “Third-harmonic generation enhancement by film-coupled plasmonic stripe resonators,” ACS Photonics 1(11), 1212–1217 (2014).
[Crossref]

B. Metzger, M. Hentschel, T. Schumacher, M. Lippitz, X. Ye, C. B. Murray, B. Knabe, K. Buse, and H. Giessen, “Doubling the Efficiency of Third Harmonic Generation by Positioning ITO Nanocrystals into the Hot-Spot of Plasmonic Gap-Antennas,” Nano Lett. 14(5), 2867–2872 (2014).
[Crossref] [PubMed]

J. Lee, M. Tymchenko, C. Argyropoulos, P.-Y. Chen, F. Lu, F. Demmerle, G. Boehm, M.-C. Amann, A. Alù, and M. A. Belkin, “Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions,” Nature 511(7507), 65–69 (2014).
[Crossref] [PubMed]

A. Rose, T. B. Hoang, F. McGuire, J. J. Mock, C. Ciracì, D. R. Smith, and M. H. Mikkelsen, “Control of radiative processes using tunable plasmonic nanopatch antennas,” Nano Lett. 14(8), 4797–4802 (2014).
[Crossref] [PubMed]

H. Aouani, M. Rahmani, M. Navarro-Cía, and S. A. Maier, “Third-harmonic-upconversion enhancement from a single semiconductor nanoparticle coupled to a plasmonic antenna,” Nat. Nanotechnol. 9(4), 290–294 (2014).
[Crossref] [PubMed]

M. R. Shcherbakov, D. N. Neshev, B. Hopkins, A. S. Shorokhov, I. Staude, E. V. Melik-Gaykazyan, M. Decker, A. A. Ezhov, A. E. Miroshnichenko, I. Brener, A. A. Fedyanin, and Y. S. Kivshar, “Enhanced Third-Harmonic Generation in Silicon Nanoparticles Driven by Magnetic Response,” Nano Lett. 14(11), 6488–6492 (2014).
[Crossref] [PubMed]

2013 (3)

N. E. J. Omaghali, V. Tkachenko, A. Andreone, and G. Abbate, “Optical Sensing Using Dark Mode Excitation in an Asymmetric Dimer Metamaterial,” Sensors (Basel) 14(1), 272–282 (2013).
[Crossref] [PubMed]

P. Albella, M. A. Poyli, M. K. Schmidt, S. A. Maier, F. Moreno, J. J. Saenz, and J. Aizpurua, “Low-loss electric and magnetic field-enhanced spectroscopy with subwavelength silicon dimers,” J. Phys. Chem. C 117(26), 13573–13584 (2013).
[Crossref]

Y. Zhang, F. Wen, Y.-R. Zhen, P. Nordlander, and N. J. Halas, “Coherent fano resonances in a plasmonic nanocluster enhance optical four-wave mixing,” Proc. Natl. Acad. Sci. U.S.A. 110(23), 9215–9219 (2013).
[Crossref] [PubMed]

2012 (6)

H. Harutyunyan, G. Volpe, R. Quidant, and L. Novotny, “Enhancing the nonlinear optical response using multifrequency gold-nanowire antennas,” Phys. Rev. Lett. 108(21), 217403 (2012).
[Crossref] [PubMed]

M. Kauranen and A. V. Zayats, “Nonlinear plasmonics,” Nat. Photonics 6(11), 737–748 (2012).
[Crossref]

T. Hanke, J. Cesar, V. Knittel, A. Trügler, U. Hohenester, A. Leitenstorfer, and R. Bratschitsch, “Tailoring spatiotemporal light confinement in single plasmonic nanoantennas,” Nano Lett. 12(2), 992–996 (2012).
[Crossref] [PubMed]

F. Wang, A. Chakrabarty, F. Minkowski, K. Sun, and Q.-H. Wei, “Polarization conversion with elliptical patch nanoantennas,” Appl. Phys. Lett. 101(2), 023101 (2012).
[Crossref]

W. Ahn, S. V. Boriskina, Y. Hong, and B. M. Reinhard, “Photonic-plasmonic mode coupling in on-chip integrated optoplasmonic molecules,” ACS Nano 6(1), 951–960 (2012).
[Crossref] [PubMed]

Y.-F. Xiao, Y.-C. Liu, B.-B. Li, Y.-L. Chen, Y. Li, and Q. Gong, “Strongly enhanced light-matter interaction in a hybrid photonic-plasmonic resonator,” Phys. Rev. A 85(3), 031805 (2012).
[Crossref]

2011 (5)

M. Chamanzar and A. Adibi, “Hybrid nanoplasmonic-photonic resonators for efficient coupling of light to single plasmonic nanoresonators,” Opt. Express 19(22), 22292–22304 (2011).
[Crossref] [PubMed]

X. Yang, A. Ishikawa, X. Yin, and X. Zhang, “Hybrid photonic-plasmonic crystal nanocavities,” ACS Nano 5(4), 2831–2838 (2011).
[Crossref] [PubMed]

W. Cai, A. P. Vasudev, and M. L. Brongersma, “Electrically controlled nonlinear generation of light with plasmonics,” Science 333(6050), 1720–1723 (2011).
[Crossref] [PubMed]

L. Novotny and N. F. van Hulst, “Antennas for light,” Nat. Photonics 5(2), 83–90 (2011).
[Crossref]

N. Liu, M. L. Tang, M. Hentschel, H. Giessen, and A. P. Alivisatos, “Nanoantenna-enhanced gas sensing in a single tailored nanofocus,” Nat. Mater. 10(8), 631–636 (2011).
[Crossref] [PubMed]

2010 (7)

N. Liu, M. Mesch, T. Weiss, M. Hentschel, and H. Giessen, “Infrared perfect absorber and its application as plasmonic sensor,” Nano Lett. 10(7), 2342–2348 (2010).
[Crossref] [PubMed]

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2009 (2)

2008 (1)

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2007 (1)

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2003 (1)

D. K. Armani, T. J. Kippenberg, S. M. Spillane, and K. J. Vahala, “Ultra-high-Q toroid microcavity on a chip,” Nature 421(6926), 925–928 (2003).
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J. Lee, M. Tymchenko, C. Argyropoulos, P.-Y. Chen, F. Lu, F. Demmerle, G. Boehm, M.-C. Amann, A. Alù, and M. A. Belkin, “Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions,” Nature 511(7507), 65–69 (2014).
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J. Lee, M. Tymchenko, C. Argyropoulos, P.-Y. Chen, F. Lu, F. Demmerle, G. Boehm, M.-C. Amann, A. Alù, and M. A. Belkin, “Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions,” Nature 511(7507), 65–69 (2014).
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R. Ameling and H. Giessen, “Cavity plasmonics: large normal mode splitting of electric and magnetic particle plasmons induced by a photonic microcavity,” Nano Lett. 10(11), 4394–4398 (2010).
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N. E. J. Omaghali, V. Tkachenko, A. Andreone, and G. Abbate, “Optical Sensing Using Dark Mode Excitation in an Asymmetric Dimer Metamaterial,” Sensors (Basel) 14(1), 272–282 (2013).
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P. Anger, P. Bharadwaj, and L. Novotny, “Enhancement and quenching of single-molecule fluorescence,” Phys. Rev. Lett. 96(11), 113002 (2006).
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G. M. Akselrod, C. Argyropoulos, T. B. Hoang, C. Ciracì, C. Fang, J. Huang, D. R. Smith, and M. H. Mikkelsen, “Probing the mechanisms of large purcell enhancement in plasmonic nanoantennas,” Nat. Photonics 8(11), 835–840 (2014).
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D. K. Armani, T. J. Kippenberg, S. M. Spillane, and K. J. Vahala, “Ultra-high-Q toroid microcavity on a chip,” Nature 421(6926), 925–928 (2003).
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Artar, A.

A. A. Yanik, M. Huang, O. Kamohara, A. Artar, T. W. Geisbert, J. H. Connor, and H. Altug, “An optofluidic nanoplasmonic biosensor for direct detection of live viruses from biological media,” Nano Lett. 10(12), 4962–4969 (2010).
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Bachelot, R.

Barnard, E. S.

J. A. Schuller, E. S. Barnard, W. Cai, Y. C. Jun, J. S. White, and M. L. Brongersma, “Plasmonics for extreme light concentration and manipulation,” Nat. Mater. 9(3), 193–204 (2010).
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M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Belkin, M. A.

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H. Harutyunyan, A. B. F. Martinson, D. Rosenmann, L. K. Khorashad, L. V. Besteiro, A. O. Govorov, and G. P. Wiederrecht, “Anomalous ultrafast dynamics of hot plasmonic electrons in nanostructures with hot spots,” Nat. Nanotechnol. 10(9), 770–774 (2015).
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Bharadwaj, P.

P. Anger, P. Bharadwaj, and L. Novotny, “Enhancement and quenching of single-molecule fluorescence,” Phys. Rev. Lett. 96(11), 113002 (2006).
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Biagioni, P.

M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Boehm, G.

J. Lee, M. Tymchenko, C. Argyropoulos, P.-Y. Chen, F. Lu, F. Demmerle, G. Boehm, M.-C. Amann, A. Alù, and M. A. Belkin, “Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions,” Nature 511(7507), 65–69 (2014).
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Boriskina, S. V.

W. Ahn, S. V. Boriskina, Y. Hong, and B. M. Reinhard, “Photonic-plasmonic mode coupling in on-chip integrated optoplasmonic molecules,” ACS Nano 6(1), 951–960 (2012).
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Y. Yang, W. Wang, A. Boulesbaa, I. I. Kravchenko, D. P. Briggs, A. Puretzky, D. Geohegan, and J. Valentine, “Nonlinear fano-resonant dielectric metasurfaces,” Nano Lett. 15(11), 7388–7393 (2015).
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T. Hanke, J. Cesar, V. Knittel, A. Trügler, U. Hohenester, A. Leitenstorfer, and R. Bratschitsch, “Tailoring spatiotemporal light confinement in single plasmonic nanoantennas,” Nano Lett. 12(2), 992–996 (2012).
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Brener, I.

S. Liu, M. B. Sinclair, S. Saravi, G. A. Keeler, Y. Yang, J. Reno, G. M. Peake, F. Setzpfandt, I. Staude, T. Pertsch, and I. Brener, “Resonantly Enhanced Second-Harmonic Generation Using III-V Semiconductor All-Dielectric Metasurfaces,” Nano Lett. 16(9), 5426–5432 (2016).
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Briggs, D. P.

Y. Yang, W. Wang, A. Boulesbaa, I. I. Kravchenko, D. P. Briggs, A. Puretzky, D. Geohegan, and J. Valentine, “Nonlinear fano-resonant dielectric metasurfaces,” Nano Lett. 15(11), 7388–7393 (2015).
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Brongersma, M. L.

W. Cai, A. P. Vasudev, and M. L. Brongersma, “Electrically controlled nonlinear generation of light with plasmonics,” Science 333(6050), 1720–1723 (2011).
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B. Metzger, M. Hentschel, T. Schumacher, M. Lippitz, X. Ye, C. B. Murray, B. Knabe, K. Buse, and H. Giessen, “Doubling the Efficiency of Third Harmonic Generation by Positioning ITO Nanocrystals into the Hot-Spot of Plasmonic Gap-Antennas,” Nano Lett. 14(5), 2867–2872 (2014).
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W. Cai, A. P. Vasudev, and M. L. Brongersma, “Electrically controlled nonlinear generation of light with plasmonics,” Science 333(6050), 1720–1723 (2011).
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J. A. Schuller, E. S. Barnard, W. Cai, Y. C. Jun, J. S. White, and M. L. Brongersma, “Plasmonics for extreme light concentration and manipulation,” Nat. Mater. 9(3), 193–204 (2010).
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Carletti, L.

Celebrano, M.

V. F. Gili, L. Carletti, A. Locatelli, D. Rocco, M. Finazzi, L. Ghirardini, I. Favero, C. Gomez, A. Lemaître, M. Celebrano, C. De Angelis, and G. Leo, “Monolithic AlGaAs second-harmonic nanoantennas,” Opt. Express 24(14), 15965–15971 (2016).
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M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Cerullo, G.

M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Cesar, J.

T. Hanke, J. Cesar, V. Knittel, A. Trügler, U. Hohenester, A. Leitenstorfer, and R. Bratschitsch, “Tailoring spatiotemporal light confinement in single plasmonic nanoantennas,” Nano Lett. 12(2), 992–996 (2012).
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Chen, P.-Y.

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J. B. Lassiter, X. Chen, X. Liu, C. Ciraci, T. Hoang, S. Larouche, S.-H. Oh, M. H. Mikkelsen, and D. Smith, “Third-harmonic generation enhancement by film-coupled plasmonic stripe resonators,” ACS Photonics 1(11), 1212–1217 (2014).
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Y. Yin, Y. Chen, E. Saei Ghareh Naz, X. Lu, S. Li, V. Engemaier, L. Ma, and O. G. Schmidt, “Silver nanocap enabled conversion and tuning of hybrid photon-plasmon modes in microtubular cavities,” ACS Photonics 4(4), 736–740 (2017).
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B. Luk’yanchuk, N. I. Zheludev, S. A. Maier, N. J. Halas, P. Nordlander, H. Giessen, and C. T. Chong, “The Fano resonance in plasmonic nanostructures and metamaterials,” Nat. Mater. 9(9), 707–715 (2010).
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P. B. Johnson and R. W. Christy, “Optical constants of the noble metals,” Phys. Rev. B 6(12), 4370–4379 (1972).
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Ciccacci, F.

M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Ciraci, C.

J. B. Lassiter, X. Chen, X. Liu, C. Ciraci, T. Hoang, S. Larouche, S.-H. Oh, M. H. Mikkelsen, and D. Smith, “Third-harmonic generation enhancement by film-coupled plasmonic stripe resonators,” ACS Photonics 1(11), 1212–1217 (2014).
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G. M. Akselrod, C. Argyropoulos, T. B. Hoang, C. Ciracì, C. Fang, J. Huang, D. R. Smith, and M. H. Mikkelsen, “Probing the mechanisms of large purcell enhancement in plasmonic nanoantennas,” Nat. Photonics 8(11), 835–840 (2014).
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A. A. Yanik, M. Huang, O. Kamohara, A. Artar, T. W. Geisbert, J. H. Connor, and H. Altug, “An optofluidic nanoplasmonic biosensor for direct detection of live viruses from biological media,” Nano Lett. 10(12), 4962–4969 (2010).
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Dai, D.

De Angelis, C.

V. F. Gili, L. Carletti, A. Locatelli, D. Rocco, M. Finazzi, L. Ghirardini, I. Favero, C. Gomez, A. Lemaître, M. Celebrano, C. De Angelis, and G. Leo, “Monolithic AlGaAs second-harmonic nanoantennas,” Opt. Express 24(14), 15965–15971 (2016).
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M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Demmerle, F.

J. Lee, M. Tymchenko, C. Argyropoulos, P.-Y. Chen, F. Lu, F. Demmerle, G. Boehm, M.-C. Amann, A. Alù, and M. A. Belkin, “Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions,” Nature 511(7507), 65–69 (2014).
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Ding, W.

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Y. Yin, Y. Chen, E. Saei Ghareh Naz, X. Lu, S. Li, V. Engemaier, L. Ma, and O. G. Schmidt, “Silver nanocap enabled conversion and tuning of hybrid photon-plasmon modes in microtubular cavities,” ACS Photonics 4(4), 736–740 (2017).
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Ezhov, A. A.

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Fang, C.

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Favero, I.

Fedyanin, A. A.

M. R. Shcherbakov, D. N. Neshev, B. Hopkins, A. S. Shorokhov, I. Staude, E. V. Melik-Gaykazyan, M. Decker, A. A. Ezhov, A. E. Miroshnichenko, I. Brener, A. A. Fedyanin, and Y. S. Kivshar, “Enhanced Third-Harmonic Generation in Silicon Nanoparticles Driven by Magnetic Response,” Nano Lett. 14(11), 6488–6492 (2014).
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M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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M. Kuttge, F. J. García de Abajo, and A. Polman, “Ultrasmall mode volume plasmonic nanodisk resonators,” Nano Lett. 10(5), 1537–1541 (2010).
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Geisbert, T. W.

A. A. Yanik, M. Huang, O. Kamohara, A. Artar, T. W. Geisbert, J. H. Connor, and H. Altug, “An optofluidic nanoplasmonic biosensor for direct detection of live viruses from biological media,” Nano Lett. 10(12), 4962–4969 (2010).
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S. D. Gennaro, M. Rahmani, V. Giannini, H. Aouani, T. P. H. Sidiropoulos, M. Navarro-Cía, S. A. Maier, and R. F. Oulton, “The Interplay of Symmetry and Scattering Phase in Second Harmonic Generation from Gold Nanoantennas,” Nano Lett. 16(8), 5278–5285 (2016).
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Y. Zhang, F. Wen, Y.-R. Zhen, P. Nordlander, and N. J. Halas, “Coherent fano resonances in a plasmonic nanocluster enhance optical four-wave mixing,” Proc. Natl. Acad. Sci. U.S.A. 110(23), 9215–9219 (2013).
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Y. Zhang, F. Wen, Y.-R. Zhen, P. Nordlander, and N. J. Halas, “Coherent fano resonances in a plasmonic nanocluster enhance optical four-wave mixing,” Proc. Natl. Acad. Sci. U.S.A. 110(23), 9215–9219 (2013).
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Nanoscale (1)

Y. Zhan, D. Y. Lei, X. Li, and S. A. Maier, “Plasmonic fano resonances in nanohole quadrumers for ultra-sensitive refractive index sensing,” Nanoscale 6(9), 4705–4715 (2014).
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Nat. Mater. (3)

J. A. Schuller, E. S. Barnard, W. Cai, Y. C. Jun, J. S. White, and M. L. Brongersma, “Plasmonics for extreme light concentration and manipulation,” Nat. Mater. 9(3), 193–204 (2010).
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N. Liu, M. L. Tang, M. Hentschel, H. Giessen, and A. P. Alivisatos, “Nanoantenna-enhanced gas sensing in a single tailored nanofocus,” Nat. Mater. 10(8), 631–636 (2011).
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B. Luk’yanchuk, N. I. Zheludev, S. A. Maier, N. J. Halas, P. Nordlander, H. Giessen, and C. T. Chong, “The Fano resonance in plasmonic nanostructures and metamaterials,” Nat. Mater. 9(9), 707–715 (2010).
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H. Harutyunyan, A. B. F. Martinson, D. Rosenmann, L. K. Khorashad, L. V. Besteiro, A. O. Govorov, and G. P. Wiederrecht, “Anomalous ultrafast dynamics of hot plasmonic electrons in nanostructures with hot spots,” Nat. Nanotechnol. 10(9), 770–774 (2015).
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H. Aouani, M. Rahmani, M. Navarro-Cía, and S. A. Maier, “Third-harmonic-upconversion enhancement from a single semiconductor nanoparticle coupled to a plasmonic antenna,” Nat. Nanotechnol. 9(4), 290–294 (2014).
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M. Celebrano, X. Wu, M. Baselli, S. Großmann, P. Biagioni, A. Locatelli, C. De Angelis, G. Cerullo, R. Osellame, B. Hecht, L. Duò, F. Ciccacci, and M. Finazzi, “Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation,” Nat. Nanotechnol. 10(5), 412–417 (2015).
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Nat. Photonics (6)

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M. Kauranen and A. V. Zayats, “Nonlinear plasmonics,” Nat. Photonics 6(11), 737–748 (2012).
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Opt. Express (6)

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Y.-F. Xiao, Y.-C. Liu, B.-B. Li, Y.-L. Chen, Y. Li, and Q. Gong, “Strongly enhanced light-matter interaction in a hybrid photonic-plasmonic resonator,” Phys. Rev. A 85(3), 031805 (2012).
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Y. Zhang, F. Wen, Y.-R. Zhen, P. Nordlander, and N. J. Halas, “Coherent fano resonances in a plasmonic nanocluster enhance optical four-wave mixing,” Proc. Natl. Acad. Sci. U.S.A. 110(23), 9215–9219 (2013).
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Figures (4)

Fig. 1
Fig. 1 a) Schematic of one unit of the hybrid plasmonic/dielectric nanoantenna array; b) A representative SEM picture of the developed nanoantennas sample; c) Local E-field distribution at the resonant wavelength (1390 nm) of the antenna (Px = 540 nm, g = 60 nm); d) Local H-field at the resonant wavelength (1390 nm) of the antenna (Px = 540 nm, g = 60 nm); e) and f) are local electric field enhancement profiles along z-direction at the outer edge of the Au antenna for dimers on SOI wafer and Si wafer respectively. The inset in f) shows the wavelength-dependent local field enhancement for antennas on SOI and Si wafer respectively.
Fig. 2
Fig. 2 a) and b) show the measured and simulated reflection spectrum for hybrid antennas with fixed ~60 nm gap width but varying x-periodicity; c) The simulated local H field enhancement spectra for hybrid antennas with fixed ~60 nm gap width but varying x-periodicity; d) and e) are the measured and simulated reflection spectrum for hybrid antennas with fixed x-period of 520 nm but varying gap width g; f) The simulated local H-field enhancement spectra for hybrid antennas with fixed x-period 520 nm but varying gap width g. The reflection spectra are offset for clarity.
Fig. 3
Fig. 3 a) reference THG spectrum obtained by pumping 30 nm Au film on top of 10 nm SiO2 film on Si wafer; b) The largest measured THG signals for different periods but fixed dimer gap width 60 nm. Each THG spectrum represents the strongest observed signal for the given periodicity sample. c) Measured THG at different excitation wavelengths for the hybrid plasmonic/dielectric nano-resonator (60 nm gap, 540 nm period) around its resonant wavelength; inset the reflection spectra for the sample of Px = 540 nm /g = 60 nm (blue curve) and the sample of Px = 520 nm /g = 22 nm (red curve); d) Measured THG of the hybrid plasmonic/dielectric nano-resonator for Px = 520 nm /g = 22 nm around its resonant wavelength.
Fig. 4
Fig. 4 a) The measured (dotted curve) and simulated (solid curve) reflection spectrum for bare SOI wafer; b) Electric field distribution inside the Si device layer and the SiO2 BOX layer of the bare SOI wafer; c) Ex field distribution of the coupled plasmonic-TM0 waveguide mode; Calculated power radiation directivity for the sample of Px = 560 nm period and g = 60 nm dimer gap with d) 3000 nm SiO2 BOX layer and e) total glass substrate substituting for 3000 nm SiO2 BOX layer.

Tables (1)

Tables Icon

Table 1 Fitted Q factors for the experimentally measured and numerically simulated reflection spectra in Figs. 2(a) and 2(b) (samples with fixed dimer gap g = 60 nm but varying x-periodicities). Q stands for Q factor and E stands for the local field enhancement inside the SiO2 cladding layer.

Equations (1)

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R=a+b·× ( q 0 γ 0 2 +f f 0 ) 2 ( γ 0 2 ) 2 + ( f f 0 ) 2 × i=1 n ( γ i 2 ) 2 ( γ i 2 ) 2 + ( f f i ) 2

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