Abstract

Colloidal quantum dots which can emit red, green, and blue colors are incorporated with a micro-LED array to demonstrate a feasible choice for future display technology. The pitch of the micro-LED array is 40μm, which is sufficient for high-resolution screen applications. The method that was used to spray the quantum dots in such tight space is called Aerosol Jet technology which uses atomizer and gas flow control to obtain uniform and controlled narrow spots. The ultra-violet LEDs are used in the array to excite the red, green and blue quantum dots on the top surface. To increase the utilization of the UV photons, a layer of distributed Bragg reflector was laid down on the device to reflect most of the leaked UV photons back to the quantum dot layers. With this mechanism, the enhanced luminous flux is 194% (blue), 173% (green) and 183% (red) more than that of the samples without the reflector. The luminous efficacy of radiation (LER) was measured under various currents and a value of 165 lm/Watt was recorded.

© 2015 Optical Society of America

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2015 (3)

Y. Yang, Y. Zheng, W. Cao, A. Titov, J. Hyvonen, R. Manders Jesse, J. Xue, P. H. Holloway, and L. Qian, “High-efficiency light-emitting devices based on quantum dots with tailored nanostructures,” Nat. Photonics 9, 259–266 (2015).

J. G. Tait, E. Witkowska, M. Hirade, T.-H. Ke, P. E. Malinowski, S. Steudel, C. Adachi, and P. Heremans, “Uniform Aerosol Jet printed polymer lines with 30 μm width for 140 ppi resolution RGB organic light emitting diodes,” Org. Electron. 22, 40–43 (2015).
[Crossref]

T. Seifert, E. Sowade, F. Roscher, M. Wiemer, T. Gessner, and R. R. Baumann, “Additive Manufacturing Technologies Compared: Morphology of Deposits of Silver Ink Using Inkjet and Aerosol Jet Printing,” Ind. Eng. Chem. Res. 54(2), 769–779 (2015).
[Crossref]

2014 (6)

R. Aga, C. Jordan, R. S. Aga, C. M. Bartsch, and E. M. Heckman, “Metal Electrode Work Function Modification Using Aerosol Jet Printing,” IEEE Electron Dev. Lett. 35(11), 1124–1126 (2014).
[Crossref]

H.-V. Han, C.-C. Lin, Y.-L. Tsai, H.-C. Chen, K.-J. Chen, Y.-L. Yeh, W.-Y. Lin, H.-C. Kuo, and P. Yu, “A Highly Efficient Hybrid GaAs Solar Cell Based on Colloidal-Quantum-Dot-Sensitization,” Sci. Rep. 4, 5734 (2014).
[PubMed]

W. Tang, L. Feng, C. Jiang, G. Yao, J. Zhao, Q. Cui, and X. Guo, “Controlling the surface wettability of the polymer dielectric for improved resolution of inkjet-printed electrodes and patterned channel regions in low-voltage solution-processed organic thin film transistors,” J. Mater. Chem. C Mater. Opt. Electron. Devices 2(28), 5553–5558 (2014).
[Crossref]

S. Ma, L. Liu, V. Bromberg, and T. J. Singler, “Fabrication of highly electrically conducting fine patterns via substrate-independent inkjet printing of mussel-inspired organic nano-material,” J. Mater. Chem. C Mater. Opt. Electron. Devices 2(20), 3885–3889 (2014).
[Crossref]

K.-J. Chen, H.-V. Han, H.-C. Chen, C.-C. Lin, S.-H. Chien, C.-C. Huang, T.-M. Chen, M.-H. Shih, and H.-C. Kuo, “White Light Emitting Diodes with Enhanced CCT Uniformity and Luminous Flux Using ZrO2 Nanoparticles,” Nanoscale 6(10), 5378–5383 (2014).
[Crossref] [PubMed]

B. Guzelturk, Y. Kelestemur, M. Z. Akgul, V. K. Sharma, and H. V. Demir, “Ultralow Threshold One-Photon- and Two-Photon-Pumped Optical Gain Media of Blue-Emitting Colloidal Quantum Dot Films,” J. Phys. Chem. Lett. 5(13), 2214–2218 (2014).
[Crossref] [PubMed]

2013 (4)

Z. L. Liu, W. C. Chong, K. M. Wong, K. H. Tam, and K. M. Lau, “A Novel BLU-Free Full-Color LED Projector using LED on Silicon Micro-Displays,” IEEE Photonics Technol. Lett. 25(23), 2267–2270 (2013).
[Crossref]

Z. J. Liu, W. C. Chong, K. M. Wong, and K. M. Lau, “360 PPI flip-chip mounted active matrix addressable light emitting diode on silicon (LEDoS) micro-displays,” J. Displ. Technol. 9(8), 678–682 (2013).
[Crossref]

Z. J. Liu, W. C. Chong, K. M. Wong, C. W. Keung, and K. M. Lau, “Investigation of Forward Voltage Uniformity in Monolithic Light-Emitting Diode Arrays,” IEEE Photonics Technol. Lett. 25(13), 1290–1293 (2013).
[Crossref]

B. S. Mashford, M. Stevenson, Z. Popovic, C. Hamilton, Z. Zhou, C. Breen, J. Steckel, V. Bulovic, M. Bawendi, S. Coe-Sullivan, and P. T. Kazlas, “High-efficiency quantum-dot light-emitting devices with enhanced charge injection,” Nat. Photonics 7(5), 407–412 (2013).
[Crossref]

2012 (7)

J. Kwak, W. K. Bae, D. Lee, I. Park, J. Lim, M. Park, H. Cho, H. Woo, Y. Yoon, K. Char, S. Lee, and C. Lee, “Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure,” Nano Lett. 12(5), 2362–2366 (2012).
[Crossref] [PubMed]

K. J. Chen, H. C. Chen, K. A. Tsai, C. C. Lin, H. H. Tsai, S. H. Chien, B. S. Cheng, Y. J. Hsu, M. H. Shih, C. H. Tsai, H.-H. Shih, and H.-C. Kuo, “Resonant‐Enhanced Full‐Color Emission of Quantum‐Dot‐Based Display Technology Using a Pulsed Spray Method,” Adv. Funct. Mater. 22(24), 5138–5143 (2012).
[Crossref]

Y. Shirasaki, G. J. Supran, M. G. Bawendi, and V. Bulovic, “Emergence of colloidal quantum-dot light-emitting technologies,” Nat. Photonics 7(1), 13–23 (2012).
[Crossref]

R. Liu, H. Ding, J. Lin, F. Shen, Z. Cui, and T. Zhang, “Fabrication of platinum-decorated single-walled carbon nanotube based hydrogen sensors by aerosol jet printing,” Nanotechnology 23(50), 505301 (2012).
[Crossref] [PubMed]

G. Cummins and M. P. Y. Desmulliez, “Inkjet printing of conductive materials: a review,” Circuit World 38(4), 193–213 (2012).
[Crossref]

J. M. Hoey, A. Lutfurakhmanov, D. L. Schulz, and I. S. Akhatov, “A Review on Aerosol-Based Direct-Write and Its Applications for Microelectronics,” J. Nanotechnol. 2012, 22 (2012).
[Crossref]

K.-J. Chen, H.-C. Chen, M.-H. Shih, C.-H. Wang, M.-Y. Kuo, Y.-C. Yang, C.-C. Lin, and H.-C. Kuo, “The Influence of the thermal effect on CdSe/ZnS quantum dots in light-emitting diodes,” J. Lightwave Technol. 30(14), 2256–2261 (2012).
[Crossref]

2011 (5)

P. Chen, Y. Fu, R. Aminirad, C. Wang, J. Zhang, K. Wang, K. Galatsis, and C. Zhou, “Fully Printed Separated Carbon Nanotube Thin Film Transistor Circuits and Its Application in Organic Light Emitting Diode Control,” Nano Lett. 11(12), 5301–5308 (2011).
[Crossref] [PubMed]

Y. T. Gizachew, L. Escoubas, J. J. Simon, M. Pasquinelli, J. Loiret, P. Y. Leguen, J. C. Jimeno, J. Martin, A. Apraiz, and J. P. Aguerre, “Towards ink-jet printed fine line front side metallization of crystalline silicon solar cells,” Sol. Energy Mater. Sol. Cells 95, S70–S82 (2011).
[Crossref]

J. Wang, X. Cheng, M. Caironi, F. Gao, X. Yang, and N. C. Greenham, “Entirely solution-processed write-once-read-many-times memory devices and their operation mechanism,” Org. Electron. 12(7), 1271–1274 (2011).
[Crossref]

L. Qian, Y. Zheng, J. Xue, and P. H. Holloway, “Stable and efficient quantum-dot light-emitting diodes based on solution-processed multilayer structures,” Nat. Photonics 5(9), 543–548 (2011).
[Crossref]

T.-H. Kim, K.-S. Cho, E. K. Lee, S. J. Lee, J. Chae, J. W. Kim, D. H. Kim, J.-Y. Kwon, G. Amaratunga, S. Y. Lee, B. L. Choi, Y. Kuk, J. M. Kim, and K. Kim, “Full-colour quantum dot displays fabricated by transfer printing,” Nat. Photonics 5(3), 176–182 (2011).
[Crossref]

2010 (3)

H. M. Haverinen, R. A. Myllyla, and G. E. Jabbour, “Inkjet Printed RGB Quantum Dot-Hybrid LED,” J. Displ. Technol. 6(3), 87–89 (2010).
[Crossref]

M. Singh, H. M. Haverinen, P. Dhagat, and G. E. Jabbour, “Inkjet printing-process and its applications,” Adv. Mater. 22(6), 673–685 (2010).
[Crossref] [PubMed]

W. K. Bae, J. Kwak, J. Lim, D. Lee, M. K. Nam, K. Char, C. Lee, and S. Lee, “Multicolored Light-Emitting Diodes Based on All-Quantum-Dot Multilayer Films Using Layer-by-Layer Assembly Method,” Nano Lett. 10(7), 2368–2373 (2010).
[Crossref] [PubMed]

2009 (5)

S. Riehemann, C. Grossmann, U. Vogel, B. Richter, R. Herold, and G. Notni, “Ultra small OLED pico projector,” Optik Photonik 4(2), 34–36 (2009).
[Crossref]

V. Wood, M. J. Panzer, J. E. Halpert, J.-M. Caruge, M. G. Bawendi, and V. Bulović, “Selection of metal oxide charge transport layers for colloidal quantum dot LEDs,” ACS Nano 3(11), 3581–3586 (2009).
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H. M. Haverinen, R. A. Myllylä, and G. E. Jabbour, “Inkjet printing of light emitting quantum dots,” Appl. Phys. Lett. 94(7), 073108 (2009).
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S. Pimputkar, J. S. Speck, S. P. DenBaars, and S. Nakamura, “Prospects for LED lighting,” Nat. Photonics 3(4), 180–182 (2009).
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M. Wu, Z. Gong, A. J. Kuehne, A. L. Kanibolotsky, Y. J. Chen, I. F. Perepichka, A. R. Mackintosh, E. Gu, P. J. Skabara, R. A. Pethrick, and M. D. Dawson, “Hybrid GaN/organic microstructured light-emitting devices via ink-jet printing,” Opt. Express 17(19), 16436–16443 (2009).
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2008 (3)

C. N. Hoth, P. Schilinsky, S. A. Choulis, and C. J. Brabec, “Printing highly efficient organic solar cells,” Nano Lett. 8(9), 2806–2813 (2008).
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Z. Gong, E. Gu, S. R. Jin, D. Massoubre, B. Guilhabert, H. X. Zhang, M. D. Dawson, V. Poher, G. T. Kennedy, P. M. W. French, and M. A. A. Neil, “Efficient flip-chip InGaN micro-pixellated light-emitting diode arrays: Promising candidates for micro-displays and colour conversion,” J. Phys. D Appl. Phys. 41(9), 094002 (2008).
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L. Kim, P. O. Anikeeva, S. A. Coe-Sullivan, J. S. Steckel, M. G. Bawendi, and V. Bulović, “Contact Printing of Quantum Dot Light-Emitting Devices,” Nano Lett. 8(12), 4513–4517 (2008).
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2007 (3)

S. Günes, H. Neugebauer, and N. S. Sariciftci, “Conjugated polymer-based organic solar cells,” Chem. Rev. 107(4), 1324–1338 (2007).
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I. Robel, M. Kuno, and P. V. Kamat, “Size-dependent electron injection from excited CdSe quantum dots into TiO2 nanoparticles,” J. Am. Chem. Soc. 129(14), 4136–4137 (2007).
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A. Mette, P. Richter, M. Hörteis, and S. Glunz, “Metal aerosol jet printing for solar cell metallization,” Prog. Photovolt. Res. Appl. 15(7), 621–627 (2007).
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2006 (2)

C. de Mello Donegá, M. Bode, and A. Meijerink, “Size- and temperature-dependence of exciton lifetimes in CdSe quantum dots,” Phys. Rev. B 74(8), 085320 (2006).
[Crossref]

J. Zhao, J. A. Bardecker, A. M. Munro, M. S. Liu, Y. Niu, I.-K. Ding, J. Luo, B. Chen, A. K.-Y. Jen, and D. S. Ginger, “Efficient CdSe/CdS quantum dot light-emitting diodes using a thermally polymerized hole transport layer,” Nano Lett. 6(3), 463–467 (2006).
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2005 (2)

I. L. Medintz, H. T. Uyeda, E. R. Goldman, and H. Mattoussi, “Quantum dot bioconjugates for imaging, labelling and sensing,” Nat. Mater. 4(6), 435–446 (2005).
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E. F. Schubert and J. K. Kim, “Solid-State Light Sources Getting Smart,” Science 308(5726), 1274–1278 (2005).
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2004 (1)

J. K. Park, C. H. Kim, S. H. Park, H. D. Park, and S. Y. Choi, “Application of strontium silicate yellow phosphor for white light-emitting diodes,” Appl. Phys. Lett. 84(10), 1647–1649 (2004).
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2003 (1)

T. Shimoda, K. Morii, S. Seki, and H. Kiguchi, “Inkjet printing of light-emitting polymer displays,” MRS Bull. 28(11), 821–827 (2003).
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2002 (2)

S. Coe, W.-K. Woo, M. Bawendi, and V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
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P. Reiss, J. Bleuse, and A. Pron, “Highly luminescent CdSe/ZnSe core/shell nanocrystals of low size dispersion,” Nano Lett. 2(7), 781–784 (2002).
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2001 (1)

T.-F. Wu, Y.-C. Wu, and Z.-Y. Su, “Design considerations for single-stage electronic ballast with dimming feature,” IEEE Transactions on Industry Applications,  37(5), 1537–1543 (2001).

2000 (2)

H. Mattoussi, J. M. Mauro, E. R. Goldman, G. P. Anderson, V. C. Sundar, F. V. Mikulec, and M. G. Bawendi, “Self-assembly of CdSe-ZnS quantum dot bioconjugates using an engineered recombinant protein,” J. Am. Chem. Soc. 122(49), 12142–12150 (2000).
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P. Waltereit, O. Brandt, A. Trampert, H. T. Grahn, J. Menniger, M. Ramsteiner, M. Reiche, and K. H. Ploog, “Nitride semiconductors free of electrostatic fields for efficient white light-emitting diodes,” Nature 406(6798), 865–868 (2000).
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1999 (1)

S.-C. Chang, J. Liu, J. Bharathan, Y. Yang, J. Onohara, and J. Kido, “Multicolor organic light-emitting diodes processed by hybrid inkjet printing,” Adv. Mater. 11(9), 734–737 (1999).
[Crossref]

1997 (1)

B. Dabbousi, J. Rodriguez-Viejo, F. V. Mikulec, J. Heine, H. Mattoussi, R. Ober, K. Jensen, and M. Bawendi, “(CdSe) ZnS core-shell quantum dots: synthesis and characterization of a size series of highly luminescent nanocrystallites,” J. Phys. Chem. B 101(46), 9463–9475 (1997).
[Crossref]

1996 (1)

M. A. Hines and P. Guyot-Sionnest, “Synthesis and Characterization of Strongly Luminescing ZnS-Capped CdSe Nanocrystals,” J. Phys. Chem. 100(2), 468–471 (1996).
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Adachi, C.

J. G. Tait, E. Witkowska, M. Hirade, T.-H. Ke, P. E. Malinowski, S. Steudel, C. Adachi, and P. Heremans, “Uniform Aerosol Jet printed polymer lines with 30 μm width for 140 ppi resolution RGB organic light emitting diodes,” Org. Electron. 22, 40–43 (2015).
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Aga, R.

R. Aga, C. Jordan, R. S. Aga, C. M. Bartsch, and E. M. Heckman, “Metal Electrode Work Function Modification Using Aerosol Jet Printing,” IEEE Electron Dev. Lett. 35(11), 1124–1126 (2014).
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Aga, R. S.

R. Aga, C. Jordan, R. S. Aga, C. M. Bartsch, and E. M. Heckman, “Metal Electrode Work Function Modification Using Aerosol Jet Printing,” IEEE Electron Dev. Lett. 35(11), 1124–1126 (2014).
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Aguerre, J. P.

Y. T. Gizachew, L. Escoubas, J. J. Simon, M. Pasquinelli, J. Loiret, P. Y. Leguen, J. C. Jimeno, J. Martin, A. Apraiz, and J. P. Aguerre, “Towards ink-jet printed fine line front side metallization of crystalline silicon solar cells,” Sol. Energy Mater. Sol. Cells 95, S70–S82 (2011).
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Akgul, M. Z.

B. Guzelturk, Y. Kelestemur, M. Z. Akgul, V. K. Sharma, and H. V. Demir, “Ultralow Threshold One-Photon- and Two-Photon-Pumped Optical Gain Media of Blue-Emitting Colloidal Quantum Dot Films,” J. Phys. Chem. Lett. 5(13), 2214–2218 (2014).
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Akhatov, I. S.

J. M. Hoey, A. Lutfurakhmanov, D. L. Schulz, and I. S. Akhatov, “A Review on Aerosol-Based Direct-Write and Its Applications for Microelectronics,” J. Nanotechnol. 2012, 22 (2012).
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Amaratunga, G.

T.-H. Kim, K.-S. Cho, E. K. Lee, S. J. Lee, J. Chae, J. W. Kim, D. H. Kim, J.-Y. Kwon, G. Amaratunga, S. Y. Lee, B. L. Choi, Y. Kuk, J. M. Kim, and K. Kim, “Full-colour quantum dot displays fabricated by transfer printing,” Nat. Photonics 5(3), 176–182 (2011).
[Crossref]

Aminirad, R.

P. Chen, Y. Fu, R. Aminirad, C. Wang, J. Zhang, K. Wang, K. Galatsis, and C. Zhou, “Fully Printed Separated Carbon Nanotube Thin Film Transistor Circuits and Its Application in Organic Light Emitting Diode Control,” Nano Lett. 11(12), 5301–5308 (2011).
[Crossref] [PubMed]

Anderson, G. P.

H. Mattoussi, J. M. Mauro, E. R. Goldman, G. P. Anderson, V. C. Sundar, F. V. Mikulec, and M. G. Bawendi, “Self-assembly of CdSe-ZnS quantum dot bioconjugates using an engineered recombinant protein,” J. Am. Chem. Soc. 122(49), 12142–12150 (2000).
[Crossref]

Anikeeva, P. O.

L. Kim, P. O. Anikeeva, S. A. Coe-Sullivan, J. S. Steckel, M. G. Bawendi, and V. Bulović, “Contact Printing of Quantum Dot Light-Emitting Devices,” Nano Lett. 8(12), 4513–4517 (2008).
[Crossref] [PubMed]

Apraiz, A.

Y. T. Gizachew, L. Escoubas, J. J. Simon, M. Pasquinelli, J. Loiret, P. Y. Leguen, J. C. Jimeno, J. Martin, A. Apraiz, and J. P. Aguerre, “Towards ink-jet printed fine line front side metallization of crystalline silicon solar cells,” Sol. Energy Mater. Sol. Cells 95, S70–S82 (2011).
[Crossref]

Bae, W. K.

J. Kwak, W. K. Bae, D. Lee, I. Park, J. Lim, M. Park, H. Cho, H. Woo, Y. Yoon, K. Char, S. Lee, and C. Lee, “Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure,” Nano Lett. 12(5), 2362–2366 (2012).
[Crossref] [PubMed]

W. K. Bae, J. Kwak, J. Lim, D. Lee, M. K. Nam, K. Char, C. Lee, and S. Lee, “Multicolored Light-Emitting Diodes Based on All-Quantum-Dot Multilayer Films Using Layer-by-Layer Assembly Method,” Nano Lett. 10(7), 2368–2373 (2010).
[Crossref] [PubMed]

Bardecker, J. A.

J. Zhao, J. A. Bardecker, A. M. Munro, M. S. Liu, Y. Niu, I.-K. Ding, J. Luo, B. Chen, A. K.-Y. Jen, and D. S. Ginger, “Efficient CdSe/CdS quantum dot light-emitting diodes using a thermally polymerized hole transport layer,” Nano Lett. 6(3), 463–467 (2006).
[Crossref] [PubMed]

Bartsch, C. M.

R. Aga, C. Jordan, R. S. Aga, C. M. Bartsch, and E. M. Heckman, “Metal Electrode Work Function Modification Using Aerosol Jet Printing,” IEEE Electron Dev. Lett. 35(11), 1124–1126 (2014).
[Crossref]

Baumann, R. R.

T. Seifert, E. Sowade, F. Roscher, M. Wiemer, T. Gessner, and R. R. Baumann, “Additive Manufacturing Technologies Compared: Morphology of Deposits of Silver Ink Using Inkjet and Aerosol Jet Printing,” Ind. Eng. Chem. Res. 54(2), 769–779 (2015).
[Crossref]

Bawendi, M.

B. S. Mashford, M. Stevenson, Z. Popovic, C. Hamilton, Z. Zhou, C. Breen, J. Steckel, V. Bulovic, M. Bawendi, S. Coe-Sullivan, and P. T. Kazlas, “High-efficiency quantum-dot light-emitting devices with enhanced charge injection,” Nat. Photonics 7(5), 407–412 (2013).
[Crossref]

S. Coe, W.-K. Woo, M. Bawendi, and V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[Crossref] [PubMed]

B. Dabbousi, J. Rodriguez-Viejo, F. V. Mikulec, J. Heine, H. Mattoussi, R. Ober, K. Jensen, and M. Bawendi, “(CdSe) ZnS core-shell quantum dots: synthesis and characterization of a size series of highly luminescent nanocrystallites,” J. Phys. Chem. B 101(46), 9463–9475 (1997).
[Crossref]

Bawendi, M. G.

Y. Shirasaki, G. J. Supran, M. G. Bawendi, and V. Bulovic, “Emergence of colloidal quantum-dot light-emitting technologies,” Nat. Photonics 7(1), 13–23 (2012).
[Crossref]

V. Wood, M. J. Panzer, J. E. Halpert, J.-M. Caruge, M. G. Bawendi, and V. Bulović, “Selection of metal oxide charge transport layers for colloidal quantum dot LEDs,” ACS Nano 3(11), 3581–3586 (2009).
[Crossref] [PubMed]

L. Kim, P. O. Anikeeva, S. A. Coe-Sullivan, J. S. Steckel, M. G. Bawendi, and V. Bulović, “Contact Printing of Quantum Dot Light-Emitting Devices,” Nano Lett. 8(12), 4513–4517 (2008).
[Crossref] [PubMed]

H. Mattoussi, J. M. Mauro, E. R. Goldman, G. P. Anderson, V. C. Sundar, F. V. Mikulec, and M. G. Bawendi, “Self-assembly of CdSe-ZnS quantum dot bioconjugates using an engineered recombinant protein,” J. Am. Chem. Soc. 122(49), 12142–12150 (2000).
[Crossref]

Bharathan, J.

S.-C. Chang, J. Liu, J. Bharathan, Y. Yang, J. Onohara, and J. Kido, “Multicolor organic light-emitting diodes processed by hybrid inkjet printing,” Adv. Mater. 11(9), 734–737 (1999).
[Crossref]

Bleuse, J.

P. Reiss, J. Bleuse, and A. Pron, “Highly luminescent CdSe/ZnSe core/shell nanocrystals of low size dispersion,” Nano Lett. 2(7), 781–784 (2002).
[Crossref]

Bode, M.

C. de Mello Donegá, M. Bode, and A. Meijerink, “Size- and temperature-dependence of exciton lifetimes in CdSe quantum dots,” Phys. Rev. B 74(8), 085320 (2006).
[Crossref]

Brabec, C. J.

C. N. Hoth, P. Schilinsky, S. A. Choulis, and C. J. Brabec, “Printing highly efficient organic solar cells,” Nano Lett. 8(9), 2806–2813 (2008).
[Crossref] [PubMed]

Brandt, O.

P. Waltereit, O. Brandt, A. Trampert, H. T. Grahn, J. Menniger, M. Ramsteiner, M. Reiche, and K. H. Ploog, “Nitride semiconductors free of electrostatic fields for efficient white light-emitting diodes,” Nature 406(6798), 865–868 (2000).
[Crossref] [PubMed]

Breen, C.

B. S. Mashford, M. Stevenson, Z. Popovic, C. Hamilton, Z. Zhou, C. Breen, J. Steckel, V. Bulovic, M. Bawendi, S. Coe-Sullivan, and P. T. Kazlas, “High-efficiency quantum-dot light-emitting devices with enhanced charge injection,” Nat. Photonics 7(5), 407–412 (2013).
[Crossref]

Bromberg, V.

S. Ma, L. Liu, V. Bromberg, and T. J. Singler, “Fabrication of highly electrically conducting fine patterns via substrate-independent inkjet printing of mussel-inspired organic nano-material,” J. Mater. Chem. C Mater. Opt. Electron. Devices 2(20), 3885–3889 (2014).
[Crossref]

Bulovic, V.

B. S. Mashford, M. Stevenson, Z. Popovic, C. Hamilton, Z. Zhou, C. Breen, J. Steckel, V. Bulovic, M. Bawendi, S. Coe-Sullivan, and P. T. Kazlas, “High-efficiency quantum-dot light-emitting devices with enhanced charge injection,” Nat. Photonics 7(5), 407–412 (2013).
[Crossref]

Y. Shirasaki, G. J. Supran, M. G. Bawendi, and V. Bulovic, “Emergence of colloidal quantum-dot light-emitting technologies,” Nat. Photonics 7(1), 13–23 (2012).
[Crossref]

V. Wood, M. J. Panzer, J. E. Halpert, J.-M. Caruge, M. G. Bawendi, and V. Bulović, “Selection of metal oxide charge transport layers for colloidal quantum dot LEDs,” ACS Nano 3(11), 3581–3586 (2009).
[Crossref] [PubMed]

L. Kim, P. O. Anikeeva, S. A. Coe-Sullivan, J. S. Steckel, M. G. Bawendi, and V. Bulović, “Contact Printing of Quantum Dot Light-Emitting Devices,” Nano Lett. 8(12), 4513–4517 (2008).
[Crossref] [PubMed]

S. Coe, W.-K. Woo, M. Bawendi, and V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[Crossref] [PubMed]

Caironi, M.

J. Wang, X. Cheng, M. Caironi, F. Gao, X. Yang, and N. C. Greenham, “Entirely solution-processed write-once-read-many-times memory devices and their operation mechanism,” Org. Electron. 12(7), 1271–1274 (2011).
[Crossref]

Cao, W.

Y. Yang, Y. Zheng, W. Cao, A. Titov, J. Hyvonen, R. Manders Jesse, J. Xue, P. H. Holloway, and L. Qian, “High-efficiency light-emitting devices based on quantum dots with tailored nanostructures,” Nat. Photonics 9, 259–266 (2015).

Caruge, J.-M.

V. Wood, M. J. Panzer, J. E. Halpert, J.-M. Caruge, M. G. Bawendi, and V. Bulović, “Selection of metal oxide charge transport layers for colloidal quantum dot LEDs,” ACS Nano 3(11), 3581–3586 (2009).
[Crossref] [PubMed]

Chae, J.

T.-H. Kim, K.-S. Cho, E. K. Lee, S. J. Lee, J. Chae, J. W. Kim, D. H. Kim, J.-Y. Kwon, G. Amaratunga, S. Y. Lee, B. L. Choi, Y. Kuk, J. M. Kim, and K. Kim, “Full-colour quantum dot displays fabricated by transfer printing,” Nat. Photonics 5(3), 176–182 (2011).
[Crossref]

Chang, S.-C.

S.-C. Chang, J. Liu, J. Bharathan, Y. Yang, J. Onohara, and J. Kido, “Multicolor organic light-emitting diodes processed by hybrid inkjet printing,” Adv. Mater. 11(9), 734–737 (1999).
[Crossref]

Char, K.

J. Kwak, W. K. Bae, D. Lee, I. Park, J. Lim, M. Park, H. Cho, H. Woo, Y. Yoon, K. Char, S. Lee, and C. Lee, “Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure,” Nano Lett. 12(5), 2362–2366 (2012).
[Crossref] [PubMed]

W. K. Bae, J. Kwak, J. Lim, D. Lee, M. K. Nam, K. Char, C. Lee, and S. Lee, “Multicolored Light-Emitting Diodes Based on All-Quantum-Dot Multilayer Films Using Layer-by-Layer Assembly Method,” Nano Lett. 10(7), 2368–2373 (2010).
[Crossref] [PubMed]

Chen, B.

J. Zhao, J. A. Bardecker, A. M. Munro, M. S. Liu, Y. Niu, I.-K. Ding, J. Luo, B. Chen, A. K.-Y. Jen, and D. S. Ginger, “Efficient CdSe/CdS quantum dot light-emitting diodes using a thermally polymerized hole transport layer,” Nano Lett. 6(3), 463–467 (2006).
[Crossref] [PubMed]

Chen, H. C.

K. J. Chen, H. C. Chen, K. A. Tsai, C. C. Lin, H. H. Tsai, S. H. Chien, B. S. Cheng, Y. J. Hsu, M. H. Shih, C. H. Tsai, H.-H. Shih, and H.-C. Kuo, “Resonant‐Enhanced Full‐Color Emission of Quantum‐Dot‐Based Display Technology Using a Pulsed Spray Method,” Adv. Funct. Mater. 22(24), 5138–5143 (2012).
[Crossref]

Chen, H.-C.

H.-V. Han, C.-C. Lin, Y.-L. Tsai, H.-C. Chen, K.-J. Chen, Y.-L. Yeh, W.-Y. Lin, H.-C. Kuo, and P. Yu, “A Highly Efficient Hybrid GaAs Solar Cell Based on Colloidal-Quantum-Dot-Sensitization,” Sci. Rep. 4, 5734 (2014).
[PubMed]

K.-J. Chen, H.-V. Han, H.-C. Chen, C.-C. Lin, S.-H. Chien, C.-C. Huang, T.-M. Chen, M.-H. Shih, and H.-C. Kuo, “White Light Emitting Diodes with Enhanced CCT Uniformity and Luminous Flux Using ZrO2 Nanoparticles,” Nanoscale 6(10), 5378–5383 (2014).
[Crossref] [PubMed]

K.-J. Chen, H.-C. Chen, M.-H. Shih, C.-H. Wang, M.-Y. Kuo, Y.-C. Yang, C.-C. Lin, and H.-C. Kuo, “The Influence of the thermal effect on CdSe/ZnS quantum dots in light-emitting diodes,” J. Lightwave Technol. 30(14), 2256–2261 (2012).
[Crossref]

Chen, K. J.

K. J. Chen, H. C. Chen, K. A. Tsai, C. C. Lin, H. H. Tsai, S. H. Chien, B. S. Cheng, Y. J. Hsu, M. H. Shih, C. H. Tsai, H.-H. Shih, and H.-C. Kuo, “Resonant‐Enhanced Full‐Color Emission of Quantum‐Dot‐Based Display Technology Using a Pulsed Spray Method,” Adv. Funct. Mater. 22(24), 5138–5143 (2012).
[Crossref]

Chen, K.-J.

H.-V. Han, C.-C. Lin, Y.-L. Tsai, H.-C. Chen, K.-J. Chen, Y.-L. Yeh, W.-Y. Lin, H.-C. Kuo, and P. Yu, “A Highly Efficient Hybrid GaAs Solar Cell Based on Colloidal-Quantum-Dot-Sensitization,” Sci. Rep. 4, 5734 (2014).
[PubMed]

K.-J. Chen, H.-V. Han, H.-C. Chen, C.-C. Lin, S.-H. Chien, C.-C. Huang, T.-M. Chen, M.-H. Shih, and H.-C. Kuo, “White Light Emitting Diodes with Enhanced CCT Uniformity and Luminous Flux Using ZrO2 Nanoparticles,” Nanoscale 6(10), 5378–5383 (2014).
[Crossref] [PubMed]

K.-J. Chen, H.-C. Chen, M.-H. Shih, C.-H. Wang, M.-Y. Kuo, Y.-C. Yang, C.-C. Lin, and H.-C. Kuo, “The Influence of the thermal effect on CdSe/ZnS quantum dots in light-emitting diodes,” J. Lightwave Technol. 30(14), 2256–2261 (2012).
[Crossref]

Chen, P.

P. Chen, Y. Fu, R. Aminirad, C. Wang, J. Zhang, K. Wang, K. Galatsis, and C. Zhou, “Fully Printed Separated Carbon Nanotube Thin Film Transistor Circuits and Its Application in Organic Light Emitting Diode Control,” Nano Lett. 11(12), 5301–5308 (2011).
[Crossref] [PubMed]

Chen, T.-M.

K.-J. Chen, H.-V. Han, H.-C. Chen, C.-C. Lin, S.-H. Chien, C.-C. Huang, T.-M. Chen, M.-H. Shih, and H.-C. Kuo, “White Light Emitting Diodes with Enhanced CCT Uniformity and Luminous Flux Using ZrO2 Nanoparticles,” Nanoscale 6(10), 5378–5383 (2014).
[Crossref] [PubMed]

Chen, Y. J.

Cheng, B. S.

K. J. Chen, H. C. Chen, K. A. Tsai, C. C. Lin, H. H. Tsai, S. H. Chien, B. S. Cheng, Y. J. Hsu, M. H. Shih, C. H. Tsai, H.-H. Shih, and H.-C. Kuo, “Resonant‐Enhanced Full‐Color Emission of Quantum‐Dot‐Based Display Technology Using a Pulsed Spray Method,” Adv. Funct. Mater. 22(24), 5138–5143 (2012).
[Crossref]

Cheng, X.

J. Wang, X. Cheng, M. Caironi, F. Gao, X. Yang, and N. C. Greenham, “Entirely solution-processed write-once-read-many-times memory devices and their operation mechanism,” Org. Electron. 12(7), 1271–1274 (2011).
[Crossref]

Chien, S. H.

K. J. Chen, H. C. Chen, K. A. Tsai, C. C. Lin, H. H. Tsai, S. H. Chien, B. S. Cheng, Y. J. Hsu, M. H. Shih, C. H. Tsai, H.-H. Shih, and H.-C. Kuo, “Resonant‐Enhanced Full‐Color Emission of Quantum‐Dot‐Based Display Technology Using a Pulsed Spray Method,” Adv. Funct. Mater. 22(24), 5138–5143 (2012).
[Crossref]

Chien, S.-H.

K.-J. Chen, H.-V. Han, H.-C. Chen, C.-C. Lin, S.-H. Chien, C.-C. Huang, T.-M. Chen, M.-H. Shih, and H.-C. Kuo, “White Light Emitting Diodes with Enhanced CCT Uniformity and Luminous Flux Using ZrO2 Nanoparticles,” Nanoscale 6(10), 5378–5383 (2014).
[Crossref] [PubMed]

Cho, H.

J. Kwak, W. K. Bae, D. Lee, I. Park, J. Lim, M. Park, H. Cho, H. Woo, Y. Yoon, K. Char, S. Lee, and C. Lee, “Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure,” Nano Lett. 12(5), 2362–2366 (2012).
[Crossref] [PubMed]

Cho, K.-S.

T.-H. Kim, K.-S. Cho, E. K. Lee, S. J. Lee, J. Chae, J. W. Kim, D. H. Kim, J.-Y. Kwon, G. Amaratunga, S. Y. Lee, B. L. Choi, Y. Kuk, J. M. Kim, and K. Kim, “Full-colour quantum dot displays fabricated by transfer printing,” Nat. Photonics 5(3), 176–182 (2011).
[Crossref]

Choi, B. L.

T.-H. Kim, K.-S. Cho, E. K. Lee, S. J. Lee, J. Chae, J. W. Kim, D. H. Kim, J.-Y. Kwon, G. Amaratunga, S. Y. Lee, B. L. Choi, Y. Kuk, J. M. Kim, and K. Kim, “Full-colour quantum dot displays fabricated by transfer printing,” Nat. Photonics 5(3), 176–182 (2011).
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R. Liu, H. Ding, J. Lin, F. Shen, Z. Cui, and T. Zhang, “Fabrication of platinum-decorated single-walled carbon nanotube based hydrogen sensors by aerosol jet printing,” Nanotechnology 23(50), 505301 (2012).
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Zhao, J.

W. Tang, L. Feng, C. Jiang, G. Yao, J. Zhao, Q. Cui, and X. Guo, “Controlling the surface wettability of the polymer dielectric for improved resolution of inkjet-printed electrodes and patterned channel regions in low-voltage solution-processed organic thin film transistors,” J. Mater. Chem. C Mater. Opt. Electron. Devices 2(28), 5553–5558 (2014).
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Y. Yang, Y. Zheng, W. Cao, A. Titov, J. Hyvonen, R. Manders Jesse, J. Xue, P. H. Holloway, and L. Qian, “High-efficiency light-emitting devices based on quantum dots with tailored nanostructures,” Nat. Photonics 9, 259–266 (2015).

L. Qian, Y. Zheng, J. Xue, and P. H. Holloway, “Stable and efficient quantum-dot light-emitting diodes based on solution-processed multilayer structures,” Nat. Photonics 5(9), 543–548 (2011).
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Zhou, C.

P. Chen, Y. Fu, R. Aminirad, C. Wang, J. Zhang, K. Wang, K. Galatsis, and C. Zhou, “Fully Printed Separated Carbon Nanotube Thin Film Transistor Circuits and Its Application in Organic Light Emitting Diode Control,” Nano Lett. 11(12), 5301–5308 (2011).
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L. Qian, Y. Zheng, J. Xue, and P. H. Holloway, “Stable and efficient quantum-dot light-emitting diodes based on solution-processed multilayer structures,” Nat. Photonics 5(9), 543–548 (2011).
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Figures (11)

Fig. 1
Fig. 1 UV-visible absorption and PL emission spectra of QDs with the emission colors of (a) blue, (c) green and (e) red. (b) blue, (d) green and (f) red are the photos of quantum dot solution under UV excitation.
Fig. 2
Fig. 2 Typical TEM images of QDs with the emission colors of (a) blue, (c) green, and (e) red. The corresponding HRTEM images are shown in (b), (d), and (f), respectively.
Fig. 3
Fig. 3 The process flow of the full-color emission of quantum-dot-based micro LED display.
Fig. 4
Fig. 4 (a) The image of aerosol jet printing. (b) The schematic pictures of aerosol jet printing.
Fig. 5
Fig. 5 (a) The deposition profiles for our RGB QDs on the UV LED, (b) The surface profile image of jet-printed QDs scanned by the laser microscopy.
Fig. 6
Fig. 6 The photo image of sprayed QDs micro LED array under the fluorescence microscopy.
Fig. 7
Fig. 7 (a)Measured reflectance spectrum of 17.5-pair HfO2/SiO2 distributed Bragg reflector (DBR). (b)The relative PL intensity of the sprayed QDs samples with and without DBR.
Fig. 8
Fig. 8 (a) The emission spectra with and without the DBR structure. (b) Top: the sprayed RBG QDs micro LED display device in action; bottom: representative image of RGB pixels.
Fig. 9
Fig. 9 (a)-(c) The large area monochromatic light emission (red, green, and blue) of the QD micro LED arrays.
Fig. 10
Fig. 10 The CIE1976 color space chromaticity diagram of the QD display technology and NTSC.
Fig. 11
Fig. 11 (a) The relative emission spectrum of the micro LED array with RGB QDs and DBR structure under various drive currents (from 100 mA to 1 A, from bottom to top curves). (b) The zoom-in traces of CIE1976 chromaticity diagram of our structure under different driving current. (c) The CCT and (d) the luminous efficacy of optical radiation of UV micro LED array with RGB QDs and DBR structure under currents between 100 mA and 1 A.

Equations (1)

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LER=683 lm W V(λ) P white ( λ )dλ P white ( λ )dλ .

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