Abstract

We report on a polarization-dependent plasmonic aluminum-based high-density metasurface operating at blue wavelengths. The fabricated sub-wavelength structures, tailored in size and geometry, possess strong, localized, plasmonic resonances able to control linear polarization. Best performance is achieved by rotating an elongated rectangular structure of length 180 nm and width 110 nm inside a square lattice of period 250 nm. In the case of 45 degrees rotation of the structure with respect to the lattice, the normal-incidence reflectance drops around the resonance wavelength of 457 nm from about 60 percent to below 2 percent.

© 2015 Optical Society of America

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2015 (5)

W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
[Crossref] [PubMed]

D. Gérard and S. K. Gray, “Aluminium plasmonics,” J. Phys. D. Appl. Phys. 184001, 184001 (2015).
[Crossref]

C. Vannahme, M. Dufva, and A. Kristensen, “High frame rate multi-resonance imaging refractometry with distributed feedback dye laser sensor,” Light Sci. Appl. 4, e269 (2015).
[Crossref]

P. G. Hermannsson, K. T. Sørensen, C. Vannahme, C. L. Smith, J. J. Klein, M.-M. Russew, G. Grützner, and A. Kristensen, “All-polymer photonic crystal slab sensor,” Opt. Express 23, 16529 (2015).
[Crossref] [PubMed]

S. Raza, S. I. Bozhevolnyi, M. Wubs, and N. A. Mortensen, “Nonlocal optical response in metallic nanostructures,” J. Phys. Condens. Matter 27, 183204 (2015).
[Crossref] [PubMed]

2014 (6)

E. Højlund-Nielsen, J. Weirich, J. Nørregaard, J. Garnaes, N. A. Mortensen, and A. Kristensen, “Angle-independent structural colors of silicon,” J. Nanophotonics 8, 083988 (2014).
[Crossref]

M. W. Knight, N. S. King, L. Liu, H. O. Everitt, P. Nordlander, and N. J. Halas, “Aluminum for plasmonics,” ACS Nano 8, 834–840 (2014).
[Crossref]

S. J. Tan, L. Zhang, D. Zhu, X. M. Goh, Y. M. Wang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Plasmonic color palettes for photorealistic printing with aluminum nanostructures,” Nano Lett. 14, 4023–4029 (2014).
[Crossref] [PubMed]

J. Olson, A. Manjavacas, L. Liu, W.-S. Chang, B. Foerster, N. S. King, M. W. Knight, P. Nordlander, N. J. Halas, and S. Link, “Vivid, full-color aluminum plasmonic pixels,” Proc. Natl. Acad. Sci. U.S.A. 111, 14348–14353 (2014).
[Crossref] [PubMed]

J. S. Clausen, E. Højlund-Nielsen, A. B. Christiansen, S. Yazdi, M. Grajower, H. Taha, U. Levy, A. Kristensen, and N. A. Mortensen, “Plasmonic metasurfaces for coloration of plastic consumer products,” Nano Lett. 14, 4499–4504 (2014).
[Crossref] [PubMed]

X. M. Goh, Y. Zheng, S. J. Tan, L. Zhang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Three-dimensional plasmonic stereoscopic prints in full colour,” Nat. Commun. 5, 5361 (2014).
[Crossref] [PubMed]

2013 (1)

2012 (2)

2011 (3)

J. Zhang, J.-Y. Ou, N. Papasimakis, Y. Chen, K. F. MacDonald, and N. I. Zheludev, “Continuous metal plasmonic frequency selective surfaces,” Opt. Express 19, 23279–23285 (2011).
[Crossref] [PubMed]

E. Petryayeva and U. J. Krull, “Localized surface plasmon resonance: nanostructures, bioassays and biosensing - a review,” Anal. Chim. Acta 706, 8–24 (2011).
[Crossref] [PubMed]

I. Zorić, M. Zäch, B. Kasemo, and C. Langhammer, “Gold, platinum, and aluminum nanodisk plasmons: material independence, subradiance, and damping mechanisms,” ACS Nano 5, 2535–2546 (2011).
[Crossref]

2010 (1)

P. West, S. Ishii, G. Naik, N. Emani, V. Shalaev, and A. Boltasseva, “Searching for better plasmonic materials,” Laser Photonics Rev. 4, 795–808 (2010).
[Crossref]

2009 (1)

R. Adato, A. A. Yanik, J. J. Amsden, D. L. Kaplan, F. G. Omenetto, M. K. Hong, S. Erramilli, and H. Altug, “Ultra-sensitive vibrational spectroscopy of protein monolayers with plasmonic nanoantenna arrays,” Proc. Natl. Acad. Sci. U. S. A. 106, 19227–19232 (2009).
[Crossref] [PubMed]

2008 (5)

F.-J. Haug, T. Soderstrom, O. Cubero, V. Terrazzoni-Daudrix, and C. Ballif, “Plasmonic absorption in textured silver back reflectors of thin film solar cells,” J. Appl. Phys. 104, 064509 (2008).
[Crossref]

F. Le, D. W. Brandl, Y. A. Urzhumov, H. Wang, J. Kundu, N. J. Halas, J. Aizpurua, and P. Nordlander, “Metallic nanoparticle arrays: a common substrate for both surface-enhanced Raman scattering and surface-enhanced infrared absorption,” ACS Nano 2, 707–718 (2008).
[Crossref]

C. Langhammer, M. Schwind, B. Kasemo, and I. Zorić, “Localized surface plasmon resonances in aluminum nanodisks,” Nano Lett. 8, 1461–1471 (2008).
[Crossref] [PubMed]

G. H. Chan, J. Zhao, G. C. Schatz, and R. P. Van Duyne, “Localized surface plasmon resonance spectroscopy of triangular aluminum nanoparticles,” J. Phys. Chem. C 112, 13958–13963 (2008).
[Crossref]

M. E. Stewart, C. R. Anderton, L. B. Thompson, J. Maria, S. K. Gray, J. A. Rogers, and R. G. Nuzzo, “Nanostructured plasmonic sensors,” Chem. Rev. 108, 494–521 (2008).
[Crossref] [PubMed]

2005 (1)

A. L. Ramaswamy and P. Kaste, “A nanovision of the physiochemical phenomena occurring in nanoparticles of aluminum,” J. Energ. Mater. 23, 1–25 (2005).
[Crossref]

2003 (1)

E. Prodan, C. Radloff, N. J. Halas, and P. Nordlander, “A hybridization model for the plasmon response of complex nanostructures,” Science 302, 419–422 (2003).
[Crossref] [PubMed]

2000 (2)

L. Jeurgens, W. Sloof, F. Tichelaar, and E. Mittemeijer, “Thermodynamic stability of amorphous oxide films on metals: application to aluminum oxide films on aluminum substrates,” Phys. Rev. B 62, 4707–4719 (2000).
[Crossref]

S. Link and M. A. El-Sayed, “Shape and size dependence of radiative, non-radiative and photothermal properties of gold nanocrystals,” Int. Rev. Phys. Chem. 19, 409–453 (2000).
[Crossref]

1995 (1)

M. A. Green and M. J. Keevers, “Optical properties of intrinsic silicon at 300 K,” Prog. Photovoltaics Res. Appl. 3, 189–192 (1995).
[Crossref]

1979 (1)

G. Papavassiliou, “Optical properties of small inorganic and organic metal particles,” Prog. Solid State Chem. 12, 185–271 (1979).
[Crossref]

1912 (1)

R. Gans, “Über die Form ultramikroskopischer Goldteilchen,” Ann. Phys. 342, 881–900 (1912).
[Crossref]

Adato, R.

R. Adato, A. A. Yanik, J. J. Amsden, D. L. Kaplan, F. G. Omenetto, M. K. Hong, S. Erramilli, and H. Altug, “Ultra-sensitive vibrational spectroscopy of protein monolayers with plasmonic nanoantenna arrays,” Proc. Natl. Acad. Sci. U. S. A. 106, 19227–19232 (2009).
[Crossref] [PubMed]

Aizpurua, J.

F. Le, D. W. Brandl, Y. A. Urzhumov, H. Wang, J. Kundu, N. J. Halas, J. Aizpurua, and P. Nordlander, “Metallic nanoparticle arrays: a common substrate for both surface-enhanced Raman scattering and surface-enhanced infrared absorption,” ACS Nano 2, 707–718 (2008).
[Crossref]

Altug, H.

R. Adato, A. A. Yanik, J. J. Amsden, D. L. Kaplan, F. G. Omenetto, M. K. Hong, S. Erramilli, and H. Altug, “Ultra-sensitive vibrational spectroscopy of protein monolayers with plasmonic nanoantenna arrays,” Proc. Natl. Acad. Sci. U. S. A. 106, 19227–19232 (2009).
[Crossref] [PubMed]

Alu, A.

W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
[Crossref] [PubMed]

Amsden, J. J.

R. Adato, A. A. Yanik, J. J. Amsden, D. L. Kaplan, F. G. Omenetto, M. K. Hong, S. Erramilli, and H. Altug, “Ultra-sensitive vibrational spectroscopy of protein monolayers with plasmonic nanoantenna arrays,” Proc. Natl. Acad. Sci. U. S. A. 106, 19227–19232 (2009).
[Crossref] [PubMed]

Anderton, C. R.

M. E. Stewart, C. R. Anderton, L. B. Thompson, J. Maria, S. K. Gray, J. A. Rogers, and R. G. Nuzzo, “Nanostructured plasmonic sensors,” Chem. Rev. 108, 494–521 (2008).
[Crossref] [PubMed]

Ballif, C.

F.-J. Haug, T. Soderstrom, O. Cubero, V. Terrazzoni-Daudrix, and C. Ballif, “Plasmonic absorption in textured silver back reflectors of thin film solar cells,” J. Appl. Phys. 104, 064509 (2008).
[Crossref]

Boltasseva, A.

P. West, S. Ishii, G. Naik, N. Emani, V. Shalaev, and A. Boltasseva, “Searching for better plasmonic materials,” Laser Photonics Rev. 4, 795–808 (2010).
[Crossref]

Bozhevolnyi, S. I.

S. Raza, S. I. Bozhevolnyi, M. Wubs, and N. A. Mortensen, “Nonlocal optical response in metallic nanostructures,” J. Phys. Condens. Matter 27, 183204 (2015).
[Crossref] [PubMed]

Brandl, D. W.

F. Le, D. W. Brandl, Y. A. Urzhumov, H. Wang, J. Kundu, N. J. Halas, J. Aizpurua, and P. Nordlander, “Metallic nanoparticle arrays: a common substrate for both surface-enhanced Raman scattering and surface-enhanced infrared absorption,” ACS Nano 2, 707–718 (2008).
[Crossref]

Chan, G. H.

G. H. Chan, J. Zhao, G. C. Schatz, and R. P. Van Duyne, “Localized surface plasmon resonance spectroscopy of triangular aluminum nanoparticles,” J. Phys. Chem. C 112, 13958–13963 (2008).
[Crossref]

Chang, W.-S.

J. Olson, A. Manjavacas, L. Liu, W.-S. Chang, B. Foerster, N. S. King, M. W. Knight, P. Nordlander, N. J. Halas, and S. Link, “Vivid, full-color aluminum plasmonic pixels,” Proc. Natl. Acad. Sci. U.S.A. 111, 14348–14353 (2014).
[Crossref] [PubMed]

Chen, W.

W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
[Crossref] [PubMed]

Chen, Y.

Christiansen, A. B.

J. S. Clausen, E. Højlund-Nielsen, A. B. Christiansen, S. Yazdi, M. Grajower, H. Taha, U. Levy, A. Kristensen, and N. A. Mortensen, “Plasmonic metasurfaces for coloration of plastic consumer products,” Nano Lett. 14, 4499–4504 (2014).
[Crossref] [PubMed]

Clausen, J. S.

J. S. Clausen, E. Højlund-Nielsen, A. B. Christiansen, S. Yazdi, M. Grajower, H. Taha, U. Levy, A. Kristensen, and N. A. Mortensen, “Plasmonic metasurfaces for coloration of plastic consumer products,” Nano Lett. 14, 4499–4504 (2014).
[Crossref] [PubMed]

Cubero, O.

F.-J. Haug, T. Soderstrom, O. Cubero, V. Terrazzoni-Daudrix, and C. Ballif, “Plasmonic absorption in textured silver back reflectors of thin film solar cells,” J. Appl. Phys. 104, 064509 (2008).
[Crossref]

Dufva, M.

C. Vannahme, M. Dufva, and A. Kristensen, “High frame rate multi-resonance imaging refractometry with distributed feedback dye laser sensor,” Light Sci. Appl. 4, e269 (2015).
[Crossref]

El-Sayed, M. A.

S. Link and M. A. El-Sayed, “Shape and size dependence of radiative, non-radiative and photothermal properties of gold nanocrystals,” Int. Rev. Phys. Chem. 19, 409–453 (2000).
[Crossref]

Emani, N.

P. West, S. Ishii, G. Naik, N. Emani, V. Shalaev, and A. Boltasseva, “Searching for better plasmonic materials,” Laser Photonics Rev. 4, 795–808 (2010).
[Crossref]

Erramilli, S.

R. Adato, A. A. Yanik, J. J. Amsden, D. L. Kaplan, F. G. Omenetto, M. K. Hong, S. Erramilli, and H. Altug, “Ultra-sensitive vibrational spectroscopy of protein monolayers with plasmonic nanoantenna arrays,” Proc. Natl. Acad. Sci. U. S. A. 106, 19227–19232 (2009).
[Crossref] [PubMed]

Everitt, H. O.

M. W. Knight, N. S. King, L. Liu, H. O. Everitt, P. Nordlander, and N. J. Halas, “Aluminum for plasmonics,” ACS Nano 8, 834–840 (2014).
[Crossref]

Foerster, B.

J. Olson, A. Manjavacas, L. Liu, W.-S. Chang, B. Foerster, N. S. King, M. W. Knight, P. Nordlander, N. J. Halas, and S. Link, “Vivid, full-color aluminum plasmonic pixels,” Proc. Natl. Acad. Sci. U.S.A. 111, 14348–14353 (2014).
[Crossref] [PubMed]

Gans, R.

R. Gans, “Über die Form ultramikroskopischer Goldteilchen,” Ann. Phys. 342, 881–900 (1912).
[Crossref]

Garnaes, J.

E. Højlund-Nielsen, J. Weirich, J. Nørregaard, J. Garnaes, N. A. Mortensen, and A. Kristensen, “Angle-independent structural colors of silicon,” J. Nanophotonics 8, 083988 (2014).
[Crossref]

Gérard, D.

D. Gérard and S. K. Gray, “Aluminium plasmonics,” J. Phys. D. Appl. Phys. 184001, 184001 (2015).
[Crossref]

Goh, X. M.

X. M. Goh, Y. Zheng, S. J. Tan, L. Zhang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Three-dimensional plasmonic stereoscopic prints in full colour,” Nat. Commun. 5, 5361 (2014).
[Crossref] [PubMed]

S. J. Tan, L. Zhang, D. Zhu, X. M. Goh, Y. M. Wang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Plasmonic color palettes for photorealistic printing with aluminum nanostructures,” Nano Lett. 14, 4023–4029 (2014).
[Crossref] [PubMed]

Gopalan, P.

W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
[Crossref] [PubMed]

Grajower, M.

J. S. Clausen, E. Højlund-Nielsen, A. B. Christiansen, S. Yazdi, M. Grajower, H. Taha, U. Levy, A. Kristensen, and N. A. Mortensen, “Plasmonic metasurfaces for coloration of plastic consumer products,” Nano Lett. 14, 4499–4504 (2014).
[Crossref] [PubMed]

Gray, S. K.

D. Gérard and S. K. Gray, “Aluminium plasmonics,” J. Phys. D. Appl. Phys. 184001, 184001 (2015).
[Crossref]

M. E. Stewart, C. R. Anderton, L. B. Thompson, J. Maria, S. K. Gray, J. A. Rogers, and R. G. Nuzzo, “Nanostructured plasmonic sensors,” Chem. Rev. 108, 494–521 (2008).
[Crossref] [PubMed]

Green, M. A.

M. A. Green and M. J. Keevers, “Optical properties of intrinsic silicon at 300 K,” Prog. Photovoltaics Res. Appl. 3, 189–192 (1995).
[Crossref]

Grützner, G.

Halas, N. J.

J. Olson, A. Manjavacas, L. Liu, W.-S. Chang, B. Foerster, N. S. King, M. W. Knight, P. Nordlander, N. J. Halas, and S. Link, “Vivid, full-color aluminum plasmonic pixels,” Proc. Natl. Acad. Sci. U.S.A. 111, 14348–14353 (2014).
[Crossref] [PubMed]

M. W. Knight, N. S. King, L. Liu, H. O. Everitt, P. Nordlander, and N. J. Halas, “Aluminum for plasmonics,” ACS Nano 8, 834–840 (2014).
[Crossref]

F. Le, D. W. Brandl, Y. A. Urzhumov, H. Wang, J. Kundu, N. J. Halas, J. Aizpurua, and P. Nordlander, “Metallic nanoparticle arrays: a common substrate for both surface-enhanced Raman scattering and surface-enhanced infrared absorption,” ACS Nano 2, 707–718 (2008).
[Crossref]

E. Prodan, C. Radloff, N. J. Halas, and P. Nordlander, “A hybridization model for the plasmon response of complex nanostructures,” Science 302, 419–422 (2003).
[Crossref] [PubMed]

Hansen, O.

Haug, F.-J.

F.-J. Haug, T. Soderstrom, O. Cubero, V. Terrazzoni-Daudrix, and C. Ballif, “Plasmonic absorption in textured silver back reflectors of thin film solar cells,” J. Appl. Phys. 104, 064509 (2008).
[Crossref]

Hermannsson, P. G.

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P. West, S. Ishii, G. Naik, N. Emani, V. Shalaev, and A. Boltasseva, “Searching for better plasmonic materials,” Laser Photonics Rev. 4, 795–808 (2010).
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M. E. Stewart, C. R. Anderton, L. B. Thompson, J. Maria, S. K. Gray, J. A. Rogers, and R. G. Nuzzo, “Nanostructured plasmonic sensors,” Chem. Rev. 108, 494–521 (2008).
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F. Le, D. W. Brandl, Y. A. Urzhumov, H. Wang, J. Kundu, N. J. Halas, J. Aizpurua, and P. Nordlander, “Metallic nanoparticle arrays: a common substrate for both surface-enhanced Raman scattering and surface-enhanced infrared absorption,” ACS Nano 2, 707–718 (2008).
[Crossref]

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G. H. Chan, J. Zhao, G. C. Schatz, and R. P. Van Duyne, “Localized surface plasmon resonance spectroscopy of triangular aluminum nanoparticles,” J. Phys. Chem. C 112, 13958–13963 (2008).
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C. Vannahme, M. Dufva, and A. Kristensen, “High frame rate multi-resonance imaging refractometry with distributed feedback dye laser sensor,” Light Sci. Appl. 4, e269 (2015).
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S. J. Tan, L. Zhang, D. Zhu, X. M. Goh, Y. M. Wang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Plasmonic color palettes for photorealistic printing with aluminum nanostructures,” Nano Lett. 14, 4023–4029 (2014).
[Crossref] [PubMed]

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E. Højlund-Nielsen, J. Weirich, J. Nørregaard, J. Garnaes, N. A. Mortensen, and A. Kristensen, “Angle-independent structural colors of silicon,” J. Nanophotonics 8, 083988 (2014).
[Crossref]

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P. West, S. Ishii, G. Naik, N. Emani, V. Shalaev, and A. Boltasseva, “Searching for better plasmonic materials,” Laser Photonics Rev. 4, 795–808 (2010).
[Crossref]

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W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
[Crossref] [PubMed]

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S. Raza, S. I. Bozhevolnyi, M. Wubs, and N. A. Mortensen, “Nonlocal optical response in metallic nanostructures,” J. Phys. Condens. Matter 27, 183204 (2015).
[Crossref] [PubMed]

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Yang, J. K. W.

X. M. Goh, Y. Zheng, S. J. Tan, L. Zhang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Three-dimensional plasmonic stereoscopic prints in full colour,” Nat. Commun. 5, 5361 (2014).
[Crossref] [PubMed]

S. J. Tan, L. Zhang, D. Zhu, X. M. Goh, Y. M. Wang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Plasmonic color palettes for photorealistic printing with aluminum nanostructures,” Nano Lett. 14, 4023–4029 (2014).
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J. S. Clausen, E. Højlund-Nielsen, A. B. Christiansen, S. Yazdi, M. Grajower, H. Taha, U. Levy, A. Kristensen, and N. A. Mortensen, “Plasmonic metasurfaces for coloration of plastic consumer products,” Nano Lett. 14, 4499–4504 (2014).
[Crossref] [PubMed]

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W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
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I. Zorić, M. Zäch, B. Kasemo, and C. Langhammer, “Gold, platinum, and aluminum nanodisk plasmons: material independence, subradiance, and damping mechanisms,” ACS Nano 5, 2535–2546 (2011).
[Crossref]

Zhang, J.

Zhang, L.

S. J. Tan, L. Zhang, D. Zhu, X. M. Goh, Y. M. Wang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Plasmonic color palettes for photorealistic printing with aluminum nanostructures,” Nano Lett. 14, 4023–4029 (2014).
[Crossref] [PubMed]

X. M. Goh, Y. Zheng, S. J. Tan, L. Zhang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Three-dimensional plasmonic stereoscopic prints in full colour,” Nat. Commun. 5, 5361 (2014).
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Zhang, M.

W. Chen, M. Tymchenko, P. Gopalan, X. Ye, Y. Wu, M. Zhang, C. B. Murray, A. Alu, and C. R. Kagan, “Large-area nanoimprinted colloidal Au nanocrystal-based nanoantennas for ultrathin polarizing plasmonic metasurfaces,” Nano Lett. 15, 5254–5260 (2015).
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G. H. Chan, J. Zhao, G. C. Schatz, and R. P. Van Duyne, “Localized surface plasmon resonance spectroscopy of triangular aluminum nanoparticles,” J. Phys. Chem. C 112, 13958–13963 (2008).
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Zheng, Y.

X. M. Goh, Y. Zheng, S. J. Tan, L. Zhang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Three-dimensional plasmonic stereoscopic prints in full colour,” Nat. Commun. 5, 5361 (2014).
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S. J. Tan, L. Zhang, D. Zhu, X. M. Goh, Y. M. Wang, K. Kumar, C.-W. Qiu, and J. K. W. Yang, “Plasmonic color palettes for photorealistic printing with aluminum nanostructures,” Nano Lett. 14, 4023–4029 (2014).
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Figures (4)

Fig. 1
Fig. 1 Hybrid transverse mode concept by elongation of base plasmonic structure. a) Energy hybridization diagrams of circular and elongated structures at transverse polarization. b–e Representative reflectance spectra for different polarizations of various structures with CIE/sRGB calculated color coding. Top dashed lines show spectrum for non-structured surface.
Fig. 2
Fig. 2 Fabrication process for 250 nm periodic structures from pattern definition to metalized polymer replica. a–e) Sketch of fabrication process, see text. f) SEM image of metalized polymer replica for 45° rotation inside unit-cell. Corresponding SEM image of Si master can be seen as inset.
Fig. 3
Fig. 3 Measured normal incidence reflectance spectra for metalized polymer samples. a) Definition of coordinate system and angles. b) Schematic illustration of optical setup. c) Reflectance as function of wavelength for different polarizations in the case of structure ”n” with CIE/sRGB calculated color coding. Top dashed line shows spectrum for non-structured surface. d) Reflectance as function of polarization angle at resonance wavelength for elongated structures ”l”, ”m”, and ”n”. e) Resonance wavelengths as function of rotation angle. f–n) Reflectance as function of wavelength and polarization angle for all nine investigated topographies. Arrows indicate transverse (450 nm) and longitudinal (630 nm) resonances.
Fig. 4
Fig. 4 Simulations. a) Reflectance spectra for structure ”n” at 40° and 130° polarization angle. b) Reflectance contour-plot for structure ”n”. c) Absolute electric field intensity for structure ”n”. d) Scale for absolute field intensity with maximum of 800 mV/nm. e) Scale for z-component of electric field for input field of 76.6 mV/nm. f–n) Plots of the electric field z-component inside the unit-cell, with inserts of the corresponding absolute field intensity for structures ”f”–”n” at the high-energy resonance for optimal polarization angle (90°, 113°, 135°) and phase. The hybrid transverse mode can be seen.

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