Abstract

In this study, non-toxic and highly stable silica coated ZnCuInS NCs were synthesized by a reverse microemulsion method. The single NCs were uniformly encapsulated in a silica shell with a diameter of ~30nm. Although hydrolyzed TEOS caused a QY reduction, and a 12.5nm red shift occurred after silica coating, the photo and thermal stabilities were extremely improved. For LED application, the silica coated ZnCuInS NCs phosphor layer was arrayed on the InGaN LED surface by layer-by-layer deposition utilizing electrostatic attraction. When the ZnCuInS/SiO2 NCs single monolayer was fabricated, 6.73% high color conversion efficiency was achieved.

© 2014 Optical Society of America

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    [CrossRef]
  25. S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
    [CrossRef]
  26. D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
    [CrossRef] [PubMed]
  27. M. Darbandi, G. Urban, M. Krüger, “Bright luminescent, colloidal stable silica coated CdSe/ZnS nanocomposite by an in situ, one-pot surface functionalization,” J. Colloid Interface Sci. 365(1), 41–45 (2012).
    [CrossRef] [PubMed]

2013 (1)

2012 (5)

M. Darbandi, G. Urban, M. Krüger, “Bright luminescent, colloidal stable silica coated CdSe/ZnS nanocomposite by an in situ, one-pot surface functionalization,” J. Colloid Interface Sci. 365(1), 41–45 (2012).
[CrossRef] [PubMed]

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

W. Song, H. Yang, “Efficient white-light-emitting diodes fabricated from highly fluorescent copper indium sulfide core/shell quantum dots,” Chem. Mater. 24(10), 1961–1967 (2012).
[CrossRef]

W. Song, H. Yang, “Fabrication of white light-emitting diodes based on solvotherrmally synthesized copper indium sulfide quantum dots as color converters,” Appl. Phys. Lett. 100(18), 183104 (2012).
[CrossRef]

W. Chung, H. Jung, C. H. Lee, S. H. Kim, “Fabrication of high color rendering index white LED using Cd-free wavelength tunable Zn doped CuInS2 nanocrystals,” Opt. Express 20(22), 25071–25076 (2012).
[CrossRef] [PubMed]

2011 (5)

J. Park, S. Kim, “CuInS2/ZnS core/shell quantum dots by cation exchange and their blue-shifted photoluminescence,” J. Mater. Chem. 21(11), 3745–3750 (2011).
[CrossRef]

J. Zhang, R. Xie, W. Yang, “A simple route for highly luminescent quaternary Cu-Zn-In-S nanocrystal emitter,” Chem. Mater. 23(14), 3357–3361 (2011).
[CrossRef]

D. Nam, W. Song, H. Yang, “Facile, air-insensitive solvothermal synthesis of emission-tunable CuInS2/ZnS quantum dots with high quantum yields,” J. Mater. Chem. 21(45), 18220–18226 (2011).
[CrossRef]

J. M. Yang, H. Yang, L. Lin, “Quantum dot nano thermometers reveal heterogeneous local thermogenesis in living cells,” ACS Nano 5(6), 5067–5071 (2011).
[CrossRef] [PubMed]

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

2010 (1)

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

2009 (1)

R. Xie, M. Rutherford, X. Peng, “Formation of high-quality I-III-VI semiconductor nanocrystals by tuning relative reactivity of cationic precursors,” J. Am. Chem. Soc. 131(15), 5691–5697 (2009).
[CrossRef] [PubMed]

2008 (2)

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

2007 (2)

S. Nizamoglu, T. Ozel, E. Sari, H. Demir, “White light generation using CdSe/ZnS core–shell nanocrystals hybridized with InGaN/GaN light emitting diodes,” Nanotechnology 18(6), 065709 (2007).
[CrossRef]

P. O. Anikeeva, J. E. Halpert, M. G. Bawendi, V. Bulović, “Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer,” Nano Lett. 7(8), 2196–2200 (2007).
[CrossRef] [PubMed]

2006 (2)

H. Chen, C. Hsu, H. Hong, “InGaN–CdSe–ZnSe quantum dots white LEDs,” IEEE Photon. Technol. Lett. 18(1), 193–195 (2006).
[CrossRef]

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

2005 (1)

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

2004 (3)

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

2002 (1)

S. Coe, W. K. Woo, M. Bawendi, V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[CrossRef] [PubMed]

2000 (1)

A. Rogach, D. Koktysh, M. Harrison, N. Kotov, “Layer-by-Layer assembled films of HgTe nanocrystals with strong infrared emission,” Chem. Mater. 12(6), 1526–1528 (2000).
[CrossRef]

1997 (2)

G. Decher, “Fuzzy nanoassemblies: toward layered polymeric multicomposites,” Science 277(5330), 1232–1237 (1997).
[CrossRef]

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Achermann, M.

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Akhavan, V.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Anikeeva, P. O.

P. O. Anikeeva, J. E. Halpert, M. G. Bawendi, V. Bulović, “Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer,” Nano Lett. 7(8), 2196–2200 (2007).
[CrossRef] [PubMed]

Ariga, K.

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Baffou, G.

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

Bailey, S.

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

Banger, K.

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

Barbara, P. F.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Bawendi, M.

S. Coe, W. K. Woo, M. Bawendi, V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[CrossRef] [PubMed]

Bawendi, M. G.

P. O. Anikeeva, J. E. Halpert, M. G. Bawendi, V. Bulović, “Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer,” Nano Lett. 7(8), 2196–2200 (2007).
[CrossRef] [PubMed]

Belcher, A.

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

Bulovic, V.

P. O. Anikeeva, J. E. Halpert, M. G. Bawendi, V. Bulović, “Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer,” Nano Lett. 7(8), 2196–2200 (2007).
[CrossRef] [PubMed]

S. Coe, W. K. Woo, M. Bawendi, V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[CrossRef] [PubMed]

Castro, S.

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

Chen, B.

Chen, H.

H. Chen, C. Hsu, H. Hong, “InGaN–CdSe–ZnSe quantum dots white LEDs,” IEEE Photon. Technol. Lett. 18(1), 193–195 (2006).
[CrossRef]

Cho, Y. H.

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

Chung, W.

Coe, S.

S. Coe, W. K. Woo, M. Bawendi, V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[CrossRef] [PubMed]

Crawford, M. H.

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

Darbandi, M.

M. Darbandi, G. Urban, M. Krüger, “Bright luminescent, colloidal stable silica coated CdSe/ZnS nanocomposite by an in situ, one-pot surface functionalization,” J. Colloid Interface Sci. 365(1), 41–45 (2012).
[CrossRef] [PubMed]

Decher, G.

G. Decher, “Fuzzy nanoassemblies: toward layered polymeric multicomposites,” Science 277(5330), 1232–1237 (1997).
[CrossRef]

Demir, H.

S. Nizamoglu, T. Ozel, E. Sari, H. Demir, “White light generation using CdSe/ZnS core–shell nanocrystals hybridized with InGaN/GaN light emitting diodes,” Nanotechnology 18(6), 065709 (2007).
[CrossRef]

Demir, H. V.

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

Dodabalapur, A.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Donner, J. S.

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

Dunn, L.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Erdem, T.

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

Eychmüller, A.

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

Gaponik, N.

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

Goodfellow, B.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Halpert, J. E.

P. O. Anikeeva, J. E. Halpert, M. G. Bawendi, V. Bulović, “Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer,” Nano Lett. 7(8), 2196–2200 (2007).
[CrossRef] [PubMed]

Harrison, M.

A. Rogach, D. Koktysh, M. Harrison, N. Kotov, “Layer-by-Layer assembled films of HgTe nanocrystals with strong infrared emission,” Chem. Mater. 12(6), 1526–1528 (2000).
[CrossRef]

Hepp, A.

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

Hong, C. H.

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

Hong, H.

H. Chen, C. Hsu, H. Hong, “InGaN–CdSe–ZnSe quantum dots white LEDs,” IEEE Photon. Technol. Lett. 18(1), 193–195 (2006).
[CrossRef]

Hsu, C.

H. Chen, C. Hsu, H. Hong, “InGaN–CdSe–ZnSe quantum dots white LEDs,” IEEE Photon. Technol. Lett. 18(1), 193–195 (2006).
[CrossRef]

Ichinose, I.

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Jaffar, S.

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

Jang, E.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Jang, H.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Jun, S.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Jung, H.

Khademhosseini, A.

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

Kim, B.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Kim, S.

J. Park, S. Kim, “CuInS2/ZnS core/shell quantum dots by cation exchange and their blue-shifted photoluminescence,” J. Mater. Chem. 21(11), 3745–3750 (2011).
[CrossRef]

Kim, S. H.

Kim, Y.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Klimov, V. I.

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Koktysh, D.

A. Rogach, D. Koktysh, M. Harrison, N. Kotov, “Layer-by-Layer assembled films of HgTe nanocrystals with strong infrared emission,” Chem. Mater. 12(6), 1526–1528 (2000).
[CrossRef]

Koleske, D. D.

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Korgel, B. A.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Kos, S.

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Kotov, N.

A. Rogach, D. Koktysh, M. Harrison, N. Kotov, “Layer-by-Layer assembled films of HgTe nanocrystals with strong infrared emission,” Chem. Mater. 12(6), 1526–1528 (2000).
[CrossRef]

Kreuzer, M. P.

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

Krüger, M.

M. Darbandi, G. Urban, M. Krüger, “Bright luminescent, colloidal stable silica coated CdSe/ZnS nanocomposite by an in situ, one-pot surface functionalization,” J. Colloid Interface Sci. 365(1), 41–45 (2012).
[CrossRef] [PubMed]

Kundaliya, D.

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

Kunitake, T.

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Langer, R.

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

Lee, C. H.

Lee, K. S.

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

Lee, S. S.

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

Li, J.

Lim, J.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Lin, L.

J. M. Yang, H. Yang, L. Lin, “Quantum dot nano thermometers reveal heterogeneous local thermogenesis in living cells,” ACS Nano 5(6), 5067–5071 (2011).
[CrossRef] [PubMed]

Liu, R.

Lvov, Y.

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Mutlugun, E.

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

Nam, D.

D. Nam, W. Song, H. Yang, “Facile, air-insensitive solvothermal synthesis of emission-tunable CuInS2/ZnS quantum dots with high quantum yields,” J. Mater. Chem. 21(45), 18220–18226 (2011).
[CrossRef]

Nam, K.

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

Nizamoglu, S.

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

S. Nizamoglu, T. Ozel, E. Sari, H. Demir, “White light generation using CdSe/ZnS core–shell nanocrystals hybridized with InGaN/GaN light emitting diodes,” Nanotechnology 18(6), 065709 (2007).
[CrossRef]

Onda, M.

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Ozel, T.

S. Nizamoglu, T. Ozel, E. Sari, H. Demir, “White light generation using CdSe/ZnS core–shell nanocrystals hybridized with InGaN/GaN light emitting diodes,” Nanotechnology 18(6), 065709 (2007).
[CrossRef]

Panthani, M. G.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Papaefthymiou, G. C.

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

Park, J.

J. Park, S. Kim, “CuInS2/ZnS core/shell quantum dots by cation exchange and their blue-shifted photoluminescence,” J. Mater. Chem. 21(11), 3745–3750 (2011).
[CrossRef]

Peng, X.

R. Xie, M. Rutherford, X. Peng, “Formation of high-quality I-III-VI semiconductor nanocrystals by tuning relative reactivity of cationic precursors,” J. Am. Chem. Soc. 131(15), 5691–5697 (2009).
[CrossRef] [PubMed]

Petruska, M. A.

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Quidant, R.

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

Raffaelle, R.

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

Rogach, A.

A. Rogach, D. Koktysh, M. Harrison, N. Kotov, “Layer-by-Layer assembled films of HgTe nanocrystals with strong infrared emission,” Chem. Mater. 12(6), 1526–1528 (2000).
[CrossRef]

Rutherford, M.

R. Xie, M. Rutherford, X. Peng, “Formation of high-quality I-III-VI semiconductor nanocrystals by tuning relative reactivity of cationic precursors,” J. Am. Chem. Soc. 131(15), 5691–5697 (2009).
[CrossRef] [PubMed]

Ryu, J. H.

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

Sari, E.

S. Nizamoglu, T. Ozel, E. Sari, H. Demir, “White light generation using CdSe/ZnS core–shell nanocrystals hybridized with InGaN/GaN light emitting diodes,” Nanotechnology 18(6), 065709 (2007).
[CrossRef]

Schmidtke, J. P.

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

Selvan, S. T.

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

Smith, D. L.

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Song, W.

W. Song, H. Yang, “Efficient white-light-emitting diodes fabricated from highly fluorescent copper indium sulfide core/shell quantum dots,” Chem. Mater. 24(10), 1961–1967 (2012).
[CrossRef]

W. Song, H. Yang, “Fabrication of white light-emitting diodes based on solvotherrmally synthesized copper indium sulfide quantum dots as color converters,” Appl. Phys. Lett. 100(18), 183104 (2012).
[CrossRef]

D. Nam, W. Song, H. Yang, “Facile, air-insensitive solvothermal synthesis of emission-tunable CuInS2/ZnS quantum dots with high quantum yields,” J. Mater. Chem. 21(45), 18220–18226 (2011).
[CrossRef]

Thompson, S. A.

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

Urban, G.

M. Darbandi, G. Urban, M. Krüger, “Bright luminescent, colloidal stable silica coated CdSe/ZnS nanocomposite by an in situ, one-pot surface functionalization,” J. Colloid Interface Sci. 365(1), 41–45 (2012).
[CrossRef] [PubMed]

Wang, H.

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

Woo, W. K.

S. Coe, W. K. Woo, M. Bawendi, V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[CrossRef] [PubMed]

Xie, R.

J. Zhang, R. Xie, W. Yang, “A simple route for highly luminescent quaternary Cu-Zn-In-S nanocrystal emitter,” Chem. Mater. 23(14), 3357–3361 (2011).
[CrossRef]

R. Xie, M. Rutherford, X. Peng, “Formation of high-quality I-III-VI semiconductor nanocrystals by tuning relative reactivity of cationic precursors,” J. Am. Chem. Soc. 131(15), 5691–5697 (2009).
[CrossRef] [PubMed]

Xing, J.

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

Yang, H.

W. Song, H. Yang, “Fabrication of white light-emitting diodes based on solvotherrmally synthesized copper indium sulfide quantum dots as color converters,” Appl. Phys. Lett. 100(18), 183104 (2012).
[CrossRef]

W. Song, H. Yang, “Efficient white-light-emitting diodes fabricated from highly fluorescent copper indium sulfide core/shell quantum dots,” Chem. Mater. 24(10), 1961–1967 (2012).
[CrossRef]

D. Nam, W. Song, H. Yang, “Facile, air-insensitive solvothermal synthesis of emission-tunable CuInS2/ZnS quantum dots with high quantum yields,” J. Mater. Chem. 21(45), 18220–18226 (2011).
[CrossRef]

J. M. Yang, H. Yang, L. Lin, “Quantum dot nano thermometers reveal heterogeneous local thermogenesis in living cells,” ACS Nano 5(6), 5067–5071 (2011).
[CrossRef] [PubMed]

Yang, J. M.

J. M. Yang, H. Yang, L. Lin, “Quantum dot nano thermometers reveal heterogeneous local thermogenesis in living cells,” ACS Nano 5(6), 5067–5071 (2011).
[CrossRef] [PubMed]

Yang, W.

J. Zhang, R. Xie, W. Yang, “A simple route for highly luminescent quaternary Cu-Zn-In-S nanocrystal emitter,” Chem. Mater. 23(14), 3357–3361 (2011).
[CrossRef]

Yi, D. K.

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

Ying, J. Y.

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

Zhang, F.

Zhang, J.

J. Zhang, R. Xie, W. Yang, “A simple route for highly luminescent quaternary Cu-Zn-In-S nanocrystal emitter,” Chem. Mater. 23(14), 3357–3361 (2011).
[CrossRef]

Zhong, H.

Zhou, Q.

Zou, B.

ACS Nano (1)

J. M. Yang, H. Yang, L. Lin, “Quantum dot nano thermometers reveal heterogeneous local thermogenesis in living cells,” ACS Nano 5(6), 5067–5071 (2011).
[CrossRef] [PubMed]

Adv. Mater. (1)

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Appl. Phys. Lett. (1)

W. Song, H. Yang, “Fabrication of white light-emitting diodes based on solvotherrmally synthesized copper indium sulfide quantum dots as color converters,” Appl. Phys. Lett. 100(18), 183104 (2012).
[CrossRef]

Chem. Mater. (3)

J. Zhang, R. Xie, W. Yang, “A simple route for highly luminescent quaternary Cu-Zn-In-S nanocrystal emitter,” Chem. Mater. 23(14), 3357–3361 (2011).
[CrossRef]

W. Song, H. Yang, “Efficient white-light-emitting diodes fabricated from highly fluorescent copper indium sulfide core/shell quantum dots,” Chem. Mater. 24(10), 1961–1967 (2012).
[CrossRef]

A. Rogach, D. Koktysh, M. Harrison, N. Kotov, “Layer-by-Layer assembled films of HgTe nanocrystals with strong infrared emission,” Chem. Mater. 12(6), 1526–1528 (2000).
[CrossRef]

IEEE Photon. Technol. Lett. (1)

H. Chen, C. Hsu, H. Hong, “InGaN–CdSe–ZnSe quantum dots white LEDs,” IEEE Photon. Technol. Lett. 18(1), 193–195 (2006).
[CrossRef]

J. Am. Chem. Soc. (3)

R. Xie, M. Rutherford, X. Peng, “Formation of high-quality I-III-VI semiconductor nanocrystals by tuning relative reactivity of cationic precursors,” J. Am. Chem. Soc. 131(15), 5691–5697 (2009).
[CrossRef] [PubMed]

M. G. Panthani, V. Akhavan, B. Goodfellow, J. P. Schmidtke, L. Dunn, A. Dodabalapur, P. F. Barbara, B. A. Korgel, “Synthesis of CulnS2, CulnSe2, and Cu(InxGa1-x)Se2 (CIGS) nanocrystal “Inks” for printable photovoltaics,” J. Am. Chem. Soc. 130(49), 16770–16777 (2008).
[CrossRef] [PubMed]

D. K. Yi, S. T. Selvan, S. S. Lee, G. C. Papaefthymiou, D. Kundaliya, J. Y. Ying, “Silica-coated nanocomposites of magnetic nanoparticles and quantum dots,” J. Am. Chem. Soc. 127(14), 4990–4991 (2005).
[CrossRef] [PubMed]

J. Colloid Interface Sci. (1)

M. Darbandi, G. Urban, M. Krüger, “Bright luminescent, colloidal stable silica coated CdSe/ZnS nanocomposite by an in situ, one-pot surface functionalization,” J. Colloid Interface Sci. 365(1), 41–45 (2012).
[CrossRef] [PubMed]

J. Mater. Chem. (2)

J. Park, S. Kim, “CuInS2/ZnS core/shell quantum dots by cation exchange and their blue-shifted photoluminescence,” J. Mater. Chem. 21(11), 3745–3750 (2011).
[CrossRef]

D. Nam, W. Song, H. Yang, “Facile, air-insensitive solvothermal synthesis of emission-tunable CuInS2/ZnS quantum dots with high quantum yields,” J. Mater. Chem. 21(45), 18220–18226 (2011).
[CrossRef]

J. Phys. Chem. B (1)

S. Castro, S. Bailey, R. Raffaelle, K. Banger, A. Hepp, “Synthesis and characterization of colloidal CuInS2 nanoparticles from a molecular single-source precursor,” J. Phys. Chem. B 108(33), 12429–12435 (2004).
[CrossRef]

Langmuir (1)

Y. Lvov, K. Ariga, M. Onda, I. Ichinose, T. Kunitake, “Alternate assembly of ordered multilayers of SiO2 and other nanoparticles and polyions,” Langmuir 13(23), 6195–6203 (1997).
[CrossRef]

Nano Lett. (4)

M. Achermann, M. A. Petruska, D. D. Koleske, M. H. Crawford, V. I. Klimov, “Nanocrystal-based light-emitting diodes utilizing high-efficiency nonradiative energy transfer for color conversion,” Nano Lett. 6(7), 1396–1400 (2006).
[CrossRef] [PubMed]

S. Jaffar, K. Nam, A. Khademhosseini, J. Xing, R. Langer, A. Belcher, “Layer-by-Layer surface modification and patterned electrostatic deposition of quantum dots,” Nano Lett. 4(8), 1421–1425 (2004).
[CrossRef]

P. O. Anikeeva, J. E. Halpert, M. G. Bawendi, V. Bulović, “Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer,” Nano Lett. 7(8), 2196–2200 (2007).
[CrossRef] [PubMed]

J. S. Donner, S. A. Thompson, M. P. Kreuzer, G. Baffou, R. Quidant, “Mapping intracellular temperature using green fluorescent protein,” Nano Lett. 12(4), 2107–2111 (2012).
[CrossRef] [PubMed]

Nano Today (1)

H. V. Demir, S. Nizamoglu, T. Erdem, E. Mutlugun, N. Gaponik, A. Eychmüller, “Quantum dot integrated LEDs using photonic and excitonic color conversion,” Nano Today 6(6), 632–647 (2011).
[CrossRef]

Nanotechnology (2)

S. Nizamoglu, T. Ozel, E. Sari, H. Demir, “White light generation using CdSe/ZnS core–shell nanocrystals hybridized with InGaN/GaN light emitting diodes,” Nanotechnology 18(6), 065709 (2007).
[CrossRef]

H. Wang, K. S. Lee, J. H. Ryu, C. H. Hong, Y. H. Cho, “White light emitting diodes realized by using an active packaging method with CdSe/ZnS quantum dots dispersed in photosensitive epoxy resins,” Nanotechnology 19(14), 145202 (2008).
[CrossRef] [PubMed]

Nature (2)

S. Coe, W. K. Woo, M. Bawendi, V. Bulović, “Electroluminescence from single monolayers of nanocrystals in molecular organic devices,” Nature 420(6917), 800–803 (2002).
[CrossRef] [PubMed]

M. Achermann, M. A. Petruska, S. Kos, D. L. Smith, D. D. Koleske, V. I. Klimov, “Energy-transfer pumping of semiconductor nanocrystals using an epitaxial quantum well,” Nature 429(6992), 642–646 (2004).
[CrossRef] [PubMed]

Opt. Express (2)

Science (1)

G. Decher, “Fuzzy nanoassemblies: toward layered polymeric multicomposites,” Science 277(5330), 1232–1237 (1997).
[CrossRef]

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Figures (5)

Fig. 1
Fig. 1

The HR-TEM image of (a) ZnCuInS NCs, and (b) silica coated ZnCuInS NCs. (c) The X-ray diffraction of ZnCuInS NCs, and silica coated ZnCuInS NCs.

Fig. 2
Fig. 2

(a) The absorption, and (b) emission spectra of ZnCuInS NCs and ZnCuInS/SiO2 NCs.

Fig. 3
Fig. 3

(a) Photo-stability, and (b) thermal-stability of ZnCuInS NCs and ZnCuInS/SiO2 NCs.

Fig. 4
Fig. 4

FE-SEM image of ZnCuInS/SiO2 NCs monolayer with different NaCl concentration. (a) 0M NaCl; (b) 0.1M NaCl; (c) 1M NaCl.

Fig. 5
Fig. 5

The emission spectrum of fabricated color conversion LEDs. 430nm InGaN LED pumped with ZnCuInS/SiO2 NCs monolayer phosphor.

Equations (1)

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Q Y = Q Y s t 1 10 A s t 1 10 A × η 2 η 2 s t × I I s t

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