Abstract

We present a numerical parametric study of single-cycle electromagnetic pulse generation in a DAST/SiO2 multilayer structure via collinear optical rectification of 800 nm femtosecond laser pulses. It is shown that modifications of the thicknesses of the DAST and SiO2 layers allow tuning of the average frequency of the generated THz pulses in the frequency range from 3 to 6 THz. The laser-to-THz energy conversion efficiency in the proposed structures is compared with that in a bulk DAST crystal and a quasi-phase-matching periodically poled DAST crystal and shows significant enhancement.

© 2014 Optical Society of America

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  3. C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
    [Crossref]
  4. N. Stojanovic and M. Drescher, “Accelerator- and laser-based sources of high-field terahertz pulses,” J. Phys. At. Mol. Opt. Phys. 46(19), 192001 (2013).
    [Crossref]
  5. E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
    [Crossref]
  6. A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
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    [Crossref]
  9. C. Vicario, B. Monoszlai, Cs. Lombosi, A. Mareczko, A. Courjaud, J. A. Fülöp, and C. P. Hauri, “Pump pulse width and temperature effects in lithium niobate for efficient THz generation,” Opt. Lett. 38(24), 5373–5376 (2013).
    [Crossref] [PubMed]
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    [Crossref] [PubMed]
  11. K. Y. Kim, J. H. Glownia, A. J. Taylor, and G. Rodriguez, “High-power broadband terahertz generation via two-color photoionization in gases,” IEEE J. Quantum Electron. 48(6), 797–805 (2012).
    [Crossref]
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    [Crossref]
  13. C. Ruchert, C. Vicario, and C. P. Hauri, “Scaling submillimeter single-cycle transients toward megavolts per centimeter field strength via optical rectification in the organic crystal OH1,” Opt. Lett. 37(5), 899–901 (2012).
    [Crossref] [PubMed]
  14. C. Ruchert, C. Vicario, and C. P. Hauri, “Spatiotemporal focusing dynamics of intense supercontinuum THz pulses,” Phys. Rev. Lett. 110(12), 123902 (2013).
    [Crossref] [PubMed]
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    [Crossref]
  16. C. Vicario, B. Monoszlai, and C. P. Hauri, “GV/m single-cycle terahertz fields from a laser-driven large-size partitioned organic crystal,” Phys. Rev. Lett. 112(21), 213901 (2014).
    [Crossref]
  17. B. Monoszlai, C. Vicario, M. Jazbinsek, and C. P. Hauri, “High-energy terahertz pulses from organic crystals: DAST and DSTMS pumped at Ti:sapphire wavelength,” Opt. Lett. 38(23), 5106–5109 (2013).
    [Crossref] [PubMed]
  18. A. G. Stepanov, L. Bonacina, and J.-P. Wolf, “DAST/SiO2 multilayer structure for efficient generation of 6 THz quasi-single-cycle electromagnetic pulses,” Opt. Lett. 37(13), 2439–2441 (2012).
    [Crossref] [PubMed]
  19. J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
    [Crossref]
  20. Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
    [Crossref]
  21. F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
    [Crossref]
  22. P. D. Cunningham and L. M. Hayden, “Optical properties of DAST in the THz range,” Opt. Express 18(23), 23620–23625 (2010).
    [Crossref] [PubMed]
  23. G. Ghosh, “Dispersion-equation coefficients for the refractive index and birefringence of calcite and quartz crystals,” Opt. Commun. 163(1–3), 95–102 (1999).
    [Crossref]
  24. E. E. Russel and E. E. Bell, “Measurement of the optical constants of crystal quartz in the far infrared with the asymmetric Fourier-transform method,” JOSA 57(3), 341–348 (1967).
    [Crossref]
  25. M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
    [Crossref]
  26. S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
    [Crossref]

2014 (1)

C. Vicario, B. Monoszlai, and C. P. Hauri, “GV/m single-cycle terahertz fields from a laser-driven large-size partitioned organic crystal,” Phys. Rev. Lett. 112(21), 213901 (2014).
[Crossref]

2013 (8)

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

N. Stojanovic and M. Drescher, “Accelerator- and laser-based sources of high-field terahertz pulses,” J. Phys. At. Mol. Opt. Phys. 46(19), 192001 (2013).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Spatiotemporal focusing dynamics of intense supercontinuum THz pulses,” Phys. Rev. Lett. 110(12), 123902 (2013).
[Crossref] [PubMed]

C. Vicario, C. Ruchert, and C. P. Hauri, “High field broadband THz generation in organic materials,” J. Mod. Opt. 2013, 1–6 (2013).
[Crossref]

S.-W. Huang, E. Granados, W. R. Huang, K.-H. Hong, L. E. Zapata, and F. X. Kärtner, “High conversion efficiency, high energy terahertz pulses by optical rectification in cryogenically cooled lithium niobate,” Opt. Lett. 38(5), 796–798 (2013).
[Crossref] [PubMed]

B. Monoszlai, C. Vicario, M. Jazbinsek, and C. P. Hauri, “High-energy terahertz pulses from organic crystals: DAST and DSTMS pumped at Ti:sapphire wavelength,” Opt. Lett. 38(23), 5106–5109 (2013).
[Crossref] [PubMed]

C. Vicario, B. Monoszlai, Cs. Lombosi, A. Mareczko, A. Courjaud, J. A. Fülöp, and C. P. Hauri, “Pump pulse width and temperature effects in lithium niobate for efficient THz generation,” Opt. Lett. 38(24), 5373–5376 (2013).
[Crossref] [PubMed]

2012 (3)

2011 (1)

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

2010 (3)

2006 (1)

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

2004 (1)

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

2000 (1)

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

1999 (2)

G. Ghosh, “Dispersion-equation coefficients for the refractive index and birefringence of calcite and quartz crystals,” Opt. Commun. 163(1–3), 95–102 (1999).
[Crossref]

M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
[Crossref]

1996 (1)

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

1967 (1)

E. E. Russel and E. E. Bell, “Measurement of the optical constants of crystal quartz in the far infrared with the asymmetric Fourier-transform method,” JOSA 57(3), 341–348 (1967).
[Crossref]

1962 (1)

J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
[Crossref]

Almasi, G.

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

Araki, T.

Ardana, F.

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

Ardana-Lamas, F.

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

Armstrong, J. A.

J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
[Crossref]

Averitt, R. D.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Bartal, B.

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

Bell, E. E.

E. E. Russel and E. E. Bell, “Measurement of the optical constants of crystal quartz in the far infrared with the asymmetric Fourier-transform method,” JOSA 57(3), 341–348 (1967).
[Crossref]

Bhowmik, A.

M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
[Crossref]

Bloembergen, N.

J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
[Crossref]

Bonacina, L.

A. G. Stepanov, L. Bonacina, and J.-P. Wolf, “DAST/SiO2 multilayer structure for efficient generation of 6 THz quasi-single-cycle electromagnetic pulses,” Opt. Lett. 37(13), 2439–2441 (2012).
[Crossref] [PubMed]

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

Bosshard, C.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Brahadeeswaran, S.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Brandt, N. C.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Courjaud, A.

Cunningham, P. D.

Derlet, P. M.

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

Drescher, M.

N. Stojanovic and M. Drescher, “Accelerator- and laser-based sources of high-field terahertz pulses,” J. Phys. At. Mol. Opt. Phys. 46(19), 192001 (2013).
[Crossref]

Ducuing, J.

J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
[Crossref]

Fan, K.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Fleischer, S.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Follonier, S.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Fujio, M.

Fülöp, J. A.

Galvanauskas, A.

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

Ghosh, G.

G. Ghosh, “Dispersion-equation coefficients for the refractive index and birefringence of calcite and quartz crystals,” Opt. Commun. 163(1–3), 95–102 (1999).
[Crossref]

Glownia, J. H.

K. Y. Kim, J. H. Glownia, A. J. Taylor, and G. Rodriguez, “High-power broadband terahertz generation via two-color photoionization in gases,” IEEE J. Quantum Electron. 48(6), 797–805 (2012).
[Crossref]

Granados, E.

Günter, P.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Hangyo, M.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Hauri, C. P.

C. Vicario, B. Monoszlai, and C. P. Hauri, “GV/m single-cycle terahertz fields from a laser-driven large-size partitioned organic crystal,” Phys. Rev. Lett. 112(21), 213901 (2014).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Spatiotemporal focusing dynamics of intense supercontinuum THz pulses,” Phys. Rev. Lett. 110(12), 123902 (2013).
[Crossref] [PubMed]

C. Vicario, C. Ruchert, and C. P. Hauri, “High field broadband THz generation in organic materials,” J. Mod. Opt. 2013, 1–6 (2013).
[Crossref]

C. Vicario, B. Monoszlai, Cs. Lombosi, A. Mareczko, A. Courjaud, J. A. Fülöp, and C. P. Hauri, “Pump pulse width and temperature effects in lithium niobate for efficient THz generation,” Opt. Lett. 38(24), 5373–5376 (2013).
[Crossref] [PubMed]

B. Monoszlai, C. Vicario, M. Jazbinsek, and C. P. Hauri, “High-energy terahertz pulses from organic crystals: DAST and DSTMS pumped at Ti:sapphire wavelength,” Opt. Lett. 38(23), 5106–5109 (2013).
[Crossref] [PubMed]

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Scaling submillimeter single-cycle transients toward megavolts per centimeter field strength via optical rectification in the organic crystal OH1,” Opt. Lett. 37(5), 899–901 (2012).
[Crossref] [PubMed]

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

Hayden, L. M.

Hebling, J.

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

Henin, S.

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

Hong, K.-H.

Huang, S.-W.

Huang, W. R.

Hwang, H. Y.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Ito, H.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Jazbinsek, M.

Kärtner, F. X.

Kasparian, J.

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

Kim, K. Y.

K. Y. Kim, J. H. Glownia, A. J. Taylor, and G. Rodriguez, “High-power broadband terahertz generation via two-color photoionization in gases,” IEEE J. Quantum Electron. 48(6), 797–805 (2012).
[Crossref]

Knöpfle, G.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Kuhl, J.

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

Lee, Y.-S.

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

Liu, M.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Lombosi, Cs.

Luning, J.

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

Mareczko, A.

Meade, T.

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

Minami, M.

Miura, J.

Monoszlai, B.

Mori, Y.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Nashima, S.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Nelson, K. A.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Norris, T. B.

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

Okada, S.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Pan, F.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Perkins, B. G.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Perlin, V.

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

Pershan, P. S.

J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
[Crossref]

Petit, Y.

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

Rodriguez, G.

K. Y. Kim, J. H. Glownia, A. J. Taylor, and G. Rodriguez, “High-power broadband terahertz generation via two-color photoionization in gases,” IEEE J. Quantum Electron. 48(6), 797–805 (2012).
[Crossref]

Roman, E.

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

Ruchert, C.

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

C. Vicario, C. Ruchert, and C. P. Hauri, “High field broadband THz generation in organic materials,” J. Mod. Opt. 2013, 1–6 (2013).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Spatiotemporal focusing dynamics of intense supercontinuum THz pulses,” Phys. Rev. Lett. 110(12), 123902 (2013).
[Crossref] [PubMed]

C. Ruchert, C. Vicario, and C. P. Hauri, “Scaling submillimeter single-cycle transients toward megavolts per centimeter field strength via optical rectification in the organic crystal OH1,” Opt. Lett. 37(5), 899–901 (2012).
[Crossref] [PubMed]

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

Russel, E. E.

E. E. Russel and E. E. Bell, “Measurement of the optical constants of crystal quartz in the far infrared with the asymmetric Fourier-transform method,” JOSA 57(3), 341–348 (1967).
[Crossref]

Sasaki, T.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Schirmer, M.

Souza, I.

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

Spreiter, R.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Stepanov, A. G.

A. G. Stepanov, L. Bonacina, and J.-P. Wolf, “DAST/SiO2 multilayer structure for efficient generation of 6 THz quasi-single-cycle electromagnetic pulses,” Opt. Lett. 37(13), 2439–2441 (2012).
[Crossref] [PubMed]

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

Sternbach, A.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Stojanovic, N.

N. Stojanovic and M. Drescher, “Accelerator- and laser-based sources of high-field terahertz pulses,” J. Phys. At. Mol. Opt. Phys. 46(19), 192001 (2013).
[Crossref]

Takahashi, Y.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Tani, M.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Taylor, A. J.

K. Y. Kim, J. H. Glownia, A. J. Taylor, and G. Rodriguez, “High-power broadband terahertz generation via two-color photoionization in gases,” IEEE J. Quantum Electron. 48(6), 797–805 (2012).
[Crossref]

Thakur, M.

M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
[Crossref]

Tudu, B.

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

Vanderbilt, D.

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

Veithen, M.

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

Vicario, C.

C. Vicario, B. Monoszlai, and C. P. Hauri, “GV/m single-cycle terahertz fields from a laser-driven large-size partitioned organic crystal,” Phys. Rev. Lett. 112(21), 213901 (2014).
[Crossref]

C. Vicario, C. Ruchert, and C. P. Hauri, “High field broadband THz generation in organic materials,” J. Mod. Opt. 2013, 1–6 (2013).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Spatiotemporal focusing dynamics of intense supercontinuum THz pulses,” Phys. Rev. Lett. 110(12), 123902 (2013).
[Crossref] [PubMed]

B. Monoszlai, C. Vicario, M. Jazbinsek, and C. P. Hauri, “High-energy terahertz pulses from organic crystals: DAST and DSTMS pumped at Ti:sapphire wavelength,” Opt. Lett. 38(23), 5106–5109 (2013).
[Crossref] [PubMed]

C. Vicario, B. Monoszlai, Cs. Lombosi, A. Mareczko, A. Courjaud, J. A. Fülöp, and C. P. Hauri, “Pump pulse width and temperature effects in lithium niobate for efficient THz generation,” Opt. Lett. 38(24), 5373–5376 (2013).
[Crossref] [PubMed]

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Scaling submillimeter single-cycle transients toward megavolts per centimeter field strength via optical rectification in the organic crystal OH1,” Opt. Lett. 37(5), 899–901 (2012).
[Crossref] [PubMed]

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

Winful, H.

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

Wolf, J.-P.

A. G. Stepanov, L. Bonacina, and J.-P. Wolf, “DAST/SiO2 multilayer structure for efficient generation of 6 THz quasi-single-cycle electromagnetic pulses,” Opt. Lett. 37(13), 2439–2441 (2012).
[Crossref] [PubMed]

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

Wong, M. S.

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

Xu, J.

M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
[Crossref]

Yasui, T.

Yates, J. R.

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

Yoshimura, M.

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

Zapata, L. E.

Zhang, X.

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

Zhou, L.

M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
[Crossref]

Appl. Phys. B (2)

A. G. Stepanov, S. Henin, Y. Petit, L. Bonacina, J. Kasparian, and J.-P. Wolf, “Mobile source of high-energy single-cycle terahertz pulses,” Appl. Phys. B 101(1–2), 11–14 (2010).
[Crossref]

J. Hebling, A. G. Stepanov, G. Almasi, B. Bartal, and J. Kuhl, “Tunable THz pulse generation by optical rectification of ultrashort laser pulses with tilted pulse fronts,” Appl. Phys. B 78(5), 593–599 (2004).
[Crossref]

Appl. Phys. Lett. (4)

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

Y.-S. Lee, T. Meade, V. Perlin, H. Winful, T. B. Norris, and A. Galvanauskas, “Generation of narrow-band terahertz radiation via optical rectification of femtosecond pulses in periodically poled lithium niobate,” Appl. Phys. Lett. 76(18), 2505–2507 (2000).
[Crossref]

F. Pan, G. Knöpfle, C. Bosshard, S. Follonier, R. Spreiter, M. S. Wong, and P. Günter, “Electro-optic properties of the organic salt 4-N,N-dimethylamino-4-N-methylstilbazolium tosylate,” Appl. Phys. Lett. 69(1), 13–15 (1996).
[Crossref]

M. Thakur, J. Xu, A. Bhowmik, and L. Zhou, “Single-pass thin-film electro-optic modulator based on an organic molecular salt,” Appl. Phys. Lett. 74(5), 635–637 (1999).
[Crossref]

Biomed. Opt. Express (1)

Cryst. Growth Des. (1)

S. Brahadeeswaran, Y. Takahashi, M. Yoshimura, M. Tani, S. Okada, S. Nashima, Y. Mori, M. Hangyo, H. Ito, and T. Sasaki, “Growth of ultrathin and highly efficient organic nonlinear optical crystal 4′-dimethylamino-N-methyl-4-stilbazolium p-chlorobenzenesulfonate for enhanced terahertz efficiency at higher frequencies,” Cryst. Growth Des. 13(2), 415–421 (2013).
[Crossref]

IEEE J. Quantum Electron. (1)

K. Y. Kim, J. H. Glownia, A. J. Taylor, and G. Rodriguez, “High-power broadband terahertz generation via two-color photoionization in gases,” IEEE J. Quantum Electron. 48(6), 797–805 (2012).
[Crossref]

J. Mod. Opt. (1)

C. Vicario, C. Ruchert, and C. P. Hauri, “High field broadband THz generation in organic materials,” J. Mod. Opt. 2013, 1–6 (2013).
[Crossref]

J. Phys. At. Mol. Opt. Phys. (1)

N. Stojanovic and M. Drescher, “Accelerator- and laser-based sources of high-field terahertz pulses,” J. Phys. At. Mol. Opt. Phys. 46(19), 192001 (2013).
[Crossref]

JOSA (1)

E. E. Russel and E. E. Bell, “Measurement of the optical constants of crystal quartz in the far infrared with the asymmetric Fourier-transform method,” JOSA 57(3), 341–348 (1967).
[Crossref]

Nat. Photonics (1)

C. Vicario, C. Ruchert, F. Ardana-Lamas, P. M. Derlet, B. Tudu, J. Luning, and C. P. Hauri, “Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient,” Nat. Photonics 7(9), 720–723 (2013).
[Crossref]

Opt. Commun. (1)

G. Ghosh, “Dispersion-equation coefficients for the refractive index and birefringence of calcite and quartz crystals,” Opt. Commun. 163(1–3), 95–102 (1999).
[Crossref]

Opt. Express (1)

Opt. Lett. (5)

Phys. Rev. (1)

J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, “Interactions between light waves in a nonlinear dielectric,” Phys. Rev. 127(6), 1918–1939 (1962).
[Crossref]

Phys. Rev. B (1)

E. Roman, J. R. Yates, M. Veithen, D. Vanderbilt, and I. Souza, “Ab initio study of the nonlinear optics of III-V semiconductors in the terahertz regime,” Phys. Rev. B 74(24), 245204 (2006).
[Crossref]

Phys. Rev. Lett. (2)

C. Vicario, B. Monoszlai, and C. P. Hauri, “GV/m single-cycle terahertz fields from a laser-driven large-size partitioned organic crystal,” Phys. Rev. Lett. 112(21), 213901 (2014).
[Crossref]

C. Ruchert, C. Vicario, and C. P. Hauri, “Spatiotemporal focusing dynamics of intense supercontinuum THz pulses,” Phys. Rev. Lett. 110(12), 123902 (2013).
[Crossref] [PubMed]

Other (2)

H. Y. Hwang, S. Fleischer, N. C. Brandt, B. G. Perkins, M. Liu, K. Fan, A. Sternbach, X. Zhang, R. D. Averitt, and K. A. Nelson, “A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses,” J. Mod. Opt., doi:.
[Crossref]

J. A. Fülöp and J. Hebling, Applications of Tilted-Pulse-Front Excitation; in Recent Optical and Photonic Technologies, edited by K. Y. Kim (NTECH, 2010).

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Figures (4)

Fig. 1
Fig. 1

THz generation via collinear optical rectification of 800 nm femtosecond laser pulses in studied samples: bulk DAST crystal (thickness ~100 μm) (a), multilayer DAST/SiO2 structure (b), quasi-phase-matching periodically poled DAST crystal (c), see Table1. for details.

Fig. 2
Fig. 2

Temporal profiles of THz pulses calculated for three different DAST/SiO2 multilayer structures (curves i, ii, and iii; see text for details) and for a quasi-phase-matching periodically poled DAST crystal (curve iv).

Fig. 3
Fig. 3

FFT spectra of THz pulses calculated for three different DAST/SiO2 multilayer structures (i, ii, and iii; see text for details) and for a quasi-phase-matching periodically poled DAST crystal (iv).

Fig. 4
Fig. 4

Laser-to-THz energy conversion efficiency as a function of laser pulse propagation distance calculated for three different DAST/SiO2 multilayer structures (traces i, ii, and iii), a quasi-phase-matching periodically poled DAST crystal (trace iv), and a bulk DAST crystal (trace v) pumped with the output of a Ti:sapphire laser (0.8 μm).

Tables (1)

Tables Icon

Table1 Parameters of the investigated multilayer DAST/SiO2 structures (i-iii) and the quasi-phase-matching periodically poled DAST crystal (iv).

Equations (1)

Equations on this page are rendered with MathJax. Learn more.

z E(z, ω THz )=  α( ω THz ) 2 E(z, ω THz )+ i 2 ω THz d eff n( ω THz )c ω L2 ω L1 E( ω L + ω THz ) E * ( ω L ) e iΔkz d ω L

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