Abstract

We fabricate a saturable absorber mirror by coating a graphene- film on an output coupler mirror. This is then used to obtain Q-switched mode-locking from a diode-pumped linear cavity channel waveguide laser inscribed in Ytterbium-doped Bismuthate Glass. The laser produces 1.06 ps pulses at ~1039 nm, with a 1.5 GHz repetition rate, 48% slope efficiency and 202 mW average output power. This performance is due to the combination of the graphene saturable absorber and the high quality optical waveguides in the laser glass.

© 2013 OSA

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2013 (1)

A. A. Lagatsky, Z. Sun, T. S. Kulmala, R. S. Sundaram, S. Milana, F. Torrisi, O. L. Antipov, Y. Lee, J. H. Ahn, C. T. A. Brown, W. Sibbett, and A. C. Ferrari, “2μm Solid-State Laser Mode-locked By Single-Layer Graphene,” Appl. Phys. Lett.102(1), 013113 (2013).
[CrossRef]

2012 (8)

F. Bonaccorso, A. Lombardo, T. Hasan, Z. Sun, L. Colombo, and A. C. Ferrari, “Production and processing of graphene and 2d crystals,” Mater. Today15(12), 564–589 (2012).
[CrossRef]

D. Popa, Z. Sun, T. Hasan, W. B. Cho, F. Wang, F. Torrisi, and A. C. Ferrari, “74-fs nanotube-mode-locked fiber laser,” Appl. Phys. Lett.101(15), 153107 (2012).
[CrossRef]

Z. Sun, T. Hasan, and A. C. Ferrari, “Ultrafast lasers mode-locked by nanotubes and graphene,” Physica E44(6), 1082–1091 (2012).
[CrossRef]

M. Zhang, E. J. R. Kelleher, F. Torrisi, Z. Sun, T. Hasan, D. Popa, F. Wang, A. C. Ferrari, S. V. Popov, and J. R. Taylor, “Tm-doped fiber laser mode-locked by graphene-polymer composite,” Opt. Express20(22), 25077–25084 (2012).
[CrossRef] [PubMed]

J. Ma, G. Q. Xie, P. Lv, W. L. Gao, P. Yuan, L. J. Qian, H. H. Yu, H. J. Zhang, J. Y. Wang, and D. Y. Tang, “Graphene mode-locked femtosecond laser at 2 μm wavelength,” Opt. Lett.37(11), 2085–2087 (2012).
[CrossRef] [PubMed]

A. Choudhary, A. A. Lagatsky, P. Kannan, W. Sibbett, C. T. A. Brown, and D. P. Shepherd, “Diode-pumped femtosecond solid-state waveguide laser with a 4.9 GHz pulse repetition rate,” Opt. Lett.37(21), 4416–4418 (2012).
[CrossRef] [PubMed]

J. Liu, Y. G. Wang, Z. S. Qu, L. H. Zheng, L. B. Su, and J. Xu, “Graphene oxide absorber for 2 µm passive mode-locking Tm:YAlO3 laser,” Laser Phys. Lett.9(1), 15–19 (2012).
[CrossRef]

R. Mary, S. J. Beecher, G. Brown, R. R. Thomson, D. Jaque, S. Ohara, and A. K. Kar, “Compact, highly efficient ytterbium doped bismuthate glass waveguide laser,” Opt. Lett.37(10), 1691–1693 (2012).
[CrossRef] [PubMed]

2011 (4)

W. B. Cho, J. W. Kim, H. W. Lee, S. Bae, B. H. Hong, S. Y. Choi, I. H. Baek, K. Kim, D.-I. Yeom, and F. Rotermund, “High-quality, large-area monolayer graphene for efficient bulk laser mode-locking near 1.25 μm,” Opt. Lett.36(20), 4089–4091 (2011).
[CrossRef] [PubMed]

A. Martinez, K. Fuse, and S. Yamashita, “Mechanical exfoliation of graphene for the passive mode-locking of fiber lasers,” Appl. Phys. Lett.99(12), 121107 (2011).
[CrossRef]

M. P. Moreno and S. S. Vianna, “Femtosecond 1 GHz Ti:sapphire laser as a tool for coherent spectroscopy in atomic vapor,” J. Opt. Soc. Am. B28(9), 2066–2069 (2011).
[CrossRef]

D. Popa, Z. Sun, T. Hasan, F. Torrisi, F. Wang, and A. C. Ferrari, “Graphene Q-switched, tunable fiber laser,” Appl. Phys. Lett.98(7), 073106 (2011).
[CrossRef]

2010 (10)

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, “Graphene photonics and optoelectronics,” Nat. Photonics4(9), 611–622 (2010).
[CrossRef]

L. M. Zhao, D. Y. Tang, H. Zhang, X. Wu, Q. Bao, and K. P. Loh, “Dissipative soliton operation of an ytterbium-doped fiber laser mode locked with atomic multilayer graphene,” Opt. Lett.35(21), 3622–3624 (2010).
[CrossRef] [PubMed]

D. Popa, Z. Sun, F. Torrisi, T. Hasan, F. Wang, and A. C. Ferrari, “Sub 200 fs pulse generation from a graphene mode-locked fiber laser,” Appl. Phys. Lett.97(20), 203106 (2010).
[CrossRef]

Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
[CrossRef] [PubMed]

Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
[CrossRef]

S. J. Beecher, R. R. Thomson, N. D. Psaila, Z. Sun, T. Hasan, A. G. Rozhin, A. C. Ferrari, and A. K. Kar, “320 fs pulse generation from an ultrafast laser inscribed waveguide laser mode-locked by a nanotube saturable absorber,” Appl. Phys. Lett.97(11), 111114 (2010).
[CrossRef]

H. Yu, X. Chen, H. Zhang, X. Xu, X. Hu, Z. Wang, J. Wang, S. Zhuang, and M. Jiang, “Large energy pulse generation modulated by graphene epitaxially grown on silicon carbide,” ACS Nano4(12), 7582–7586 (2010).
[CrossRef] [PubMed]

T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
[CrossRef]

S. A. Diddams, “The evolving optical frequency comb,” J. Opt. Soc. Am. B27(11), B51–B62 (2010).
[CrossRef]

V. G. Kravets, A. N. Grigorenko, R. R. Nair, P. Blake, S. Anissimova, K. S. Novoselov, and A. K. Geim, “Spectroscopic ellipsometry of graphene and an exciton-shifted van Hove peak in absorption,” Phys. Rev. B81(15), 155413 (2010).
[CrossRef]

2009 (7)

D. M. Basko, S. Piscanec, and A. C. Ferrari, “Electron-electron interactions and doping dependence of the two-phonon Raman intensity in graphene,” Phys. Rev. B80(16), 165413 (2009).
[CrossRef]

M. Lotya, Y. Hernandez, P. J. King, R. J. Smith, V. Nicolosi, L. S. Karlsson, F. M. Blighe, S. De, Z. Wang, I. T. McGovern, G. S. Duesberg, and J. N. Coleman, “Liquid phase production of graphene by exfoliation of graphite in surfactant/water solutions,” J. Am. Chem. Soc.131(10), 3611–3620 (2009).
[CrossRef] [PubMed]

C. Casiraghi, A. Hartschuh, H. Qian, S. Piscanec, C. Georgi, A. Fasoli, K. S. Novoselov, D. M. Basko, and A. C. Ferrari, “Raman spectroscopy of graphene edges,” Nano Lett.9(4), 1433–1441 (2009).
[CrossRef] [PubMed]

C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
[CrossRef]

G. Della Valle, R. Osellame, and P. Laporta, “Micromachining of photonic devices by femtosecond laser pulses,” J. Opt. A, Pure Appl. Opt.11(1), 013001 (2009).
[CrossRef]

S. H. Chung and E. Mazur, “Surgical applications of femtosecond lasers,” J Biophotonics2(10), 557–572 (2009).
[CrossRef] [PubMed]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
[CrossRef]

2008 (5)

F. Wang, A. G. Rozhin, V. Scardaci, Z. Sun, F. Hennrich, I. H. White, W. I. Milne, and A. C. Ferrari, “Wideband-tuneable, nanotube mode-locked, fibre laser,” Nat. Nanotechnol.3(12), 738–742 (2008).
[CrossRef] [PubMed]

Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
[CrossRef] [PubMed]

K. F. Mak, M. Y. Sfeir, Y. Wu, C. H. Lui, J. A. Misewich, and T. F. Heinz, “Measurement of the optical conductivity of graphene,” Phys. Rev. Lett.101(19), 196405 (2008).
[CrossRef] [PubMed]

Z. Q. Li, E. A. Henriksen, Z. Jiang, Z. Hao, M. C. Martin, P. Kim, H. L. Stormer, and D. N. Basov, “Dirac charge dynamics in graphene by infrared spectroscopy,” Nat. Phys.4(7), 532–535 (2008).
[CrossRef]

A. Das, S. Pisana, B. Chakraborty, S. Piscanec, S. K. Saha, U. V. Waghmare, K. S. Novoselov, H. R. Krishnamurthy, A. K. Geim, A. C. Ferrari, and A. K. Sood, “Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor,” Nat. Nanotechnol.3(4), 210–215 (2008).
[CrossRef] [PubMed]

2007 (1)

S. Latil, V. Meunier, and L. Henrard, “Massless fermions in multilayer graphitic systems with misoriented layers: Ab initio calculations and experimental fingerprints,” Phys. Rev. B76(20), 201402 (2007).
[CrossRef]

2006 (2)

A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, “Raman spectrum of graphene and graphene layers,” Phys. Rev. Lett.97(18), 187401 (2006).
[CrossRef] [PubMed]

G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
[CrossRef]

2005 (1)

2004 (3)

M. Haiml, R. Grange, and U. Keller, “Optical characterization of semiconductor saturable absorbers,” Appl. Phys. B79(3), 331–339 (2004).
[CrossRef]

O. Okhotnikov, A. Grudinin, and M. Pessa, “Ultra-fast fibre laser systems based on SESAM technology: new horizons and applications,” New J. Phys.6, 177 (2004).
[CrossRef]

J. Mertz, “Nonlinear microscopy: new techniques and applications,” Curr. Opin. Neurobiol.14(5), 610–616 (2004).
[CrossRef] [PubMed]

2001 (1)

A. C. Ferrari and J. Robertson, “Resonant Raman spectroscopy of disordered, amorphous, and diamondlike carbon,” Phys. Rev. B64(7), 075414 (2001).
[CrossRef]

2000 (1)

A. C. Ferrari and J. Robertson, “Interpretation of Raman spectra of disordered and amorphous carbon,” Phys. Rev. B61(20), 14095–14107 (2000).
[CrossRef]

1999 (1)

1997 (1)

1986 (1)

D. V. Linde, “Characterization of the noise in continuously operating mode-locked lasers,” Appl. Phys. B39(4), 201–217 (1986).
[CrossRef]

Agnoli, S.

C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
[CrossRef]

Ahn, J. H.

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D. M. Basko, S. Piscanec, and A. C. Ferrari, “Electron-electron interactions and doping dependence of the two-phonon Raman intensity in graphene,” Phys. Rev. B80(16), 165413 (2009).
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V. G. Kravets, A. N. Grigorenko, R. R. Nair, P. Blake, S. Anissimova, K. S. Novoselov, and A. K. Geim, “Spectroscopic ellipsometry of graphene and an exciton-shifted van Hove peak in absorption,” Phys. Rev. B81(15), 155413 (2010).
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M. Lotya, Y. Hernandez, P. J. King, R. J. Smith, V. Nicolosi, L. S. Karlsson, F. M. Blighe, S. De, Z. Wang, I. T. McGovern, G. S. Duesberg, and J. N. Coleman, “Liquid phase production of graphene by exfoliation of graphite in surfactant/water solutions,” J. Am. Chem. Soc.131(10), 3611–3620 (2009).
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Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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F. Bonaccorso, A. Lombardo, T. Hasan, Z. Sun, L. Colombo, and A. C. Ferrari, “Production and processing of graphene and 2d crystals,” Mater. Today15(12), 564–589 (2012).
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Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
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F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, “Graphene photonics and optoelectronics,” Nat. Photonics4(9), 611–622 (2010).
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T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
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T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
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A. A. Lagatsky, Z. Sun, T. S. Kulmala, R. S. Sundaram, S. Milana, F. Torrisi, O. L. Antipov, Y. Lee, J. H. Ahn, C. T. A. Brown, W. Sibbett, and A. C. Ferrari, “2μm Solid-State Laser Mode-locked By Single-Layer Graphene,” Appl. Phys. Lett.102(1), 013113 (2013).
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C. Casiraghi, A. Hartschuh, H. Qian, S. Piscanec, C. Georgi, A. Fasoli, K. S. Novoselov, D. M. Basko, and A. C. Ferrari, “Raman spectroscopy of graphene edges,” Nano Lett.9(4), 1433–1441 (2009).
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A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, “Raman spectrum of graphene and graphene layers,” Phys. Rev. Lett.97(18), 187401 (2006).
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C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
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G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
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A. Das, S. Pisana, B. Chakraborty, S. Piscanec, S. K. Saha, U. V. Waghmare, K. S. Novoselov, H. R. Krishnamurthy, A. K. Geim, A. C. Ferrari, and A. K. Sood, “Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor,” Nat. Nanotechnol.3(4), 210–215 (2008).
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C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
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Chiodo, N.

G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
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Choi, S. Y.

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S. H. Chung and E. Mazur, “Surgical applications of femtosecond lasers,” J Biophotonics2(10), 557–572 (2009).
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M. Lotya, Y. Hernandez, P. J. King, R. J. Smith, V. Nicolosi, L. S. Karlsson, F. M. Blighe, S. De, Z. Wang, I. T. McGovern, G. S. Duesberg, and J. N. Coleman, “Liquid phase production of graphene by exfoliation of graphite in surfactant/water solutions,” J. Am. Chem. Soc.131(10), 3611–3620 (2009).
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Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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F. Bonaccorso, A. Lombardo, T. Hasan, Z. Sun, L. Colombo, and A. C. Ferrari, “Production and processing of graphene and 2d crystals,” Mater. Today15(12), 564–589 (2012).
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A. Das, S. Pisana, B. Chakraborty, S. Piscanec, S. K. Saha, U. V. Waghmare, K. S. Novoselov, H. R. Krishnamurthy, A. K. Geim, A. C. Ferrari, and A. K. Sood, “Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor,” Nat. Nanotechnol.3(4), 210–215 (2008).
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M. Lotya, Y. Hernandez, P. J. King, R. J. Smith, V. Nicolosi, L. S. Karlsson, F. M. Blighe, S. De, Z. Wang, I. T. McGovern, G. S. Duesberg, and J. N. Coleman, “Liquid phase production of graphene by exfoliation of graphite in surfactant/water solutions,” J. Am. Chem. Soc.131(10), 3611–3620 (2009).
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Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
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Duesberg, G.

Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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M. Lotya, Y. Hernandez, P. J. King, R. J. Smith, V. Nicolosi, L. S. Karlsson, F. M. Blighe, S. De, Z. Wang, I. T. McGovern, G. S. Duesberg, and J. N. Coleman, “Liquid phase production of graphene by exfoliation of graphite in surfactant/water solutions,” J. Am. Chem. Soc.131(10), 3611–3620 (2009).
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C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
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C. Casiraghi, A. Hartschuh, H. Qian, S. Piscanec, C. Georgi, A. Fasoli, K. S. Novoselov, D. M. Basko, and A. C. Ferrari, “Raman spectroscopy of graphene edges,” Nano Lett.9(4), 1433–1441 (2009).
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Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
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A. A. Lagatsky, Z. Sun, T. S. Kulmala, R. S. Sundaram, S. Milana, F. Torrisi, O. L. Antipov, Y. Lee, J. H. Ahn, C. T. A. Brown, W. Sibbett, and A. C. Ferrari, “2μm Solid-State Laser Mode-locked By Single-Layer Graphene,” Appl. Phys. Lett.102(1), 013113 (2013).
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F. Bonaccorso, A. Lombardo, T. Hasan, Z. Sun, L. Colombo, and A. C. Ferrari, “Production and processing of graphene and 2d crystals,” Mater. Today15(12), 564–589 (2012).
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M. Zhang, E. J. R. Kelleher, F. Torrisi, Z. Sun, T. Hasan, D. Popa, F. Wang, A. C. Ferrari, S. V. Popov, and J. R. Taylor, “Tm-doped fiber laser mode-locked by graphene-polymer composite,” Opt. Express20(22), 25077–25084 (2012).
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D. Popa, Z. Sun, T. Hasan, W. B. Cho, F. Wang, F. Torrisi, and A. C. Ferrari, “74-fs nanotube-mode-locked fiber laser,” Appl. Phys. Lett.101(15), 153107 (2012).
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Z. Sun, T. Hasan, and A. C. Ferrari, “Ultrafast lasers mode-locked by nanotubes and graphene,” Physica E44(6), 1082–1091 (2012).
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D. Popa, Z. Sun, T. Hasan, F. Torrisi, F. Wang, and A. C. Ferrari, “Graphene Q-switched, tunable fiber laser,” Appl. Phys. Lett.98(7), 073106 (2011).
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Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
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F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, “Graphene photonics and optoelectronics,” Nat. Photonics4(9), 611–622 (2010).
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D. Popa, Z. Sun, F. Torrisi, T. Hasan, F. Wang, and A. C. Ferrari, “Sub 200 fs pulse generation from a graphene mode-locked fiber laser,” Appl. Phys. Lett.97(20), 203106 (2010).
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S. J. Beecher, R. R. Thomson, N. D. Psaila, Z. Sun, T. Hasan, A. G. Rozhin, A. C. Ferrari, and A. K. Kar, “320 fs pulse generation from an ultrafast laser inscribed waveguide laser mode-locked by a nanotube saturable absorber,” Appl. Phys. Lett.97(11), 111114 (2010).
[CrossRef]

T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
[CrossRef]

C. Casiraghi, A. Hartschuh, H. Qian, S. Piscanec, C. Georgi, A. Fasoli, K. S. Novoselov, D. M. Basko, and A. C. Ferrari, “Raman spectroscopy of graphene edges,” Nano Lett.9(4), 1433–1441 (2009).
[CrossRef] [PubMed]

D. M. Basko, S. Piscanec, and A. C. Ferrari, “Electron-electron interactions and doping dependence of the two-phonon Raman intensity in graphene,” Phys. Rev. B80(16), 165413 (2009).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
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F. Wang, A. G. Rozhin, V. Scardaci, Z. Sun, F. Hennrich, I. H. White, W. I. Milne, and A. C. Ferrari, “Wideband-tuneable, nanotube mode-locked, fibre laser,” Nat. Nanotechnol.3(12), 738–742 (2008).
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A. Das, S. Pisana, B. Chakraborty, S. Piscanec, S. K. Saha, U. V. Waghmare, K. S. Novoselov, H. R. Krishnamurthy, A. K. Geim, A. C. Ferrari, and A. K. Sood, “Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor,” Nat. Nanotechnol.3(4), 210–215 (2008).
[CrossRef] [PubMed]

Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, “Raman spectrum of graphene and graphene layers,” Phys. Rev. Lett.97(18), 187401 (2006).
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G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
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A. C. Ferrari and J. Robertson, “Resonant Raman spectroscopy of disordered, amorphous, and diamondlike carbon,” Phys. Rev. B64(7), 075414 (2001).
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A. C. Ferrari and J. Robertson, “Interpretation of Raman spectra of disordered and amorphous carbon,” Phys. Rev. B61(20), 14095–14107 (2000).
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G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
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Garfunkel, E.

C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
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V. G. Kravets, A. N. Grigorenko, R. R. Nair, P. Blake, S. Anissimova, K. S. Novoselov, and A. K. Geim, “Spectroscopic ellipsometry of graphene and an exciton-shifted van Hove peak in absorption,” Phys. Rev. B81(15), 155413 (2010).
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A. Das, S. Pisana, B. Chakraborty, S. Piscanec, S. K. Saha, U. V. Waghmare, K. S. Novoselov, H. R. Krishnamurthy, A. K. Geim, A. C. Ferrari, and A. K. Sood, “Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor,” Nat. Nanotechnol.3(4), 210–215 (2008).
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A. C. Ferrari, J. C. Meyer, V. Scardaci, C. Casiraghi, M. Lazzeri, F. Mauri, S. Piscanec, D. Jiang, K. S. Novoselov, S. Roth, and A. K. Geim, “Raman spectrum of graphene and graphene layers,” Phys. Rev. Lett.97(18), 187401 (2006).
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C. Casiraghi, A. Hartschuh, H. Qian, S. Piscanec, C. Georgi, A. Fasoli, K. S. Novoselov, D. M. Basko, and A. C. Ferrari, “Raman spectroscopy of graphene edges,” Nano Lett.9(4), 1433–1441 (2009).
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Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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C. Mattevi, G. Eda, S. Agnoli, S. Miller, K. A. Mkhoyan, O. Celik, D. Mastrogiovanni, G. Granozzi, E. Garfunkel, and M. Chhowalla, “Evolution of electrical, chemical, and structural properties of transparent and conducting chemically derived graphene thin films,” Adv. Funct. Mater.19(16), 2577–2583 (2009).
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V. G. Kravets, A. N. Grigorenko, R. R. Nair, P. Blake, S. Anissimova, K. S. Novoselov, and A. K. Geim, “Spectroscopic ellipsometry of graphene and an exciton-shifted van Hove peak in absorption,” Phys. Rev. B81(15), 155413 (2010).
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O. Okhotnikov, A. Grudinin, and M. Pessa, “Ultra-fast fibre laser systems based on SESAM technology: new horizons and applications,” New J. Phys.6, 177 (2004).
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Y. Hernandez, V. Nicolosi, M. Lotya, F. M. Blighe, Z. Sun, S. De, I. T. McGovern, B. Holland, M. Byrne, Y. K. Gun’Ko, J. J. Boland, P. Niraj, G. Duesberg, S. Krishnamurthy, R. Goodhue, J. Hutchison, V. Scardaci, A. C. Ferrari, and J. N. Coleman, “High-yield production of graphene by liquid-phase exfoliation of graphite,” Nat. Nanotechnol.3(9), 563–568 (2008).
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C. Casiraghi, A. Hartschuh, H. Qian, S. Piscanec, C. Georgi, A. Fasoli, K. S. Novoselov, D. M. Basko, and A. C. Ferrari, “Raman spectroscopy of graphene edges,” Nano Lett.9(4), 1433–1441 (2009).
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D. Popa, Z. Sun, T. Hasan, W. B. Cho, F. Wang, F. Torrisi, and A. C. Ferrari, “74-fs nanotube-mode-locked fiber laser,” Appl. Phys. Lett.101(15), 153107 (2012).
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D. Popa, Z. Sun, T. Hasan, F. Torrisi, F. Wang, and A. C. Ferrari, “Graphene Q-switched, tunable fiber laser,” Appl. Phys. Lett.98(7), 073106 (2011).
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Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
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Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
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D. Popa, Z. Sun, F. Torrisi, T. Hasan, F. Wang, and A. C. Ferrari, “Sub 200 fs pulse generation from a graphene mode-locked fiber laser,” Appl. Phys. Lett.97(20), 203106 (2010).
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T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
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Privitera, G.

Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
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T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
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S. J. Beecher, R. R. Thomson, N. D. Psaila, Z. Sun, T. Hasan, A. G. Rozhin, A. C. Ferrari, and A. K. Kar, “320 fs pulse generation from an ultrafast laser inscribed waveguide laser mode-locked by a nanotube saturable absorber,” Appl. Phys. Lett.97(11), 111114 (2010).
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T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
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G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
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D. Popa, Z. Sun, T. Hasan, W. B. Cho, F. Wang, F. Torrisi, and A. C. Ferrari, “74-fs nanotube-mode-locked fiber laser,” Appl. Phys. Lett.101(15), 153107 (2012).
[CrossRef]

M. Zhang, E. J. R. Kelleher, F. Torrisi, Z. Sun, T. Hasan, D. Popa, F. Wang, A. C. Ferrari, S. V. Popov, and J. R. Taylor, “Tm-doped fiber laser mode-locked by graphene-polymer composite,” Opt. Express20(22), 25077–25084 (2012).
[CrossRef] [PubMed]

D. Popa, Z. Sun, T. Hasan, F. Torrisi, F. Wang, and A. C. Ferrari, “Graphene Q-switched, tunable fiber laser,” Appl. Phys. Lett.98(7), 073106 (2011).
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Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
[CrossRef] [PubMed]

Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
[CrossRef]

D. Popa, Z. Sun, F. Torrisi, T. Hasan, F. Wang, and A. C. Ferrari, “Sub 200 fs pulse generation from a graphene mode-locked fiber laser,” Appl. Phys. Lett.97(20), 203106 (2010).
[CrossRef]

S. J. Beecher, R. R. Thomson, N. D. Psaila, Z. Sun, T. Hasan, A. G. Rozhin, A. C. Ferrari, and A. K. Kar, “320 fs pulse generation from an ultrafast laser inscribed waveguide laser mode-locked by a nanotube saturable absorber,” Appl. Phys. Lett.97(11), 111114 (2010).
[CrossRef]

T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
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F. Wang, A. G. Rozhin, V. Scardaci, Z. Sun, F. Hennrich, I. H. White, W. I. Milne, and A. C. Ferrari, “Wideband-tuneable, nanotube mode-locked, fibre laser,” Nat. Nanotechnol.3(12), 738–742 (2008).
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[CrossRef]

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G. Della Valle, R. Osellame, G. Galzerano, N. Chiodo, G. Cerullo, P. Laporta, O. Svelto, U. Morgner, A. G. Rozhin, V. Scardaci, and A. C. Ferrari, “Passive mode locking by carbon nanotubes in a femtosecond laser written waveguide laser,” Appl. Phys. Lett.89(23), 231115 (2006).
[CrossRef]

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T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
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Taylor, J. R.

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[CrossRef]

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A. A. Lagatsky, Z. Sun, T. S. Kulmala, R. S. Sundaram, S. Milana, F. Torrisi, O. L. Antipov, Y. Lee, J. H. Ahn, C. T. A. Brown, W. Sibbett, and A. C. Ferrari, “2μm Solid-State Laser Mode-locked By Single-Layer Graphene,” Appl. Phys. Lett.102(1), 013113 (2013).
[CrossRef]

M. Zhang, E. J. R. Kelleher, F. Torrisi, Z. Sun, T. Hasan, D. Popa, F. Wang, A. C. Ferrari, S. V. Popov, and J. R. Taylor, “Tm-doped fiber laser mode-locked by graphene-polymer composite,” Opt. Express20(22), 25077–25084 (2012).
[CrossRef] [PubMed]

D. Popa, Z. Sun, T. Hasan, W. B. Cho, F. Wang, F. Torrisi, and A. C. Ferrari, “74-fs nanotube-mode-locked fiber laser,” Appl. Phys. Lett.101(15), 153107 (2012).
[CrossRef]

D. Popa, Z. Sun, T. Hasan, F. Torrisi, F. Wang, and A. C. Ferrari, “Graphene Q-switched, tunable fiber laser,” Appl. Phys. Lett.98(7), 073106 (2011).
[CrossRef]

Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
[CrossRef] [PubMed]

Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
[CrossRef]

D. Popa, Z. Sun, F. Torrisi, T. Hasan, F. Wang, and A. C. Ferrari, “Sub 200 fs pulse generation from a graphene mode-locked fiber laser,” Appl. Phys. Lett.97(20), 203106 (2010).
[CrossRef]

T. Hasan, F. Torrisi, Z. Sun, D. Popa, V. Nicolosi, G. Privitera, F. Bonaccorso, and A. C. Ferrari, “Solution-phase exfoliation of graphite for ultrafast photonics,” Phys. Status Solidi B247(11-12), 2953–2957 (2010).
[CrossRef]

Travers, J.

Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
[CrossRef]

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Vianna, S. S.

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[CrossRef] [PubMed]

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M. Zhang, E. J. R. Kelleher, F. Torrisi, Z. Sun, T. Hasan, D. Popa, F. Wang, A. C. Ferrari, S. V. Popov, and J. R. Taylor, “Tm-doped fiber laser mode-locked by graphene-polymer composite,” Opt. Express20(22), 25077–25084 (2012).
[CrossRef] [PubMed]

D. Popa, Z. Sun, T. Hasan, W. B. Cho, F. Wang, F. Torrisi, and A. C. Ferrari, “74-fs nanotube-mode-locked fiber laser,” Appl. Phys. Lett.101(15), 153107 (2012).
[CrossRef]

D. Popa, Z. Sun, T. Hasan, F. Torrisi, F. Wang, and A. C. Ferrari, “Graphene Q-switched, tunable fiber laser,” Appl. Phys. Lett.98(7), 073106 (2011).
[CrossRef]

Z. Sun, T. Hasan, F. Torrisi, D. Popa, G. Privitera, F. Wang, F. Bonaccorso, D. M. Basko, and A. C. Ferrari, “Graphene mode-locked ultrafast laser,” ACS Nano4(2), 803–810 (2010).
[CrossRef] [PubMed]

Z. Sun, D. Popa, T. Hasan, F. Torrisi, F. Wang, E. Kelleher, J. Travers, V. Nicolosi, and A. Ferrari, “A stable, wideband tunable, near transform-limited, graphene-mode-locked, ultrafast laser,” Nano Res.3(9), 653–660 (2010).
[CrossRef]

D. Popa, Z. Sun, F. Torrisi, T. Hasan, F. Wang, and A. C. Ferrari, “Sub 200 fs pulse generation from a graphene mode-locked fiber laser,” Appl. Phys. Lett.97(20), 203106 (2010).
[CrossRef]

T. Hasan, Z. Sun, F. Wang, F. Bonaccorso, P. H. Tan, A. G. Rozhin, and A. C. Ferrari, “Nanotube-polymer composites for ultrafast photonics,” Adv. Mater.21(38–39), 3874–3899 (2009).
[CrossRef]

F. Wang, A. G. Rozhin, V. Scardaci, Z. Sun, F. Hennrich, I. H. White, W. I. Milne, and A. C. Ferrari, “Wideband-tuneable, nanotube mode-locked, fibre laser,” Nat. Nanotechnol.3(12), 738–742 (2008).
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H. Yu, X. Chen, H. Zhang, X. Xu, X. Hu, Z. Wang, J. Wang, S. Zhuang, and M. Jiang, “Large energy pulse generation modulated by graphene epitaxially grown on silicon carbide,” ACS Nano4(12), 7582–7586 (2010).
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Wang, Y. G.

J. Liu, Y. G. Wang, Z. S. Qu, L. H. Zheng, L. B. Su, and J. Xu, “Graphene oxide absorber for 2 µm passive mode-locking Tm:YAlO3 laser,” Laser Phys. Lett.9(1), 15–19 (2012).
[CrossRef]

Wang, Z.

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Figures (5)

Fig. 1
Fig. 1

Raman spectra measured at 514 nm of (a) graphene dispersion in SDC-Water and (b) graphene film.

Fig. 2
Fig. 2

Transmittance of (a) Quartz, (b) Graphene dispersion, (c) Graphene-film, and (d) Graphene-film on quartz. (e) Nonlinear reflectivity vs pulse fluence for the GF-SA.

Fig. 3
Fig. 3

Laser schematic. L1 and L2: Coupling lenses; PM: Polarization maintaining fiber; GF-SOC: Graphene-film saturable output coupler; DM: Dichroic mirror.

Fig. 4
Fig. 4

(a) Repetition rate and energy within the Q-switched envelope, as a function of input pump power. (b) Mode-locked pulse train

Fig. 5
Fig. 5

(a) RF Spectrum measured at the maximum pump (zoom-out in the inset). (b) Corresponding optical spectrum. (c) Output autocorrelation trace. (d) Output power with launched pump power (with a slope efficiency of ~48% and a maximum output power of 202 mW).

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