Abstract

Chirality effects in optical second harmonic generation (SHG) are studied in periodic planar arrays of gold G-shaped nanostructures. We show that G-shaped structures of different handedness demonstrate different SHG efficiency for the left and right circular polarizations, as well as the opposite directions of the SHG polarization plane rotation. The observed effects are interpreted as the appearance of chirality in the SHG response which allows clear distinguishing of two enantiomers.

© 2012 OSA

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2011

2010

V. K. Valev, A. V. Silhanek, N. Verellen, W. Gillijns, P. Van Dorpe, O. A. Aktsipetrov, G. A. E. Vandenbosch, V. V. Moshchalkov, and T. Verbiest, “Asymmetric optical second-harmonic generation from chiral G-shaped gold nanostructures,” Phys. Rev. Lett.104, 127401 (2010).
[PubMed]

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

Y. Pu, R. Grange, C.-L. Hsieh, and D. Psaltis, “Nonlinear optical properties of core-shell nanocavities for enhanced second-harmonic generation,” Phys. Rev. Lett.104, 207402 (2010).
[PubMed]

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

V. K. Valev, A. V. Silhanek, N. Smisdom, B. D. Clercq, W. Gillijns, O. A. Aktsipetrov, M. Ameloot, V. V. Moshchalkov, and T. Verbiest, “Linearly polarized second harmonic generation microscopy reveals chirality,” Opt. Express18, 8286–8293 (2010).
[PubMed]

2009

2008

2007

V. A. Fedotov, A. S. Schwanecke, N. I. Zheludev, V. V. Khardikov, and S. L. Prosvirnin, “Asymmetric transmission of light and enantiomerically sensitive plasmon resonance in planar chiral nanostructures,” Nano. Lett.7, 1996–1999 (2007).

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

S. Kujala, B. K. Canfield, M. Kauranen, Y. Svirko, and J. Turunen, “Multipole interference in the second-harmonic optical radiation from gold nanoparticles,” Phys. Rev. Lett.98, 167403 (2007).
[PubMed]

2006

V. A. Fedotov, P. L. Mladyonov, S. L. Prosvirnin, A. V. Rogacheva, Y. Chen, and N. I. Zheludev, “Asymmetric propagation of electromagnetic waves through a planar chiral structure,” Phys. Rev. Lett.97, 167401 (2006).
[PubMed]

2005

2004

A. Potts, A. Papakostas, D. M. Bagnall, and N. I. Zheludev, “Planar chiral meta-materials for optical applications,” Microelectron. Eng.73–74, 367–371 (2004).

2003

A. Papakostas, A. Potts, D. M. Bagnall, S. L. Prosvirnin, H. J. Coles, and N. I. Zheludev, “Optical manifestations of planar chirality,” Phys. Rev. Lett.90, 107404 (2003).
[PubMed]

1954

W. L. Schaich, “Second harmonic generation by periodically-structured metal surfaces,” Phys. Rev. B78, 195416 (2008).

Adam, P.-M.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Aktsipetrov, O. A.

Ameloot, M.

Bachelier, G.

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

Bachelot, R.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Bagnall, D. M.

A. Potts, A. Papakostas, D. M. Bagnall, and N. I. Zheludev, “Planar chiral meta-materials for optical applications,” Microelectron. Eng.73–74, 367–371 (2004).

A. Papakostas, A. Potts, D. M. Bagnall, S. L. Prosvirnin, H. J. Coles, and N. I. Zheludev, “Optical manifestations of planar chirality,” Phys. Rev. Lett.90, 107404 (2003).
[PubMed]

Belardini, A.

Benichou, E.

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

Bertolotti, M.

Billot, L.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Bratkovsky, A.

Brevet, P.-F.

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

Butet, J.

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

Canfield, B. K.

S. Kujala, B. K. Canfield, M. Kauranen, Y. Svirko, and J. Turunen, “Multipole interference in the second-harmonic optical radiation from gold nanoparticles,” Phys. Rev. Lett.98, 167403 (2007).
[PubMed]

Centini, M.

Chen, Y.

V. A. Fedotov, P. L. Mladyonov, S. L. Prosvirnin, A. V. Rogacheva, Y. Chen, and N. I. Zheludev, “Asymmetric propagation of electromagnetic waves through a planar chiral structure,” Phys. Rev. Lett.97, 167401 (2006).
[PubMed]

Chiappe, D.

Clercq, B. D.

Coles, H. J.

A. Papakostas, A. Potts, D. M. Bagnall, S. L. Prosvirnin, H. J. Coles, and N. I. Zheludev, “Optical manifestations of planar chirality,” Phys. Rev. Lett.90, 107404 (2003).
[PubMed]

de Mongeot, F. B.

Dorkenoo, K. D.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Duboisset, J.

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

Fazio, E.

Fedotov, V. A.

V. A. Fedotov, A. S. Schwanecke, N. I. Zheludev, V. V. Khardikov, and S. L. Prosvirnin, “Asymmetric transmission of light and enantiomerically sensitive plasmon resonance in planar chiral nanostructures,” Nano. Lett.7, 1996–1999 (2007).

V. A. Fedotov, P. L. Mladyonov, S. L. Prosvirnin, A. V. Rogacheva, Y. Chen, and N. I. Zheludev, “Asymmetric propagation of electromagnetic waves through a planar chiral structure,” Phys. Rev. Lett.97, 167401 (2006).
[PubMed]

Fedyanin, A. A.

Fort, A.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Galynsky, V. M.

Gillijns, W.

V. K. Valev, A. V. Silhanek, N. Verellen, W. Gillijns, P. Van Dorpe, O. A. Aktsipetrov, G. A. E. Vandenbosch, V. V. Moshchalkov, and T. Verbiest, “Asymmetric optical second-harmonic generation from chiral G-shaped gold nanostructures,” Phys. Rev. Lett.104, 127401 (2010).
[PubMed]

V. K. Valev, A. V. Silhanek, N. Smisdom, B. D. Clercq, W. Gillijns, O. A. Aktsipetrov, M. Ameloot, V. V. Moshchalkov, and T. Verbiest, “Linearly polarized second harmonic generation microscopy reveals chirality,” Opt. Express18, 8286–8293 (2010).
[PubMed]

Gindre, D.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Grand, J.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Grange, R.

Y. Pu, R. Grange, C.-L. Hsieh, and D. Psaltis, “Nonlinear optical properties of core-shell nanocavities for enhanced second-harmonic generation,” Phys. Rev. Lett.104, 207402 (2010).
[PubMed]

Hoyer, W.

Y. Zeng, W. Hoyer, J. Liu, S. W. Koch, and J. V. Moloney, “Classical theory for second-harmonic generation from metallic nanoparticles,” Phys. Rev. B79, 235109 (2009).

Hsieh, C.-L.

Y. Pu, R. Grange, C.-L. Hsieh, and D. Psaltis, “Nonlinear optical properties of core-shell nanocavities for enhanced second-harmonic generation,” Phys. Rev. Lett.104, 207402 (2010).
[PubMed]

Hubert, C.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Inoue, M.

Ivanchenko, M. V.

Jonin, C.

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

Kapra, R. V.

Kauranen, M.

S. Kujala, B. K. Canfield, M. Kauranen, Y. Svirko, and J. Turunen, “Multipole interference in the second-harmonic optical radiation from gold nanoparticles,” Phys. Rev. Lett.98, 167403 (2007).
[PubMed]

Khardikov, V. V.

V. A. Fedotov, A. S. Schwanecke, N. I. Zheludev, V. V. Khardikov, and S. L. Prosvirnin, “Asymmetric transmission of light and enantiomerically sensitive plasmon resonance in planar chiral nanostructures,” Nano. Lett.7, 1996–1999 (2007).

Kim, E. M.

Koch, S. W.

Y. Zeng, W. Hoyer, J. Liu, S. W. Koch, and J. V. Moloney, “Classical theory for second-harmonic generation from metallic nanoparticles,” Phys. Rev. B79, 235109 (2009).

Kolmychek, I. A.

Kravets, A. F.

Kujala, S.

S. Kujala, B. K. Canfield, M. Kauranen, Y. Svirko, and J. Turunen, “Multipole interference in the second-harmonic optical radiation from gold nanoparticles,” Phys. Rev. Lett.98, 167403 (2007).
[PubMed]

Kuznetsova, S. V.

Kwon, D.-H.

Larciprete, M. C.

Li, J.

S. Zhang, Y.-S. Park, J. Li, X. Lu, W. Zhang, and X. Zhang, “Negative refractive index in chiral metamaterials,” Phys. Rev. Lett.102, 023901 (2009).
[PubMed]

Lifshits, V. G.

Liu, J.

Y. Zeng, W. Hoyer, J. Liu, S. W. Koch, and J. V. Moloney, “Classical theory for second-harmonic generation from metallic nanoparticles,” Phys. Rev. B79, 235109 (2009).

Lu, X.

S. Zhang, Y.-S. Park, J. Li, X. Lu, W. Zhang, and X. Zhang, “Negative refractive index in chiral metamaterials,” Phys. Rev. Lett.102, 023901 (2009).
[PubMed]

Mamonov, E. A.

Maydykovsky, A. I.

Mladyonov, P. L.

V. A. Fedotov, P. L. Mladyonov, S. L. Prosvirnin, A. V. Rogacheva, Y. Chen, and N. I. Zheludev, “Asymmetric propagation of electromagnetic waves through a planar chiral structure,” Phys. Rev. Lett.97, 167401 (2006).
[PubMed]

Moloney, J. V.

Y. Zeng and J. V. Moloney, “Volume electric dipole origin of second-harmonic generation from metallic membrane with noncentrosymmetric patterns,” Opt. Lett.34, 2844–2846 (2009).
[PubMed]

Y. Zeng, W. Hoyer, J. Liu, S. W. Koch, and J. V. Moloney, “Classical theory for second-harmonic generation from metallic nanoparticles,” Phys. Rev. B79, 235109 (2009).

Moshchalkov, V. V.

Murzina, T. V.

Nee, S.-M. F.

S.-M. F. Nee, “Polarization measurement,” in The Measurement, Instrumentation and Sensors Handbook, J. G. Webster, ed. (CRC and IEEE, Boca Raton, 1999).

Novitsky, A. V.

Papakostas, A.

A. Potts, A. Papakostas, D. M. Bagnall, and N. I. Zheludev, “Planar chiral meta-materials for optical applications,” Microelectron. Eng.73–74, 367–371 (2004).

A. Papakostas, A. Potts, D. M. Bagnall, S. L. Prosvirnin, H. J. Coles, and N. I. Zheludev, “Optical manifestations of planar chirality,” Phys. Rev. Lett.90, 107404 (2003).
[PubMed]

Park, Y.-S.

S. Zhang, Y.-S. Park, J. Li, X. Lu, W. Zhang, and X. Zhang, “Negative refractive index in chiral metamaterials,” Phys. Rev. Lett.102, 023901 (2009).
[PubMed]

Ponizovskaya, E.

Potts, A.

A. Potts, A. Papakostas, D. M. Bagnall, and N. I. Zheludev, “Planar chiral meta-materials for optical applications,” Microelectron. Eng.73–74, 367–371 (2004).

A. Papakostas, A. Potts, D. M. Bagnall, S. L. Prosvirnin, H. J. Coles, and N. I. Zheludev, “Optical manifestations of planar chirality,” Phys. Rev. Lett.90, 107404 (2003).
[PubMed]

Prosvirnin, S. L.

V. A. Fedotov, A. S. Schwanecke, N. I. Zheludev, V. V. Khardikov, and S. L. Prosvirnin, “Asymmetric transmission of light and enantiomerically sensitive plasmon resonance in planar chiral nanostructures,” Nano. Lett.7, 1996–1999 (2007).

V. A. Fedotov, P. L. Mladyonov, S. L. Prosvirnin, A. V. Rogacheva, Y. Chen, and N. I. Zheludev, “Asymmetric propagation of electromagnetic waves through a planar chiral structure,” Phys. Rev. Lett.97, 167401 (2006).
[PubMed]

A. Papakostas, A. Potts, D. M. Bagnall, S. L. Prosvirnin, H. J. Coles, and N. I. Zheludev, “Optical manifestations of planar chirality,” Phys. Rev. Lett.90, 107404 (2003).
[PubMed]

Psaltis, D.

Y. Pu, R. Grange, C.-L. Hsieh, and D. Psaltis, “Nonlinear optical properties of core-shell nanocavities for enhanced second-harmonic generation,” Phys. Rev. Lett.104, 207402 (2010).
[PubMed]

Pu, Y.

Y. Pu, R. Grange, C.-L. Hsieh, and D. Psaltis, “Nonlinear optical properties of core-shell nanocavities for enhanced second-harmonic generation,” Phys. Rev. Lett.104, 207402 (2010).
[PubMed]

Rogacheva, A. V.

V. A. Fedotov, P. L. Mladyonov, S. L. Prosvirnin, A. V. Rogacheva, Y. Chen, and N. I. Zheludev, “Asymmetric propagation of electromagnetic waves through a planar chiral structure,” Phys. Rev. Lett.97, 167401 (2006).
[PubMed]

Royer, P.

C. Hubert, L. Billot, P.-M. Adam, R. Bachelot, P. Royer, J. Grand, D. Gindre, K. D. Dorkenoo, and A. Fort, “Role of surface plasmon in second harmonic generation from gold nanorods,” Appl. Phys.90, 181105 (2007).

Russier-Antoine, I.

J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett.105, 077401 (2010).
[PubMed]

J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano. Lett.10, 1717–1721 (2010).
[PubMed]

Schaich, W. L.

W. L. Schaich, “Second harmonic generation by periodically-structured metal surfaces,” Phys. Rev. B78, 195416 (2008).

Schwanecke, A. S.

V. A. Fedotov, A. S. Schwanecke, N. I. Zheludev, V. V. Khardikov, and S. L. Prosvirnin, “Asymmetric transmission of light and enantiomerically sensitive plasmon resonance in planar chiral nanostructures,” Nano. Lett.7, 1996–1999 (2007).

Sibilia, C.

Silhanek, A. V.

Smisdom, N.

Svirko, Y.

S. Kujala, B. K. Canfield, M. Kauranen, Y. Svirko, and J. Turunen, “Multipole interference in the second-harmonic optical radiation from gold nanoparticles,” Phys. Rev. Lett.98, 167403 (2007).
[PubMed]

Toma, A.

Turunen, J.

S. Kujala, B. K. Canfield, M. Kauranen, Y. Svirko, and J. Turunen, “Multipole interference in the second-harmonic optical radiation from gold nanoparticles,” Phys. Rev. Lett.98, 167403 (2007).
[PubMed]

Valev, V. K.

Van Dorpe, P.

V. K. Valev, A. V. Silhanek, N. Verellen, W. Gillijns, P. Van Dorpe, O. A. Aktsipetrov, G. A. E. Vandenbosch, V. V. Moshchalkov, and T. Verbiest, “Asymmetric optical second-harmonic generation from chiral G-shaped gold nanostructures,” Phys. Rev. Lett.104, 127401 (2010).
[PubMed]

Vandenbosch, G. A. E.

V. K. Valev, A. V. Silhanek, N. Verellen, W. Gillijns, P. Van Dorpe, O. A. Aktsipetrov, G. A. E. Vandenbosch, V. V. Moshchalkov, and T. Verbiest, “Asymmetric optical second-harmonic generation from chiral G-shaped gold nanostructures,” Phys. Rev. Lett.104, 127401 (2010).
[PubMed]

Verbiest, T.

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