Abstract

We present power conversion efficiency (PCE) and luminous efficiency (LE) performance levels of high photometric quality white LEDs integrated with quantum dots (QDs) achieving an averaged color rendering index of ≥90 (with R9 at least 70), a luminous efficacy of optical radiation of ≥380 lm/Wopt a correlated color temperature of ≤4000 K, and a chromaticity difference dC <0.0054. We computationally find that the device LE levels of 100, 150, and 200 lm/Welect can be achieved with QD quantum efficiency of 43%, 61%, and 80% in film, respectively, using state-of-the-art blue LED chips (81.3% PCE). Furthermore, our computational analyses suggest that QD-LEDs can be both photometrically and electrically more efficient than phosphor based LEDs when state-of-the-art QDs are used.

© 2012 OSA

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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  13. E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
    [CrossRef]
  14. M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
    [CrossRef]
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    [CrossRef]
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2011 (3)

O. Graydon, “The new oil?” Nat. Photonics 5(1), 1 (2011).
[CrossRef]

T. Erdem and H. V. Demir, “Semiconductor nanocrystals as rare-earth alternatives,” Nat. Photonics 5(3), 126 (2011).
[CrossRef]

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

2010 (5)

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

T. Erdem, S. Nizamoglu, X. W. Sun, and H. V. Demir, “A photometric investigation of ultra-efficient LEDs with high color rendering index and high luminous efficacy employing nanocrystal quantum dot luminophores,” Opt. Express 18(1), 340–347 (2010), http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-1-340 .
[CrossRef] [PubMed]

S. Nizamoglu, T. Erdem, X. W. Sun, and H. V. Demir, “Warm-white light-emitting diodes integrated with colloidal quantum dots for high luminous efficacy and color rendering,” Opt. Lett. 35(20), 3372–3374 (2010), http://www.opticsinfobase.org/abstract.cfm?uri=ol-35-20-3372 .
[CrossRef] [PubMed]

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

2009 (1)

K. Sanderson, “Quantum dots go large,” Nature 459(7248), 760–761 (2009).
[CrossRef] [PubMed]

2007 (2)

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

2005 (1)

K. J. Nordell, E. M. Boatman, and G. C. Lisensky, “A safer, easier, faster synthesis for CdSe quantum dot nanocrystals,” J. Chem. Educ. 82(11), 1697–1699 (2005).
[CrossRef]

2000 (1)

D. S. Ginger and N. C. Greenham, “Charge injection and transport in films of CdSe nanocrystals,” J. Appl. Phys. 87(3), 1361–1368 (2000).
[CrossRef]

Boatman, E. M.

K. J. Nordell, E. M. Boatman, and G. C. Lisensky, “A safer, easier, faster synthesis for CdSe quantum dot nanocrystals,” J. Chem. Educ. 82(11), 1697–1699 (2005).
[CrossRef]

Coltrin, M. F.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Craford, M. G.

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

Crawford, M. H.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Demir, H. V.

Erdem, T.

Fischer, A. J.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Fleury, B.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Ginger, D. S.

D. S. Ginger and N. C. Greenham, “Charge injection and transport in films of CdSe nanocrystals,” J. Appl. Phys. 87(3), 1361–1368 (2000).
[CrossRef]

Graydon, O.

O. Graydon, “The new oil?” Nat. Photonics 5(1), 1 (2011).
[CrossRef]

Greenham, N. C.

D. S. Ginger and N. C. Greenham, “Charge injection and transport in films of CdSe nanocrystals,” J. Appl. Phys. 87(3), 1361–1368 (2000).
[CrossRef]

Harbers, G.

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

Hu, E.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Ichikawa, M.

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

Iza, M.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Jang, E.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Jang, H.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Jun, S.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Kim, B.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Kim, Y.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Krames, M. R.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

Kuo, H.-C.

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

Lim, J.

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Lin, S.-H.

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

Lisensky, G. C.

K. J. Nordell, E. M. Boatman, and G. C. Lisensky, “A safer, easier, faster synthesis for CdSe quantum dot nanocrystals,” J. Chem. Educ. 82(11), 1697–1699 (2005).
[CrossRef]

Matioli, E.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Mueller, G. O.

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Mueller-Mach, R.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

Mukai, T.

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

Narukawa, Y.

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

Nizamoglu, S.

Nordell, K. J.

K. J. Nordell, E. M. Boatman, and G. C. Lisensky, “A safer, easier, faster synthesis for CdSe quantum dot nanocrystals,” J. Chem. Educ. 82(11), 1697–1699 (2005).
[CrossRef]

Ohno, Y.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Pfaff, N.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Phillips, J. M.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Rangel, E.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Rohwer, L. E. S.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Sanderson, K.

K. Sanderson, “Quantum dots go large,” Nature 459(7248), 760–761 (2009).
[CrossRef] [PubMed]

Sanga, D.

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

Sano, M.

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

Shchekin, O. B.

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

Simmons, J. A.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Speck, J.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Sun, X. W.

Tsai, M.-A.

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

Tsao, J. Y.

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Wang, H.-W.

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

Weisbuch, C.

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

Yu, P.

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

Zhou, L.

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

Adv. Mater. (Deerfield Beach Fla.) (1)

E. Jang, S. Jun, H. Jang, J. Lim, B. Kim, and Y. Kim, “White-light-emitting diodes with quantum dot color converters for display backlights,” Adv. Mater. (Deerfield Beach Fla.) 22(28), 3076–3080 (2010).
[CrossRef] [PubMed]

Appl. Phys. Lett. (1)

E. Matioli, E. Rangel, M. Iza, B. Fleury, N. Pfaff, J. Speck, E. Hu, and C. Weisbuch, “High extraction efficiency light-emitting diodes based on embedded air-gap photonic-crystals,” Appl. Phys. Lett. 96(3), 031108 (2010).
[CrossRef]

J. Appl. Phys. (1)

D. S. Ginger and N. C. Greenham, “Charge injection and transport in films of CdSe nanocrystals,” J. Appl. Phys. 87(3), 1361–1368 (2000).
[CrossRef]

J. Chem. Educ. (1)

K. J. Nordell, E. M. Boatman, and G. C. Lisensky, “A safer, easier, faster synthesis for CdSe quantum dot nanocrystals,” J. Chem. Educ. 82(11), 1697–1699 (2005).
[CrossRef]

J. Disp. Technol. (1)

M. R. Krames, O. B. Shchekin, R. Mueller-Mach, G. O. Mueller, L. Zhou, G. Harbers, and M. G. Craford, “Status and future of high-power light-emitting diodes,” J. Disp. Technol. 3(2), 160–175 (2007).
[CrossRef]

J. Phys. D Appl. Phys. (1)

Y. Narukawa, M. Ichikawa, D. Sanga, M. Sano, and T. Mukai, “White light emitting diodes with super-high luminous efficacy,” J. Phys. D Appl. Phys. 43(35), 354002 (2010).
[CrossRef]

Jpn. J. Appl. Phys. (1)

M.-A. Tsai, H.-W. Wang, P. Yu, H.-C. Kuo, and S.-H. Lin, “High extraction efficiency of GaN-based vertical-injection light-emitting diodes using distinctive indium–tin-oxide nanorod by glancing-angle deposition,” Jpn. J. Appl. Phys. 50(5), 052102 (2011).
[CrossRef]

Laser Photon. Rev. (1)

J. M. Phillips, M. F. Coltrin, M. H. Crawford, A. J. Fischer, M. R. Krames, R. Mueller-Mach, G. O. Mueller, Y. Ohno, L. E. S. Rohwer, J. A. Simmons, and J. Y. Tsao, “Research challenges to ultra-efficient inorganic solid-state lighting,” Laser Photon. Rev. 1(4), 307–333 (2007).
[CrossRef]

Nat. Photonics (2)

O. Graydon, “The new oil?” Nat. Photonics 5(1), 1 (2011).
[CrossRef]

T. Erdem and H. V. Demir, “Semiconductor nanocrystals as rare-earth alternatives,” Nat. Photonics 5(3), 126 (2011).
[CrossRef]

Nature (1)

K. Sanderson, “Quantum dots go large,” Nature 459(7248), 760–761 (2009).
[CrossRef] [PubMed]

Opt. Express (1)

Opt. Lett. (1)

Other (4)

DEMA Electronic AG, http://www.zenigata.de (accessed on August 17, 2011).

Cree Inc, http://www.cree.com/press/enlarge.asp?i=1174480795673 (accessed on August 17, 2011).

OSRAM Opto Semiconductors GmbH, http://www.osram-os.com/osram_os/EN/Press/Press_Releases/Solid_State_Lighting/2011/From_the_OSRAM_laboratory_-_efficiency_record_for_warm_white.html (accessed on August 17, 2011).

Energy Savings Estimates of Light Emitting Diodes in Niche Lighting Applications, Building Technologies Program, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy (2011).

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