Abstract

Two-dimensional Fourier transform spectra of a three level model system are simulated using a non-perturbative density matrix formalism. The electric field distortions resultant from using pixelated pulse shaping devices to produce phase-locked pulse pairs are modeled and the effects on the recovered spectra are examined. To minimize spectral distortions, a temporal filtering scheme is employed which eliminates contributions from spurious sample polarizations.

© 2012 OSA

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    [CrossRef] [PubMed]
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2012 (2)

K. L. M. Lewis and J. P. Ogilvie, “Probing photosynthetic energy and charge transfer with two-dimensional electronic spectroscopy,” J. Phys. Chem. Lett.3(4), 503–510 (2012).
[CrossRef]

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

2011 (1)

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

2010 (2)

2009 (2)

2008 (1)

2007 (4)

E. M. Grumstrup, S.-H. Shim, M. A. Montgomery, N. H. Damrauer, and M. T. Zanni, “Facile collection of two-dimensional electronic spectra using femtosecond pulse-shaping technology,” Opt. Express15(25), 16681–16689 (2007).
[CrossRef] [PubMed]

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” Proc. Natl. Acad. Sci. U.S.A.104(36), 14197–14202 (2007).
[CrossRef] [PubMed]

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

H. Lee, Y.-C. Cheng, and G. R. Fleming, “Coherence dynamics in photosynthesis: Protein protection of excitonic coherence,” Science316(5830), 1462–1465 (2007).
[CrossRef] [PubMed]

2006 (5)

T. S. Mančal, A. V. Pisliakov, and G. R. Fleming, “Two-dimensional optical three-pulse photon echo spectroscopy. I. Nonperturbative approach to the calculation of spectra,” J. Chem. Phys.124(23), 234504 (2006).
[CrossRef] [PubMed]

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006).
[CrossRef] [PubMed]

J. Vaughan, T. Feurer, K. Stone, and K. Nelson, “Analysis of replica pulses in femtosecond pulse shaping with pixelated devices,” Opt. Express14(3), 1314–1328 (2006).
[CrossRef] [PubMed]

S. H. Shim, D. B. Strasfeld, E. C. Fulmer, and M. T. Zanni, “Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation,” Opt. Lett.31(6), 838–840 (2006).
[CrossRef] [PubMed]

2005 (1)

2004 (1)

H. Wang and M. Thoss, “Nonperturbative simulation of pump–probe spectra for electron transfer reactions in the condensed phase,” Chem. Phys. Lett.389(1-3), 43–50 (2004).
[CrossRef]

2003 (2)

D. M. Jonas, “Two-dimensional femtosecond spectroscopy,” Annu. Rev. Phys. Chem.54(1), 425–463 (2003).
[CrossRef] [PubMed]

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003).
[CrossRef] [PubMed]

2001 (1)

J. Hybl, Y. Christophe, and D. Jonas, “Peak shapes in femtosecond 2D correlation spectroscopy,” Chem. Phys.266(2-3), 295–309 (2001).
[CrossRef]

2000 (1)

A. Weiner, “Femtosecond pulse shaping using spatial light modulators,” Rev. Sci. Instrum.71(5), 1929–1960 (2000).
[CrossRef]

1999 (2)

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: theory and model calculations,” J. Phys. Chem. A103(49), 10489–10505 (1999).
[CrossRef]

A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999).
[CrossRef]

1998 (1)

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998).
[CrossRef]

1997 (1)

B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997).
[CrossRef]

1995 (1)

L. Seidner, G. Stock, and W. Domcke, “Nonperturbative approach to femtosecond spectroscopy: General theory and application to multidimensional nonadiabatic photoisomerization processes,” J. Chem. Phys.103(10), 3998–4011 (1995).
[CrossRef]

1985 (1)

Ahn, T.-K.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

Albrecht, A.

A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999).
[CrossRef]

Albrecht, A. W.

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998).
[CrossRef]

Blankenship, R. E.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

Brixner, T.

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006).
[CrossRef] [PubMed]

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Buback, J.

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

Calhoun, T. R.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

Cheng, Y.-C.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

H. Lee, Y.-C. Cheng, and G. R. Fleming, “Coherence dynamics in photosynthesis: Protein protection of excitonic coherence,” Science316(5830), 1462–1465 (2007).
[CrossRef] [PubMed]

Christophe, Y.

J. Hybl, Y. Christophe, and D. Jonas, “Peak shapes in femtosecond 2D correlation spectroscopy,” Chem. Phys.266(2-3), 295–309 (2001).
[CrossRef]

Cogdell, R. J.

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Damrauer, N. H.

DeSilvestri, S.

Domcke, W.

B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997).
[CrossRef]

L. Seidner, G. Stock, and W. Domcke, “Nonperturbative approach to femtosecond spectroscopy: General theory and application to multidimensional nonadiabatic photoisomerization processes,” J. Chem. Phys.103(10), 3998–4011 (1995).
[CrossRef]

Engel, G. S.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

Faeder, S.

A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999).
[CrossRef]

Feurer, T.

Fleming, G. R.

H. Lee, Y.-C. Cheng, and G. R. Fleming, “Coherence dynamics in photosynthesis: Protein protection of excitonic coherence,” Science316(5830), 1462–1465 (2007).
[CrossRef] [PubMed]

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006).
[CrossRef] [PubMed]

T. S. Mančal, A. V. Pisliakov, and G. R. Fleming, “Two-dimensional optical three-pulse photon echo spectroscopy. I. Nonperturbative approach to the calculation of spectra,” J. Chem. Phys.124(23), 234504 (2006).
[CrossRef] [PubMed]

Fuller, F. D.

Fulmer, E. C.

Gallagher Faeder, S. M.

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: theory and model calculations,” J. Phys. Chem. A103(49), 10489–10505 (1999).
[CrossRef]

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998).
[CrossRef]

Gardiner, A. T.

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Grumstrup, E. M.

Hybl, J.

J. Hybl, Y. Christophe, and D. Jonas, “Peak shapes in femtosecond 2D correlation spectroscopy,” Chem. Phys.266(2-3), 295–309 (2001).
[CrossRef]

A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999).
[CrossRef]

Hybl, J. D.

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998).
[CrossRef]

Ippen, E. P.

Jonas, D.

J. Hybl, Y. Christophe, and D. Jonas, “Peak shapes in femtosecond 2D correlation spectroscopy,” Chem. Phys.266(2-3), 295–309 (2001).
[CrossRef]

A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999).
[CrossRef]

Jonas, D. M.

D. M. Jonas, “Two-dimensional femtosecond spectroscopy,” Annu. Rev. Phys. Chem.54(1), 425–463 (2003).
[CrossRef] [PubMed]

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: theory and model calculations,” J. Phys. Chem. A103(49), 10489–10505 (1999).
[CrossRef]

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998).
[CrossRef]

Keusters, D.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003).
[CrossRef] [PubMed]

Kotur, M.

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

Kullmann, M.

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

Lee, H.

H. Lee, Y.-C. Cheng, and G. R. Fleming, “Coherence dynamics in photosynthesis: Protein protection of excitonic coherence,” Science316(5830), 1462–1465 (2007).
[CrossRef] [PubMed]

Lewis, K. L. M.

Li, C.

Ling, Y. L.

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” Proc. Natl. Acad. Sci. U.S.A.104(36), 14197–14202 (2007).
[CrossRef] [PubMed]

Mancal, T.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Mancal, T. S.

T. S. Mančal, A. V. Pisliakov, and G. R. Fleming, “Two-dimensional optical three-pulse photon echo spectroscopy. I. Nonperturbative approach to the calculation of spectra,” J. Chem. Phys.124(23), 234504 (2006).
[CrossRef] [PubMed]

Matsika, S.

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

C. H. Tseng, S. Matsika, and T. C. Weinacht, “Two-dimensional ultrafast Fourier transform spectroscopy in the deep ultraviolet,” Opt. Express17(21), 18788–18793 (2009).
[CrossRef] [PubMed]

Montgomery, M. A.

Myers, J. A.

Nelson, K.

Nuernberger, P.

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

Ogilvie, J. P.

Pisliakov, A. V.

T. S. Mančal, A. V. Pisliakov, and G. R. Fleming, “Two-dimensional optical three-pulse photon echo spectroscopy. I. Nonperturbative approach to the calculation of spectra,” J. Chem. Phys.124(23), 234504 (2006).
[CrossRef] [PubMed]

Read, E. L.

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Ruetzel, S.

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

Sándor, P.

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

Seidner, L.

B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997).
[CrossRef]

L. Seidner, G. Stock, and W. Domcke, “Nonperturbative approach to femtosecond spectroscopy: General theory and application to multidimensional nonadiabatic photoisomerization processes,” J. Chem. Phys.103(10), 3998–4011 (1995).
[CrossRef]

Semmlow, J.

Shim, S. H.

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” Proc. Natl. Acad. Sci. U.S.A.104(36), 14197–14202 (2007).
[CrossRef] [PubMed]

S. H. Shim, D. B. Strasfeld, E. C. Fulmer, and M. T. Zanni, “Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation,” Opt. Lett.31(6), 838–840 (2006).
[CrossRef] [PubMed]

Shim, S.-H.

Stiopkin, I.

I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006).
[CrossRef] [PubMed]

Stock, G.

B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997).
[CrossRef]

L. Seidner, G. Stock, and W. Domcke, “Nonperturbative approach to femtosecond spectroscopy: General theory and application to multidimensional nonadiabatic photoisomerization processes,” J. Chem. Phys.103(10), 3998–4011 (1995).
[CrossRef]

Stone, K.

Strasfeld, D. B.

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” Proc. Natl. Acad. Sci. U.S.A.104(36), 14197–14202 (2007).
[CrossRef] [PubMed]

S. H. Shim, D. B. Strasfeld, E. C. Fulmer, and M. T. Zanni, “Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation,” Opt. Lett.31(6), 838–840 (2006).
[CrossRef] [PubMed]

Suzaki, Y.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003).
[CrossRef] [PubMed]

Tekavec, P. F.

Thoss, M.

H. Wang and M. Thoss, “Nonperturbative simulation of pump–probe spectra for electron transfer reactions in the condensed phase,” Chem. Phys. Lett.389(1-3), 43–50 (2004).
[CrossRef]

Tian, P.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003).
[CrossRef] [PubMed]

Tseng, C. H.

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

C. H. Tseng, S. Matsika, and T. C. Weinacht, “Two-dimensional ultrafast Fourier transform spectroscopy in the deep ultraviolet,” Opt. Express17(21), 18788–18793 (2009).
[CrossRef] [PubMed]

Vaughan, J.

Wagner, W.

Wang, H.

H. Wang and M. Thoss, “Nonperturbative simulation of pump–probe spectra for electron transfer reactions in the condensed phase,” Chem. Phys. Lett.389(1-3), 43–50 (2004).
[CrossRef]

Warren, W.

Warren, W. S.

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003).
[CrossRef] [PubMed]

Weinacht, T. C.

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

C. H. Tseng, S. Matsika, and T. C. Weinacht, “Two-dimensional ultrafast Fourier transform spectroscopy in the deep ultraviolet,” Opt. Express17(21), 18788–18793 (2009).
[CrossRef] [PubMed]

Weiner, A.

A. Weiner, “Femtosecond pulse shaping using spatial light modulators,” Rev. Sci. Instrum.71(5), 1929–1960 (2000).
[CrossRef]

Weiner, A. M.

Wolfseder, B.

B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997).
[CrossRef]

Yang, M.

I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006).
[CrossRef] [PubMed]

Zanni, M. T.

Zigmantas, D.

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Annu. Rev. Phys. Chem. (1)

D. M. Jonas, “Two-dimensional femtosecond spectroscopy,” Annu. Rev. Phys. Chem.54(1), 425–463 (2003).
[CrossRef] [PubMed]

Chem. Phys. (2)

B. Wolfseder, L. Seidner, G. Stock, and W. Domcke, “Femtosecond pump-probe spectroscopy of electron-transfer systems: a nonperturbative approach,” Chem. Phys.217(2-3), 275–287 (1997).
[CrossRef]

J. Hybl, Y. Christophe, and D. Jonas, “Peak shapes in femtosecond 2D correlation spectroscopy,” Chem. Phys.266(2-3), 295–309 (2001).
[CrossRef]

Chem. Phys. Lett. (2)

H. Wang and M. Thoss, “Nonperturbative simulation of pump–probe spectra for electron transfer reactions in the condensed phase,” Chem. Phys. Lett.389(1-3), 43–50 (2004).
[CrossRef]

J. D. Hybl, A. W. Albrecht, S. M. Gallagher Faeder, and D. M. Jonas, “Two-dimensional electronic spectroscopy,” Chem. Phys. Lett.297(3-4), 307–313 (1998).
[CrossRef]

J. Am. Chem. Soc. (1)

M. Kullmann, S. Ruetzel, J. Buback, P. Nuernberger, and T. Brixner, “Reaction dynamics of a molecular switch unveiled by coherent two-dimensional electronic spectroscopy,” J. Am. Chem. Soc.133(33), 13074–13080 (2011).
[CrossRef] [PubMed]

J. Chem. Phys. (3)

T. S. Mančal, A. V. Pisliakov, and G. R. Fleming, “Two-dimensional optical three-pulse photon echo spectroscopy. I. Nonperturbative approach to the calculation of spectra,” J. Chem. Phys.124(23), 234504 (2006).
[CrossRef] [PubMed]

A. Albrecht, J. Hybl, S. Faeder, and D. Jonas, “Experimental distinction between phase shifts and time delays: Implications for femtosecond spectroscopy and coherent control of chemical reactions,” J. Chem. Phys.111(24), 10934–10956 (1999).
[CrossRef]

L. Seidner, G. Stock, and W. Domcke, “Nonperturbative approach to femtosecond spectroscopy: General theory and application to multidimensional nonadiabatic photoisomerization processes,” J. Chem. Phys.103(10), 3998–4011 (1995).
[CrossRef]

J. Opt. Soc. Am. B (2)

J. Phys. Chem. A (2)

S. M. Gallagher Faeder and D. M. Jonas, “Two-dimensional electronic correlation and relaxation spectra: theory and model calculations,” J. Phys. Chem. A103(49), 10489–10505 (1999).
[CrossRef]

C. H. Tseng, P. Sándor, M. Kotur, T. C. Weinacht, and S. Matsika, “Two-dimensional Fourier transform spectroscopy of adenine and uracil using shaped ultrafast laser pulses in the deep UV,” J. Phys. Chem. A116(11), 2654–2661 (2012).
[CrossRef] [PubMed]

J. Phys. Chem. B (1)

I. Stiopkin, T. Brixner, M. Yang, and G. R. Fleming, “Heterogeneous exciton dynamics revealed by two-dimensional optical spectroscopy,” J. Phys. Chem. B110(40), 20032–20037 (2006).
[CrossRef] [PubMed]

J. Phys. Chem. Lett. (1)

K. L. M. Lewis and J. P. Ogilvie, “Probing photosynthetic energy and charge transfer with two-dimensional electronic spectroscopy,” J. Phys. Chem. Lett.3(4), 503–510 (2012).
[CrossRef]

Nature (1)

G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mančal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007).
[CrossRef] [PubMed]

Opt. Express (6)

Opt. Lett. (2)

Proc. Natl. Acad. Sci. U.S.A. (2)

S. H. Shim, D. B. Strasfeld, Y. L. Ling, and M. T. Zanni, “Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide,” Proc. Natl. Acad. Sci. U.S.A.104(36), 14197–14202 (2007).
[CrossRef] [PubMed]

D. Zigmantas, E. L. Read, T. Mančal, T. Brixner, A. T. Gardiner, R. J. Cogdell, and G. R. Fleming, “Two-dimensional electronic spectroscopy of the B800-B820 light-harvesting complex,” Proc. Natl. Acad. Sci. U.S.A.103(34), 12672–12677 (2006).
[CrossRef] [PubMed]

Rev. Sci. Instrum. (1)

A. Weiner, “Femtosecond pulse shaping using spatial light modulators,” Rev. Sci. Instrum.71(5), 1929–1960 (2000).
[CrossRef]

Science (2)

P. Tian, D. Keusters, Y. Suzaki, and W. S. Warren, “Femtosecond phase-coherent two-dimensional spectroscopy,” Science300(5625), 1553–1555 (2003).
[CrossRef] [PubMed]

H. Lee, Y.-C. Cheng, and G. R. Fleming, “Coherence dynamics in photosynthesis: Protein protection of excitonic coherence,” Science316(5830), 1462–1465 (2007).
[CrossRef] [PubMed]

Other (4)

S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University Press, 1995).

D. Jonas, (personal communication, August 10, 2011).

K. Blum, Density Matrix Theory and Applications, Physics of Atoms and Molecules, 2nd ed., (Plenum Press, 1996).

R. W. Boyd, Nonlinear Optics, 3rd ed. (Elsevier/Academic Press, 2008).

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