Abstract

We demonstrate a photonic metamaterial that shows extraordinary sensitivity to the presence of a single atomic layer of graphene on its surface. Metamaterial's optical transmission increases multi-fold at the resonance frequency linked to the Fano-type plasmonic mode supported by the periodic metallic nanostructure. The experiments were performed with chemical vapor deposited (CVD) graphene covering a number of size-scaled metamaterial samples with plasmonic modes at different frequencies ranging from 167 to 187 Thz.

© 2010 OSA

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2009 (6)

M. Jablan, H. Buljan, and M. Soljacic, “Plasmonics in graphene at infrared frequencies,” Phys. Rev. B 80(24), 245435 (2009).
[CrossRef]

X. Wang, M. Zhao, and D. D. Nolte, “Optical contrast and clarity of graphene on an arbitrary substrate,” Appl. Phys. Lett. 95(8), 081102 (2009).
[CrossRef]

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

B. Lahiri, A. Z. Khokhar, R. M. De La Rue, S. G. McMeekin, and N. P. Johnson, “Asymmetric split ring resonators for optical sensing of organic materials,” Opt. Express 17(2), 1107–1115 (2009).
[CrossRef] [PubMed]

2008 (6)

H. J. Lee and J. G. Yook, “Biosensing using split-ring resonators at microwave regime,” Appl. Phys. Lett. 92(25), 254103 (2008).
[CrossRef]

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

A. Banerjee and H. Grebel, “Depositing graphene films on solid and perforated substrates,” Nanotechnology 19(36), 365303 (2008).
[CrossRef] [PubMed]

I. A. I. Al-Naib, C. Jensen, and M. Koch, “Thin-film sensing with planar asymmetric metamaterial resonators,” Appl. Phys. Lett. 93(8), 083507 (2008).
[CrossRef]

M. Freitag, “Graphene: nanoelectronics goes flat out,” Nat. Nanotechnol. 3(8), 455–457 (2008).
[CrossRef] [PubMed]

X. Du, I. Skachko, A. Barker, and E. Y. Andrei, “Approaching ballistic transport in suspended graphene,” Nat. Nanotechnol. 3(8), 491–495 (2008).
[CrossRef] [PubMed]

2007 (8)

A. K. Geim and K. S. Novoselov, “The rise of graphene,” Nat. Mater. 6(3), 183–191 (2007).
[CrossRef] [PubMed]

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

D. S. L. Abergel, A. Russell, and V. I.. Falko, “Visibility of graphene falkes on a dielectric substrate,” Appl. Phys. Lett. 91(6), 063125 (2007).
[CrossRef]

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

C. Debus and P. H. Bolivar, “Frequency selective surfaces for high sensitivity terahertz sensing,” Appl. Phys. Lett. 91(18), 184102 (2007).
[CrossRef]

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

K. Chang, J. T. Liu, J. B. Xia, and N. Dai, “Enhanced visibility of graphene: Effect of one-dimensional photonic crystal,” Appl. Phys. Lett. 91(18), 181906 (2007).
[CrossRef]

2006 (2)

A. H. Castro Neto, F. Guinea, and N. M. R. Peres, “Drawing conclusions from graphene,” Physics World 19, 33–37 (2006).

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

2005 (2)

Y. Zhang, Y. W. Tan, H. L. Stormer, and P. Kim, “Experimental observation of the quantum Hall effect and Berry’s phase in graphene,” Nature 438(7065), 201–204 (2005).
[CrossRef] [PubMed]

A. Ishimaru, S. Jaruwatanadilok, and Y. Kuga, “Generalized surface Plasmon resonance sensors using metamaterials and negative index materials,” PIERS 51, 139–152 (2005).
[CrossRef]

2004 (1)

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Abergel, D. S. L.

D. S. L. Abergel, A. Russell, and V. I.. Falko, “Visibility of graphene falkes on a dielectric substrate,” Appl. Phys. Lett. 91(6), 063125 (2007).
[CrossRef]

Al-Naib, I. A. I.

I. A. I. Al-Naib, C. Jensen, and M. Koch, “Thin-film sensing with planar asymmetric metamaterial resonators,” Appl. Phys. Lett. 93(8), 083507 (2008).
[CrossRef]

An, J. H.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Andreev, G. O.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Andrei, E. Y.

X. Du, I. Skachko, A. Barker, and E. Y. Andrei, “Approaching ballistic transport in suspended graphene,” Nat. Nanotechnol. 3(8), 491–495 (2008).
[CrossRef] [PubMed]

Banerjee, A.

A. Banerjee and H. Grebel, “Depositing graphene films on solid and perforated substrates,” Nanotechnology 19(36), 365303 (2008).
[CrossRef] [PubMed]

Banerjee, S. K.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Barker, A.

X. Du, I. Skachko, A. Barker, and E. Y. Andrei, “Approaching ballistic transport in suspended graphene,” Nat. Nanotechnol. 3(8), 491–495 (2008).
[CrossRef] [PubMed]

Bartal, G.

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

Basov, D. N.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Blake, P.

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

Bolivar, P. H.

C. Debus and P. H. Bolivar, “Frequency selective surfaces for high sensitivity terahertz sensing,” Appl. Phys. Lett. 91(18), 184102 (2007).
[CrossRef]

Booth, T. J.

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

Buljan, H.

M. Jablan, H. Buljan, and M. Soljacic, “Plasmonics in graphene at infrared frequencies,” Phys. Rev. B 80(24), 245435 (2009).
[CrossRef]

Cai, W. W.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Castro Neto, A. H.

A. H. Castro Neto, F. Guinea, and N. M. R. Peres, “Drawing conclusions from graphene,” Physics World 19, 33–37 (2006).

Chang, K.

K. Chang, J. T. Liu, J. B. Xia, and N. Dai, “Enhanced visibility of graphene: Effect of one-dimensional photonic crystal,” Appl. Phys. Lett. 91(18), 181906 (2007).
[CrossRef]

Cho, S. Y.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Colombo, L.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Cubukcu, E.

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

Dai, N.

K. Chang, J. T. Liu, J. B. Xia, and N. Dai, “Enhanced visibility of graphene: Effect of one-dimensional photonic crystal,” Appl. Phys. Lett. 91(18), 181906 (2007).
[CrossRef]

De La Rue, R. M.

Debus, C.

C. Debus and P. H. Bolivar, “Frequency selective surfaces for high sensitivity terahertz sensing,” Appl. Phys. Lett. 91(18), 184102 (2007).
[CrossRef]

Driscoll, T.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Du, X.

X. Du, I. Skachko, A. Barker, and E. Y. Andrei, “Approaching ballistic transport in suspended graphene,” Nat. Nanotechnol. 3(8), 491–495 (2008).
[CrossRef] [PubMed]

Dubonos, S. V.

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Fal’ko, V. I.

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

Falko, V. I..

D. S. L. Abergel, A. Russell, and V. I.. Falko, “Visibility of graphene falkes on a dielectric substrate,” Appl. Phys. Lett. 91(6), 063125 (2007).
[CrossRef]

Fan, H. M.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Fedotov, V. A.

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

Feng, Y. P.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Firsov, A. A.

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Freitag, M.

M. Freitag, “Graphene: nanoelectronics goes flat out,” Nat. Nanotechnol. 3(8), 455–457 (2008).
[CrossRef] [PubMed]

Fu, Y. H.

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

Geim, A. K.

A. K. Geim and K. S. Novoselov, “The rise of graphene,” Nat. Mater. 6(3), 183–191 (2007).
[CrossRef] [PubMed]

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Grebel, H.

A. Banerjee and H. Grebel, “Depositing graphene films on solid and perforated substrates,” Nanotechnology 19(36), 365303 (2008).
[CrossRef] [PubMed]

Grigorieva, I. V.

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Guinea, F.

A. H. Castro Neto, F. Guinea, and N. M. R. Peres, “Drawing conclusions from graphene,” Physics World 19, 33–37 (2006).

Guo, Z.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Hill, E. W.

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

Ishimaru, A.

A. Ishimaru, S. Jaruwatanadilok, and Y. Kuga, “Generalized surface Plasmon resonance sensors using metamaterials and negative index materials,” PIERS 51, 139–152 (2005).
[CrossRef]

Jablan, M.

M. Jablan, H. Buljan, and M. Soljacic, “Plasmonics in graphene at infrared frequencies,” Phys. Rev. B 80(24), 245435 (2009).
[CrossRef]

Jaruwatanadilok, S.

A. Ishimaru, S. Jaruwatanadilok, and Y. Kuga, “Generalized surface Plasmon resonance sensors using metamaterials and negative index materials,” PIERS 51, 139–152 (2005).
[CrossRef]

Jensen, C.

I. A. I. Al-Naib, C. Jensen, and M. Koch, “Thin-film sensing with planar asymmetric metamaterial resonators,” Appl. Phys. Lett. 93(8), 083507 (2008).
[CrossRef]

Jiang, D.

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Johnson, N. P.

Jokerst, N. M.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Jung, I.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Kasim, J.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Katsnelson, M. I.

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

Khokhar, A. Z.

Kim, P.

Y. Zhang, Y. W. Tan, H. L. Stormer, and P. Kim, “Experimental observation of the quantum Hall effect and Berry’s phase in graphene,” Nature 438(7065), 201–204 (2005).
[CrossRef] [PubMed]

Kim, S.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Koch, M.

I. A. I. Al-Naib, C. Jensen, and M. Koch, “Thin-film sensing with planar asymmetric metamaterial resonators,” Appl. Phys. Lett. 93(8), 083507 (2008).
[CrossRef]

Kuga, Y.

A. Ishimaru, S. Jaruwatanadilok, and Y. Kuga, “Generalized surface Plasmon resonance sensors using metamaterials and negative index materials,” PIERS 51, 139–152 (2005).
[CrossRef]

Lahiri, B.

Lee, H. J.

H. J. Lee and J. G. Yook, “Biosensing using split-ring resonators at microwave regime,” Appl. Phys. Lett. 92(25), 254103 (2008).
[CrossRef]

Li, X. S.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Liu, J. T.

K. Chang, J. T. Liu, J. B. Xia, and N. Dai, “Enhanced visibility of graphene: Effect of one-dimensional photonic crystal,” Appl. Phys. Lett. 91(18), 181906 (2007).
[CrossRef]

McCann, E.

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

McMeekin, S. G.

Morozov, S. V.

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Nah, J.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Neto, A. H. C.

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

Ni, Z.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Ni, Z. H.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Nolte, D. D.

X. Wang, M. Zhao, and D. D. Nolte, “Optical contrast and clarity of graphene on an arbitrary substrate,” Appl. Phys. Lett. 95(8), 081102 (2009).
[CrossRef]

Novoselov, K. S.

A. K. Geim and K. S. Novoselov, “The rise of graphene,” Nat. Mater. 6(3), 183–191 (2007).
[CrossRef] [PubMed]

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Palit, S.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Papasimakis, N.

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

Park, Y. S.

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

Peres, N. M. R.

A. H. Castro Neto, F. Guinea, and N. M. R. Peres, “Drawing conclusions from graphene,” Physics World 19, 33–37 (2006).

Piner, R. D.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Prosvirnin, S. L.

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

Rose, M.

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

Ruoff, R. S.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Russell, A.

D. S. L. Abergel, A. Russell, and V. I.. Falko, “Visibility of graphene falkes on a dielectric substrate,” Appl. Phys. Lett. 91(6), 063125 (2007).
[CrossRef]

Schedin, F.

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

Shen, Z.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Shen, Z. X.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Skachko, I.

X. Du, I. Skachko, A. Barker, and E. Y. Andrei, “Approaching ballistic transport in suspended graphene,” Nat. Nanotechnol. 3(8), 491–495 (2008).
[CrossRef] [PubMed]

Smith, D. R.

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

Soljacic, M.

M. Jablan, H. Buljan, and M. Soljacic, “Plasmonics in graphene at infrared frequencies,” Phys. Rev. B 80(24), 245435 (2009).
[CrossRef]

Stormer, H. L.

Y. Zhang, Y. W. Tan, H. L. Stormer, and P. Kim, “Experimental observation of the quantum Hall effect and Berry’s phase in graphene,” Nature 438(7065), 201–204 (2005).
[CrossRef] [PubMed]

Tan, Y. W.

Y. Zhang, Y. W. Tan, H. L. Stormer, and P. Kim, “Experimental observation of the quantum Hall effect and Berry’s phase in graphene,” Nature 438(7065), 201–204 (2005).
[CrossRef] [PubMed]

Teo, G.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Tsai, D. P.

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

Tutuc, E.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Velamakanni, A.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Wang, H.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Wang, H. M.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Wang, X.

X. Wang, M. Zhao, and D. D. Nolte, “Optical contrast and clarity of graphene on an arbitrary substrate,” Appl. Phys. Lett. 95(8), 081102 (2009).
[CrossRef]

Wu, Y.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Wu, Y. H.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Xia, J. B.

K. Chang, J. T. Liu, J. B. Xia, and N. Dai, “Enhanced visibility of graphene: Effect of one-dimensional photonic crystal,” Appl. Phys. Lett. 91(18), 181906 (2007).
[CrossRef]

Yang, D. X.

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

Yang, R.

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

Yook, J. G.

H. J. Lee and J. G. Yook, “Biosensing using split-ring resonators at microwave regime,” Appl. Phys. Lett. 92(25), 254103 (2008).
[CrossRef]

Yu, T.

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Zeitler, U.

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

Zhang, J.

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Zhang, S.

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

Zhang, X.

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

Zhang, Y.

Y. Zhang, Y. W. Tan, H. L. Stormer, and P. Kim, “Experimental observation of the quantum Hall effect and Berry’s phase in graphene,” Nature 438(7065), 201–204 (2005).
[CrossRef] [PubMed]

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Zhao, M.

X. Wang, M. Zhao, and D. D. Nolte, “Optical contrast and clarity of graphene on an arbitrary substrate,” Appl. Phys. Lett. 95(8), 081102 (2009).
[CrossRef]

Zheludev, N. I.

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

Appl. Phys. Lett. (9)

P. Blake, E. W. Hill, A. H. C. Neto, K. S. Novoselov, D. Jiang, R. Yang, T. J. Booth, and A. K. Geim, “Making graphene visible,” Appl. Phys. Lett. 91(6), 063124 (2007).
[CrossRef]

X. Wang, M. Zhao, and D. D. Nolte, “Optical contrast and clarity of graphene on an arbitrary substrate,” Appl. Phys. Lett. 95(8), 081102 (2009).
[CrossRef]

K. Chang, J. T. Liu, J. B. Xia, and N. Dai, “Enhanced visibility of graphene: Effect of one-dimensional photonic crystal,” Appl. Phys. Lett. 91(18), 181906 (2007).
[CrossRef]

I. A. I. Al-Naib, C. Jensen, and M. Koch, “Thin-film sensing with planar asymmetric metamaterial resonators,” Appl. Phys. Lett. 93(8), 083507 (2008).
[CrossRef]

T. Driscoll, G. O. Andreev, D. N. Basov, S. Palit, S. Y. Cho, N. M. Jokerst, and D. R. Smith, “Tuned permeability in terahertz split-ring resonators for devices and sensors,” Appl. Phys. Lett. 91(6), 062511 (2007).
[CrossRef]

C. Debus and P. H. Bolivar, “Frequency selective surfaces for high sensitivity terahertz sensing,” Appl. Phys. Lett. 91(18), 184102 (2007).
[CrossRef]

H. J. Lee and J. G. Yook, “Biosensing using split-ring resonators at microwave regime,” Appl. Phys. Lett. 92(25), 254103 (2008).
[CrossRef]

E. Cubukcu, S. Zhang, Y. S. Park, G. Bartal, and X. Zhang, “Split ring resonator sensors for infrared detection of single molecular monolayers,” Appl. Phys. Lett. 95(4), 043113 (2009).
[CrossRef]

D. S. L. Abergel, A. Russell, and V. I.. Falko, “Visibility of graphene falkes on a dielectric substrate,” Appl. Phys. Lett. 91(6), 063125 (2007).
[CrossRef]

J. Appl. Phys. (1)

G. Teo, H. Wang, Y. Wu, Z. Guo, J. Zhang, Z. Ni, and Z. Shen, “Visibility study of graphene multilayer structures,” J. Appl. Phys. 103(12), 124302 (2008).
[CrossRef]

Nano Lett. (1)

Z. H. Ni, H. M. Wang, J. Kasim, H. M. Fan, T. Yu, Y. H. Wu, Y. P. Feng, and Z. X. Shen, “Graphene thickness determination using reflection and contrast spectroscopy,” Nano Lett. 7(9), 2758–2763 (2007).
[CrossRef] [PubMed]

Nanotechnology (1)

A. Banerjee and H. Grebel, “Depositing graphene films on solid and perforated substrates,” Nanotechnology 19(36), 365303 (2008).
[CrossRef] [PubMed]

Nat. Mater. (1)

A. K. Geim and K. S. Novoselov, “The rise of graphene,” Nat. Mater. 6(3), 183–191 (2007).
[CrossRef] [PubMed]

Nat. Nanotechnol. (2)

M. Freitag, “Graphene: nanoelectronics goes flat out,” Nat. Nanotechnol. 3(8), 455–457 (2008).
[CrossRef] [PubMed]

X. Du, I. Skachko, A. Barker, and E. Y. Andrei, “Approaching ballistic transport in suspended graphene,” Nat. Nanotechnol. 3(8), 491–495 (2008).
[CrossRef] [PubMed]

Nat. Phys. (1)

K. S. Novoselov, E. McCann, S. V. Morozov, V. I. Fal’ko, M. I. Katsnelson, U. Zeitler, D. Jiang, F. Schedin, and A. K. Geim, “Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene,” Nat. Phys. 2(3), 177–180 (2006).
[CrossRef]

Nature (1)

Y. Zhang, Y. W. Tan, H. L. Stormer, and P. Kim, “Experimental observation of the quantum Hall effect and Berry’s phase in graphene,” Nature 438(7065), 201–204 (2005).
[CrossRef] [PubMed]

Opt. Express (1)

Phys. Rev. B (2)

N. Papasimakis, V. A. Fedotov, Y. H. Fu, D. P. Tsai, and N. I. Zheludev, “Coherent and incoherent metamaterials and order-disorderr transitions,” Phys. Rev. B 80(4), 041102 (2009).
[CrossRef]

M. Jablan, H. Buljan, and M. Soljacic, “Plasmonics in graphene at infrared frequencies,” Phys. Rev. B 80(24), 245435 (2009).
[CrossRef]

Phys. Rev. Lett. (1)

V. A. Fedotov, M. Rose, S. L. Prosvirnin, N. Papasimakis, and N. I. Zheludev, “Sharp trapped-mode resonances in planar metamaterials with a broken structural symmetry,” Phys. Rev. Lett. 99(14), 147401 (2007).
[CrossRef] [PubMed]

Physics World (1)

A. H. Castro Neto, F. Guinea, and N. M. R. Peres, “Drawing conclusions from graphene,” Physics World 19, 33–37 (2006).

PIERS (1)

A. Ishimaru, S. Jaruwatanadilok, and Y. Kuga, “Generalized surface Plasmon resonance sensors using metamaterials and negative index materials,” PIERS 51, 139–152 (2005).
[CrossRef]

Science (2)

X. S. Li, W. W. Cai, J. H. An, S. Kim, J. Nah, D. X. Yang, R. D. Piner, A. Velamakanni, I. Jung, E. Tutuc, S. K. Banerjee, L. Colombo, and R. S. Ruoff, “Large-area synthesis of high-quality and uniform graphene films on copper foils,” Science 324(5932), 1312–1314 (2009).
[CrossRef] [PubMed]

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[CrossRef] [PubMed]

Other (2)

V. V. Khardikov, E. O. Iarko, and S. L. Prosvirnin, “Trapping of light by metal arrays,” submitted for publication.

V. A. Fedotov, N. Papasimakis, E. Plum, A. Bitzer, M. Walther, P. Kuo, D. P. Tsai, and N. I. Zheludev, “Spectral collapse in ensembles of meta-molecules,” http://arxiv.org/abs/0908.2533 .

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Figures (3)

Fig. 1
Fig. 1

(a) Schematic of the fabricated complementary split-ring metamaterial. (b) Microscope photograph of six metamaterial arrays after deposition of graphene: Note the boundary between the covered and non-covered areas. (c) Raman spectrum corresponding to the marked region in (b).

Fig. 3
Fig. 3

(a) Experimental transmission spectrum of an ASR array before (dashed black line) and after (red solid line) deposition of graphene for unit cell size D = 711nm as shown in the inset. The vertical dashed lines mark the position of the trapped-mode (α) and the long-wavelength dipole (β) resonance, before and after graphene deposition. (b) Wavelength shift of the trapped-mode (α) and of the dipole (β) resonance resulting from the deposition of the graphene layer as a function of unit cell size. (c) Electric field maps at the trapped-mode (α) and the dipole (β) resonance.

Fig. 2
Fig. 2

Transmission contrast of the graphene covered metamaterial arrays for five different values of the unit cell side D, displaced along the vertical axis. Dashed black lines mark the zero contrast level.

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