Abstract

We experimentally investigate the high harmonic generation (HHG) from CH4 molecules and Xe atoms in a two-color field (using the 800nm laser and the tunable laser with the longer wavelength from 1500nm to 1900nm), and observe that the longer wavelength component can destructively suppress the HHG from CH4 molecules. By controlling the time delay between the two color laser pulses or tuning the laser intensity of the longer wavelength component, the suppressions of the HHG from CH4 molecules and the enhancements of the HHG from Xe atoms at the same laser condition are observed. The results indicate that the longer wavelength component around the molecular infrared absorption can suppress the molecular HHG process.

© 2010 OSA

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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  4. C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef] [PubMed]
  17. F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
    [CrossRef] [PubMed]
  18. C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
    [CrossRef]
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    [CrossRef] [PubMed]
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    [CrossRef]
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    [CrossRef]

2010 (1)

C. Liu, Z. Zeng, P. Wei, P. Liu, R. Li, and Z. Xu, “Driving-laser wavelength dependence of high-order harmonic generation in H2+ molecules,” Phys. Rev. A 81(3), 033426 (2010).
[CrossRef]

2009 (4)

2008 (2)

A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008).
[CrossRef] [PubMed]

Y. Zheng, Z. Zeng, X. Li, X. Chen, P. Liu, H. Xiong, H. Lu, S. Zhao, P. Wei, L. Zhang, Z. Wang, J. Liu, Y. Cheng, R. Li, and Z. Xu, “Enhancement and broadening of extreme-ultraviolet supercontinuum in a relative phase controlled two-color laser field,” Opt. Lett. 33(3), 234–236 (2008).
[CrossRef] [PubMed]

2007 (2)

2006 (3)

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

2005 (4)

T. Kanai, S. Minemoto, and H. Sakai, “Quantum interference during high-order harmonic generation from aligned molecules,” Nature 435(7041), 470–474 (2005).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

M. Lein, “Attosecond probing of vibrational dynamics with high-harmonic generation,” Phys. Rev. Lett. 94(5), 053004 (2005).
[CrossRef] [PubMed]

2004 (2)

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

1999 (1)

A. Talebpour, A. D. Bandrauk, J. Yang, and S. L. Chin, “Multiphoton ionization of inner-valence electrons and fragmentation of ethylene in an intense Ti:sapphire laser pulse,” Chem. Phys. Lett. 313(5-6), 789–794 (1999).
[CrossRef]

1994 (1)

R. Lemus and A. Frank, “Algebraic approach to vibrational spectra of tetrahedral molecules: Application to methane,” J. Chem. Phys. 101(10), 8321 (1994).
[CrossRef]

1993 (1)

P. B. Corkum, “Plasma perspective on strong field multiphoton ionization,” Phys. Rev. Lett. 71(13), 1994–1997 (1993).
[CrossRef] [PubMed]

Altucci, C.

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Auguste, T.

Avaldi, L.

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

Baker, S.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Bandrauk, A. D.

A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008).
[CrossRef] [PubMed]

A. Talebpour, A. D. Bandrauk, J. Yang, and S. L. Chin, “Multiphoton ionization of inner-valence electrons and fragmentation of ethylene in an intense Ti:sapphire laser pulse,” Chem. Phys. Lett. 313(5-6), 789–794 (1999).
[CrossRef]

Benedetti, E.

C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007).
[CrossRef] [PubMed]

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Boutu, W.

Calegari, F.

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Carré, B.

Caumes, J. P.

H. Merdji, T. Auguste, W. Boutu, J. P. Caumes, B. Carré, T. Pfeifer, A. Jullien, D. M. Neumark, and S. R. Leone, “Isolated attosecond pulses using a detuned second-harmonic field,” Opt. Lett. 32(21), 3134–3136 (2007).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Cerullo, G.

Chelkowski, S.

A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008).
[CrossRef] [PubMed]

Chen, X.

Cheng, Y.

Chin, S. L.

A. Talebpour, A. D. Bandrauk, J. Yang, and S. L. Chin, “Multiphoton ionization of inner-valence electrons and fragmentation of ethylene in an intense Ti:sapphire laser pulse,” Chem. Phys. Lett. 313(5-6), 789–794 (1999).
[CrossRef]

Chirila, C. C.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Cirmi, G.

Corkum, P. B.

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

P. B. Corkum, “Plasma perspective on strong field multiphoton ionization,” Phys. Rev. Lett. 71(13), 1994–1997 (1993).
[CrossRef] [PubMed]

De Silvestri, S.

Flammini, R.

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

Frank, A.

R. Lemus and A. Frank, “Algebraic approach to vibrational spectra of tetrahedral molecules: Application to methane,” J. Chem. Phys. 101(10), 8321 (1994).
[CrossRef]

Frassetto, F.

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

Gasilov, S.

Haworth, C. A.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Heesel, E.

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Hong, K.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Huang, Y.

Itatani, J.

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Jullien, A.

Kajumba, N.

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Kanai, T.

T. Kanai, S. Minemoto, and H. Sakai, “Quantum interference during high-order harmonic generation from aligned molecules,” Nature 435(7041), 470–474 (2005).
[CrossRef] [PubMed]

Kawai, S.

A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008).
[CrossRef] [PubMed]

Kieffer, J. C.

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Kim, C.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Kim, H.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Kim, I.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Lee, Y.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Lein, M.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

M. Lein, “Attosecond probing of vibrational dynamics with high-harmonic generation,” Phys. Rev. Lett. 94(5), 053004 (2005).
[CrossRef] [PubMed]

Lemus, R.

R. Lemus and A. Frank, “Algebraic approach to vibrational spectra of tetrahedral molecules: Application to methane,” J. Chem. Phys. 101(10), 8321 (1994).
[CrossRef]

Leng, Y.

Leone, S. R.

Levesque, J.

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Li, R.

Li, X.

Liu, C.

Liu, J.

Liu, P.

Lu, H.

Y. Zheng, Z. Zeng, X. Li, X. Chen, P. Liu, H. Xiong, H. Lu, S. Zhao, P. Wei, L. Zhang, Z. Wang, J. Liu, Y. Cheng, R. Li, and Z. Xu, “Enhancement and broadening of extreme-ultraviolet supercontinuum in a relative phase controlled two-color laser field,” Opt. Lett. 33(3), 234–236 (2008).
[CrossRef] [PubMed]

A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008).
[CrossRef] [PubMed]

Manzoni, C.

Marangos, J. P.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Merdji, H.

Minemoto, S.

T. Kanai, S. Minemoto, and H. Sakai, “Quantum interference during high-order harmonic generation from aligned molecules,” Nature 435(7041), 470–474 (2005).
[CrossRef] [PubMed]

Nam, C.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Negro, M.

Neumark, D. M.

Niikura, H.

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Nisoli, M.

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Park, J.

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Pépin, H.

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Pfeifer, T.

Poletto, L.

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

Robinson, J. S.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Sakai, H.

T. Kanai, S. Minemoto, and H. Sakai, “Quantum interference during high-order harmonic generation from aligned molecules,” Nature 435(7041), 470–474 (2005).
[CrossRef] [PubMed]

Sansone, G.

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007).
[CrossRef] [PubMed]

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Smith, R. A.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Spanner, M.

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

Stagira, S.

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007).
[CrossRef] [PubMed]

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Svelto, O.

Talebpour, A.

A. Talebpour, A. D. Bandrauk, J. Yang, and S. L. Chin, “Multiphoton ionization of inner-valence electrons and fragmentation of ethylene in an intense Ti:sapphire laser pulse,” Chem. Phys. Lett. 313(5-6), 789–794 (1999).
[CrossRef]

Teng, H.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Tisch, J. W. G.

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

Torres, R.

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Velotta, R.

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Villeneuve, D. M.

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Villoresi, P.

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

Vozzi, C.

F. Calegari, C. Vozzi, M. Negro, G. Sansone, F. Frassetto, L. Poletto, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver,” Opt. Lett. 34(20), 3125–3127 (2009).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

C. Vozzi, F. Calegari, E. Benedetti, S. Gasilov, G. Sansone, G. Cerullo, M. Nisoli, S. De Silvestri, and S. Stagira, “Millijoule-level phase-stabilized few-optical-cycle infrared parametric source,” Opt. Lett. 32(20), 2957–2959 (2007).
[CrossRef] [PubMed]

C. Vozzi, G. Cirmi, C. Manzoni, E. Benedetti, F. Calegari, G. Sansone, S. Stagira, O. Svelto, S. De Silvestri, M. Nisoli, and G. Cerullo, “High-energy, few-optical-cycle pulses at 1.5 µm with passive carrier-envelope phase stabilization,” Opt. Express 14(21), 10109–10116 (2006).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

Wang, Z.

Wei, P.

Xiong, H.

Xu, Z.

Yang, J.

A. Talebpour, A. D. Bandrauk, J. Yang, and S. L. Chin, “Multiphoton ionization of inner-valence electrons and fragmentation of ethylene in an intense Ti:sapphire laser pulse,” Chem. Phys. Lett. 313(5-6), 789–794 (1999).
[CrossRef]

Zeidler, D.

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Zeng, Z.

Zhang, C.

Zhang, L.

Zhao, S.

Zheng, Y.

Appl. Phys. B (1)

I. Kim, H. Kim, C. Kim, J. Park, Y. Lee, K. Hong, and C. Nam, “Efficient high-order harmonic generation in a two-color laser field,” Appl. Phys. B 78(7-8), 859–861 (2004).
[CrossRef]

Chem. Phys. Lett. (1)

A. Talebpour, A. D. Bandrauk, J. Yang, and S. L. Chin, “Multiphoton ionization of inner-valence electrons and fragmentation of ethylene in an intense Ti:sapphire laser pulse,” Chem. Phys. Lett. 313(5-6), 789–794 (1999).
[CrossRef]

J. Chem. Phys. (1)

R. Lemus and A. Frank, “Algebraic approach to vibrational spectra of tetrahedral molecules: Application to methane,” J. Chem. Phys. 101(10), 8321 (1994).
[CrossRef]

Nature (2)

T. Kanai, S. Minemoto, and H. Sakai, “Quantum interference during high-order harmonic generation from aligned molecules,” Nature 435(7041), 470–474 (2005).
[CrossRef] [PubMed]

J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, and D. M. Villeneuve, “Tomographic imaging of molecular orbitals,” Nature 432(7019), 867–871 (2004).
[CrossRef] [PubMed]

Opt. Express (2)

Opt. Lett. (5)

Phys. Rev. A (2)

C. Liu, Z. Zeng, P. Wei, P. Liu, R. Li, and Z. Xu, “Driving-laser wavelength dependence of high-order harmonic generation in H2+ molecules,” Phys. Rev. A 81(3), 033426 (2010).
[CrossRef]

C. Vozzi, F. Calegari, F. Frassetto, L. Poletto, G. Sansone, P. Villoresi, M. Nisoli, S. De Silvestri, and S. Stagira, “Coherent continuum generation above 100eV driven by an ir parametric source in a two-color scheme,” Phys. Rev. A 79(3), 033842 (2009).
[CrossRef]

Phys. Rev. Lett. (5)

M. Lein, “Attosecond probing of vibrational dynamics with high-harmonic generation,” Phys. Rev. Lett. 94(5), 053004 (2005).
[CrossRef] [PubMed]

A. D. Bandrauk, S. Chelkowski, S. Kawai, and H. Lu, “Effect of nuclear motion on molecular high-order harmonics and on generation of attosecond pulses in intense laser pulses,” Phys. Rev. Lett. 101(15), 153901 (2008).
[CrossRef] [PubMed]

C. Vozzi, F. Calegari, E. Benedetti, J. P. Caumes, G. Sansone, S. Stagira, M. Nisoli, R. Torres, E. Heesel, N. Kajumba, J. P. Marangos, C. Altucci, and R. Velotta, “Controlling two-center interference in molecular high harmonic generation,” Phys. Rev. Lett. 95(15), 153902 (2005).
[CrossRef] [PubMed]

J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, and P. B. Corkum, “Controlling high harmonic generation with molecular wave packets,” Phys. Rev. Lett. 94(12), 123902 (2005).
[CrossRef] [PubMed]

P. B. Corkum, “Plasma perspective on strong field multiphoton ionization,” Phys. Rev. Lett. 71(13), 1994–1997 (1993).
[CrossRef] [PubMed]

Science (2)

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

S. Baker, J. S. Robinson, C. A. Haworth, H. Teng, R. A. Smith, C. C. Chirila, M. Lein, J. W. G. Tisch, and J. P. Marangos, “Probing proton dynamics in molecules on an attosecond time scale,” Science 312(5772), 424–427 (2006).
[CrossRef] [PubMed]

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Figures (4)

Fig. 1
Fig. 1

(a) Experimental setup. The two output beams are collinearly focused with variable time delay into a gas cell located in a high-vacuum interaction chamber. The generated high-order harmonics are detected by a home-made flat-field grating spectrometer equipped with a soft-x-ray CCD. (b) The tunable OPA spectra from 1500nm to 1900nm.

Fig. 2
Fig. 2

Measured harmonic yields as functions of the time delay between the two color pulses from (a) CH4 molecules and (b) Xe atoms at the equal gas density driven by the same two-color field with the longer wavelength component tuned to 1700nm. (c)-(d) The harmonic spectra are the lineouts of (a)-(b) at the time delay of −100fs (red dotted lines), −50fs (green dashed lines) and 0fs (black solid lines).

Fig. 3
Fig. 3

Measured harmonic yields as functions of the laser intensity of the 1700nm component at the time delay of 0fs from (a) CH4 molecules and (b) Xe atoms. The laser intensity of the 800nm component is kept constant.

Fig. 4
Fig. 4

Measured harmonic yields as functions of the time delay between the two color pulses from CH4 molecules driven by the longer wavelength component tuned to (a) 1500nm, (b) 1700nm, and (c) 1900nm. (d)-(f) The wavelength effect on the harmonic spectra at the different time delay of (d) 0fs, (e) 50fs and (f) 100fs, which are the lineouts of (a)-(c).

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