Abstract

We report the CsPbI3 random lasing at room temperature fabricated by a chemical deposition method. The CsPbI3 thin films with high crystalline quality have intense PL emission and easily achieve the lasing behavior with the Q-factor value over 7000. The lasing behavior of CsPbI3 thin films can be classified as random lasing by measuring lasing spectra at different collective angles. The fast Fourier transform analysis of the lasing spectra is employed to determine the effective cavity length. Most important of all, the lasing stability investigation shows the prolonged lasing stability over 4.8 X 105 laser shots in air.

© 2020 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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    [Crossref]
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    [Crossref]
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    [Crossref]
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    [Crossref]
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    [Crossref]
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  39. H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, “Random Laser Action in Semiconductor Powder,” Phys. Rev. Lett. 82(11), 2278–2281 (1999).
    [Crossref]
  40. D. S. Wiersma, “Random lasers explained?” Nat. Photonics 3(5), 246–248 (2009).
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  41. Y. Ren, H. Zhu, Y. Wu, G. Lou, Y. Liang, S. Li, S. Su, X. Gui, Z. Qiu, and Z. Tang, “Ultraviolet Random Laser Based on a Single GaN Microwire,” ACS Photonics 5(6), 2503–2508 (2018).
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  42. Y. J. Lee, T. W. Yeh, P. Nagarjuna, C. C. Tseng, and J. Y. Yi, “A strain-gauge random laser,” APL Mater. 7(6), 061103 (2019).
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    [Crossref]

2020 (2)

C. H. Chiang, T. Y. Li, H. S. Wu, K. Y. Li, C. F. Hsu, L. F. Tsai, P. K. Yang, Y. J. Lee, H. C. Lee, C. Y. Wang, and M. L. Tsai, “High-stability inorganic perovskite quantum dot–cellulose nanocrystal hybrid films,” Nanotechnology 31(32), 324002 (2020).
[Crossref]

H. L. Hsu, B. H. Jiang, C. L. Chung, Y. Y. Yu, R. J. Jeng, and C. P. Chen, “Commercially available jeffamine additives for p–i–n perovskite solar cells,” Nanotechnology 31(27), 274002 (2020).
[Crossref]

2019 (9)

Y. C. Wang, H. Li, Y. H. Hong, K. B. Hong, F. C. Chen, C. H. Hsu, R. K. Lee, C. Conti, T. S. Kao, and T. C. Lu, “Flexible Organometal–Halide Perovskite Lasers for Speckle Reduction in Imaging Projection,” ACS Nano 13(5), 5421–5429 (2019).
[Crossref]

K. H. Wang, Y. Peng, J. Ge, S. Jiang, B. S. Zhu, J. Yao, Y. C. Yin, J. N. Yang, Q. Zhang, and H. B. Yao, “Efficient and Color-Tunable Quasi-2D CsPbBrxCl3−x Perovskite Blue Light-Emitting Diodes,” ACS Photonics 6(3), 667–676 (2019).
[Crossref]

S. Seth, T. Ahmed, A. De, and A. Samanta, “Tackling the Defects, Stability, and Photoluminescence of CsPbX3 Perovskite Nanocrystals,” ACS Energy Lett. 4(7), 1610–1618 (2019).
[Crossref]

B. Zhou, M. Jiang, H. Dong, W. Zheng, Y. Huang, J. Han, A. Pan, and L. Zhang, “High-Temperature Upconverted Single-Mode Lasing in 3D Fully Inorganic Perovskite Microcubic Cavity,” ACS Photonics 6(3), 793–801 (2019).
[Crossref]

Z. Liu, Y. Li, X. Guan, Y. Mi, A. Al-Hussain, S. T. Ha, M. H. Chiu, C. Ma, M. R. Amer, L. J. Li, J. Liu, Q. Xiong, J. Wang, X. Liu, and T. Wu, “One-Step Vapor-Phase Synthesis and Quantum-Confined Exciton in Single-Crystal Platelets of Hybrid Halide Perovskites,” J. Phys. Chem. Lett. 10(10), 2363–2371 (2019).
[Crossref]

L. N. Quan, B. P. Rand, R. H. Friend, S. G. Mhaisalkar, T. W. Lee, and E. H. Sargent, “Perovskites for Next-Generation Optical Sources,” Chem. Rev. 119(12), 7444–7477 (2019).
[Crossref]

Z. Y. Wu, B. L. Jian, and H. C. Hsu, “Photoluminescence characterizations of highly ambient-air-stable CH3NH3PbI3/PbI2 heterostructure,” Opt. Mater. Express 9(4), 1882–1892 (2019).
[Crossref]

Y. J. Lee, T. W. Yeh, P. Nagarjuna, C. C. Tseng, and J. Y. Yi, “A strain-gauge random laser,” APL Mater. 7(6), 061103 (2019).
[Crossref]

R. K. Singh, R. Kumar, N. Jain, S. R. Dash, J. Singh, and A. Srivastava, “Investigation of optical and dielectric properties of CsPbI3 inorganic lead iodide perovskite thin film,” J. Taiwan Inst. Chem. Eng. 96, 538–542 (2019).
[Crossref]

2018 (4)

Y. Ren, H. Zhu, Y. Wu, G. Lou, Y. Liang, S. Li, S. Su, X. Gui, Z. Qiu, and Z. Tang, “Ultraviolet Random Laser Based on a Single GaN Microwire,” ACS Photonics 5(6), 2503–2508 (2018).
[Crossref]

K. Wang, S. Wang, S. Xiao, and Q. Song, “Recent Advances in Perovskite Micro- and Nanolasers,” Adv. Opt. Mater. 6(18), 1800278 (2018).
[Crossref]

H. Masaki, H. Yoichi, N. Ryota, M. Tomoya, A. Ulugbek, O. Hiromi, N. Takeshi, Y. Yoshifumi, and H. Yasuhiko, “In-situ X-ray diffraction reveals the degradation of crystalline CH3NH3PbI3 by water-molecule collisions at room temperature,” Jpn. J. Appl. Phys. 57(2), 028001 (2018).
[Crossref]

A. Safdar, Y. Wang, and T. F. Krauss, “Random lasing in uniform perovskite thin films,” Opt. Express 26(2), A75–A84 (2018).
[Crossref]

2017 (4)

H. Zhou, S. Yuan, X. Wang, T. Xu, X. Wang, H. Li, W. Zheng, P. Fan, Y. Li, L. Sun, and A. Pan, “Vapor Growth and Tunable Lasing of Band Gap Engineered Cesium Lead Halide Perovskite Micro/Nanorods with Triangular Cross Section,” ACS Nano 11(2), 1189–1195 (2017).
[Crossref]

C. Li, Z. Zang, C. Han, Z. Hu, X. Tang, J. Du, Y. Leng, and K. Sun, “Highly compact CsPbBr3 perovskite thin films decorated by ZnO nanoparticles for enhanced random lasing,” Nano Energy 40, 195–202 (2017).
[Crossref]

B. Tang, H. Dong, L. Sun, W. Zheng, Q. Wang, F. Sun, X. Jiang, A. Pan, and L. Zhang, “Single-Mode Lasers Based on Cesium Lead Halide Perovskite Submicron Spheres,” ACS Nano 11(11), 10681–10688 (2017).
[Crossref]

P. Perumal, C. S. Wang, K. M. Boopathi, G. Haider, W. C. Liao, and Y. F. Chen, “Whispering Gallery Mode Lasing from Self-Assembled Hexagonal Perovskite Single Crystals and Porous Thin Films Decorated by Dielectric Spherical Resonators,” ACS Photonics 4(1), 146–155 (2017).
[Crossref]

2016 (4)

I. Lignos, S. Stavrakis, G. Nedelcu, L. Protesescu, A. J. deMello, and M. V. Kovalenko, “Synthesis of Cesium Lead Halide Perovskite Nanocrystals in a Droplet-Based Microfluidic Platform: Fast Parametric Space Mapping,” Nano Lett. 16(3), 1869–1877 (2016).
[Crossref]

Y. Fu, H. Zhu, C. C. Stoumpos, Q. Ding, J. Wang, M. G. Kanatzidis, X. Zhu, and S. Jin, “Broad Wavelength Tunable Robust Lasing from Single-Crystal Nanowires of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I),” ACS Nano 10(8), 7963–7972 (2016).
[Crossref]

Q. Zhang, R. Su, X. Liu, J. Xing, T. C. Sum, and Q. Xiong, “High-Quality Whispering-Gallery-Mode Lasing from Cesium Lead Halide Perovskite Nanoplatelets,” Adv. Funct. Mater. 26(34), 6238–6245 (2016).
[Crossref]

Z. F. Shi, X. G. Sun, D. Wu, T. T. Xu, Y. T. Tian, Y. T. Zhang, X. J. Li, and G. T. Du, “Near-infrared random lasing realized in a perovskite CH3NH3PbI3 thin film,” J. Mater. Chem. C 4(36), 8373–8379 (2016).
[Crossref]

2015 (6)

S. Yakunin, L. Protesescu, F. Krieg, M. I. Bodnarchuk, G. Nedelcu, M. Humer, G. De Luca, M. Fiebig, W. Heiss, and M. V. Kovalenko, “Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites,” Nat. Commun. 6(1), 8056 (2015).
[Crossref]

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref]

M. B. Price, J. Butkus, T. C. Jellicoe, A. Sadhanala, A. Briane, J. E. Halpert, K. Broch, J. M. Hodgkiss, R. H. Friend, and F. Deschler, “Hot-carrier cooling and photoinduced refractive index changes in organic–inorganic lead halide perovskites,” Nat. Commun. 6(1), 8420 (2015).
[Crossref]

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X. Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref]

G. R. Li, Z. K. Tan, D. W. Di, M. L. Lai, L. Jiang, J. H. W. Lim, R. H. Friend, and N. C. Greenham, “Efficient Light-Emitting Diodes Based on Nanocrystalline Perovskite in a Dielectric Polymer Matrix,” Nano Lett. 15(4), 2640–2644 (2015).
[Crossref]

J. Song, J. Li, X. Li, L. Xu, Y. Dong, and H. Zeng, “Quantum Dot Light-Emitting Diodes Based on Inorganic Perovskite Cesium Lead Halides (CsPbX3),” Adv. Mater. 27(44), 7162–7167 (2015).
[Crossref]

2014 (7)

G. Xing, N. Mathews, S. S. Lim, N. Yantara, X. Liu, D. Sabba, M. Grätzel, S. Mhaisalkar, and T. C. Sum, “Low-temperature solution-processed wavelength-tunable perovskites for lasing,” Nat. Mater. 13(5), 476–480 (2014).
[Crossref]

Z. K. Tan, R. S. Moghaddam, M. L. Lai, P. Docampo, R. Higler, F. Deschler, M. Price, A. Sadhanala, L. M. Pazos, D. Credgington, F. Hanusch, T. Bein, H. J. Snaith, and R. H. Friend, “Bright light-emitting diodes based on organometal halide perovskite,” Nat. Nanotechnol. 9(9), 687–692 (2014).
[Crossref]

Q. Zhang, S. T. Ha, X. Liu, T. C. Sum, and Q. Xiong, “Room-Temperature Near-Infrared High-Q Perovskite Whispering-Gallery Planar Nanolasers,” Nano Lett. 14(10), 5995–6001 (2014).
[Crossref]

C. Wehrenfennig, G. E. Eperon, M. B. Johnston, H. J. Snaith, and L. M. Herz, “High Charge Carrier Mobilities and Lifetimes in Organolead Trihalide Perovskites,” Adv. Mater. 26(10), 1584–1589 (2014).
[Crossref]

A. Amat, E. Mosconi, E. Ronca, C. Quarti, P. Umari, M. K. Nazeeruddin, M. Grätzel, and F. De Angelis, “Cation-Induced Band-Gap Tuning in Organohalide Perovskites: Interplay of Spin–Orbit Coupling and Octahedra Tilting,” Nano Lett. 14(6), 3608–3616 (2014).
[Crossref]

T. S. Kao, Y. H. Chou, C. H. Chou, F. C. Chen, and T. C. Lu, “Lasing behaviors upon phase transition in solution-processed perovskite thin films,” Appl. Phys. Lett. 105(23), 231108 (2014).
[Crossref]

R. Dhanker, A. N. Brigeman, A. V. Larsen, R. J. Stewart, J. B. Asbury, and N. C. Giebink, “Random lasing in organo-lead halide perovskite microcrystal networks,” Appl. Phys. Lett. 105(15), 151112 (2014).
[Crossref]

2013 (1)

G. Xing, N. Mathews, S. Sun, S. S. Lim, Y. M. Lam, M. Grätzel, S. Mhaisalkar, and T. C. Sum, “Long-Range Balanced Electron- and Hole-Transport Lengths in Organic-Inorganic CH3NH3PbI3,” Science 342(6156), 344–347 (2013).
[Crossref]

2009 (2)

A. Kojima, K. Teshima, Y. Shirai, and T. Miyasaka, “Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells,” J. Am. Chem. Soc. 131(17), 6050–6051 (2009).
[Crossref]

D. S. Wiersma, “Random lasers explained?” Nat. Photonics 3(5), 246–248 (2009).
[Crossref]

1999 (1)

H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, “Random Laser Action in Semiconductor Powder,” Phys. Rev. Lett. 82(11), 2278–2281 (1999).
[Crossref]

1997 (1)

D. S. Wiersma, P. Bartolini, A. Lagendijk, and R. Righini, “Localization of light in a disordered medium,” Nature 390(6661), 671–673 (1997).
[Crossref]

1995 (1)

D. B. Mitzi, C. A. Feild, Z. Schlesinger, and R. B. Laibowitz, “Transport, Optical, and Magnetic Properties of the Conducting Halide Perovskite CH3NH3SnI3,” J. Solid State Chem. 114(1), 159–163 (1995).
[Crossref]

1958 (1)

P. W. Anderson, “Absence of Diffusion in Certain Random Lattices,” Phys. Rev. 109(5), 1492–1505 (1958).
[Crossref]

Ahmed, T.

S. Seth, T. Ahmed, A. De, and A. Samanta, “Tackling the Defects, Stability, and Photoluminescence of CsPbX3 Perovskite Nanocrystals,” ACS Energy Lett. 4(7), 1610–1618 (2019).
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ACS Energy Lett. (1)

S. Seth, T. Ahmed, A. De, and A. Samanta, “Tackling the Defects, Stability, and Photoluminescence of CsPbX3 Perovskite Nanocrystals,” ACS Energy Lett. 4(7), 1610–1618 (2019).
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ACS Nano (4)

Y. Fu, H. Zhu, C. C. Stoumpos, Q. Ding, J. Wang, M. G. Kanatzidis, X. Zhu, and S. Jin, “Broad Wavelength Tunable Robust Lasing from Single-Crystal Nanowires of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I),” ACS Nano 10(8), 7963–7972 (2016).
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Y. C. Wang, H. Li, Y. H. Hong, K. B. Hong, F. C. Chen, C. H. Hsu, R. K. Lee, C. Conti, T. S. Kao, and T. C. Lu, “Flexible Organometal–Halide Perovskite Lasers for Speckle Reduction in Imaging Projection,” ACS Nano 13(5), 5421–5429 (2019).
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ACS Photonics (4)

P. Perumal, C. S. Wang, K. M. Boopathi, G. Haider, W. C. Liao, and Y. F. Chen, “Whispering Gallery Mode Lasing from Self-Assembled Hexagonal Perovskite Single Crystals and Porous Thin Films Decorated by Dielectric Spherical Resonators,” ACS Photonics 4(1), 146–155 (2017).
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K. H. Wang, Y. Peng, J. Ge, S. Jiang, B. S. Zhu, J. Yao, Y. C. Yin, J. N. Yang, Q. Zhang, and H. B. Yao, “Efficient and Color-Tunable Quasi-2D CsPbBrxCl3−x Perovskite Blue Light-Emitting Diodes,” ACS Photonics 6(3), 667–676 (2019).
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Adv. Funct. Mater. (1)

Q. Zhang, R. Su, X. Liu, J. Xing, T. C. Sum, and Q. Xiong, “High-Quality Whispering-Gallery-Mode Lasing from Cesium Lead Halide Perovskite Nanoplatelets,” Adv. Funct. Mater. 26(34), 6238–6245 (2016).
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Adv. Mater. (2)

C. Wehrenfennig, G. E. Eperon, M. B. Johnston, H. J. Snaith, and L. M. Herz, “High Charge Carrier Mobilities and Lifetimes in Organolead Trihalide Perovskites,” Adv. Mater. 26(10), 1584–1589 (2014).
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J. Song, J. Li, X. Li, L. Xu, Y. Dong, and H. Zeng, “Quantum Dot Light-Emitting Diodes Based on Inorganic Perovskite Cesium Lead Halides (CsPbX3),” Adv. Mater. 27(44), 7162–7167 (2015).
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Adv. Opt. Mater. (1)

K. Wang, S. Wang, S. Xiao, and Q. Song, “Recent Advances in Perovskite Micro- and Nanolasers,” Adv. Opt. Mater. 6(18), 1800278 (2018).
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APL Mater. (1)

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Figures (6)

Fig. 1.
Fig. 1. (a) SEM image of the CsPbI3 thin film. (b) XRD patterns of the CsPbI3 thin film and the XRD standard line for γ-CsPbI3 (JCPDS card No. 18-0376).
Fig. 2.
Fig. 2. The absorbance and steady-state PL emission of the CsPbI3 thin film.
Fig. 3.
Fig. 3. (a) Lasing spectra of the CsPbI3 thin film under increasing excitation fluence. (b) PL intensity and FWHM of the CsPbI3 thin film as a function of excitation fluence. (c) The zoom-in lasing spectra from 718.2 nm to 719.4 nm just well above threshold. (d) The lasing spectrum at 718.8 nm near threshold with the Lorentz fitting curve.
Fig. 4.
Fig. 4. (a) Schematic diagram to illustrate the principle of random lasing. (b) Angle-dependent lasing spectra of the CsPbI3 film in two directions: (a) 0$^\circ $ and (b) 30$^\circ $. form the surface of the CsPbI3 thin film.
Fig. 5.
Fig. 5. FFT spectra for the CsPbI3 random laser under different excitation fluence.
Fig. 6.
Fig. 6. (a) Lasing spectra of the CsPbI3 thin film during different time under a fixed excitation energy density. (b) Lasing intensity of the CsPbI3 thin film as a function of laser shots.

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