Abstract

We report the first experimental demonstration of a-periodic multilayer mirrors controlling the frequency sweep (chirp) of isolated attosecond XUV pulses. The concept was proven with about 200-attosecond pulses in the photon energy range of 100-130 eV measured via photoelectron streaking in neon. The demonstrated attosecond dispersion control is engineerable in a wide range of XUV photon energies and bandwidths. The resultant tailor-made attosecond pulses with highly enhanced photon flux are expected to significantly advance attosecond metrology and spectroscopy and broaden their range of applications.

© 2011 OSA

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  1. M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291(5510), 1923–1927 (2001).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  3. M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
    [CrossRef] [PubMed]
  4. M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  9. M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
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    [CrossRef]
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    [CrossRef] [PubMed]
  14. V. Pervak, A. V. Tikhonravov, M. K. Trubetskov, S. Naumov, F. Krausz, and A. Apolonski, “1.5-octave chirped mirror for pulse compression down to sub-3 fs,” Appl. Phys. B 87(1), 5–12 (2007).
    [CrossRef]
  15. E. Gustafsson, T. Ruchon, M. Swoboda, T. Remetter, E. Pourtal, R. López-Martens, Ph. Balcou, and A. L’Huillier, “Broadband attosecond pulse shaping,” Opt. Lett. 32(11), 1353–1355 (2007).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  17. G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
    [CrossRef] [PubMed]
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    [CrossRef] [PubMed]
  19. M. Drescher, M. Hentschel, R. Kienberger, M. Uiberacker, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, and F. Krausz, “Time-resolved atomic inner-shell spectroscopy,” Nature 419(6909), 803–807 (2002).
    [CrossRef] [PubMed]
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    [CrossRef]
  21. M. Hofstetter, M. Schultze, M. Fieß, A. Guggenmos, J. Gagnon, E. Magerl, E. Botschafter, R. Ernstorfer, R. Kienberger, E. M. Gullikson, F. Krausz, and U. Kleineberg, “First attosecond pulse control by multilayer mirrors above 100 eV photon energy,“ in Ultrafast Phenomena XVII, 11.17, M. Chergui, D. Jonas, E. Riedle, B. Schönlein, A. Taylor (Oxford University Press, New York, 2010).
  22. A. V. Tikhonravov, M. K. Trubetskov, and G. W. DeBell, “Optical coating design approaches based on the needle optimization technique,” Appl. Opt. 46(5), 704–710 (2007).
    [CrossRef] [PubMed]
  23. B. L. Henke, E. M. Gullikson, and J. C. Davis, “X-ray interactions: photoabsorption, scattering, transmission, and reflection at E=50-30000 eV, Z=1-92,” At. Data Nucl. Data Tables 54(2), 181–342 (1993).
    [CrossRef]
  24. E. M. Gullikson, J. H. Underwood, P. Batson, and V. Nikitin, “A soft x-ray/EUV reflectometer based on a laser produced plasma source,” J. XRay Sci. Technol. 3(4), 283–299 (1992).
    [PubMed]
  25. A. Aquila, F. Salmassi, and E. Gullikson, “Metrologies for the phase characterization of attosecond extreme ultraviolet optics,” Opt. Lett. 33(5), 455–457 (2008).
    [CrossRef] [PubMed]
  26. M. Kitzler, N. Milosevic, A. Scrinzi, F. Krausz, and T. Brabec, “Quantum theory of attosecond XUV pulse measurement by laser dressed photoionization,” Phys. Rev. Lett. 88(17), 173904 (2002).
    [CrossRef] [PubMed]
  27. R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
    [CrossRef] [PubMed]
  28. M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
    [CrossRef]
  29. M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
    [CrossRef]
  30. R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbügel, B. A. Richman, and D. J. Kane, “Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating,” Rev. Sci. Instrum. 68(9), 3277 (1997).
    [CrossRef]
  31. A download link of the program can be found at http://www.attoworld.de/Home/ourResearch/Downloads/index.html
  32. Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
    [CrossRef] [PubMed]
  33. J. Gagnon, E. Goulielmakis, and V. S. Yakovlev, “The accurate FROG characterization of attosecond pulses from streaking measurements,” Appl. Phys. B 92(1), 25–32 (2008).
    [CrossRef]
  34. J. Gagnon and V. S. Yakovlev, “The robustness of attosecond streaking measurements,” Opt. Express 17(20), 17678–17693 (2009).
    [CrossRef] [PubMed]
  35. L. Y. Peng, F. Tan, Q. Gong, E. A. Pronin, and A. F. Starace, “Few-cycle attosecond pulse chirp effects on asymmetries in ionized electron momentum distributions,” Phys. Rev. A 80(1), 013407 (2009).
    [CrossRef]
  36. V. S. Yakovlev, J. Gagnon, N. Karpowicz, and F. Krausz, “Attosecond streaking enables the measurement of quantum phase,” Phys. Rev. Lett. 105(7), 073001 (2010).
    [CrossRef] [PubMed]
  37. Y. Li, J. Lewellen, Z. Huang, V. Sajaev, and S. V. Milton, “Time-resolved measurement of a self-amplified free-electron laser,” NIM A 507(1-2), 413–416 (2003).
    [CrossRef]

2010

M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

E. Goulielmakis, Z. H. Loh, A. Wirth, R. Santra, N. Rohringer, V. S. Yakovlev, S. Zherebtsov, T. Pfeifer, A. M. Azzeer, M. F. Kling, S. R. Leone, and F. Krausz, “Real-time observation of valence electron motion,” Nature 466(7307), 739–743 (2010).
[CrossRef] [PubMed]

Y. Ménesguen, S. de Rossi, E. Meltchakov, and F. Delmotte, “Aperiodic multilayer mirrors for efficient broadband reflection in the extreme ultraviolet,” Appl. Phys., A Mater. Sci. Process. 98(2), 305–309 (2010).
[CrossRef]

M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
[CrossRef]

V. S. Yakovlev, J. Gagnon, N. Karpowicz, and F. Krausz, “Attosecond streaking enables the measurement of quantum phase,” Phys. Rev. Lett. 105(7), 073001 (2010).
[CrossRef] [PubMed]

2009

J. Gagnon and V. S. Yakovlev, “The robustness of attosecond streaking measurements,” Opt. Express 17(20), 17678–17693 (2009).
[CrossRef] [PubMed]

L. Y. Peng, F. Tan, Q. Gong, E. A. Pronin, and A. F. Starace, “Few-cycle attosecond pulse chirp effects on asymmetries in ionized electron momentum distributions,” Phys. Rev. A 80(1), 013407 (2009).
[CrossRef]

M. Suman, G. Monaco, M.-G. Pelizzo, D. L. Windt, and P. Nicolosi, “Realization and characterization of an XUV multilayer coating for attosecond pulses,” Opt. Express 17(10), 7922–7932 (2009).
[CrossRef] [PubMed]

F. Krausz and M. Ivanov, “Attosecond physics,” Rev. Mod. Phys. 81(1), 163–234 (2009).
[CrossRef]

2008

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

J. Gagnon, E. Goulielmakis, and V. S. Yakovlev, “The accurate FROG characterization of attosecond pulses from streaking measurements,” Appl. Phys. B 92(1), 25–32 (2008).
[CrossRef]

A. Aquila, F. Salmassi, and E. Gullikson, “Metrologies for the phase characterization of attosecond extreme ultraviolet optics,” Opt. Lett. 33(5), 455–457 (2008).
[CrossRef] [PubMed]

2007

M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
[CrossRef]

A. V. Tikhonravov, M. K. Trubetskov, and G. W. DeBell, “Optical coating design approaches based on the needle optimization technique,” Appl. Opt. 46(5), 704–710 (2007).
[CrossRef] [PubMed]

V. Pervak, A. V. Tikhonravov, M. K. Trubetskov, S. Naumov, F. Krausz, and A. Apolonski, “1.5-octave chirped mirror for pulse compression down to sub-3 fs,” Appl. Phys. B 87(1), 5–12 (2007).
[CrossRef]

E. Gustafsson, T. Ruchon, M. Swoboda, T. Remetter, E. Pourtal, R. López-Martens, Ph. Balcou, and A. L’Huillier, “Broadband attosecond pulse shaping,” Opt. Lett. 32(11), 1353–1355 (2007).
[CrossRef] [PubMed]

A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
[CrossRef] [PubMed]

M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

2006

A. Wonisch, U. Neuhäusler, N. M. Kabachnik, T. Uphues, M. Uiberacker, V. Yakovlev, F. Krausz, M. Drescher, U. Kleineberg, and U. Heinzmann, “Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses,” Appl. Opt. 45(17), 4147–4156 (2006).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

2005

A.-S. Morlens, P. Balcou, P. Zeitoun, C. Valentin, V. Laude, and S. Kazamias, “Compression of attosecond harmonic pulses by extreme-ultraviolet chirped mirrors,” Opt. Lett. 30(12), 1554–1556 (2005).
[CrossRef] [PubMed]

R. López-Martens, K. Varjú, P. Johnsson, J. Mauritsson, Y. Mairesse, P. Salières, M. B. Gaarde, K. J. Schafer, A. Persson, S. Svanberg, C.-G. Wahlström, and A. L’huillier, “Amplitude and phase control of attosecond light pulses,” Phys. Rev. Lett. 94(3), 033001 (2005).
[CrossRef] [PubMed]

2004

E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
[CrossRef] [PubMed]

R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
[CrossRef] [PubMed]

2003

Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
[CrossRef] [PubMed]

Y. Li, J. Lewellen, Z. Huang, V. Sajaev, and S. V. Milton, “Time-resolved measurement of a self-amplified free-electron laser,” NIM A 507(1-2), 413–416 (2003).
[CrossRef]

2002

M. Kitzler, N. Milosevic, A. Scrinzi, F. Krausz, and T. Brabec, “Quantum theory of attosecond XUV pulse measurement by laser dressed photoionization,” Phys. Rev. Lett. 88(17), 173904 (2002).
[CrossRef] [PubMed]

R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
[CrossRef] [PubMed]

M. Drescher, M. Hentschel, R. Kienberger, M. Uiberacker, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, and F. Krausz, “Time-resolved atomic inner-shell spectroscopy,” Nature 419(6909), 803–807 (2002).
[CrossRef] [PubMed]

2001

M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291(5510), 1923–1927 (2001).
[CrossRef] [PubMed]

M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
[CrossRef] [PubMed]

1997

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, “High-Harmonic Generation of Attosecond Pulses in the “Single-Cycle” Regime,” Phys. Rev. Lett. 78(7), 1251–1254 (1997).
[CrossRef]

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbügel, B. A. Richman, and D. J. Kane, “Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating,” Rev. Sci. Instrum. 68(9), 3277 (1997).
[CrossRef]

1993

B. L. Henke, E. M. Gullikson, and J. C. Davis, “X-ray interactions: photoabsorption, scattering, transmission, and reflection at E=50-30000 eV, Z=1-92,” At. Data Nucl. Data Tables 54(2), 181–342 (1993).
[CrossRef]

1992

E. M. Gullikson, J. H. Underwood, P. Batson, and V. Nikitin, “A soft x-ray/EUV reflectometer based on a laser produced plasma source,” J. XRay Sci. Technol. 3(4), 283–299 (1992).
[PubMed]

Agostini, P.

Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
[CrossRef] [PubMed]

Altucci, C.

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

Apolonski, A.

V. Pervak, A. V. Tikhonravov, M. K. Trubetskov, S. Naumov, F. Krausz, and A. Apolonski, “1.5-octave chirped mirror for pulse compression down to sub-3 fs,” Appl. Phys. B 87(1), 5–12 (2007).
[CrossRef]

Aquila, A.

A. Aquila, F. Salmassi, and E. Gullikson, “Metrologies for the phase characterization of attosecond extreme ultraviolet optics,” Opt. Lett. 33(5), 455–457 (2008).
[CrossRef] [PubMed]

Aquila, A. L.

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

Attwood, D. T.

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

Avaldi, L.

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

Azzeer, A. M.

M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

E. Goulielmakis, Z. H. Loh, A. Wirth, R. Santra, N. Rohringer, V. S. Yakovlev, S. Zherebtsov, T. Pfeifer, A. M. Azzeer, M. F. Kling, S. R. Leone, and F. Krausz, “Real-time observation of valence electron motion,” Nature 466(7307), 739–743 (2010).
[CrossRef] [PubMed]

Balcou, P.

A.-S. Morlens, P. Balcou, P. Zeitoun, C. Valentin, V. Laude, and S. Kazamias, “Compression of attosecond harmonic pulses by extreme-ultraviolet chirped mirrors,” Opt. Lett. 30(12), 1554–1556 (2005).
[CrossRef] [PubMed]

Balcou, Ph.

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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
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A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
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A. Wonisch, U. Neuhäusler, N. M. Kabachnik, T. Uphues, M. Uiberacker, V. Yakovlev, F. Krausz, M. Drescher, U. Kleineberg, and U. Heinzmann, “Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses,” Appl. Opt. 45(17), 4147–4156 (2006).
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R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
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E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
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R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
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M. Drescher, M. Hentschel, R. Kienberger, M. Uiberacker, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, and F. Krausz, “Time-resolved atomic inner-shell spectroscopy,” Nature 419(6909), 803–807 (2002).
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M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
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M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291(5510), 1923–1927 (2001).
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A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
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R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbügel, B. A. Richman, and D. J. Kane, “Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating,” Rev. Sci. Instrum. 68(9), 3277 (1997).
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G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
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Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
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R. López-Martens, K. Varjú, P. Johnsson, J. Mauritsson, Y. Mairesse, P. Salières, M. B. Gaarde, K. J. Schafer, A. Persson, S. Svanberg, C.-G. Wahlström, and A. L’huillier, “Amplitude and phase control of attosecond light pulses,” Phys. Rev. Lett. 94(3), 033001 (2005).
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V. S. Yakovlev, J. Gagnon, N. Karpowicz, and F. Krausz, “Attosecond streaking enables the measurement of quantum phase,” Phys. Rev. Lett. 105(7), 073001 (2010).
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M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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J. Gagnon and V. S. Yakovlev, “The robustness of attosecond streaking measurements,” Opt. Express 17(20), 17678–17693 (2009).
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J. Gagnon, E. Goulielmakis, and V. S. Yakovlev, “The accurate FROG characterization of attosecond pulses from streaking measurements,” Appl. Phys. B 92(1), 25–32 (2008).
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E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
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Goulielmakis, E.

M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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E. Goulielmakis, Z. H. Loh, A. Wirth, R. Santra, N. Rohringer, V. S. Yakovlev, S. Zherebtsov, T. Pfeifer, A. M. Azzeer, M. F. Kling, S. R. Leone, and F. Krausz, “Real-time observation of valence electron motion,” Nature 466(7307), 739–743 (2010).
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J. Gagnon, E. Goulielmakis, and V. S. Yakovlev, “The accurate FROG characterization of attosecond pulses from streaking measurements,” Appl. Phys. B 92(1), 25–32 (2008).
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E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
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M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
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E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
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R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
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B. L. Henke, E. M. Gullikson, and J. C. Davis, “X-ray interactions: photoabsorption, scattering, transmission, and reflection at E=50-30000 eV, Z=1-92,” At. Data Nucl. Data Tables 54(2), 181–342 (1993).
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E. M. Gullikson, J. H. Underwood, P. Batson, and V. Nikitin, “A soft x-ray/EUV reflectometer based on a laser produced plasma source,” J. XRay Sci. Technol. 3(4), 283–299 (1992).
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E. Gustafsson, T. Ruchon, M. Swoboda, T. Remetter, E. Pourtal, R. López-Martens, Ph. Balcou, and A. L’Huillier, “Broadband attosecond pulse shaping,” Opt. Lett. 32(11), 1353–1355 (2007).
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M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
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A. Wonisch, U. Neuhäusler, N. M. Kabachnik, T. Uphues, M. Uiberacker, V. Yakovlev, F. Krausz, M. Drescher, U. Kleineberg, and U. Heinzmann, “Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses,” Appl. Opt. 45(17), 4147–4156 (2006).
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E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
[CrossRef] [PubMed]

R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
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R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
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M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
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M. Drescher, M. Hentschel, R. Kienberger, M. Uiberacker, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, and F. Krausz, “Time-resolved atomic inner-shell spectroscopy,” Nature 419(6909), 803–807 (2002).
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R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
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M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291(5510), 1923–1927 (2001).
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M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
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M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
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E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
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M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
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A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
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A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
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A. Wonisch, U. Neuhäusler, N. M. Kabachnik, T. Uphues, M. Uiberacker, V. Yakovlev, F. Krausz, M. Drescher, U. Kleineberg, and U. Heinzmann, “Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses,” Appl. Opt. 45(17), 4147–4156 (2006).
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V. S. Yakovlev, J. Gagnon, N. Karpowicz, and F. Krausz, “Attosecond streaking enables the measurement of quantum phase,” Phys. Rev. Lett. 105(7), 073001 (2010).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
[CrossRef]

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
[CrossRef] [PubMed]

R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
[CrossRef] [PubMed]

E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
[CrossRef] [PubMed]

M. Drescher, M. Hentschel, R. Kienberger, M. Uiberacker, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, and F. Krausz, “Time-resolved atomic inner-shell spectroscopy,” Nature 419(6909), 803–807 (2002).
[CrossRef] [PubMed]

R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
[CrossRef] [PubMed]

M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
[CrossRef] [PubMed]

M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291(5510), 1923–1927 (2001).
[CrossRef] [PubMed]

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M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
[CrossRef]

Kim, J.

M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
[CrossRef]

Kitzler, M.

R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
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M. Kitzler, N. Milosevic, A. Scrinzi, F. Krausz, and T. Brabec, “Quantum theory of attosecond XUV pulse measurement by laser dressed photoionization,” Phys. Rev. Lett. 88(17), 173904 (2002).
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M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
[CrossRef]

M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
[CrossRef] [PubMed]

A. Wonisch, U. Neuhäusler, N. M. Kabachnik, T. Uphues, M. Uiberacker, V. Yakovlev, F. Krausz, M. Drescher, U. Kleineberg, and U. Heinzmann, “Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses,” Appl. Opt. 45(17), 4147–4156 (2006).
[CrossRef] [PubMed]

R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
[CrossRef] [PubMed]

E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
[CrossRef] [PubMed]

R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
[CrossRef] [PubMed]

M. Drescher, M. Hentschel, R. Kienberger, M. Uiberacker, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, and F. Krausz, “Time-resolved atomic inner-shell spectroscopy,” Nature 419(6909), 803–807 (2002).
[CrossRef] [PubMed]

Kling, M. F.

E. Goulielmakis, Z. H. Loh, A. Wirth, R. Santra, N. Rohringer, V. S. Yakovlev, S. Zherebtsov, T. Pfeifer, A. M. Azzeer, M. F. Kling, S. R. Leone, and F. Krausz, “Real-time observation of valence electron motion,” Nature 466(7307), 739–743 (2010).
[CrossRef] [PubMed]

M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

Komninos, Y.

M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

Kompa, K. L.

M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

Korbman, M.

M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

Kovacev, M.

Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
[CrossRef] [PubMed]

Krausz, F.

V. S. Yakovlev, J. Gagnon, N. Karpowicz, and F. Krausz, “Attosecond streaking enables the measurement of quantum phase,” Phys. Rev. Lett. 105(7), 073001 (2010).
[CrossRef] [PubMed]

M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
[CrossRef]

M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

E. Goulielmakis, Z. H. Loh, A. Wirth, R. Santra, N. Rohringer, V. S. Yakovlev, S. Zherebtsov, T. Pfeifer, A. M. Azzeer, M. F. Kling, S. R. Leone, and F. Krausz, “Real-time observation of valence electron motion,” Nature 466(7307), 739–743 (2010).
[CrossRef] [PubMed]

F. Krausz and M. Ivanov, “Attosecond physics,” Rev. Mod. Phys. 81(1), 163–234 (2009).
[CrossRef]

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

M. Schultze, E. Goulielmakis, M. Uiberacker, M. Hofstetter, J. Kim, D. Kim, F. Krausz, and U. Kleineberg, “Powerful 170-attosecond XUV pulses generated with few-cycle laser pulses and broadband multilayer optics,” N. J. Phys. 9(7), 243 (2007).
[CrossRef]

V. Pervak, A. V. Tikhonravov, M. K. Trubetskov, S. Naumov, F. Krausz, and A. Apolonski, “1.5-octave chirped mirror for pulse compression down to sub-3 fs,” Appl. Phys. B 87(1), 5–12 (2007).
[CrossRef]

M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
[CrossRef] [PubMed]

A. Wonisch, U. Neuhäusler, N. M. Kabachnik, T. Uphues, M. Uiberacker, V. Yakovlev, F. Krausz, M. Drescher, U. Kleineberg, and U. Heinzmann, “Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses,” Appl. Opt. 45(17), 4147–4156 (2006).
[CrossRef] [PubMed]

E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
[CrossRef] [PubMed]

R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
[CrossRef] [PubMed]

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R. Kienberger, E. Goulielmakis, M. Uiberacker, A. Baltuška, V. Yakovlev, F. Bammer, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Atomic transient recorder,” Nature 427(6977), 817–821 (2004).
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R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
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M. Suman, G. Monaco, M.-G. Pelizzo, D. L. Windt, and P. Nicolosi, “Realization and characterization of an XUV multilayer coating for attosecond pulses,” Opt. Express 17(10), 7922–7932 (2009).
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M. Hentschel, R. Kienberger, Ch. Spielmann, G. A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond metrology,” Nature 414(6863), 509–513 (2001).
[CrossRef] [PubMed]

A. L. Cavalieri, N. Müller, T. Uphues, V. S. Yakovlev, A. Baltuška, B. Horvath, B. Schmidt, L. Blümel, R. Holzwarth, S. Hendel, M. Drescher, U. Kleineberg, P. M. Echenique, R. Kienberger, F. Krausz, and U. Heinzmann, “Attosecond spectroscopy in condensed matter,” Nature 449(7165), 1029–1032 (2007).
[CrossRef] [PubMed]

M. Uiberacker, Th. Uphues, M. Schultze, A. J. Verhoef, V. Yakovlev, M. F. Kling, J. Rauschenberger, N. M. Kabachnik, H. Schröder, M. Lezius, K. L. Kompa, H.-G. Muller, M. J. J. Vrakking, S. Hendel, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Attosecond real-time observation of electron tunnelling in atoms,” Nature 446(7136), 627–632 (2007).
[CrossRef] [PubMed]

E. Goulielmakis, Z. H. Loh, A. Wirth, R. Santra, N. Rohringer, V. S. Yakovlev, S. Zherebtsov, T. Pfeifer, A. M. Azzeer, M. F. Kling, S. R. Leone, and F. Krausz, “Real-time observation of valence electron motion,” Nature 466(7307), 739–743 (2010).
[CrossRef] [PubMed]

NIM A

Y. Li, J. Lewellen, Z. Huang, V. Sajaev, and S. V. Milton, “Time-resolved measurement of a self-amplified free-electron laser,” NIM A 507(1-2), 413–416 (2003).
[CrossRef]

Opt. Express

J. Gagnon and V. S. Yakovlev, “The robustness of attosecond streaking measurements,” Opt. Express 17(20), 17678–17693 (2009).
[CrossRef] [PubMed]

M. Suman, G. Monaco, M.-G. Pelizzo, D. L. Windt, and P. Nicolosi, “Realization and characterization of an XUV multilayer coating for attosecond pulses,” Opt. Express 17(10), 7922–7932 (2009).
[CrossRef] [PubMed]

Opt. Lett.

E. Gustafsson, T. Ruchon, M. Swoboda, T. Remetter, E. Pourtal, R. López-Martens, Ph. Balcou, and A. L’Huillier, “Broadband attosecond pulse shaping,” Opt. Lett. 32(11), 1353–1355 (2007).
[CrossRef] [PubMed]

A.-S. Morlens, P. Balcou, P. Zeitoun, C. Valentin, V. Laude, and S. Kazamias, “Compression of attosecond harmonic pulses by extreme-ultraviolet chirped mirrors,” Opt. Lett. 30(12), 1554–1556 (2005).
[CrossRef] [PubMed]

A. Aquila, F. Salmassi, and E. Gullikson, “Metrologies for the phase characterization of attosecond extreme ultraviolet optics,” Opt. Lett. 33(5), 455–457 (2008).
[CrossRef] [PubMed]

Phys. Rev. A

L. Y. Peng, F. Tan, Q. Gong, E. A. Pronin, and A. F. Starace, “Few-cycle attosecond pulse chirp effects on asymmetries in ionized electron momentum distributions,” Phys. Rev. A 80(1), 013407 (2009).
[CrossRef]

Phys. Rev. Lett.

V. S. Yakovlev, J. Gagnon, N. Karpowicz, and F. Krausz, “Attosecond streaking enables the measurement of quantum phase,” Phys. Rev. Lett. 105(7), 073001 (2010).
[CrossRef] [PubMed]

M. Kitzler, N. Milosevic, A. Scrinzi, F. Krausz, and T. Brabec, “Quantum theory of attosecond XUV pulse measurement by laser dressed photoionization,” Phys. Rev. Lett. 88(17), 173904 (2002).
[CrossRef] [PubMed]

I. P. Christov, M. M. Murnane, and H. C. Kapteyn, “High-Harmonic Generation of Attosecond Pulses in the “Single-Cycle” Regime,” Phys. Rev. Lett. 78(7), 1251–1254 (1997).
[CrossRef]

R. López-Martens, K. Varjú, P. Johnsson, J. Mauritsson, Y. Mairesse, P. Salières, M. B. Gaarde, K. J. Schafer, A. Persson, S. Svanberg, C.-G. Wahlström, and A. L’huillier, “Amplitude and phase control of attosecond light pulses,” Phys. Rev. Lett. 94(3), 033001 (2005).
[CrossRef] [PubMed]

Rev. Mod. Phys.

F. Krausz and M. Ivanov, “Attosecond physics,” Rev. Mod. Phys. 81(1), 163–234 (2009).
[CrossRef]

Rev. Sci. Instrum.

M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger, and F. Krausz, “Versatile apparatus for attosecond metrology and spectroscopy,” Rev. Sci. Instrum. 81, 1 (2010).
[CrossRef]

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbügel, B. A. Richman, and D. J. Kane, “Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating,” Rev. Sci. Instrum. 68(9), 3277 (1997).
[CrossRef]

Science

R. Kienberger, M. Hentschel, M. Uiberacker, Ch. Spielmann, M. Kitzler, A. Scrinzi, M. Wieland, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Steering attosecond electron wave packets with light,” Science 297(5584), 1144–1148 (2002).
[CrossRef] [PubMed]

Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovačev, R. Taïeb, B. Carré, H. G. Muller, P. Agostini, and P. Salières, “Attosecond synchronization of high-harmonic soft x-rays,” Science 302(5650), 1540–1543 (2003).
[CrossRef] [PubMed]

E. Goulielmakis, M. Uiberacker, R. Kienberger, A. Baltuška, V. Yakovlev, A. Scrinzi, Th. Westerwalbesloh, U. Kleineberg, U. Heinzmann, M. Drescher, and F. Krausz, “Direct measurement of light waves,” Science 305(5688), 1267–1269 (2004).
[CrossRef] [PubMed]

G. Sansone, E. Benedetti, F. Calegari, C. Vozzi, L. Avaldi, R. Flammini, L. Poletto, P. Villoresi, C. Altucci, R. Velotta, S. Stagira, S. De Silvestri, and M. Nisoli, “Isolated single-cycle attosecond pulses,” Science 314(5798), 443–446 (2006).
[CrossRef] [PubMed]

E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg, “Single-cycle nonlinear optics,” Science 320(5883), 1614–1617 (2008).
[CrossRef] [PubMed]

M. Drescher, M. Hentschel, R. Kienberger, G. Tempea, C. Spielmann, G. A. Reider, P. B. Corkum, and F. Krausz, “X-ray pulses approaching the attosecond frontier,” Science 291(5510), 1923–1927 (2001).
[CrossRef] [PubMed]

M. Schultze, M. Fieß, N. Karpowicz, J. Gagnon, M. Korbman, M. Hofstetter, S. Neppl, A. L. Cavalieri, Y. Komninos, Th. Mercouris, C. A. Nicolaides, R. Pazourek, S. Nagele, J. Feist, J. Burgdörfer, A. M. Azzeer, R. Ernstorfer, R. Kienberger, U. Kleineberg, E. Goulielmakis, F. Krausz, and V. S. Yakovlev, “Delay in photoemission,” Science 328(5986), 1658–1662 (2010).
[CrossRef] [PubMed]

Other

M. Hofstetter, M. Schultze, M. Fieß, A. Guggenmos, J. Gagnon, E. Magerl, E. Botschafter, R. Ernstorfer, R. Kienberger, E. M. Gullikson, F. Krausz, and U. Kleineberg, “First attosecond pulse control by multilayer mirrors above 100 eV photon energy,“ in Ultrafast Phenomena XVII, 11.17, M. Chergui, D. Jonas, E. Riedle, B. Schönlein, A. Taylor (Oxford University Press, New York, 2010).

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Figures (5)

Fig. 1
Fig. 1

Operational principle of XUV chirped multilayers: Calculated square of the electric field amplitude of the standing wave formed in the multilayer structure upon reflection in the 94–133 eV photon energy range, normalized to that of the incident wave. Following the energy dependent maxima of the standing field, it is obvious that the penetration depth is wavelength dependent. Thus the mirrors introduce positive (a) and negative (b) chirp, resulting in an increasing and decreasing group delay for increasing photon energy respectively as the energy-dependent penetration depth signifies as depicted by the coloured arrows. The multilayer structure assumed here resembles the experimentally realized a-periodic multilayer mirrors as displayed in Fig. 2 (a/d) and (c/f).

Fig. 2
Fig. 2

Characteristics of XUV chirped multilayer coatings designed and manufactured for the experiments: Set of XUV multilayers with positive (a), near zero (b) and negative (c) group delay dispersion. The diagrams compare the measured (solid black) with the designed (dotted green) reflectivity curves. The calculated group delays (derivative of the spectral phase with respect to angular frequency) are also displayed (dashed red curve). The transmittivity of a 150-nm palladium foil is additionally qualitatively plotted in panel (b), depicted by the blue dash-dotted line. The lower panels (d), (e) and (f) show the corresponding mirror-designs of the appropriate mirrors above. Each colour represents one material as explained by the legend in 2(e).

Fig. 3
Fig. 3

Measured and retrieved attosecond electron streaking spectrograms, upper and lower row, respectively. Panels (a)-(c) and (d)-(f) display spectrograms recorded with attosecond pulses reflected off the mirrors described in Fig. 2(a)2(c), respectively. The energy shift in the recorded spectra is proportional to the vector potential AL(t) of the streaking laser field at the instant of photoemission, hence the dependence of this energy shift on the delay between the attosecond XUV pulse and the NIR laser field reflects the temporal evolution of the NIR laser field’s vector potential, AL(t). Narrowing and broadening in the streaked electron spectra at the zero crossings is displayed by enhanced and diminished electron count rates, respectively. The small insets show the energy calibrated raw data before subtraction of the background.

Fig. 4
Fig. 4

Qualitative analysis of attosecond streak images of a linearly negatively-chirped attosecond pulse. For explanation, see text.

Fig. 5
Fig. 5

Retrieved spectral and temporal characteristics of the attosecond XUV pulse, upper row and lower row, respectively. Panels (a), (b) and (c) display the intensity spectrum (green dotted line) and group delay (red dashed line) of the attosecond XUV pulse reflected off the mirrors described in Fig. 2(a), 2(b), and 2(c), respectively, as retrieved from the measured streaking spectrograms shown in Fig. 3(a), 3(b), and 3(c), respectively. The black full lines depict the corresponding XUV spectra measured directly with an XUV spectrometer. The evaluated effective group-delay dispersions weighted by the final spectral XUV intensity are also shown. Panels (d), (e), (f) show the temporal intensity profile (black line) and temporal phase (red dashed line) retrieved from the streaking spectrograms of Fig. 3(a), 3(b), and 3(c), respectively. The XUV pulse duration (full width at intensity half maximum) has been evaluated and is displayed at the bottom of each panel.

Tables (1)

Tables Icon

Table 1 Comparison of XUV mirror designed and FROG retrieved pulse parameters*

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