Abstract

Based on a comparative analysis of the formulas of the stochastic and dynamic theories for a homogeneous optical band of an impurity center, the interactions of the impurity center with the tunnel excitations that exist in glasses and polymers are investigated. It is shown that the formulas of the dynamic theory make it possible to explain the contribution to the spectral diffusion effect from separate groups of two-level systems and to judge the character of the interaction of the impurity center with the tunnel excitations in glasses and polymers.

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  1. I. S. Osad’ko, “Optical dephasing and homogeneous optical bands in crystals and amorphous solids,” Phys. Rep. 206, No. 2, 43 (1991).
    [CrossRef]
  2. A. Heuer and R. J. Silbey, “Collective dynamics in glasses and its relation to the low-temperature anomalies,” Phys. Rev. B 53, 609 (1996).
    [CrossRef]
  3. A. V. Naumov, “Low-temperature optical dynamics of impurity organic glasses: studies by means of the spectroscopy of single molecules and photon echo,” candidate’s dissertation (Troitsk, Moscow Oblast, 2003).
  4. Yu. G. Va?ner, “Dynamics of disordered molecular solid-state media: studies by means of photon echo and the spectroscopy of single molecules,” doctoral dissertation (Troitsk, Moscow Oblast, 2005).
  5. A. V. Naumov, “Spectroscopy of single molecules as a method of studying the low-temperature dynamics of disordered solid-state media,” doctoral dissertation (Troitsk, Moscow Oblast, 2009).
  6. I. S. Osad’ko and M. A. Mikhailov, “Dynamical theory for spectral diffusion in optical spectra of single molecules and molecular ensembles,” Phys. Lett. A 208, 231 (1995).
    [CrossRef]
  7. I. S. Osad’ko, M. A. Mikha?lov, and N. N. Za?tsev, “Study of spectral diffusion by means of stimulated photon echo and hole burning,” Izv. Akad. Nauk Ser. Fiz. 62, 268 (1998).
  8. K. A. Littau and M. D. Fayer, “Probing low-temperature glass dynamics by fast generation and detection of optical holes,” Chem. Phys. Lett. 176, 551 (1991).
    [CrossRef]
  9. H. C. Meijers and D. A. Wiersma, “Glass dynamics probed by the long-lived stimulated photon echo,” Phys. Rev. Lett. 68, 381 (1992).
    [CrossRef] [PubMed]
  10. P. Hu and S. R. Hartmann, “Theory of spectral diffusion decay using an uncorrelated-sudden-jump model,” Phys. Rev. B 9, 1 (1974).
    [CrossRef]
  11. P. Hu and L. R. Walker, “Spectral-diffusion decay in echo experiments,” Phys. Rev. B 18, 1300 (1978).
    [CrossRef]
  12. Y. S. Bai and M. D. Fayer, “Time scales and optical dephasing measurements: Investigation of dynamics in complex systems,” Phys. Rev. B 39, 11066 (1989).
    [CrossRef]
  13. I. S. Osad’ko, “Theory of the absorption and emission of light by organic impurity centers,” in Spectroscopy and Excitation Dynamics of Condensed Molecular Systems, V. M. Agranovich and R. M. Hochstrasser, eds. (Elsevier, St. Louis, 1983; Nauka, Moscow, 1987), pp. 263–314.
  14. I. S. Osad’ko, “Determination of electron–phonon coupling from structured optical spectra of impurity centers,” Usp. Fiz. Nauk 128, No. 1, 31 (1979). [Sov. Phys. Usp. 22, 311 (1979)].
    [CrossRef]
  15. W. P. Ambrose, Th. Basche, and W. E. Moerner, “Detection and spectroscopy of single pentacene molecules in a p-terphenyl crystal by means of fluorescence excitation,” J. Chem. Phys. 95, 7150 (1991).
    [CrossRef]

1998 (1)

I. S. Osad’ko, M. A. Mikha?lov, and N. N. Za?tsev, “Study of spectral diffusion by means of stimulated photon echo and hole burning,” Izv. Akad. Nauk Ser. Fiz. 62, 268 (1998).

1996 (1)

A. Heuer and R. J. Silbey, “Collective dynamics in glasses and its relation to the low-temperature anomalies,” Phys. Rev. B 53, 609 (1996).
[CrossRef]

1995 (1)

I. S. Osad’ko and M. A. Mikhailov, “Dynamical theory for spectral diffusion in optical spectra of single molecules and molecular ensembles,” Phys. Lett. A 208, 231 (1995).
[CrossRef]

1992 (1)

H. C. Meijers and D. A. Wiersma, “Glass dynamics probed by the long-lived stimulated photon echo,” Phys. Rev. Lett. 68, 381 (1992).
[CrossRef] [PubMed]

1991 (3)

I. S. Osad’ko, “Optical dephasing and homogeneous optical bands in crystals and amorphous solids,” Phys. Rep. 206, No. 2, 43 (1991).
[CrossRef]

K. A. Littau and M. D. Fayer, “Probing low-temperature glass dynamics by fast generation and detection of optical holes,” Chem. Phys. Lett. 176, 551 (1991).
[CrossRef]

W. P. Ambrose, Th. Basche, and W. E. Moerner, “Detection and spectroscopy of single pentacene molecules in a p-terphenyl crystal by means of fluorescence excitation,” J. Chem. Phys. 95, 7150 (1991).
[CrossRef]

1989 (1)

Y. S. Bai and M. D. Fayer, “Time scales and optical dephasing measurements: Investigation of dynamics in complex systems,” Phys. Rev. B 39, 11066 (1989).
[CrossRef]

1979 (1)

I. S. Osad’ko, “Determination of electron–phonon coupling from structured optical spectra of impurity centers,” Usp. Fiz. Nauk 128, No. 1, 31 (1979). [Sov. Phys. Usp. 22, 311 (1979)].
[CrossRef]

1978 (1)

P. Hu and L. R. Walker, “Spectral-diffusion decay in echo experiments,” Phys. Rev. B 18, 1300 (1978).
[CrossRef]

1974 (1)

P. Hu and S. R. Hartmann, “Theory of spectral diffusion decay using an uncorrelated-sudden-jump model,” Phys. Rev. B 9, 1 (1974).
[CrossRef]

Ambrose, W. P.

W. P. Ambrose, Th. Basche, and W. E. Moerner, “Detection and spectroscopy of single pentacene molecules in a p-terphenyl crystal by means of fluorescence excitation,” J. Chem. Phys. 95, 7150 (1991).
[CrossRef]

Bai, Y. S.

Y. S. Bai and M. D. Fayer, “Time scales and optical dephasing measurements: Investigation of dynamics in complex systems,” Phys. Rev. B 39, 11066 (1989).
[CrossRef]

Basche, Th.

W. P. Ambrose, Th. Basche, and W. E. Moerner, “Detection and spectroscopy of single pentacene molecules in a p-terphenyl crystal by means of fluorescence excitation,” J. Chem. Phys. 95, 7150 (1991).
[CrossRef]

Fayer, M. D.

K. A. Littau and M. D. Fayer, “Probing low-temperature glass dynamics by fast generation and detection of optical holes,” Chem. Phys. Lett. 176, 551 (1991).
[CrossRef]

Y. S. Bai and M. D. Fayer, “Time scales and optical dephasing measurements: Investigation of dynamics in complex systems,” Phys. Rev. B 39, 11066 (1989).
[CrossRef]

Hartmann, S. R.

P. Hu and S. R. Hartmann, “Theory of spectral diffusion decay using an uncorrelated-sudden-jump model,” Phys. Rev. B 9, 1 (1974).
[CrossRef]

Heuer, A.

A. Heuer and R. J. Silbey, “Collective dynamics in glasses and its relation to the low-temperature anomalies,” Phys. Rev. B 53, 609 (1996).
[CrossRef]

Hu, P.

P. Hu and L. R. Walker, “Spectral-diffusion decay in echo experiments,” Phys. Rev. B 18, 1300 (1978).
[CrossRef]

P. Hu and S. R. Hartmann, “Theory of spectral diffusion decay using an uncorrelated-sudden-jump model,” Phys. Rev. B 9, 1 (1974).
[CrossRef]

Littau, K. A.

K. A. Littau and M. D. Fayer, “Probing low-temperature glass dynamics by fast generation and detection of optical holes,” Chem. Phys. Lett. 176, 551 (1991).
[CrossRef]

Meijers, H. C.

H. C. Meijers and D. A. Wiersma, “Glass dynamics probed by the long-lived stimulated photon echo,” Phys. Rev. Lett. 68, 381 (1992).
[CrossRef] [PubMed]

Mikhailov, M. A.

I. S. Osad’ko, M. A. Mikha?lov, and N. N. Za?tsev, “Study of spectral diffusion by means of stimulated photon echo and hole burning,” Izv. Akad. Nauk Ser. Fiz. 62, 268 (1998).

I. S. Osad’ko and M. A. Mikhailov, “Dynamical theory for spectral diffusion in optical spectra of single molecules and molecular ensembles,” Phys. Lett. A 208, 231 (1995).
[CrossRef]

Moerner, W. E.

W. P. Ambrose, Th. Basche, and W. E. Moerner, “Detection and spectroscopy of single pentacene molecules in a p-terphenyl crystal by means of fluorescence excitation,” J. Chem. Phys. 95, 7150 (1991).
[CrossRef]

Naumov, A. V.

A. V. Naumov, “Spectroscopy of single molecules as a method of studying the low-temperature dynamics of disordered solid-state media,” doctoral dissertation (Troitsk, Moscow Oblast, 2009).

A. V. Naumov, “Low-temperature optical dynamics of impurity organic glasses: studies by means of the spectroscopy of single molecules and photon echo,” candidate’s dissertation (Troitsk, Moscow Oblast, 2003).

Osad’ko, I. S.

I. S. Osad’ko, M. A. Mikha?lov, and N. N. Za?tsev, “Study of spectral diffusion by means of stimulated photon echo and hole burning,” Izv. Akad. Nauk Ser. Fiz. 62, 268 (1998).

I. S. Osad’ko and M. A. Mikhailov, “Dynamical theory for spectral diffusion in optical spectra of single molecules and molecular ensembles,” Phys. Lett. A 208, 231 (1995).
[CrossRef]

I. S. Osad’ko, “Optical dephasing and homogeneous optical bands in crystals and amorphous solids,” Phys. Rep. 206, No. 2, 43 (1991).
[CrossRef]

I. S. Osad’ko, “Determination of electron–phonon coupling from structured optical spectra of impurity centers,” Usp. Fiz. Nauk 128, No. 1, 31 (1979). [Sov. Phys. Usp. 22, 311 (1979)].
[CrossRef]

I. S. Osad’ko, “Theory of the absorption and emission of light by organic impurity centers,” in Spectroscopy and Excitation Dynamics of Condensed Molecular Systems, V. M. Agranovich and R. M. Hochstrasser, eds. (Elsevier, St. Louis, 1983; Nauka, Moscow, 1987), pp. 263–314.

Silbey, R. J.

A. Heuer and R. J. Silbey, “Collective dynamics in glasses and its relation to the low-temperature anomalies,” Phys. Rev. B 53, 609 (1996).
[CrossRef]

Vainer, Yu. G.

Yu. G. Va?ner, “Dynamics of disordered molecular solid-state media: studies by means of photon echo and the spectroscopy of single molecules,” doctoral dissertation (Troitsk, Moscow Oblast, 2005).

Walker, L. R.

P. Hu and L. R. Walker, “Spectral-diffusion decay in echo experiments,” Phys. Rev. B 18, 1300 (1978).
[CrossRef]

Wiersma, D. A.

H. C. Meijers and D. A. Wiersma, “Glass dynamics probed by the long-lived stimulated photon echo,” Phys. Rev. Lett. 68, 381 (1992).
[CrossRef] [PubMed]

Zaitsev, N. N.

I. S. Osad’ko, M. A. Mikha?lov, and N. N. Za?tsev, “Study of spectral diffusion by means of stimulated photon echo and hole burning,” Izv. Akad. Nauk Ser. Fiz. 62, 268 (1998).

Chem. Phys. Lett. (1)

K. A. Littau and M. D. Fayer, “Probing low-temperature glass dynamics by fast generation and detection of optical holes,” Chem. Phys. Lett. 176, 551 (1991).
[CrossRef]

Izv. Akad. Nauk Ser. Fiz. (1)

I. S. Osad’ko, M. A. Mikha?lov, and N. N. Za?tsev, “Study of spectral diffusion by means of stimulated photon echo and hole burning,” Izv. Akad. Nauk Ser. Fiz. 62, 268 (1998).

J. Chem. Phys. (1)

W. P. Ambrose, Th. Basche, and W. E. Moerner, “Detection and spectroscopy of single pentacene molecules in a p-terphenyl crystal by means of fluorescence excitation,” J. Chem. Phys. 95, 7150 (1991).
[CrossRef]

Phys. Lett. A (1)

I. S. Osad’ko and M. A. Mikhailov, “Dynamical theory for spectral diffusion in optical spectra of single molecules and molecular ensembles,” Phys. Lett. A 208, 231 (1995).
[CrossRef]

Phys. Rep. (1)

I. S. Osad’ko, “Optical dephasing and homogeneous optical bands in crystals and amorphous solids,” Phys. Rep. 206, No. 2, 43 (1991).
[CrossRef]

Phys. Rev. B (4)

A. Heuer and R. J. Silbey, “Collective dynamics in glasses and its relation to the low-temperature anomalies,” Phys. Rev. B 53, 609 (1996).
[CrossRef]

P. Hu and S. R. Hartmann, “Theory of spectral diffusion decay using an uncorrelated-sudden-jump model,” Phys. Rev. B 9, 1 (1974).
[CrossRef]

P. Hu and L. R. Walker, “Spectral-diffusion decay in echo experiments,” Phys. Rev. B 18, 1300 (1978).
[CrossRef]

Y. S. Bai and M. D. Fayer, “Time scales and optical dephasing measurements: Investigation of dynamics in complex systems,” Phys. Rev. B 39, 11066 (1989).
[CrossRef]

Phys. Rev. Lett. (1)

H. C. Meijers and D. A. Wiersma, “Glass dynamics probed by the long-lived stimulated photon echo,” Phys. Rev. Lett. 68, 381 (1992).
[CrossRef] [PubMed]

Usp. Fiz. Nauk (1)

I. S. Osad’ko, “Determination of electron–phonon coupling from structured optical spectra of impurity centers,” Usp. Fiz. Nauk 128, No. 1, 31 (1979). [Sov. Phys. Usp. 22, 311 (1979)].
[CrossRef]

Other (4)

I. S. Osad’ko, “Theory of the absorption and emission of light by organic impurity centers,” in Spectroscopy and Excitation Dynamics of Condensed Molecular Systems, V. M. Agranovich and R. M. Hochstrasser, eds. (Elsevier, St. Louis, 1983; Nauka, Moscow, 1987), pp. 263–314.

A. V. Naumov, “Low-temperature optical dynamics of impurity organic glasses: studies by means of the spectroscopy of single molecules and photon echo,” candidate’s dissertation (Troitsk, Moscow Oblast, 2003).

Yu. G. Va?ner, “Dynamics of disordered molecular solid-state media: studies by means of photon echo and the spectroscopy of single molecules,” doctoral dissertation (Troitsk, Moscow Oblast, 2005).

A. V. Naumov, “Spectroscopy of single molecules as a method of studying the low-temperature dynamics of disordered solid-state media,” doctoral dissertation (Troitsk, Moscow Oblast, 2009).

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