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Vibrational Stark effect for matrix-isolated CN molecules

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Abstract

Stark measurements have been made on persistent IR spectral holes in the stretch mode of the CN:Na+ center in KBr. A simple model in which the anharmonic CN molecule is coupled harmonically to the lattice qualitatively explains both the magnitude of the zero-field frequency difference for the two molecular arrangements in the crystal as well as the absence of a Stark tuning curve for one of these configurations.

© 1992 Optical Society of America

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