Abstract

The linear and nonlinear optical properties of ${\rm{BaG}}{{\rm{a}}_4}{{\rm{S}}_7}$, ${\rm{BaG}}{{\rm{a}}_4}{\rm{S}}{{\rm{e}}_7}$, ${\rm{BaG}}{{\rm{a}}_2}{\rm{Ge}}{{\rm{S}}_6}$, and ${\rm{BaG}}{{\rm{a}}_2}{\rm{GeSe}}_{6}$ are reviewed, highlighting their potential for frequency downconversion of powerful laser sources from the near- to the mid-IR. Examples of successful applications are summarized and briefly discussed.

© 2021 Optical Society of America

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